Sapphire Laser Research Articles

Generation of 13.9-mJ Terahertz Radiation from Lithium Niobate Materials.

Extremely strong-field terahertz (THz) radiation in free space has compelling applications in nonequilibrium condensed matter state regulation, all-optical THz electron acceleration and manipulation, THz biological effects, etc. However, these practical applications are constrained by the absence of high-intensity, high-efficiency, high-beam-quality, and stable solid-state THz light sources. Here, the generation of single-cycle 13.9-mJ extreme THz pulses from cryogenically cooled lithium niobate crystals and a 1.2% energy conversion efficiency from 800nm to THz are demonstrated experimentally using the tilted pulse-front technique driven by a home-built 30-fs, 1.2-Joule Ti:sapphire laser amplifier. The focused peak electric field strength is estimated to be 7.5MVcm-1 . A record of 1.1-mJ THz single-pulse energy at a 450 mJ pump at room temperature is produced and observed that the self-phase modulation of the optical pump can induce THz saturation behavior from the crystals in the substantially nonlinear pump regime. This study lays the foundation for the generation of sub-Joule THz radiation from lithium niobate crystals and will inspire more innovations in extreme THz science and applications.

High-resolution Cs-Rb two-photon spectrometer for directly stabilizing a Ti:sapphire comb laser.

In this paper, we present a simple scheme for efficiently removing the residual Doppler background of a comb laser based two-photon spectrometer to be better than 10-3 background-to-signal ratio. We applied this scheme to stabilize the frequencies of a mode-locked Ti:sapphire laser directly referring to the cesium 6S-8S transition and rubidium 5S-5D transition. We suggest a standard operation procedure (SOP) for the fully direct comb laser stabilization and evaluate the frequency of two spectral lines at a certain temperature, by which we demonstrate an all-atomic-transition-based Ti:sapphire comb laser merely via a 6-cm glass cell.

Mid-infrared frequency domain optical parametric amplifier.

We report on an optical architecture delivering sub-120 femtosecond laser pulses of 20 µJ tunable from 5.5 µm to 13 µm in the mid-infrared range (mid-IR). The system is based on a dual-band frequency domain optical parametric amplifier (FOPA) optically pumped by a Ti:Sapphire laser and amplifying 2 synchronized femtosecond pulses each with a widely tunable wavelength around 1.6 and 1.9 µm respectively. These amplified pulses are then combined in a GaSe crystal to produce the mid-IR few-cycle pulses by means of difference frequency generation (DFG). The architecture provides a passively stabilized carrier-envelope phase (CEP) whose fluctuations has been characterized to 370 mrad RMS.

Frequency-doubled Q-switched 4 × 4 multicore fiber laser system.

Frequency doubling of a Q-switched Yb-doped rod-type 4 × 4 multicore fiber (MCF) laser system is reported. A second harmonic generation (SHG) efficiency of up to 52% was achieved with type I non-critically phase-matched lithium triborate (LBO), with a total SHG pulse energy of up to 17 mJ obtained at 1 kHz repetition rate. The dense parallel arrangement of amplifying cores into a shared pump cladding enables a significant increase in the energy capacity of active fibers. The frequency-doubled MCF architecture is compatible with high-repetition-rate and high-average-power operation and may provide an efficient alternative to bulk solid-state systems as pump sources for high-energy titanium-doped sapphire lasers.

Integrated titanium:sapphire laser

Integrated titanium:sapphire laser

Nanopatterning of the dielectric surface by a pair of femtosecond laser pulses of different colors through a monolayer of microspheres.

This paper considers the nanostructuring of the surface of dielectrics under the effect of two successive femtosecond laser pulses, one of the fundamental frequency (FF) and the other of the second harmonic (SH) of a Ti:sapphire laser, through a layer of polystyrene microspheres 1 µm in diameter, which act as microlenses. Polymers with strong (PMMA) and weak (TOPAS) absorption at the frequency of the third harmonic of a Ti:sapphire laser (sum frequency FF + SH) were used as targets. Laser irradiation led to the removal of microspheres and the formation of ablation craters with characteristic dimensions of about 100 nm. Depending on the variable delay time between pulses, the resulting structures differed in their geometric parameters and shape. Based on statistical processing of the depths of the obtained craters, the optimal delay times for the most effective structuring of the surfaces of these polymers was found.

Laser performance of high optical quality 4 at.% Pr3+: Sr0.7La0.3Mg0.3Al11.7O19 (Pr:ASL) single crystals.

In this work, we present the visible laser performance of improved optical quality Czochralski-grown 4 at.% Pr3+-doped Sr0.7La0.3Mg0.3Al11.7O19 (Pr:ASL) single crystals in the deep red (726 nm), the red (645 nm) and the orange (620 nm) range using two different pumping sources. Using a high beam quality frequency doubled Ti:sapphire laser with 1 W output power as pump source, deep red laser emission was reached at a wavelength of 726 nm with 40 mW of output power and a laser threshold of 86 mW. The corresponding slope efficiency was 9%. At 645 nm in the red, up to 41 mW of laser output power were obtained with 15% slope efficiency. Moreover, orange laser emission at 620 nm was demonstrated with 5 mW output power and 4.4% slope efficiency. Using a 10 W multi-diode module as pumping source allowed to obtain the highest output power of a red and deep-red diode-pumped Pr:ASL laser to date. The respective output powers at 726 and 645 nm reached 206 mW and 90 mW.

Sub-picosecond timing jitter between optically synchronized femtosecond and picosecond laser systems

Synchronized optical pulses are widely used. We report here characterization and measurement of synchronized femtosecond and picosecond pulses from a Ti:Sapphire laser (nominally 800 nm) and a Nd:YAG laser (1064 nm), respectively. Synchronization is achieved by utilizing soliton self-frequency shift in a photonic-crystal fiber that allows the 800 nm femtosecond oscillator to seed the third-harmonic generation (355 nm) of picosecond regenerative amplifier. The relative timing jitter between the amplified femtosecond and the third-harmonic generation of picosecond pulses is (710 ± 160) fs, which is only (1.17 ± 0.26)% of the picosecond pulse duration. This work paves way for applications in stimulated Raman scattering spectroscopy and amplification.

Laser-driven low energy electron beams for single-shot ultra-fast probing of meso-scale materials and warm dense matter

Laser wakefield acceleration has proven to be an excellent source of electrons and X-rays suitable for ultra-fast probing of matter. These novel beams have demonstrated unprecedented spatial and temporal resolution allowing for new discoveries in material science and plasma physics. In particular, the study of dynamic processes such as non-thermal melt and lattice changes on femtosecond time-scales have paved a way to completely new scientific horizons. Here, we demonstrate the first single-shot electron radiography measurement using an femtosecond electron source based on the downramp-density gradient laser-wakefield-acceleration with the use of a compact Ti:sapphire laser. A quasi-monoenergetic electron beam with mean energy of 1.9 ± 0.4 MeV and charge 77 ± 47 pC per shot was generated by the laser incident onto a gas target and collimated using a two ring-magnet beam path. High quality electron radiography of solid objects with spatial resolution better than 150 upmum was demonstrated. Further developments of this scheme have the potential to obtain single-shot ultrafast electron diffraction from dynamic lattices. This scheme poses a great promise for smaller scale university laboratories and facilities for efficient single-shot probing of warm dense matter, medical imaging and the study of dynamic processes in matter with broad application to inertial confinement fusion and meso-scale materials (mg g/cm^2).

Laser emission at 428 nm in N2+: Competition between two- and three-level amplification

Lasing of N2+ at 428 nm is studied as a function of the delay dt between two 800 nm ultrashort pumping pulses from a Ti:sapphire laser. This lasing corresponds to a population-inverted transition between levels B2Σu+(0) and X2Σg+(1) of a singly ionized nitrogen molecule. An important erasing of laser emission is observed under pumping with two consecutive pulses separated by large delays −20 ps < dt < +20 ps. From an analysis of the quenching results, we conclude that the mechanism of lasing corresponds to a coherent two-photon amplification scheme. Our results show that a two-photon process can dominate over a population-inverted one-photon amplification.

OH planar laser-induced fluorescence imaging system using a kilohertz-rate 283 nm UV Ti:sapphire laser.

A narrow linewidth Ti:sapphire laser is developed and characterized for the generation of an ultraviolet nanosecond laser pulses for the planar laser-induced fluorescence (PLIF) imaging of hydroxyl (OH). With a pump power of 11.4W at 1kHz, the Ti:sapphire laser produces 3.5mJ at 849nm with pulse duration of 17ns and achieves a conversion efficiency of 28.2%. Accordingly, its third-harmonic generation outputs 0.56mJ at 283nm in BBO with type I phase match. An OH PLIF imaging system has been built; a 1 to 4kHz fluorescent image of OH of a propane Bunsen burner has been captured based on this laser system.

Machine learning algorithms predict experimental output of chaotic lasers.

We apply an artificial neural network (ANN) of 20 hidden layers and backpropagation regression to the forecast of experimental time series from a Kerr lens mode locking (KLM) Ti:sapphire laser and a Nd:vanadate with modulation losses. In both cases the neural network is able to predict up to 10 steps ahead. In the Ti:sapphire laser the prediction in pulse amplitude is accurate even when the pulse is an extreme event. In the Nd:vanadate laser we forecast both pulse amplitude and pulse-to-pulse time separation. In both cases the prediction goes beyond the Lyapunov prediction horizon.

Development of a 671 nm injection-locked CW Ti:sapphire laser

We developed an injection-locked Ti:sapphire laser at a wavelength of 671 nm where the fluorescence gain of the Ti:sapphire crystal is quite low. We obtained an output of more than 500 mW at a pump power of 10 W. The injection-locked lasing operates at a single-frequency and unidirectionally lasing with no intracavity optical components. The spectral property and the stability condition for the unidirectional lasing of the injection-locked Ti:sapphire laser are reported. The developed laser will produce the powerful light source required for the laser cooling of lithium atoms.

Hyperfine structure and isotope shifts of xenon measured for near-infrared transitions with Doppler-free saturated absorption spectroscopy

Hyperfine structure and isotope shifts of Xe were investigated with Doppler-free saturated absorption spectroscopy for all transitions in the 820-841 nm spectral interval. The Xe samples were commercial gases of natural isotopic abundances. The measurements were performed by employing a widely tunable narrow line Ti:sapphire laser. The hyperfine structures for 129Xe and 131Xe were well resolved. For the transitions with the wavelengths in vacuum near 820.860 nm and 841.150 nm also isotope shifts of the even isotopes were clearly observed. The modeling of the shapes of the observed absorption lines qualitatively reproduces experimental spectral profiles. The measured absorption peaks of the hyperfine structure and isotope shifts of Xe isotopes present characteristic spectral fingerprints for their identification. Eventually, quantitative spectral analysis will provide isotopic abundances of natural, as well as radioactive Xe gas samples.

Optical and Microwave Metrology at the 10−18 Level with an Er/Yb:glass Frequency Comb

AbstractOptical frequency combs are essential tools for precision metrology experiments ranging in application from remote spectroscopic sensing of trace gases to the characterization and comparison of optical atomic clocks for precision time‐keeping and searches for physics beyond the standard model. Presented here is a description of the architecture and a full characterization of a telecom‐band, self‐modelocking frequency comb based on a free‐space laser with an Er/Yb co‐doped glass gain medium. The laser provides a robust and cost‐effective alternative to Er:fibre laser based frequency combs, while offering stability and noise performance similar to Ti:sapphire laser systems. Finally, the utility of the Er/Yb:glass frequency comb is demonstrated in high‐stability frequency synthesis using two ultra‐stable optical references at 1157 nm and 1070 nm and in low‐noise photonic microwave generation by dividing these references to the microwave domain.

Optical Waveform Synthesis and Its Applications

AbstractThe quest for ever‐shorter optical pulses has been ongoing for over half a century. Although few‐cycle pulses have been generated for nearly 40 years, pulse lengths below the single‐cycle limit have remained an elusive goal for a long time. For this purpose, optical waveform synthesizers, generating high‐energy, high‐average‐power pulses via coherent combination of multiple pulses covering different spectral regions, have been recently developed. They allow unprecedented control over the generated optical waveforms, spanning an extremely broad spectral range from ultraviolet to infrared. Such control allows for steering strong‐field interactions with increased degrees of freedom. When driving high‐harmonic generation, tailored waveforms can produce bright attosecond pulse trains and even isolated attosecond pulses with tunable spectra up to the soft X‐ray range. In this paper recent progress on parametric and hollow‐core fiber waveform synthesizers is discussed. Newly developed seeding schemes; absolute, relative, and spectral phase measurement; and control techniques suitable for synthesizers are described. The progress on serial and parallel waveform synthesis based on Ti:sapphire and Ytterbium laser systems and their latest applications in high‐harmonic generation in gaseous and solid media, attosecond science, and laser wakefield acceleration is discussed.

Transverse-pumping approach for a powerful single-mode Ti:sapphire laser for near infrared lidar applications: publisher's note.

This publisher's note contains corrections to Appl. Opt.61, 8553 (2022)APOPAI0003-693510.1364/AO.463257.

Design, construction and characterisation of a diode-pumped, three-element, 1-GHz Kerr-lens-modelocked Ti:sapphire oscillator

We present a design and construction prescription for a 1-GHz repetition rate Ti:sapphire laser pumped with a single green pump diode and with a resonator comprising as few as three optical elements. In a three-element configuration, the laser produces 111-fs pulses and exhibits self-starting Kerr-lens modelocking at pump powers above 850 mW. At 1.1 W of pump power, the average output of the laser is over 116 mW, and the slope efficiency is measured to be 13%. With the addition of a fourth dispersion-compensating element to optimise the second-order group-delay intracavity dispersion, we have demonstrated a reduction of the pulse durations to 87 fs with an average power of 108 mW.

Spectrally combined four-diode-pumped femtosecond Ti:sapphire laser with 16.3 nJ pulse and its application to video-rate coherent anti-Stokes Raman scattering spectro-microscopy.

We demonstrate the generation of high-energy femtosecond pulses by a spectrally combined four-diode-pumped Ti:sapphire laser with semi-conductor saturable absorber mirror mode locking. To achieve energy scaling, the laser cavity was extended using a design based on the Herriott multipass cell. The laser operates at a 17.5 MHz repetition rate and generates pulses with energies as high as 16.3 nJ and 80 fs in duration. The signal-to-noise ratio at the fundamental frequency showed an extinction ratio of >50 dB relative to the carrier. This compact single laser was applied to video-rate forward and backward coherent anti-Stokes Raman scattering spectro-microscopy with a pixel dwell time of 122 ns, which is the lowest dwell time ever achieved, to the best of our knowledge.

Diamond Photoconductive Antenna for Terahertz Generation Equipped with Buried Graphite Electrodes

It has been shown recently that a photoconductive antenna (PCA) based on a nitrogen-doped diamond can be effectively excited by the second harmonic of a Ti:sapphire laser (λ = 400 nm). The THz emission performance of the PCA can be significantly increased if a much stronger electric field is created between the close-located electrodes. To produce a homogeneous electric field over the entire excited diamond volume, the laser fabrication of deep-buried graphite electrodes inside the diamond crystal was proposed. Several electrodes consisting of the arrays of buried pillars connected by the surface graphite stripes were produced inside an HPHT diamond crystal using femtosecond and nanosecond laser pulses. Combining different pairs of the electrodes, a series of PCAs with various electrode interspaces was formed. The THz emission of the PCAs equipped with the buried electrodes was measured at different values of excitation fluence and bias voltage (DC and pulsed) and compared with the emission of the same diamond crystal when the bias voltage was applied to the surface electrodes on the opposite faces. All examined PCAs have demonstrated the square-law dependencies of the THz fluence on the field strength, while the saturation fluence fluctuated in the range of 1200–1600 µJ/cm2. The THz emission performance was found to be approximately the same for the PCAs with the surface electrodes and with the buried electrodes spaced at a distance of 1.4–3.5 mm. However, it noticeably decreased when the distance between the buried electrodes was reduced to 0.5 mm.