This article investigates the utilization of copper sulfide (CuS) based nanomaterials functionalized with rhodium (Rh) and palladium (Pd) nanoparticles for gas sensing and energy generation applications. CuS nanoparticles, known for their unique properties, were combined with Rh and Pd nanoparticles to enhance hydrogen (H2) gas sensing capabilities. Gas sensing experiments revealed that CuS/Rh/Pd nanocomposites exhibited the highest sensing response of 58.33% to H2, indicating the significant improvement in gas sensing properties due to the combined presence of Rh and Pd nanoparticles in CuS matrices. Moreover, temperature-dependent responses provided insights into optimal operating conditions for effective gas sensing with CuS-based nanocomposites. Comprehensive characterization studies including XPS, Raman, and morphology analysis confirmed the successful synthesis of CuS/Rh/Pd nanomaterials with high purity and desirable structural properties. Dye-sensitized solar cell (DSSC) performance studies demonstrated that CuS/Rh/Pd nanocomposites enhanced the efficiency by minimizing light over-absorption and improving photoanode stability. Overall, this study highlighted the potential of metal nanoparticle-decorated CuS nanocomposites for advanced gas sensing and energy generation applications, paving the way for the development of highly sensitive and efficient gas sensors and solar energy conversion technologies.