Recoil Proton Energy Research Articles

Measurement of Photoneutrons from Depleted Uranium and Comparison Study Using MCNPX-PoliMi

High-energy photon interrogation is a nondestructive technique that is used to detect special nuclear materials and characterize nuclear waste. The development of such systems is complex and requires Monte Carlo simulations to optimize system performance. Monte Carlo simulations rely on various scattering, absorption, and photonuclear cross-section data. While the scattering and absorption cross-section data have been extensively studied and validated with experiments, the results obtained from photonuclear simulations are often found to underpredict measured results, indicating uncertainties in the photonuclear cross sections themselves. Thus, there is a need for new measured results that can be used to quantify underpredictions in simulations using photonuclear cross-section data. In the present work, we interrogated depleted uranium with a 9-MV electron linac and detected photoneutrons with trans-stilbene organic scintillators. The measurement of photoneutrons with organic scintillators is challenging due to the presence of the intense photon flux, which causes issues such as pulse pile-up, detector saturation, and poor signal-to-background ratio. To mitigate these challenges, we used iron and polyethylene shielding of varying thicknesses around the depleted uranium target and a neural network–based digital pulse processing algorithm to recover neutron and photon information from piled-up events. Our goal was to compare the measured photoneutron count rate with the simulated rate obtained using the MCNPX-PoliMi transport code. For a light output window of 0.28 to 2.67 MeVee (1.66- to 6.85-MeV proton recoil energy), we found that the simulated count rate obtained using the ENDF/B-VII photonuclear cross-section library underpredicts the measured rate by 32.8% ± 3.2%. Additionally, we compared the simulated and measured photoneutron light output distributions. For the least thicknesses of shielding, the simulation was found to underpredict measurements in the 0.70- to 2.67-MeVee light output window. For the greatest thicknesses of shielding, the simulation was found to underpredict the measurement across the entire light output window of 0.28 to 2.67 MeVee.

Synergy of Organic and Inorganic Sites in 2D Perovskite for Fast Neutron and X‐Ray Imaging

AbstractFast neutron and X‐ray imaging are considered complementary nondestructive detection technologies. However, due to their opposite cross‐sections, development of a scintillator that is sensitive to both fast neutrons and X‐rays within a single‐material framework remains challenging. Herein, an organic–inorganic hybrid perovskite (C4H9NH3)2PbBr4 (BPB) is demonstrated as a scintillator that fully meets the requirements for both fast neutron and X‐ray detection. The hydrogen‐rich organic component acts as a fast neutron converter and produces detectable recoil protons. The heavy atom‐rich inorganic fraction efficiently deposits the energy of charged recoil protons and directly provides a large X‐ray cross‐section. Due to the synergy of these organic and inorganic components, the BPB scintillator exhibits high light yields (86% of the brightness of a commercial ZnS (Ag)/6LiF scintillator for fast neutrons; 22 000 photons per MeV for X‐rays) and fast response times (τdecay = 10.3 ns). More importantly, energy‐selective fast neutron and X‐ray imaging are also demonstrated, with high resolutions of ≈1 lp mm−1 for fast neutrons and 17.3 lp mm−1 for X‐rays; these are among the highest resolution levels for 2D perovskite scintillators. This study highlights the potential of 2D perovskite materials for use in combined fast neutron and X‐ray imaging applications.

Development of a multi-channel gamma-blind fast neutron detector based on wavelength shifting fibers embedded in a ZnS:Ag epoxy mixture

This paper presents a fast neutron detector based on elastic scattering with hydrogen, a silver-activated zinc sulfide scintillator to convert the recoil proton energy to light, and wavelength-shifting fibers (WLSFs) to collect the scintillation light. The detector uses silicon photomultipliers (SiPMs) to recognize individual scintillation photons and a digital filter algorithm based on single photon counting to find clusters of photons belonging to neutron events. The detector presented in this paper features four detection channels, arranged in a 2 × 2 square. The sensitive volume of each detection channel covers a ∼5mm by ∼5mm area from the frontal direction, is 3 cm long, and contains 49 WLSFs. The detector is versatile and performs well under different conditions. Its performance can be tuned to match different applications by simply changing some parameters of the digital filter algorithm. This is illustrated in this paper by extensive measurements in different environments. Using one set of parameters, the detector achieved a gamma-blindness of 10−8 with an intrinsic neutron detection efficiency of ∼1%. With another set of parameters and with lower requirements for gamma blindness, the intrinsic neutron detection efficiency was increased to ∼11%. Yet another set of parameters allows the detector to time incoming fast neutrons with an accuracy of ∼60ns. Additionally, the decay time of the scintillation light created by neutron events was measured, falling to 10% of its peak value in ∼10 μs. Finally, the detector was exposed to strong gamma radiation for a prolonged time to test its radiation resistance. The detection efficiency dropped about linearly with the accumulated gamma fluence, reaching a drop of 40% compared to the initial efficiency at a total gamma fluence of ∼2⋅1013 cm−2.

Neutron-based calibration of a Recoil Proton Telescope for fast neutrons spectroscopy

A Recoil Proton Telescope (RPT), allowing real-time fast neutron spectrometry, has been developed at the IPHC laboratory (Strasbourg, France). The set-up includes a neutron converter, a three-planes tracking part made of pixelated CMOS sensors and a final Si(Li) diode to measure recoil proton energy. The diode calibration is a key component for a precise neutron spectrum reconstruction. The relationship between the charge measured in the diode and the corresponding energy is a function of the temperature and radiation damage, so it must be verified periodically. However, the difficulties to access facilities providing protons with calibrated energies limit the possibility to reassess this calibration on a regular basis. In this paper, we present a straightforward method for RPT neutron-based calibration of the Si(Li) diode which is interesting for high precision measurements at reference neutron sources.

Measurement of light output response in scintillator based neutron detectors using quasi-monoenergetic neutrons

Conventional liquid scintillator (BC501A) and pulse shape discrimination capable plastic scintillator (EJ-299-33A) based detector of dimension; 5 inch diameter and 5 inch long, have been used to study pulse height response for quasi-monoenergetic neutrons of energy in the range 3 to 15 MeV generated using 7Li(p,n)7Be reaction. Scintillation light output of plastic scintillator having pulse shape discrimination property is found to be 75% of the liquid scintillator at neutron energy (maximum recoil proton energy) of 3 MeV which improves with the increase in energy. Functional dependence of the scintillation light output in terms of recoil protons energy has been determined for the liquid and the plastic scintillator detectors for neutron energy in the range 3 to 15 MeV. This functional dependences were used in the Geant4 simulation to calculate the pulse height responses at several neutron energies.

Fast neutron energy based modelling of biological effectiveness with implications for proton and ion beams

A practical neutron energy dependent RBE model has been developed, based on the relationship between a mono-energetic neutron energy and its likely recoil proton energy. Essentially, the linear energy transfer (LET) values of the most appropriate recoil proton energies are then used to modify the linear quadratic model radiosensitivities (α and β) from their reference LET radiation values to provide the RBE estimates. Experimental neutron studies published by Hall (including some mono-energetic beams ranging from 0.2 to 15 MeV), Broerse, Berry, and data from the Clatterbridge and Detroit clinical neutron beams, which all contain some data from a spectrum of neutron energies, are used to derive single effective neutron energies (NEeff) for each spectral beam. These energies yield a recoil proton spectrum, but with an effective mean proton energy (being around 50% of NEeff). The fractional increase in LET is given by the recoil proton LET divided by the proton (LETU) value which provides the highest RBE. This ratio is then used to determine the change in the linear-quadratic model α and β parameters, from those of the reference radiation, to estimate the RBE. The predicted proton recoil RBE is then reasonably close to the experimental neutron RBE values found when taking into account the variation inherent in biological experiments. The work has some important consequences. The data of Hall et al (1975 Radiat. Res. 64 245–55) shows that the highest RBE values are found with neutron energies around 0.3–0.4 MeV, but this energy cannot possibly generate recoil proton energies which are higher, as necessary for a 0.68 MeV proton with a 30.5 keV μm−1 LETU (the LET value which provides the maximum obtainable RBE for a specified ion). For 0.4 MeV neutrons with proton recoil energies of around 0.2 MeV, the latter have a LET of around 62.88 keV μm−1. This could have an impact on proton beam RBE modelling. However, this is compensated by finding that the maximum radiosensitivity for mono-energetic neutrons was around 1.7 times larger than previously suggested from experimental ion beam studies, probably due to the necessary spreading out of Bragg peaks for ion beam experimental purposes, sampling errors and particle range considerations. This semi-empirical model can be used with minimal computer support and could have applications in ionic beams and in radioprotection.

Evaluation of a position-sensitive prototype detector unit for fast neutron imaging and spectroscopy

A novel fast neutron scatter camera with capabilities of neutron imaging and spectroscopy is under development. The detection principle is based on multiple neutron–proton (n–p) elastic scattering interactions in organic scintillator. In order to improve position measurement accuracy of recoil protons, a position-sensitive prototype detector unit has been designed and characterized experimentally. The presented detector unit consisted of a plastic scintillator sheet of 10 cm × 10 cm × 1 cm dimensions and two groups (6 × 2) of wavelength-shifting fibers with orthogonal directions embedded into grooves on two opposite scintillator surfaces. Scintillation signals were read out by silicon photomultipliers (SiPMs). A collimated Sr-90 radioactive source was utilized for system calibration and position resolution measurement. Light output of the unidimensional six fiber channels from one side of the detector unit was calibrated to be 14.45 photoelectrons per MeVee. Position resolution of the detector unit was measured to be 0.35–0.44 times fiber pitch, corresponding to 5.48 mm for proton recoil energy interval of 1.63–2.60 MeV, and 4.60 mm for proton recoil energy interval of 4.82–5.50 MeV. Energy threshold for recoil proton localization was estimated to be 1.18 MeV. The results shown satisfy basic requirements of the scatter camera, while space exists for further improvements. The positioning performance optimization consists of three aspects. The first one is to increase the fiber diameter so as to reduce signal loss. The second one is to depress dark rate of the SiPMs. The last one is to decrease the number of channels involved in position reconstruction by narrowing the scintillation signal distribution function of the detector unit.

Proton Light Yield of Fast Plastic Scintillators for Neutron Imaging

Plastic organic scintillators have been tailored in composition to achieve ultra-fast temporal response, thereby enabling the design and development of fast neutron detection systems with high timing resolution. Eljen Technology's plastic organic scintillators -- EJ-230, EJ-232, and EJ-232Q -- are prospective candidates for use in emerging neutron imaging systems, where fast timing is paramount. To support the neutron response characterization of these materials, the relative proton light yields of EJ-230, EJ-232, and EJ-232Q were measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the proton light yield relations were obtained over a proton recoil energy range of approximately 300 keV to 4 MeV. The EJ-230, EJ-232, and EJ-232Q scintillators exhibited similar proton light yield relations to each other as well as to other plastic scintillators with the same polymer base material. A comparison of the relative proton light yield of different sized cylindrical EJ-232 and EJ-232Q scintillators also revealed consistent results. This work provides key input data for the realistic computational modeling of neutron detection technologies employing these materials, thereby supporting new capabilities in near-field radionuclide detection for national security applications.

Neutron detection and [formula omitted]-ray suppression using artificial neural networks with the liquid scintillators BC-501A and BC-537

In this work we present a comparison between the two liquid scintillators BC-501A and BC-537 in terms of their performance regarding the pulse-shape discrimination between neutrons and γ rays. Special emphasis is put on the application of artificial neural networks. The results show a systematically higher γ-ray rejection ratio for BC-501A compared to BC-537 applying the commonly used charge comparison method. Using the artificial neural network approach the discrimination quality was improved to more than 95% rejection efficiency of γ rays over the energy range 150 to 1000 keV for both BC-501A and BC-537. However, due to the larger light output of BC-501A compared to BC-537, neutrons could be identified in BC-501A using artificial neural networks down to a recoil proton energy of 800 keV compared to a recoil deuteron energy of 1200 keV for BC-537. We conclude that using artificial neural networks it is possible to obtain the same γ-ray rejection quality from both BC-501A and BC-537 for neutrons above a low-energy threshold. This threshold is, however, lower for BC-501A, which is important for nuclear structure spectroscopy experiments of rare reaction channels where low-energy interactions dominates.

High-precision characterization of the neutron light output of stilbene along the directions of maximum and minimum response

The scintillation light output response of stilbene crystals has been measured for protons recoiling along the a, b, and c’ crystalline axes with energies between 1.3 and 10 MeV using neutrons produced with the tandem Van de Graaff accelerator at Triangle Universities Nuclear Laboratory. The proton recoil energy and direction were measured using the coincident detection of neutrons between a stilbene scintillator and an array of EJ-309 liquid scintillators spanning arranged neutron recoil angles. The maximum light output was found to coincide with proton recoils along the a-axis, in disagreement with other published measurements, which reported the b-axis as the direction of the maximum light output. Additional measurements were conducted using two different stilbene crystals to confirm these results: a second measurement using the coincident detection of neutrons; measurements of neutron full energy deposition events along the a and b axes; and measurements of the count rate for 252Cf neutrons traveling along the a and b axes directions. All measurements found that recoils along the a-axis produce the maximum light output.

Liquid scintillator response to proton recoils in the 10–100 keV range

We study the response of EJ-301 liquid scintillator to monochromatic 244.6 $\pm$ 8.4 keV neutrons, targeting the 10-100 keV proton recoil energy interval. Limited experimental information exists for proton light yield in this range, for this or any other organic scintillator. Our results confirm the adequacy of a modified Birks' model, common to all organic scintillator formulations, predicting a marked increase in quenching factor as proton energy approaches the few keV regime. The relevance of this behavior within the context of searches for low-mass particle dark matter is mentioned.

A Neutron Spectrometer for Experiments with Radioactive Beams on the ACCULINNA-2 Fragment Separator

A neutron spectrometer based on stilbene crystals has been developed by the Flerov Laboratory of Nuclear Reactions at the Joint Institute for Nuclear Research (Dubna, Russia). The timing resolution is determined as a function of the signal amplitude (σT = 0.18 ns at an amplitude of 1 MeV in the electron equivalent). The measured energy resolution of the detecting modules for γ rays is σE/E = 4.5% at E = 1 MeV. The quality of the n–γ discrimination is investigated. It is shown that reliable discrimination is possible, beginning with a deposited energy of 100 keV in the electron equivalent, which corresponds to the kinetic energy of recoil protons of ∼700 keV. The neutron spectrometer helps to significantly expand the experimental capabilities and to carry out correlation experiments with radioactive beams on the ACCULINNA-2 fragment separator at a new level of quality.

Conception of a New Recoil Proton Telescope for Real-Time Neutron Spectrometry in Proton-Therapy

Neutrons are the main type of secondary particles emitted in proton-therapy. Because of the risk of secondary cancer and other late occurring effects, the neutron dose should be included in the out-of-field dose calculations. A neutron spectrometer has to be used to take into account the energy dependence of the neutron radiological weighting factor. Due to its high dependence on various parameters of the irradiation (beam, accelerator, patient), the neutron spectrum should be measured independently for each treatment. The current reference method for the measurement of the neutron energy, the Bonner Sphere System, consists of several homogeneous polyethylene spheres with increasing diameters equipped with a proportional counter. It provides a highresolution reconstruction of the neutron spectrum but requires a time-consuming work of signal deconvolution. New neutron spectrometers are being developed, but the main experimental limitation remains the high neutron flux in proton therapy treatment rooms. A new model of a real-time neutron spectrometer, based on a Recoil Proton Telescope technology, has been developed at the IPHC. It enables a real-time high-rate reconstruction of the neutron spectrum from the measurement of the recoil proton trajectory and energy. A new fast-readout microelectronic integrated sensor, called FastPixN, has been developed for this specific purpose.A first prototype, able to detect neutrons between 5 and 20 MeV, has already been validated for metrology with the AMANDE facility at Cadarache. The geometry of the new Recoil Proton Telescope has been optimized via extensive Geant4 Monte Carlo simulations. Uncertainty sources have been carefully studied in order to improve simultaneously efficiency and energy resolution, and solutions have been found to suppress the various expected backgrounds. We are currently upgrading the prototype for secondary neutron detection in proton therapy applications.

Model-based design evaluation of a compact, high-efficiency neutron scatter camera

This paper presents the model-based design and evaluation of an instrument that estimates incident neutron direction using the kinematics of neutron scattering by hydrogen-1 nuclei in an organic scintillator. The instrument design uses a single, nearly contiguous volume of organic scintillator that is internally subdivided only as necessary to create optically isolated pillars, i.e., long, narrow parallelepipeds of organic scintillator. Scintillation light emitted in a given pillar is confined to that pillar by a combination of total internal reflection and a specular reflector applied to the four sides of the pillar transverse to its long axis. The scintillation light is collected at each end of the pillar using a photodetector, e.g., a microchannel plate photomultiplier (MCP-PM) or a silicon photomultiplier (SiPM). In this optically segmented design, the (x,y) position of scintillation light emission (where the x and y coordinates are transverse to the long axis of the pillars) is estimated as the pillar’s (x,y) position in the scintillator “block”, and the z-position (the position along the pillar’s long axis) is estimated from the amplitude and relative timing of the signals produced by the photodetectors at each end of the pillar. The neutron’s incident direction and energy is estimated from the (x,y,z)-positions of two sequential neutron–proton scattering interactions in the scintillator block using elastic scatter kinematics. For proton recoils greater than 1 MeV, we show that the (x,y,z)-position of neutron–proton scattering can be estimated with < 1 cm root-mean-squared [RMS] error and the proton recoil energy can be estimated with < 50 keV RMS error by fitting the photodetectors’ response time history to models of optical photon transport within the scintillator pillars. Finally, we evaluate several alternative designs of this proposed single-volume scatter camera made of pillars of plastic scintillator (SVSC-PiPS), studying the effect of pillar dimensions, scintillator material (EJ-204, EJ-232Q and stilbene), and photodetector (MCP-PM vs. SiPM) response vs. time. We demonstrate that the most precise estimates of incident neutron direction and energy can be obtained using a combination of scintillator material with high luminosity and a photodetector with a narrow impulse response. Specifically, we conclude that an SVSC-PiPS constructed using EJ-204 (a high luminosity plastic scintillator) and an MCP-PM will produce the most precise estimates of incident neutron direction and energy.

Potential reduction interior point algorithm unfolding of neutron energy spectrum measured by recoil proton method**supported by Fundamental Research Funds for Central Universities (2016XS61), and Opening Foundation of State Key Laboratory of Intense Pulsed Radiation Simulation and Effect.

A reconstruction algorithm for unfolding neutron energy spectra has been developed, based for the first time on the potential reduction interior point algorithm. This algorithm can be easily applied to neutron energy spectrum reconstruction in the recoil proton method. We transform the neutron energy spectrum unfolding problem into a typical nonnegative linear complementarity problem. The recoil proton energy spectrum and response matrix at angles of 0° and 30° are generated by the Geant4 simulation toolkit. Several different neutron energy test spectra are also employed. It is found that this unfolding algorithm is stable and provides efficient, accurate results.

Neutron spectroscopy by thermalization light yield measurement in a composite heterogeneous scintillator

An exothermic neutron capture reaction can be used to uniquely identify neutrons in particle detectors. With the use of a capture-gated coincidence technique, the sequence of scatter events that lead to neutron thermalization prior to the neutron capture can also be used to measure neutron energy. We report on the measurement of thermalization light yield via a time-of-flight technique in a polyvinyl toluene-based scintillator EJ-290 within a heterogeneous composite detector that also includes 6Li-doped glass scintillator. The thermalization light output exhibits a strong correlation with neutron energy because of the preference for near-complete energy deposition prior to the 6Li(n,t)4He neutron capture reaction. The nonproportionality of the light yield from nuclear recoils contributes to the observed broadening of the distribution of thermalization light output. The nonproportional dependence of the scintillation light output in the EJ-290 scintillator as a function of proton recoil energy has been characterized in the range of 0.3–14.1MeV via the Birks parametrization through a combination of time-of-flight measurement and previously conducted measurements with monoenergetic neutron sources.

A telescope detection system for direct and high resolution spectrometry of intense neutron fields

A high energy- and spatial-resolution telescope detector was designed and constructed for neutron spectrometry of intense neutron fields. The detector is constituted by a plastic scintillator coupled to a monolithic silicon telescope (MST), in turn consisting of a ΔE and an E stage. The scintillator behaves as an “active” recoil-proton converter, since it measures the deposited energy of the recoil-protons generated across. The MST measures the residual energy of recoil-protons downstream of the converter and also discriminates recoil-protons from photons associated to the neutron field. The lay-out of the scintillator/MST system was optimized through an analytical model for selecting the angular range of the scattered protons. The use of unfolding techniques for reconstructing the neutron energy distribution was thus avoided with reasonable uncertainty (about 1.6% in neutron energy) and efficiency (of the order of 10−6 counts per unit neutron fluence). A semi-empirical procedure was also developed for correcting the non-linearity in light emission from the organic scintillator. The spectrometer was characterized with quasi-monoenergetic and continuous fields of neutrons generated at the CN Van De Graaff accelerator of the INFN-Legnaro National Laboratory, Italy, showing satisfactory agreement with literature data.

Study of an unfolding algorithm for D-T neutron energy spectra measurement using a recoil proton method**Supported by National Natural Science Foundations of China (11375077, 21327801) and National Key Scientific Instrument And Equipment Development Project (2013YQ40861)

A proton recoil method for measuring D-T neutron energy spectra using polyethylene film and a Si(Au) surface barrier detector is presented. An iteration algorithm for unfolding the recoil proton energy spectrum to the neutron energy spectrum is investigated. The response matrices R of the polyethylene film at angles of 0° and 45° were obtained by simulating the recoil proton energy spectra from mono-energetic neutrons using the MCNPX code. With an assumed D-T neutron spectrum, the recoil proton spectra from the polyethylene film at angles of 0° and 45° were also simulated using the MCNPX code. Based on the response matrices R and the simulated recoil proton spectra at 0° and 45°, the respective unfolded neutron spectra were obtained using the iteration algorithm, and compared with the assumed neutron spectrum. The results show that the iteration algorithm method can be applied to unfold the recoil proton energy spectrum to the neutron energy spectrum for D-T neutron energy spectra measurement using the recoil proton method.

Investigation of the structure of light exotic nuclei by proton elastic scattering in inverse kinematics

In order to study the spatial structure of exotic nuclei, it was proposed at the Petersburg Nuclear Physics Institute (PNPI) to measure the differential cross section for small-angle proton elastic scattering in inverse kinematics. Several experiments in beams of 0.7-GeV/nucleon exotic nuclei were performed at the heavy-ion accelerator facility of GSI (Gesellschaft fur Schwerionenforschung, Darmstadt, Germany) by using the IKAR ionization spectrometer developed at PNPI. The IKAR ionization chamber filled with hydrogen at a pressure of 10 bar served simultaneously as a target and as a recoil-proton detector, which measured the recoil-proton energy. The beam-particle scattering angle was also measured. The results obtained for the cross sections in question were analyzed on the basis of the Glauber-Sitenko theory using phenomenological nuclear-density distributions with two free parameters. Nuclear-matter distributions and root-mean-square radii were found for the nuclei under investigation. The size of the halo in the 6He, 8He, 11Li, and 14Be nuclei was determined among other things. Information about neutron distributions in nuclei was deduced by combining the data obtained here with the known values of the radii of proton distributions. A sizable neutron skin was revealed in the 8Li, 9Li, and 12Be nuclei.

Measurement of proton momentum distributions using a direct geometry instrument

We report the results of inelastic neutron scattering measurements on bulk water and ice using the direct geometry SEQUOIA chopper spectrometer at the Spallation Neutron Source (USA), with incident energy Ei= 6 eV. In this set up the measurements allow to access the Deep Inelastic Neutron Scattering regime. The scattering is centred at the proton recoil energy given by the impulse approximation, and the shape of the recoil peak conveys information on the proton momentum distribution in the system. The comparison with the performance of inverse geometry instruments, such as VESUVIO at the ISIS source (UK), shows that complementary information can be accessed by the use of direct and inverse geometry instruments. Analysis of the neutron Compton profiles shows that the proton kinetic energy in ice at 271 K is larger than in room temperature liquid water, in agreement with previous measurements on VESUVIO.