Interface Roughness Research Articles

Exploring the effects of molecular beam epitaxy growth characteristics on the temperature performance of state-of-the-art terahertz quantum cascade lasers

This study conducts a comparative analysis, using non-equilibrium Green’s functions (NEGF), of two state-of-the-art two-well (TW) Terahertz Quantum Cascade Lasers (THz QCLs) supporting clean 3-level systems. The devices have nearly identical parameters and the NEGF calculations with an abrupt-interface roughness height of 0.12 nm predict a maximum operating temperature (Tmax) of ~ 250 K for both devices. However, experimentally, one device reaches a Tmax of ~ 250 K and the other a Tmax of only ~ 134 K. Both devices were fabricated and measured under identical conditions in the same laboratory, with high quality processes as verified by reference devices. The main difference between the two devices is that they were grown in different MBE reactors. Our NEGF-based analysis considered all parameters related to MBE growth, including the maximum estimated variation in aluminum content, growth rate, doping density, background doping, and abrupt-interface roughness height. From our NEGF calculations it is evident that the sole parameter to which a drastic drop in Tmax could be attributed is the abrupt-interface roughness height. We can also learn from the simulations that both devices exhibit high-quality interfaces, with one having an abrupt-interface roughness height of approximately an atomic layer and the other approximately a monolayer. However, these small differences in interface sharpness are the cause of the large performance discrepancy. This underscores the sensitivity of device performance to interface roughness and emphasizes its strategic role in achieving higher operating temperatures for THz QCLs. We suggest Atom Probe Tomography (APT) as a path to analyze and measure the (graded)-interfaces roughness (IFR) parameters for THz QCLs, and subsequently as a design tool for higher performance THz QCLs, as was done for mid-IR QCLs. Our study not only addresses challenges faced by other groups in reproducing the record Tmax of ~ 250 K and ~ 261 K but also proposes a systematic pathway for further improving the temperature performance of THz QCLs beyond the state-of-the-art.

An experimental test of endfire synthetic aperture sonar for sediment characterisation

AbstractThe validation of seafloor scattering models used for seabed characterisation requires quantifying the contributions from the sediment interface and volume to the total acoustic returns. At low‐frequencies, direct measurements of sediment volume scattering have rarely been made, due to the bias in interface roughness scattering caused by large beamwidths of low‐frequency sonars. Endfire Synthetic Aperture Sonar (EF‐SAS) can achieve narrower beamwidths by forming a vertically oriented synthetic array as a transmitter and/or receiver and moving it through the water column. The narrower beamwidths achieved by EF‐SAS allow for more accurate measurements of volume scattering by reducing interface scattering bias in acoustic returns. The application of EF‐SAS for sediment characterisation is explored for the first time. The authors demonstrate that EF‐SAS can be used to construct the angular response curve for both interface and volume scattering as well as to estimate the attenuation and reflection coefficients, which can be inverted for grain size.

Mesoscale modeling of new-to-old concrete interface under combined shear and compressive loads

A mesoscale model of new-to-old concrete interface under combined shear and compressive loads is established, and a parameter study is conducted to evaluate the influence of interface roughness, bond strength, and fracture energy. The mesoscale model is numerically generated using a random aggregate technique, in which the number of aggregates is calculated using the Fuller grading curve and Walraven formula and the aggregates are randomly placed using the Monte Carlo simulation. The concrete damaged plasticity model is employed to simulate the mechanical behaviors of new and old mortars, as well as the interfacial transition zone between the mortar and aggregate. The linear elastic model is utilized to simulate the behavior of aggregates, while the cohesive-friction model is employed to represent the behavior of new-to-old concrete interface. The effect of interface roughness, bond strength, and fracture energy on the interface shear strength and post-peak shear strength using the double-shear test specimens is investigated. The results indicate that increasing the roughness of old concrete surface leads to significant increases in both the interface shear strength and post-peak shear strength, but the larger interface roughness is not necessarily better. As the interface bond strength increases, the interface shear strength remains the same, whereas the post-peak shear strength shows a large increase with the lower interface roughness. Moreover, the interface fracture energy imparts the minimal influence on the interface shear strength and post-peak shear strength, but the higher interface fracture energy can improve the overall constitutive behavior of new-to-old concrete interface if the roughness of old concrete surface is low. The numerical mesoscale model presented can provide the theoretical guidance and technical support for effective design and construction of new-to-old concrete interface and structures.

Interfacial cohesion model of ultra‐high performance concrete wet joints under the influence of multiple factors

AbstractThe interfacial cohesion between precast normal concrete (NC) and cast‐in‐place ultra‐high performance concrete (UHPC) is an important index to evaluate their interfacial bond strength, which is of great importance for the application of UHPC as a connection material for precast structural bridges. Interfacial cohesion is related to several influencing factors. However, there needs to be more research on the interrelationship model between multiple influencing factors and interfacial cohesion. This study took the UHPC wet joint in a precast concrete structure as the object. First, the relationship between the interface cohesion of UHPC wet joint and substrate strength, UHPC age, interfacial roughness, interfacial moisture content, and curing method was studied; The result shows that the key factors affecting interfacial cohesion include UHPC age, interface roughness, and substrate strength, with interfacial moisture content potentially playing a secondary role. Second, the failure types of the interface zone surface by using digital image correlation (DIC) are divided into three categories. Finally, the quantitative mathematical model of interfacial cohesion under the coupling effect of multiple factors was established based on the above four factors. The model is in good agreement with the experimental data.

Shear study on the interface between ultra-high durability concrete and low-cement-lightweight concrete for precast composite walls

Precast wall system is one of the solutions with great potential, as it makes it possible to build structures in a simple and quick way, without using columns and beams. Considering the advantages of this system, an innovative composite structural precast wall has been developed, using a layer of ultra-high durability concrete (UHDC) on the outside and another layer of low cement lightweight concrete (LCLWAC) on the inside. This provides a triple benefit: (a) a reduction in dead weight, (b) an increase in durability and therefore a higher life of the structure, and (c) a reduction in cement dosage and consequently a reduction of the carbon footprint of the product. The main topic of this research is the study of the interface shear strength between a low cement lightweight aggregate concrete (LCLWAC) and an eco-efficient ultra-high durability concrete (UHDC). An experimental program was carried out to evaluate this shear strength, considering two parameters: i) the roughness interface and (ii) the transversal reinforcement crossing the interface; and using two types of tests, push-off and flexural tests. Results were compared with the predictions of Eurocode 2 and fib Model Code 2010, including the new versions of both codes, to assess how suitable are the models and coefficients for this situation. The shear strength between LCLWAC-UHDC is quite effective, and the predictions are conservative for this combination, at least 2 times lower than the experimental results and close to 7 times in some cases.

Heat Transport at Silicon Grain Boundaries

AbstractEngineering microstructural defects, like grain boundaries, offers superior control over transport properties in energy materials. However, technological advancement requires establishing microstructure‐property relations at the micron or finer scales, where most of these defects operate. Here, the first experimental evidence of thermal resistance for individual silicon grain boundaries, estimated with a Gibbs excess approach, is provided. Coincident site lattice boundaries exhibit uniform excess thermal resistance along the same boundary, but notable variations from one boundary to another. Boundaries associated with low interface energy generally exhibit lower resistances, aligning with theoretical expectations and previous simulations, but several exceptions are observed. Transmission electron microscopy reveals that factors like interface roughness and presence of nanotwinning can significantly alter the observed resistance, which ranges from ∼0 to up to ∼2.3 m2K/GW. In stark contrast, significantly larger and less uniform values ‐ from 5 to 30 m2K/GW ‐ are found for high‐angle boundaries in spark‐plasma‐sintered polycrystalline silicon. Further, finite element analysis suggests that boundary planes that strongly deviate from the sample vertical (beyond ∼45°) can show up to 3‐times larger excess resistance. Direct correlations of properties with individual defects enable the design of materials with superior thermal performance for applications in energy harvesting and heat management.

Contribution to the experimental and theoretical study of the behavior of soil-structure interfaces

Designing civil engineering works often requires taking into consideration the contact and interface conditions between the soil and structure. These may refer to the discontinuity surfaces between the soil and a structure such as foundations, geotechnical works, and others. Current research aims to improve the calculation methods for structures through a better understanding of the behavior of materials and interfaces. The present work falls into this context. It involves two parts. The main purpose of the first part is to present the results of the monotonic and cyclic soil-structure interface tests which were carried out using a modified direct shear box apparatus. The tests were conducted using a local material, namely the sand from the town of Messâad in the Wilaya of Djelfa (Algeria), in accordance with a constant normal stress path. In addition, a parametric study, dealing with the effect of density, interface roughness, and type of adhesive used on the behavior of the interfaces, was carried out as well. As for the second part, it primarily aims to validate the Modjoin interface model, which was developed at the Lille Mechanical Laboratory, based on the tests that were carried out in the first part. It is important to know that this model includes the main concepts used in soil modeling, such as isotropic hardening, characteristic state, critical state, softening, and others. Moreover, several validation tests are also presented in this work in order to describe the behavior of the soil-structure interface under monotonic loading to assess the performance of the model.

Contact stress ultrasonic detection method based on contact acoustic resistance model

The size and distribution of the contact stress at the assembly interface will directly affect the connection performance of the mechanical joint. However, the rough assembly interface presents strong dielectric discontinuity and material nonlinearity, which become the bottleneck restricting the development of contact stress detection. How to obtain contact stress by nondestructive testing means has become an urgent problem to be solved. In this paper, a multi-layer interface contact stress detection method based on contact acoustic resistance model is proposed to solve the difficult problem of rough interface contact stress detection. Firstly, based on the formation mechanism of contact acoustic resistance of rough assembly interface, the equivalent contact acoustic resistance expression of contact layer is derived. Secondly, the contact mechanism of rough assembly interface is clarified, and the mapping relationship model between contact acoustic resistance and contact stress is constructed. On this basis, according to the transmission law of ultrasonic wave at different interfaces of multilayer acoustic impedance, the expression of acoustic transmission coefficient at the interface of variable acoustic impedance is obtained. A contact stress detection method based on contact stress-contact acoustic resistance coefficient and acoustic transmission coefficient is proposed. The correctness of the theoretical model is verified by the tensile testing machine, and the maximum error is 15.52 %. This method will provide powerful data support for the evaluation of assembly interface connection state.

Zero-field magnetic skyrmions in exchange-biased ferromagnetic–antiferromagnetic bilayers

We report on the stabilization of ferromagnetic skyrmions in zero external magnetic fields, in exchange-biased systems composed of ferromagnetic–antiferromagnetic (FM-AFM) bilayers. By performing atomistic spin dynamics simulations, we study cases of compensated, uncompensated, and partly uncompensated FM-AFM interfaces, and investigate the impact of important parameters such as temperature, inter-plane exchange interaction, Dzyaloshinskii–Moriya interaction, and magnetic anisotropy on the skyrmions appearance and stability. The model with an uncompensated FM-AFM interface leads to the stabilization of individual skyrmions and skyrmion lattices in the FM layer, caused by the effective field from the AFM instead of an external magnetic field. Similarly, in the case of a fully compensated FM-AFM interface, we show that FM skyrmions can be stabilized. We also demonstrate that accounting for interface roughness leads to stabilization of skyrmions both in compensated and uncompensated interface. Moreover, in bilayers with a rough interface, skyrmions in the FM layer are observed for a wide range of exchange interaction values through the FM-AFM interface, and the chirality of the skyrmions depends critically on the exchange interaction.

Combined effect of WS2 and Ti3C2Tx MXene favors oil-based ultra-low friction on rough steel-steel interface at elevated temperatures

Combined effect of WS2 and Ti3C2Tx MXene favors oil-based ultra-low friction on rough steel-steel interface at elevated temperatures

Explicit frictional stick–slip dynamics of elastic contact problem incorporating the LuGre model

Dynamical contact problem with friction is of continuous concern and have been investigated over the years. The effective and accurate description of the development of the friction force is the key to this problem. However, the stick–slip phenomenon, as typical dynamical behaviour, has rarely been considered when developing contact algorithms for frictional contact problems of elastic bodies. The conventionally used Coulomb’s model, with differentiating the static and kinetic coefficient of friction, can lead to inaccurate results due to errors generated when switch between the stick or slip states. In this work, a three-dimensional mortar-based frictional contact algorithm is proposed in an explicit scheme. The proposed algorithm incorporates the LuGre model to account for dynamical frictional behaviours such as stick–slip. The effectiveness and accuracy of the proposed algorithm are validated through several simplified two-dimensional cases. The sticking time ratio and the evolution of the global coefficient of friction with time of a three-dimensional contact problem with a randomly rough contact interface are investigated as an application.

Bonding characteristics between existing concrete substrate and high ductility geopolymer overlays under direct shear loading

High ductility geopolymer (HDG) looks promising as an exceptional repair material due to the faultless mechanical properties and environmental benefits. The interfacial bonding characteristics between existing normal concrete (NC) substrate and HDG overlay are the vital impact on the overall performance of repaired structures. This study presented the NC-HDG bonding behavior under the direct shear tests, and totally 45 specimens were designed with various concrete strength grades, interface roughness and elongations of HDG. To capture the fracture characteristics, the digital image correlation (DIC) technique was employed. Test results showed that the direct shear bonding strength (τu) had an increasing trend as the NC strength dropped or the interface roughness and elongations of HDG were increased, among the interface roughness affected the τu mostly, with the improvement amount of 185.07 %∼343.28 %. The direct shear strength ratio (defined as the ratio of τu to the inherent shear strength of NC) was ranged as 0.110∼0.489, i.e., at least half of shear strength of NC was lost during repairing. Based on the DIC measured results, the improvement of NC strength, interface roughness and elongations of HDG all delayed the interfacial crack initiation under direct shear loading. Moreover, the upper-bound limit analysis was adopted, a simplified method for predicting the direct shear bonding strength of NC-HDG interface was proposed and showed a sufficient precision.

Mineral asperities reinforce nacre through interlocking and friction-like sliding

While the surface asperities of mineral platelets are widely believed to play important roles in stiffening, strengthening, and toughening nacre, their effects have not been thoroughly investigated. Here, a computationally efficient bar-spring model is adopted to simulate, as platelets with multiple interfacial asperities slide over each other, the tensile force versus elongation behaviors as well as the effective mechanical properties such as modulus, strength, and work-to-fracture in nacre or nacre-like composites. The model employs an effective cohesive law derived from a micromechanical model based on the kinematic and deformation analysis of a single pair of contacting asperities to characterize the traction-separation relationship during the asperity inter-climbing. Strikingly, we find that the mineral asperities and resulting interfacial roughness can elevate the composites’ strength and toughness by up to 2–3 orders of magnitude through a combination of mechanical interlocking and multimodal friction-like mechanisms. Of particular interest is that the asperity-induced strengthening and toughening mechanisms are insensitive to the asperity shapes such as ellipse, hyperbolic cosine, cosine, and parabola. These findings may provide useful guidelines for developing advanced engineering composites with nacre-inspired interface designs.

Gamma-ray irradiation effect on planar defect evolution of lattice-matched InGaAsN/GaAs/Ge grown by MOVPE

This study explores structural changes in lattice-matched InGaAsN/GaAs/Ge films grown by MOVPE under gamma-ray irradiation. Exposure to a 60Co gamma rays at doses ranging from 0 to 2.0 MGy improved crystal uniformity by increasing surface grain size, reducing roughness from 8.328 nm to 3.512 nm. Planar defects in the GaAs layer traversed the InGaAsN layer, causing interface roughness. Electron diffraction patterns along the [110]-zone axis showed uniform alloy composition. TEM images revealed line contrasts at the GaAs/Ge interface extending into the InGaAsN layer, with boundary-like defects parallel to the growth direction. Additionally, (002) and (002‾) reflections, along with {111} planes, indicated planar defects, possibly antiphase boundaries. AFM and FESEM confirmed submicron-sized domains, characteristic of antiphase boundaries, in the InGaAsN film.

Three-dimensional hard X-ray ptychographic reflectometry imaging on extended mesoscopic surface structures

Many nanodevices and quantum devices, with their sizes often spanning from millimeters down to sub-nanometer, have intricate low-dimensional, non-uniform, or hierarchical structures on surfaces and interfaces. Since their functionalities are dependent on these structures, high-resolution surface-sensitive characterization becomes imperative to gain a comprehensive understanding of the function–structure relationship. We thus developed hard x-ray ptychographic reflectometry imaging, a new technique that merges the high-resolution two-dimensional imaging capabilities of hard x-ray ptychography for extended objects, with the high-resolution depth profiling capabilities of x-ray reflectivity for layered structures. The synergy of these two methods fully leverages both amplitude and phase information from ptychography reconstruction to not only reveal surface topography and localized structures, such as shapes and electron densities, but also yields statistical details, such as interfacial roughness that is not readily accessible through coherent imaging solely. The hard x-ray ptychographic reflectometry imaging is well-suited for three-dimensional imaging of mesoscopic samples, particularly those comprising planar or layered nanostructures on opaque supports, and could also offer a high-resolution surface metrology and defect analysis on semiconductor devices, such as integrated nanocircuits and lithographic photomasks for microchip fabrications.

Theoretical characterization of the magnetoresistance in magnetic multilayers with antiferromagnetic coupling

Spin-valves (SVs) constitute a significant class of magnetic metal structures with a large range of technological applications. This class of structure offers interesting magnetic properties due to their alternation with the non-magnetic layers. The SVs fortunately have good magnetic properties at room temperature (RT). This study intends to use Boltzmann Approach–BA, to treat the magetotransport properties of Co-based SV. Outer-surface scattering effects on magnetoresistance (MR) performance encountered in these structures are investigated by varying the interfacial chemical composition. Analysis of the results reveals the existence of a significant improvement of magnetic phenomenon for a scattering that is more and more specular of the conduction electrons through outer-surface. A giant MR (GMR) of amplitude 136.9 % is obtained for an interfacial geometric roughness of magnitude 2 Å. The GMR ratio is the result of large asymmetry in the spin-dependent interfacial scattering and a completely specular outer-surface scattering.

Analysis of the Sand-Concrete Interface Shear Behaviors Considering the Soil Unloading and Interface Roughness Effects

Analysis of the Sand-Concrete Interface Shear Behaviors Considering the Soil Unloading and Interface Roughness Effects

Dependence of a Hydrogen Buffer Layer on the Properties of Top-Gate IGZO TFT.

In this paper, the effect of a buffer layer created using different hydrogen-containing ratios of reactive gas on the electrical properties of a top-gate In-Ga-Zn-O thin-film transistor was thoroughly investigated. The interface roughness between the buffer layer and active layer was characterized using atomic force microscopy and X-ray reflection. The results obtained using Fourier transform infrared spectroscopy show that the hydrogen content of the buffer layer increases with the increase in the hydrogen content of the reaction gas. With the increase in the hydrogen-containing materials in the reactive gas, field effect mobility and negative bias illumination stress stability improve nearly twofold. The reasons for these results are explained using technical computer-aided design simulations.

Surface Evolution of Polymer Films Grown by Vapor Deposition: Growth of Local and Global Slopes of Interfaces.

The kinetic roughening of polymer films grown by vapor deposition polymerization was analyzed using the widely accepted classification framework of "generic scaling ansatz" given for the structure factor. Over the past two decades, this method has played a pivotal role in classifying diverse forms of dynamic scaling and understanding the mechanisms driving interface roughening. The roughness exponents of the polymer films were consistently determined as α=1.25±0.09, αloc=0.73±0.02, and αs=0.99±0.06. However, the inability to unambiguously assign these roughness exponent values to a specific scaling subclass prompts the proposal of a practical alternative. This report illustrates how all potential dynamic scaling can be consistently identified and classified based on the relationship between two temporal scaling exponents measured in real space: the average local slope and the global slope of the interface. The intrinsic anomalous roughening class is conclusively assigned to polymer film growth characterized by anomalous "native (background slope-removed) local height fluctuations". Moreover, the new analysis reveals that interfaces exhibiting anomalous scaling, previously classified as intrinsic anomalous roughening, could potentially belong to the super-rough class, particularly when the spectral roughness exponent αs is equal to 1.

Discrete element modeling of effect of interfacial roughness and pre-crack on crack propagation in thermal barrier coatings

Discrete element modeling of effect of interfacial roughness and pre-crack on crack propagation in thermal barrier coatings