Rydberg Atom Quantum Simulators Research Articles

Long-Lived Circular Rydberg Qubits of Alkaline-Earth Atoms in Optical Tweezers

Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of magnitude, as they can be effectively protected from decay due to their maximum angular momentum. We report the first realization of alkaline-earth circular Rydberg atoms trapped in optical tweezers, which provide unique and novel control possibilities due to the optically active ionic core. Specifically, we demonstrate creation of very high-n (n=79) circular states of Sr88. We measure lifetimes as long as 2.55 ms at room temperature, which are achieved via cavity-assisted suppression of black-body radiation. We show coherent control of a microwave qubit encoded in circular states of nearby manifolds, and characterize the qubit coherence time via Ramsey and spin-echo spectroscopy. Finally, circular-state tweezer trapping exploiting the Sr+ core polarizability is quantified via measurements of the trap-induced light shift on the qubit. Our work opens routes for quantum simulations with circular Rydberg states of divalent atoms, exploiting the emergent toolbox associated with the optically active core ion. Published by the American Physical Society 2024

A randomized measurement toolbox for an interacting Rydberg-atom quantum simulator

We present a toolbox to probe quantum many-body states implemented on Rydberg-atoms quantum hardware via randomized measurements. We illustrate the efficacy of this measurement toolbox in the context of probing entanglement, via the estimation of the purity, and of verifying a ground-state preparation using measurements of the Hamiltonian variance. To achieve this goal, we develop and discuss in detail a protocol to realize independent, local unitary rotations. We benchmark the protocol by investigating the ground state of the one-dimensional Su–Schrieffer–Heeger model, recently realized on a chain of Rydberg atom, and the state resulting after a sudden quench in a staggered XY chain. We probe the robustness of our toolbox by taking into account experimental imperfections, such as pulse fluctuations and measurement errors.

Weak ergodicity breaking in non-Hermitian many-body systems

The recent discovery of persistent revivals in the Rydberg-atom quantum simulator has revealed a weakly ergodicity-breaking mechanism dubbed quantum many-body scars, which are a set of nonthermal states embedded in otherwise thermal spectra. Until now, such a mechanism has been mainly studied in Hermitian systems. Here, we establish the non-Hermitian quantum many-body scars and systematically characterize their nature from dynamic revivals, entanglement entropy, physical observables, and energy level statistics. Notably, we find the non-Hermitian quantum many-body scars exhibit significantly enhanced coherent revival dynamics when approaching the exceptional point. The signatures of non-Hermitian scars switch from the real-energy axis to the imaginary-energy axis after a real-to-complex spectrum transition driven by increasing non-Hermiticity, where an exceptional point and a quantum tricritical point emerge simultaneously. We further examine the stability of non-Hermitian quantum many-body scars against external fields, reveal the non-Hermitian quantum criticality and eventually set up the whole phase diagram. The possible connection to the open quantum many-body systems is also explored. Our findings offer insights for realizing long-lived coherent states in non-Hermitian many-body systems.

Classical shadow tomography with locally scrambled quantum dynamics

We generalize the classical shadow tomography scheme to a broad class of finite-depth or finite-time local unitary ensembles, known as locally scrambled quantum dynamics, where the unitary ensemble is invariant under local-basis transformations. In this case, the reconstruction map for the classical shadow tomography depends only on the average entanglement feature of classical snapshots. We provide an unbiased estimator of the quantum state as a linear combination of reduced classical snapshots in all subsystems, where the combination coefficients are solely determined by the entanglement feature. We also bound the number of experimental measurements required for the tomography scheme, so-called sample complexity, by formulating the operator shadow norm in the entanglement feature formalism. We numerically demonstrate our approach for finite-depth local unitary circuits and finite-time local-Hamiltonian generated evolutions. The shallow-circuit measurement can achieve a lower tomography complexity compared to the existing method based on Pauli or Clifford measurements. Our approach is also applicable to approximately locally scrambled unitary ensembles with a controllable bias that vanishes quickly. Surprisingly, we find a single instance of time-dependent local Hamiltonian evolution is sufficient to perform an approximate tomography as we numerically demonstrate it using a paradigmatic spin chain Hamiltonian modeled after trapped ion or Rydberg atom quantum simulators. Our approach significantly broadens the application of classical shadow tomography on near-term quantum devices.

Superdiffusive Energy Transport in Kinetically Constrained Models

Universal nonequilibrium properties of isolated quantum systems are typically probed by studying transport of conserved quantities, such as charge or spin, while transport of energy has received considerably less attention. Here, we study infinite-temperature energy transport in the kinetically-constrained PXP model describing Rydberg atom quantum simulators. Our state-of-the-art numerical simulations, including exact diagonalization and time-evolving block decimation methods, reveal the existence of two distinct transport regimes. At moderate times, the energy-energy correlation function displays periodic oscillations due to families of eigenstates forming different su(2) representations hidden within the spectrum. These families of eigenstates generalize the quantum many-body scarred states found in previous works and leave an imprint on the infinite-temperature energy transport. At later times, we observe a broad superdiffusive transport regime that we attribute to the proximity of a nearby integrable point. Intriguingly, strong deformations of the PXP model by the chemical potential do not restore diffusion, but instead lead to a stable superdiffusive exponent $z\approx3/2$. Our results suggest constrained models to be potential hosts of novel transport regimes and call for developing an analytic understanding of their energy transport.

Extensive Multipartite Entanglement from su(2) Quantum Many-Body Scars.

Recent experimental observation of weak ergodicity breaking in Rydberg atom quantum simulators has sparked interest in quantum many-body scars-eigenstates which evade thermalization at finite energy densities due to novel mechanisms that do not rely on integrability or protection by a global symmetry. A salient feature of some quantum many-body scars is their subvolume bipartite entanglement entropy. In this Letter, we demonstrate that such exact many-body scars also possess extensive multipartite entanglement structure if they stem from an su(2) spectrum generating algebra. We show this analytically, through scaling of the quantum Fisher information, which is found to be superextensive for exact scarred eigenstates in contrast to generic thermal states. Furthermore, we numerically study signatures of multipartite entanglement in the PXP model of Rydberg atoms, showing that extensive quantum Fisher information density can be generated dynamically by performing a global quench experiment. Our results identify a rich multipartite correlation structure of scarred states with significant potential as a resource in quantum enhanced metrology.

Hypergrid subgraphs and the origin of scarred quantum walks in many-body Hilbert space

Following the recent observation of wave function revivals in large Rydberg atom quantum simulators, much effort has focused on understanding the emergence of many-body scars in non-integrable quantum systems. Here we explore the origin of scarred wavefunction revivals in a family of models obtained by deforming the graph adjacency matrix of the PXP model - the effective model of Rydberg atoms in the strong Rydberg blockade regime. We consider deformations that either enhance the Rydberg constraint, ultimately resulting in an effective tight-binding model of two hypercubes joined at a single vertex, or relax the constraint until reaching the free spin-1/2 model. In the former case, we argue that the model of two joined hypercubes captures the essential features of many-body scarring present in the PXP model. On the other hand, relaxing the constraint leads to a sequence of new scarred models, some with more robust scarring signatures than the PXP model, as can be understood from the graph-theoretic viewpoint. Our results shed light on the nature of scarring in the PXP model by identifying its simple parent model, while also highlighting its distinction from the free-spin precession.

Quantum information scrambling in quantum many-body scarred systems

Quantum many-body scarred systems host special nonthermal eigenstates that support periodic revival dynamics and weakly break the ergodicity. Here, we study the quantum information scrambling dynamics in quantum many-body scarred systems, with a focus on the ``PXP'' model. We use the out-of-time-ordered correlator (OTOC) and Holevo information as measures of the information scrambling and apply an efficient numerical method based on matrix product operators to compute them up to 41 spins. We find that both the OTOC and Holevo information exhibit a linear light cone and periodic oscillations inside the light cone for initial states within the scarred subspace, which is in sharp contrast to thermal or many-body localized systems. The periodic revivals of OTOCs and Holevo information signify unusual breakdown of quantum chaos and are not equivalent to the revival dynamics of state fidelity or local observables studied in the previous literature. To explain the formation of the linear light-cone structure, we provide a perturbation-type calculation based on a phenomenological model. In addition, we demonstrate that the OTOC and Holevo information dynamics of the PXP model can be measured using the Rydberg-atom quantum simulators with current experimental technologies and numerically identify the measurable signatures using experimental parameters.

Rainbow scars: From area to volume law

Quantum many-body scars (QMBS) constitute a new quantum dynamical regime in which rare "scarred" eigenstates mediate weak ergodicity breaking. One open question is to understand the most general setting in which these states arise. In this work, we develop a generic construction that embeds a new class of QMBS, rainbow scars, into the spectrum of an arbitrary Hamiltonian. Unlike other examples of QMBS, rainbow scars display extensive bipartite entanglement entropy while retaining a simple entanglement structure. Specifically, the entanglement scaling is volume-law for a random bipartition, while scaling for a fine-tuned bipartition is sub-extensive. When internal symmetries are present, the construction leads to multiple, and even towers of rainbow scars revealed through distinctive non-thermal dynamics. Remarkably, certain symmetries can lead rainbow scars to arise in translation-invariant models. To this end, we provide an experimental road map for realizing rainbow scar states in a Rydberg-atom quantum simulator, leading to coherent oscillations distinct from the strictly sub-volume-law QMBS previously realized in the same system.

Quantum simulation of Cayley-tree Ising Hamiltonians with three-dimensional Rydberg atoms

Significant efforts are being directed towards developing a quantum annealer capable of solving combinatorial optimization problems. The challenges are Hamiltonian programming and large-scale implementations. Here we report quantum annealing demonstration of Ising Hamiltonians programmed with up to $N=22$ spins mapped on various Cayley tree graphs. Experiments are performed with a Rydberg-atom quantum simulator, in which rubidium single atoms are arranged in three dimensional space in such a way that their Rydberg atoms and blockaded strong couplings respectively represent the nodes and edges of each graph. Three different Cayley-tree graphs of $Z=3$ neighbors and of up to $S=4$ shells are constructed, and their ground-state phases and N\'{e}el's order formations are probed. In good agreement with model calculations, the anti-ferromagnetic phase in regular Cayley trees and frustrated competing ground-states in a dual-center Cayley tree are directly observed. This demonstrates the possibilities of high-dimensional qubit connection programming in quantum simulators.

Quantum Ising Hamiltonian Programming in Trio, Quartet, and Sextet Qubit Systems

Rydberg-atom quantum simulators are of keen interest because of their possibilities towards high-dimensional qubit architectures. Here we report three-dimensional conformation spectra of quantum-Ising Hamiltonian systems with programmed qubit connections. With a Rydberg-atom quantum simulator, various connected graphs, in which vertices and edges represent atoms and blockaded couplings, respectively, are constructed in two or three-dimensional space and their eigenenergies are probed during their topological transformations. Star, complete, cyclic, and diamond graphs, and their geometric intermediates, are tested for four atoms and antiprism structures for six atoms. Spectroscopic resolution (dE/E) less than 10% is achieved and the observed energy level shifts and merges through structural transformations are in good agreement with the model few-body quantum-Ising Hamiltonian.

Lattice Gauge Theories and String Dynamics in Rydberg Atom Quantum Simulators

Gauge theories are the cornerstone of our understanding of fundamental interactions among particles. Their properties are often probed in dynamical experiments, such as those performed at ion colliders and high-intensity laser facilities. Describing the evolution of these strongly coupled systems is a formidable challenge for classical computers, and represents one of the key open quests for quantum simulation approaches to particle physics phenomena. Here, we show how recent experiments done on Rydberg atom chains naturally realize the real-time dynamics of a lattice gauge theory at system sizes at the boundary of classical computational methods. We prove that the constrained Hamiltonian dynamics induced by strong Rydberg interactions maps exactly onto the one of a $U(1)$ lattice gauge theory. Building on this correspondence, we show that the recently observed anomalously slow dynamics corresponds to a string-inversion mechanism, reminiscent of the string-breaking typically observed in gauge theories. This underlies the generality of this slow dynamics, which we illustrate in the context of one-dimensional quantum electrodynamics on the lattice. Within the same platform, we propose a set of experiments that generically show long-lived oscillations, including the evolution of particle-antiparticle pairs. Our work shows that the state of the art for quantum simulation of lattice gauge theories is at 51 qubits, and connects the recently observed slow dynamics in atomic systems to archetypal phenomena in particle physics

Real-time-dynamics quantum simulation of (1+1)-dimensional lattice QED with Rydberg atoms

We show how to implement a Rydberg-atom quantum simulator to study the non-equilibrium dynamics of an Abelian (1+1)-D lattice gauge theory. The implementation locally codifies the degrees of freedom of a $\mathbf{Z}_3$ gauge field, once the matter field is integrated out by means of the Gauss' local symmetries. The quantum simulator scheme is based on current available technology and scalable to considerable lattice sizes. It allows, within experimentally reachable regimes, to explore different string dynamics and to infer information about the Schwinger $U(1)$ model.

Quantum many-body scars from magnon condensation

We study the eigenstate properties of a nonintegrable spin chain that was recently realized experimentally in a Rydberg-atom quantum simulator. In the experiment, long-lived coherent many-body oscillations were observed only when the system was initialized in a particular product state. This pronounced coherence has been attributed to the presence of special "scarred" eigenstates with nearly equally-spaced energies and putative nonergodic properties despite their finite energy density. In this paper we uncover a surprising connection between these scarred eigenstates and low-lying quasiparticle excitations of the spin chain. In particular, we show that these eigenstates can be accurately captured by a set of variational states containing a macroscopic number of magnons with momentum $\pi$. This leads to an interpretation of the scarred eigenstates as finite-energy-density condensates of weakly interacting $\pi$-magnons. One natural consequence of this interpretation is that the scarred eigenstates possess long-range order in both space and time, providing a rare example of the spontaneous breaking of continuous time-translation symmetry. We verify numerically the presence of this space-time crystalline order and explain how it is consistent with established no-go theorems precluding its existence in ground states and at thermal equilibrium.

Systematic Construction of Scarred Many-Body Dynamics in 1D Lattice Models.

We introduce a family of nonintegrable 1D lattice models that feature robust periodic revivals under a global quench from certain initial product states, thus generalizing the phenomenon of many-body scarring recently observed in Rydberg atom quantum simulators. Our construction is based on a systematic embedding of the single-site unitary dynamics into a kinetically constrained many-body system. We numerically demonstrate that this construction yields new families of models with robust wave-function revivals, and it includes kinetically constrained quantum clock models as a special case. We show that scarring dynamics in these models can be decomposed into a period of nearly free clock precession and an interacting bottleneck, shedding light on their anomalously slow thermalization when quenched from special initial states.

Quantum Kibble-Zurek mechanism and critical dynamics on a programmable Rydberg simulator.

Quantum phase transitions (QPTs) involve transformations between different states of matter that are driven by quantum fluctuations1. These fluctuations play a dominant part in the quantum critical region surrounding the transition point, where the dynamics is governed by the universal properties associated with the QPT. Although time-dependent phenomena associated with classical, thermally driven phase transitions have been extensively studied in systems ranging from the early Universe to Bose-Einstein condensates2-5, understanding critical real-time dynamics in isolated, non-equilibrium quantum systems remains a challenge6. Here we use a Rydberg atom quantum simulator with programmable interactions to study the quantum critical dynamics associated with several distinct QPTs. By studying the growth of spatial correlations when crossing the QPT, we experimentally verify the quantum Kibble-Zurek mechanism (QKZM)7-9 for an Ising-type QPT, explore scaling universality and observe corrections beyond QKZM predictions. This approach is subsequently used to measure the critical exponents associated with chiral clock models10,11, providing new insights into exotic systems that were not previously understood and opening the door to precision studies of critical phenomena, simulations of lattice gauge theories12,13 and applications to quantum optimization14,15.

Synthetic lattices, flat bands and localization in Rydberg quantum simulators

The most recent manifestation of cold Rydberg atom quantum simulators that employs tailored optical tweezer arrays enables the study of many-body dynamics under so-called facilitation conditions. We show how the facilitation mechanism yields a Hilbert space structure in which the many-body states organize into synthetic lattices which feature in general one or several flat bands and may support immobile localized states. We focus our discussion on the case of a ladder geometry for which we analyze the influence of disorder generated by the uncertainty of the atomic positions. The localization properties of this system are characterized through two length scales (localization lengths) which are found to display anomalous scaling behavior at certain energies. Moreover, we discuss the experimental preparation of an immobile localized state, and analyze disorder-induced propagation effects.

Many-body spectral reflection symmetry and protected infinite-temperature degeneracy

Protected zero modes in quantum physics traditionally arise in the context of ground states of many-body Hamiltonians. Here we study the case where zero modes exist in the center of a reflection-symmetric many-body spectrum, giving rise to the notion of a protected "infinite-temperature" degeneracy. For a certain class of nonintegrable spin chains, we show that the number of zero modes is determined by a chiral index that grows exponentially with system size. We propose a dynamical protocol, feasible in ongoing experiments in Rydberg atom quantum simulators, to detect these many-body zero modes and their protecting spectral reflection symmetry. Finally, we consider whether the zero energy states obey the eigenstate thermalization hypothesis, as is expected of states in the middle of the many-body spectrum. We find intriguing differences in their eigenstate properties relative to those of nearby nonzero-energy eigenstates at finite system sizes.

Weak ergodicity breaking from quantum many-body scars

Certain wave functions of non-interacting quantum chaotic systems can exhibit "scars" in the fabric of their real-space density profile. Quantum scarred wave functions concentrate in the vicinity of unstable periodic classical trajectories. We introduce the notion of many-body quantum scars which reflect the existence of a subset of special many-body eigenstates concentrated in certain parts of the Hilbert space. We demonstrate the existence of scars in the Fibonacci chain -- the one- dimensional model with a constrained local Hilbert space realized in the 51 Rydberg atom quantum simulator [H. Bernien et al., arXiv:1707.04344]. The quantum scarred eigenstates are embedded throughout the thermalizing many-body spectrum, but surprisingly lead to direct experimental signatures such as robust oscillations following a quench from a charge-density wave state found in experiment. We develop a model based on a single particle hopping on the Hilbert space graph, which quantitatively captures the scarred wave functions up to large systems of L = 32 atoms. Our results suggest that scarred many-body bands give rise to a new universality class of quantum dynamics, which opens up opportunities for creating and manipulating novel states with long-lived coherence in systems that are now amenable to experimental study.

Detailed Balance of Thermalization Dynamics in Rydberg-Atom Quantum Simulators.

Dynamics of large complex systems, such as relaxation towards equilibrium in classical statistical mechanics, often obeys a master equation that captures essential information from the complexities. Here, we find that thermalization of an isolated many-body quantum state can be described by a master equation. We observe sudden quench dynamics of quantum Ising-like models implemented in our quantum simulator, defect-free single-atom tweezers in conjunction with Rydberg-atom interaction. Saturation of their local observables, a thermalization signature, obeys a master equation experimentally constructed by monitoring the occupation probabilities of prequench states and imposing the principle of the detailed balance. Our experiment agrees with theories and demonstrates the detailed balance in a thermalization dynamics that does not require coupling to baths or postulated randomness.