Decoherence Rate Research Articles

A mechanical qubit.

Although strong nonlinear interactions between quantized excitations are an important resource for quantum technologies based on bosonic oscillator modes, most electromagnetic and mechanical nonlinearities are far too weak to allow for nonlinear effects to be observed at the single-quantum level. This limitation has been overcome in electromagnetic resonators by coupling them to other strongly nonlinear quantum systems such as atoms and superconducting qubits. We demonstrate the realization of the single-phonon nonlinear regime in a solid-state mechanical system. The single-phonon anharmonicity in our system exceeds the decoherence rate by a factor of 6.8, allowing us to use it as a mechanical qubit and demonstrate initialization, readout, and single-qubit gates. Our approach provides a powerful quantum acoustics platform for quantum simulations, sensing, and information processing.

Testing Whether Gravity Acts as a Quantum Entity When Measured.

A defining signature of classical systems is "in principle measurability" without disturbance: a feature manifestly violated by quantum systems. We describe a multi-interferometer experimental setup that can, in principle, reveal the nonclassicality of a spatial superposition-sourced gravitational field if an irreducible disturbance is caused by a measurement of gravity. While one interferometer sources the field, the others are used to measure the gravitational field created by the superposition. This requires neither any specific form of nonclassical gravity, nor the generation of entanglement between any relevant degrees of freedom at any stage, thus distinguishing it from the experiments proposed so far. This test, when added to the recent entanglement-witness based proposals, enlarges the domain of quantum postulates being tested for gravity. Moreover, the proposed test yields a signature of quantum measurement induced disturbance for any finite rate of decoherence, and is device independent.

Probing Bioinorganic Electron Spin Decoherence Mechanisms with an Fe2S2 Metalloprotein.

Recent efforts have sought to develop paramagnetic molecular quantum bits (qubits) as a means to store and manipulate quantum information. Emerging structure-property relationships have shed light on electron spin decoherence mechanisms. While insights within molecular quantum information science have derived from synthetic systems, biomolecular platforms would allow for the study of decoherence phenomena in more complex chemical environments and further leverage molecular biology and protein engineering approaches. Here we have employed the exchange-coupled ST = 1/2 Fe2S2 active site of putidaredoxin, an electron transfer metalloprotein, as a platform for fundamental mechanistic studies of electron spin decoherence toward spin-based biological quantum sensing. At low temperatures, decoherence rates were anisotropic, reflecting a hyperfine-dominated decoherence mechanism, standing in contrast to the anisotropy of molecular systems observed previously. This mechanism provided a pathway for probing spatial effects on decoherence, such as protein vs solvent contributions. Furthermore, we demonstrated spatial sensitivity to single point mutations via site-directed mutagenesis and temporal sensitivity for monitoring solvent isotope exchange. Thus, this study demonstrates a step toward the design and construction of biomolecular quantum sensors.

Cosmological Bell tests with decoherence effects

The inflationary universe creates particle pairs, which are entangled in their momenta due to momentum conservation. Operators involving the momenta of the fluctuations can be rewritten into pseudo-spin operators, such as the Gour-Khanna-Mann-Revzen (GKMR) pseudo-spin. Making use of these pseudo-spin operators, cosmological Bell inequalities can be formulated. The violation of these Bell inequalities indicates the quantum nature of primordial fluctuations.In this work, we focus on primordial curvature perturbations. Since curvature perturbations arise from gravity, their action includes the Gibbons-Hawking-York boundary term. We clarify the role of the boundary term in selecting suitable initial conditions for linear perturbations.After that, we proceed to the interactions of cosmological perturbations, including the bulk and boundary interaction terms, which introduce decoherence effects. These decoherence effects change the expectation value of the Bell operator, and gradually restore the Bell inequality. We describe this process by a “Bell test curve”, which offers a window around 5 e-folds for testing the quantum origin of cosmological perturbations. We also explore the possibility of extracting the information of the decoherence rate and the structure of primordial interactions from the Bell test curve.

Quantum-assisted rendezvous on graphs: explicit algorithms and quantum computer simulations

Abstract We study quantum advantage in one-step rendezvous games on simple graphs analytically, numerically, and using noisy intermediate-scale quantum (NISQ) processors. Our protocols realise the recently discovered (Mironowicz 2023 New J. Phys. 25 013023) optimal bounds for small cycle graphs and cubic graphs. In the case of cycle graphs, we generalise the protocols to arbitrary graph size. The NISQ processor experiments realise the expected quantum advantage with high accuracy for rendezvous on the complete graph K 3. In contrast, for the graph 2 K 4 , formed by two disconnected 4-vertex complete graphs, the performance of the NISQ hardware is sub-classical, consistent with the deeper circuit and known qubit decoherence and gate error rates.

Characterization of entanglement on superconducting quantum computers of up to 414 qubits

As quantum technology advances and the size of quantum computers grow, it becomes increasingly important to understand the extent of quality in the devices. As large-scale entanglement is a quantum resource crucial for achieving quantum advantage, the challenge in its generation makes it a valuable benchmark for measuring the performance of universal quantum devices. In this paper, we study entanglement in Greenberger-Horne-Zeilinger (GHZ) and graph states prepared on the range of IBM Quantum devices. We generate GHZ states and investigate their coherence times with respect to state size and dynamical decoupling techniques. A GHZ fidelity of 0.519±0.014 is measured on a 32-qubit GHZ state, certifying its genuine multipartite entanglement (GME). We show a substantial improvement in GHZ decoherence rates for a seven-qubit GHZ state after implementing dynamical decoupling, and observe a linear trend in the decoherence rate of α=(7.13N+5.54)×10−3µs−1 for up to N=15 qubits, confirming the absence of superdecoherence. Additionally, we prepare and characterize fully bipartite entangled native-graph states on 22 superconducting quantum devices with qubit counts as high as 414 qubits, all active qubits of the 433-qubit IBM Osprey device. Analysis of the decay of two-qubit entanglement within the prepared states shows suppression of coherent noise signals with the implementation of dynamical decoupling techniques. Additionally, we observe that the entanglement in some qubit pairs oscillates over time, which is likely caused by residual ZZ-interactions. Characterizing entanglement in native-graph states, along with detecting entanglement oscillations, can be an effective approach to low-level device benchmarking that encapsulates two-qubit error rates along with additional sources of noise, with possible applications to quantum circuit compilation. We develop several tools to automate the preparation and entanglement characterization of GHZ and graph states. In particular, a method to characterize graph state bipartite entanglement using just 36 circuits, constant with respect to the number of qubits. Published by the American Physical Society 2024

Enhanced optical pumping using mutually orthogonal magnetic fields for quantum sensing

The atomic population trapped in irrelevant atomic states is a limiting factor for sensors based on laser-atom interaction. Using a bi-chromatic light field along with a specific combination of magnetic fields, we show a significant increase in the amplitude (i.e., more than seven times) of a two-photon coherent population trapping (CPT) resonance, which can be effectively used for atomic magnetometry. This increase in amplitude can be explained through enhanced optical pumping via the transfer of population to the relevant Zeeman states. Our experimental observations are consistent with the theoretical calculations carried out for a realistic three-level atomic system using density matrix formalism. We further discuss the optimum condition for enhanced optical pumping by adjusting the ground-state decoherence rate. Enhanced optical pumping through the manipulation of the magnetic field is quite important and is of great interest in the field of quantum technology.

Inherent Thermal-Noise Problem in Addressing Qubits

Qubit-specific measurement in a superconducting quantum processor requires physical interconnects that traverse 4 orders of magnitude in temperature from 293 K to 10 mK. Although the quantum processor can be thermalized and shielded from electromagnetic noise, the interconnects themselves introduce an unavoidable remote heat bath that causes decoherence of quantum states. In the present work, we report quantitative and device-independent measurements of the power radiated to the quantum processor from its control lines. Our results have been obtained using a calibrated bolometer that operates within a millikelvin environment with time-resolved measurement capability. In the limit of zero applied power, the noise power emitted to the quantum processor is equivalent to that of a blackbody with temperature 63–71 mK for the prototypical drive lines in the study. Experimentally, we increase the applied power of a simulated control signal to map out the resulting temperature rise and thermal time constant of five prototypical drive-line varieties. We input the data to an open quantum system model to demonstrate the trade-off between dissipated signal power, transmon-qubit lifetime, pure dephasing, gate fidelity, and the implied decoherence rates due to self-heating during microwave operations. Beyond explaining dephasing rates observed in the literature, our work sets the stage for accurate noise modeling in novel quantum computer interfacing methods due to our device-agnostic approach. Published by the American Physical Society 2024

Thresholds for the distributed surface code in the presence of memory decoherence

In the search for scalable, fault-tolerant quantum computing, distributed quantum computers are promising candidates. These systems can be realized in large-scale quantum networks or condensed onto a single chip with closely situated nodes. We present a framework for numerical simulations of a memory channel using the distributed toric surface code, where each data qubit of the code is part of a separate node, and the error-detection performance depends on the quality of four-qubit Greenberger–Horne–Zeilinger (GHZ) states generated between the nodes. We quantitatively investigate the effect of memory decoherence and evaluate the advantage of GHZ creation protocols tailored to the level of decoherence. We do this by applying our framework for the particular case of color centers in diamond, employing models developed from experimental characterization of nitrogen-vacancy centers. For diamond color centers, coherence times during entanglement generation are orders of magnitude lower than coherence times of idling qubits. These coherence times represent a limiting factor for applications, but previous surface code simulations did not treat them as such. Introducing limiting coherence times as a prominent noise factor makes it imperative to integrate realistic operation times into simulations and incorporate strategies for operation scheduling. Our model predicts error probability thresholds for gate and measurement reduced by at least a factor of three compared to prior work with more idealized noise models. We also find a threshold of 4×102 in the ratio between the entanglement generation and the decoherence rates, setting a benchmark for experimental progress.

Decoherence rate in random Lindblad dynamics

Open quantum systems undergo decoherence, which is responsible for the transition from quantum to classical behavior. The time scale in which decoherence takes place can be analyzed using upper limits to its rate. We examine the dynamics of open chaotic quantum systems governed by random Lindblad operators sourced from Gaussian and Ginibre ensembles with Wigner-Dyson symmetry classes. In these systems, the ensemble-averaged purity decays monotonically as a function of time. This decay is governed by the decoherence rate, which is upper-bounded by the dimension of their Hilbert space and is independent of the ensemble symmetry. These findings hold upon mixing different ensembles, indicating the universal character of the decoherence rate limit. Moreover, our findings reveal that open chaotic quantum systems governed by random Lindbladians tend to exhibit the most rapid decoherence, regardless of the initial state. This phenomenon is associated with the concentration of the decoherence rate near its upper bound. Our work identifies primary features of decoherence in dissipative quantum chaos, with applications ranging from quantum foundations to high-energy physics and quantum technologies. Published by the American Physical Society 2024

Quantum sensing with tunable superconducting qubits: optimization and speed-up

Abstract Sensing and metrology are crucial in both fundamental science and practical applications. They meet the constant demand for precise data, enabling more dependable assessments of theoretical models’ validity. Sensors, now a common feature in many fields, play a vital role in applications like gravity imaging, geology, navigation, security, timekeeping, spectroscopy, chemistry, magnetometry, healthcare, and medicine. The advancements in quantum technologies have sparked interest in employing quantum systems as sensors, offering enhanced capabilities and new possibilities. This article describes the optimization of the quantum-enhanced sensing
of magnetic fluxes with a Kitaev phase estimation algorithm based on frequency tunable transmon qubits. It provides the optimal flux biasing point for sensors with different qubit transition frequencies and gives an estimation of decoherence rates and achievable sensitivity. The use of 2- and 3-qubit entangled states are compared in simulation with the single-qubit case. The flux sensing accuracy reaches 10-8·Φ0 and scales inversely with time, which proves the speed-up of sensing with high ultimate accuracy.

Theory of electron spin resonance in scanning tunneling microscopy

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating coherent manipulation of single spins. Despite this remarkable success, the field could still be greatly advanced by a more quantitative understanding of the ESR-STM physical mechanisms. Here, we present a theory of ESR-STM that quantitatively models not only the ESR signal itself, but also the full background tunneling current, from which the ESR signal is derived. Our theory is based on a combination of Green's function techniques to describe the electron tunneling and a quantum master equation for the dynamics of the spin system along with microwave radiation interacting with both the tunneling current and the magnetic system. We show that this theory is able to quantitatively reproduce the experimental results for a spin-1/2 system (TiH molecules on MgO) across many orders of magnitude in tunneling current, providing access to the relaxation and decoherence rates that govern the spin dynamics due to intrinsic mechanisms and to the applied bias voltage. More importantly, our work establishes that (i) sizable ESR signals, which are a measure of microwave-induced changes in the junction magnetoresistance, require surprisingly high tip spin polarizations, and (ii) the coupling of the magnetization dynamics to the microwave field gives rise to the asymmetric ESR spectra often observed in this spectroscopy. Additionally, our theory provides very specific predictions for the dependence of the relaxation and decoherence times on the bias voltage and the tip-sample distance. Finally, with the help of electromagnetic simulations, we find that the transitions in our ESR-STM experiments, in which the tunnel junction is irradiated by a nearby microwave antenna, can be driven by the ac magnetic field at the junction. Published by the American Physical Society 2024

Effect of relaxation on the transfer of orbital angular momentum via four-wave mixing process in the four-level double lambda atomic system

In this work, we have theoretically studied the resonant four-wave mixing (FWM) in a four-level double Lambda (Λ) atomic system in connection with orbital angular momentum (OAM) transfer from probe to generated signal beam. The effect of the relaxation process is studied in the forward as well as backward FWM. Based on the semiclassical model, our analysis shows a strong dependence of conversion efficiency on spontaneous decay and decoherence rates. From the intensity and phase profile, we have confirmed the OAM nature of the generated signal beam. The physical explanation is given for the dependence of efficiency on the decay rate of the excited atomic state. We have shown that decoherence present in the system always leads to a deleterious effect on conversion efficiency. Our presentation treats forward and backward FWM in a unified way in the context of OAM transfer and sheds light on the parameter dependence of conversion efficiency.

Spatially correlated classical and quantum noise in driven qubits.

Correlated noise across multiple qubits poses a significant challenge for achieving scalable and fault-tolerant quantum processors. Despite recent experimental efforts to quantify this noise in various qubit architectures, a comprehensive understanding of its role in qubit dynamics remains elusive. Here, we present an analytical study of the dynamics of driven qubits under spatially correlated noise, including both Markovian and non-Markovian noise. Surprisingly, we find that by operating the qubit system at low temperatures, where correlated quantum noise plays an important role, significant long-lived entanglement between qubits can be generated. Importantly, this generation process can be controlled on-demand by turning the qubit driving on and off. On the other hand, we demonstrate that by operating the system at a higher temperature, the crosstalk between qubits induced by the correlated noise is unexpectedly suppressed. We finally reveal the impact of spatio-temporally correlated 1/f noise on the decoherence rate, and how its temporal correlations restore lost entanglement. Our findings provide critical insights into not only suppressing crosstalk between qubits caused by correlated noise but also in effectively leveraging such noise as a beneficial resource for controlled entanglement generation.

Loss of coherence and coherence protection from a graviton bath

We consider a quantum harmonic oscillator coupled with a graviton bath. We discuss the loss of coherence in the matter sector due to the matter-graviton vertex interaction, which leads to a loss of coherence provided that the matter-wave system is allowed to gravitons by the kinematics. Working in the quantum-field-theory framework, we obtain a master equation by tracing away the gravitational field at the leading order ∼O(G) and ∼O(c−2). We find that the decoherence rate is proportional to the cube of the harmonic trapping frequency and vanishes for a free particle, as expected for a system without a mass quadrupole. Furthermore, our quantum model of graviton emission recovers the known classical formula for gravitational radiation from a classical harmonic oscillator for coherent states with a large occupation number. In addition, we find that the quantum harmonic oscillator eventually settles in a steady state with of the ground and first excited states. While classical emission of gravitational waves would make the harmonic system loose all of its energy, our quantum field theory model does not allow the number states |1⟩ and |0⟩ to decay via graviton emission. In particular, the superposition of number states 12[|0⟩+|1⟩] is a steady state and never decoheres. Published by the American Physical Society 2024

Decoherence from horizons: General formulation and rotating black holes

Recent work by Danielson, Satishchandran, and Wald (DSW) has shown that black holes—and, in fact, Killing horizons more generally—impart a fundamental rate of decoherence on all nearby quantum superpositions. The effect can be understood from measurement and causality: An observer (Bob) in the black hole should be able to disturb outside quantum superpositions by measuring their superposed gravitational fields, but since his actions cannot (by causality) have this effect, the superpositions must automatically disturb themselves. DSW calculated the rate of decoherence up to an unknown numerical factor for distant observers in Schwarzschild spacetime, Rindler observers in flat spacetime, and static observers in de Sitter spacetime. Working in electromagnetic and Klein-Gordon analogs, we flesh out and generalize their calculation to derive a general formula for the precise decoherence rate for Killing observers near bifurcate Killing horizons. We evaluate the rate in closed form for an observer at an arbitrary location on the symmetry axis of a Kerr black hole. This fixes the numerical factor in the distant-observer Schwarzschild result, while allowing new exploration of near-horizon and/or near-extremal behavior. In the electromagnetic case we find that the decoherence vanishes entirely in the extremal limit, due to the “black hole Meissner effect” screening the Coulomb field from entering the black hole. This supports the causality picture: Since Bob is unable to measure the field of the outside superposition, no decoherence is necessary—and indeed none occurs. Published by the American Physical Society 2024

Real-time adaptive estimation of decoherence timescales for a single qubit

Characterizing the time over which quantum coherence survives is critical for any implementation of quantum bits, memories, and sensors. The usual method for determining a quantum system’s decoherence rate involves a suite of experiments probing the entire expected range of this parameter, and extracting the resulting estimation in postprocessing. Here we present an adaptive multiparameter Bayesian approach, based on a simple analytical update rule, to estimate the key decoherence timescales (T1, T2∗, and T2) and the corresponding decay exponent of a quantum system in real time, using information gained in preceding experiments. This approach reduces the time required to reach a given uncertainty by a factor up to an order of magnitude, depending on the specific experiment, compared to the standard protocol of curve fitting. A further speedup of a factor approximately 2 can be realized by performing our optimization with respect to sensitivity as opposed to variance. Published by the American Physical Society 2024

Strong coupling between a microwave photon and a singlet-triplet qubit

Combining superconducting resonators and quantum dots has triggered tremendous progress in quantum information, however, attempts at coupling a resonator to even charge parity spin qubits have resulted only in weak spin-photon coupling. Here, we integrate a zincblende InAs nanowire double quantum dot with strong spin-orbit interaction in a magnetic-field resilient, high-quality resonator. The quantum confinement in the nanowire is achieved using deterministically grown wurtzite tunnel barriers. Our experiments on even charge parity states and at large magnetic fields, allow us to identify the relevant spin states and to measure the spin decoherence rates and spin-photon coupling strengths. We find an anti-crossing between the resonator mode in the single photon limit and a singlet-triplet qubit with a spin-photon coupling strength of g/2π = 139 ± 4 MHz. This coherent coupling exceeds the resonator decay rate κ/2π = 19.8 ± 0.2 MHz and the qubit dephasing rate γ/2π = 116 ± 7 MHz, putting our system in the strong coupling regime.

Quantum correlations and coherence in a mixed spin- (12,1) Heisenberg dimer under intrinsic decoherence

This research delves into the dynamical behavior of quantum correlations and coherence within a mixed Heisenberg dimer system under the intrinsic decoherence. Our approach involves the application of logarithmic negativity, local quantum uncertainty, and the ℓ 1 norm-based coherence as quantifiers for entanglement, skew information correlations, and quantum coherence in this qubit-qutrit model. Our primary objective is to explore the impact of various factors on the dynamics of quantum correlations and quantum coherence. These factors encompass the initial density matrix and its mixing parameter, the intrinsic decoherence rate (γ), the external magnetic field, as well as intrinsic system parameters, notably the XXZ and uniaxial single-ion anisotropies. Our results demonstrate that the introduction of intrinsic decoherence (ID) significantly erodes quantum resources. Particularly, for high values of the ID rate (γ), excessive damping occurs, leading to the absence of oscillations or a rapid decay of quantum resources, ultimately stabilizing in steady states. Furthermore, the presence of an external homogeneous magnetic field further diminishes quantum resources within the system. However, despite the degradation induced by the combined influence of intrinsic decoherence and high external magnetic field intensities, the judicious selection of the initial density matrix and precise adjustment of the uniaxial single-ion anisotropy enable the preservation of quantum resources within the mixed spin-(1/2, 1) Heisenberg dimer.

Phonon-induced decoherence in color-center qubits

Electron spin states of solid-state defects such as nitrogen- and silicon-vacancy in diamond are a leading quantum-memory candidate for quantum communications and computing. Via open-quantum-systems modeling of spin-phonon coupling—the major contributor of decoherence—at a given temperature, we derive the time dynamics of the density operator of an electron-spin qubit. We use our model to corroborate experimentally measured decoherence rates. We further derive the temporal decay of distillable entanglement in spin-spin entangled states heralded via photonic Bell-state measurements. Extensions of our model to include other decoherence mechanisms, e.g., undesired hyperfine couplings to the neighboring nuclear-spin environment, will pave the way to a rigorous predictive model for engineering artificial-atom qubits with desirable properties. Published by the American Physical Society 2024