The prediction of the ablation rate of silicone rubber-based composites is of great significance to accelerate the development of flexible thermal protection materials. Herein, a method which combines uniform design experimentation, active learning, and virtual sample generation was proposed to establish a prediction model of the mass ablation rate based on a small dataset. Briefly, a small number of sample points were collected using uniform design experimentation, which were marked to construct the initial dataset and primitive model. Then, data points were acquired from the sample pool and iterated using various integrated algorithms through active learning to update the above dataset and model. Finally, a large number of virtual samples were generated based on the optimal model, and a further optimized prediction model was achieved. The results showed that after introducing 300 virtual samples, the average percentage error of the gradient boosting decision tree (GBDT) prediction model on the test set decreased to 3.1%, which demonstrates the effectiveness of the proposed method in building prediction models based on a small dataset.
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