Rare Isotope Accelerator Research Articles

Erratum: Acceleration of uranium beam to record power of 10.4 kW and observation of new isotopes at Facility for Rare Isotope Beams [Phys. Rev. Accel. beams 27 , 060101 (2024)

Erratum: Acceleration of uranium beam to record power of 10.4 kW and observation of new isotopes at Facility for Rare Isotope Beams [Phys. Rev. Accel. beams <b>27</b> , 060101 (2024)

Design and commissioning of the ISOL beamline at the RAON facility

The Rare isotope Accelerator complex for ON-line experiment (RAON) located at the Daejeon site of the Institute for Basic Science (IBS) is the first Radioactive Isotope (RI) beam facility in Korea. The RAON facility employs an in-flight method using RI beams produced using an Isotope Separator On-Line (ISOL) method to explore unstable nuclei in uncharted regions. A high-power ISOL facility is critical for providing the required high-quality, intense RI beams. The design, construction, and installation of the ISOL system have been completed, and the beam transport line commissioning with stable isotope beams has been conducted. As a result, all requirements, such as the transmission and the mass-resolving power, for the beamlines were satisfied, and the beams from the Target Ion Source (TIS) were transported to the end of the ISOL beamline, which is the entrance to the superconducting linear accelerator system. The ISOL beamline is now ready for the transport of RI beams.

Acceleration of uranium beam to record power of 10.4 kW and observation of new isotopes at Facility for Rare Isotope Beams

The Facility for Rare Isotope Beams (FRIB) is a major nuclear physics facility for research with fast, stopped, and reaccelerated beams that was successfully commissioned in May 2022. A key capability of FRIB is the production of an acceleration of the uranium beam, but this capability requires the facility to work at the design limits of the lowest charge-to-mass ratio and the highest power density on the beam intercepting devices. This paper presents techniques for overcoming the significant challenges in accelerating the uranium beam, culminating in the demonstration of 10.4 kW on target, and the discovery of three new isotopes. The high-power uranium beam enabled us to produce and identify G88a, A93s, and S96e, within the first 24 h of operation. The successful uranium operation at FRIB sets a new record for accelerated uranium beam power above 10 kW and opens a new avenue of research with rare isotopes. Published by the American Physical Society 2024

Beam Commissioning of the Heavy-ion Accelerator RAON

RAON (Rare-isotope Accelerator complex for ON-line experiments) is the superconducting linac (SCL3 and SCL2) facility in Korea. It consists of an injector, a superconducting linac, and user facilities. It is designed to accelerate various ion beams from proton (A/Q=1) to uranium (A/Q=7.2). The ECR ion source in the injector system generates ion beams with the energy of 10 keV/u. They are accelerated to the energy of 500 keV/u by the RFQ (Radio-Frequency Quadrupole) in the injector. The superconducting linac (SCL3) includes 22 QWR (Quater-Wave Resonator) cavities and 102 HWR (Half-Wave Resonator) cavities. The energy becomes 18.5 MeV/u for uranium beams after the linac. The beam commissioning of the injector started from August 2021. The first beam commissioning of the superconducting linac was performed from October 2022 to June 2, 2023. Research and development of the cavities for the high-energy part (SCL2) of the superconducting linac is in progress. This work explains some characteristic features of the beam dynamics for RAON linac and some beam commissioning results.

Process design for FRIB’s experimental refrigeration system

The experimental system (ES) for the Facility for Rare Isotope Beams (FRIB) at Michigan State University (MSU) has several segments. Following the acceleration through the three superconducting LINAC segments, the heavy ion beam is guided through the target, a fragment pre-separator and (the A1900) separator segments. There are many beam lines and then it can be split and sent to various experimental vaults and instrumentation, e.g. S800 spectrograph, and the newly proposed High Rigidity Spectrometer (HRS). Presently, superconducting magnets at the target and fragment pre-separator segments, along with the LINAC superconducting cryo-modules, are supported by FRIB’s main central helium liquefier/refrigerator (CHL). The remainder of the cryogenic loads are supported by the legacy NSCL Cryogenic Refrigerator (a re-commissioned Bureau of Mines helium liquefier from the mid 1970’s) and has many obsolete components for reliable operation. Considering the operational reliability of the accelerator, maintainability of the entire cryogenic system at FRIB and ever-growing experimental beam lines – it is logical to segregate the experimental system loads from the accelerator system loads. A new 4.5 K refrigerator along with a thermal shield (55 K) refrigerator are planned to support the operation of these experimental system (ES) loads and make plans for the CHL maintenance. These refrigerators will be able to support a combination of 4.5 K isothermal refrigeration, 4.5 K liquefaction (for magnet lead cooling and transients) and thermal radiation shield loads. The design loads, modes of operation and the planned operation of the FRIB cryogenic system with these refrigeration systems are discussed. This paper outlines the key selection parameters and design modes for the major components, such as the warm compressors, turbo-expanders and heat exchangers.

Development of a low-pressure Multi-Mesh THGEM detector for fission experiments at FRIB

A small-area imaging detector prototype for position measurement of fission fragments produced in low energy heavy-ion reactions is presented in this study. The detector readout is equipped with a 2-dimensional, position-sensitive gaseous avalanche readout based on the novel Multi-Mesh Thick-GEM (MM-THGEM), and is coupled to a delay-line board for particle localization. The prototype has an effective area of 10 × 10 cm2 and is operated in isobutane at low pressure (7–10 Torr). We present and discuss a series of systematic evaluation tests performed by irradiating the detector with α-particles and fission fragments emitted by small-rate sources (241Am, 249Cf and 252Cf). Position and time resolutions of about 0.42 mm and 1 ns were achieved, respectively. This work serves as a benchmark for the development of a large-scale array of detectors for experiments with fission and fission-like reaction products at the Facility for Rare Isotope Beams (FRIB).

Technological developments and accelerator improvements for the FRIB beam power ramp-up

The Facility for Rare Isotope Beams (FRIB) began operation with 1 kW beam power for scientific users in May 2022 upon completion of 8 years of project construction. The ramp-up to the ultimate beam power of 400 kW, planned over a 6-year period, will enable the facility to reach its full potential for scientific discovery in isotope science and applications. In December 2023, a record-high beam power of 10.4 kW uranium was delivered to the target. Technological developments and accelerator improvements are being made over the entire facility and are key to completion of the power ramp-up. Major technological developments entail the phased deployment of high-power beam-intercepting systems, including the charge strippers, the charge selection systems, the production target, and the beam dump, along with support systems, including non-conventional utilities (NCU) and remote handling facilities. Major accelerator improvements include renovations to aging legacy systems associated with experimental beam lines and system automation for improved operational efficiency and better machine availability. Experience must be gained to safely handle the increased radiological impacts associated with high beam power; extensive machine studies and advanced beam tuning procedures are needed to minimize uncontrolled beam losses for the desired operating conditions. This paper discusses the technological developments and accelerator improvements with emphasis on major R&D efforts.

Mechanical and process design of the interface to a 20,000 liter liquid helium dewar

A new 20,000-liter (20 kL) liquid helium dewar is being integrated in to the existing cryogenic system at the Facility for Rare Isotope Beams at Michigan State University (MSU-FRIB). This dewar will mainly be used for the helium inventory management at FRIB (preserving helium inventory during unplanned / planned maintenance of the cryogenic system) and also in sharing the capacity to support the various cryogenic refrigeration systems to increase the operational efficiency and availability. It is also designed to interface to future cryogenic system upgrades (i.e., new 4.5 K refrigerators). This dewar has a single large penetration, or ‘neck’, that all the process lines and instrumentation pass through. On top of the ‘neck’ is a vacuum insulated interface box, or ‘neck can’, which houses all the connections between the dewar and the connecting distribution system. Though not generally common, this design approach has been successfully implemented on 5 to 10 kL liquid helium dewars at the Spallation Neutron Source (SNS), Jefferson Lab (JLab), and also at FRIB. It has been found that this approach greatly simplifies the mechanical design, while allowing for multiple process and instrumentation interfaces and still permitting a low heat in-leak. This paper presents an overview of the mechanical and process design of this neck can.

High-Current Capability and Upgrades of the EBIS/T Charge-Breeding System in the Reaccelerator at the Facility for Rare-Isotope Beams

The Reaccelerator (ReA) of the Facility for Rare-Isotope Beams (FRIB) at Michigan State University uses a Beam Cooler/Buncher (BCB) and an Electron-Beam Ion Trap (EBIT) as a charge-breeding injector system. The rare isotopes produced by In-flight Separation are selected by the Advanced Rare Isotope Separator (ARIS) and stopped in a helium gas cell. Long-lived and stable-isotope beams can also be extracted from a Batch-Mode Ion Source (BMIS). The continuous beams transported at low energy to ReA are injected into the BCB. The pulsed beams are then injected into the EBIT, charge bred, ejected, and accelerated by ReA’s LINAC. The EBIT electron current (300 - 600 mA) is a factor that limits its capacity to ∼2×1010 elementary charges, which restricts the maximum EBIT-extracted rates to less than 2×1010 particles per second for light ions. An upgrade of the EBIT electron gun is expected to provide 2 A in current. In parallel, a High-Current Electron-Beam Ion Source (HCEBIS) is being commissioned. The HCEBIS can presently provide an electron current of 2 A. An upgrade will increase the current to 4 A. The implementation of these two upgrades is expected to allow for maximum rates to be ∼1011 pps, compatible with FRIB projected rates and user demands. We review the high-current capabilities and upgrades of ReA’s charge-breeding system.

Status of the High-Current Electron-Beam Ion Source Charge Breeder for the Facility for Rare-Isotope Beams

The Reaccelerator (ReA) of the Facility for Rare-Isotope Beams (FRIB) employs an Electron-Beam Ion Trap (EBIT) as a charge breeder to reaccelerate rare-isotope beams up to 12 MeV/u. The ReA EBIT produces an electron current of 300 – 600 mA. The maximum trap capacity of the ReA EBIT is 1010 elementary charges. FRIB production rates are expected to exceed 1010 particles/s in some cases in the future. There is also a user demand for reaccelerated stable-isotope beams of more than 1010 pps. To handle these rates and provide redundancy, a High Current Electron-Beam Ion Source (HCEBIS) has been built and is now being commissioned. An electron-beam current of 2 A with a 50 % duty cycle has been transported through a 4-T field. An upcoming upgrade to increase the electron-beam current up to 4 A will allow for a maximum trap capacity of 2.4×1011 elementary charges. We present the status of the HCEBIS, including the results of the electron-beam commissioning and systematic studies.

The first cooldown of SCL3 cryogenic system

RAON, Rare isotope Accelerator complex for ON-line experiments, is the first superconducting linear accelerators in S. Korea. It will have three linear accelerators (Linac), SCL1, SCL2, and SCL3. Now, construction of the SCL3, the third superconducting Linac was finished in the middle of 2022 and the commissioning of its cryogenic system was done July, 2022. The first cooldown of the Linac with the cryogenic system was started from September, 2022 and their temperature was reached at 2.05 K in January, 2023. The first cooldown was successfully completed and the static and dynamic heat loads of the Linac were measured. This paper shows the results of the first cooldown and the heat load tests.

Parallel-plate avalanche counters for heavy-ion beam tracking: History and mysteries

Despite being an old detector concept, position-sensitive parallel-plate avalanche counters (PPACs) remain widely used today for heavy-ion position and timing measurements. In modern rare isotope beam facilities and large-acceptance fragment separators, PPACs are used to characterize beam properties (diagnostics), facilitate beam delivery (tuning), and provide event-by-event beam tracking for particle identification (PID). Most popular particle localization methods in PPAC detectors are based on strip electrodes electrically connected to resistive-chain circuits or delay lines. More exotic systems include optical readouts based on recording electroluminescence light with high-granularity photodetector arrays or high-resolution resistive anode electrodes. PPACs with conventional resistive-chain or delay-line readouts achieve typical position and time resolutions of below 1 mm (σ) and around 150 ps (σ), respectively. In addition, delay-line systems are capable of counting rates above several hundred kHz for beam areas of a few millimeters square, and around 1 MHz for larger beam sizes. Resistive-chain readouts have limited rates of a few tens of kHz. A review of the operation principles and performance of PPAC detectors is presented in this paper. We will discuss decades-long experience building and operating PPACs developed at the National Superconducting Cyclotron Laboratory, and then refined at the Facility for Rare Isotope Beams (FRIB), mostly focusing on the delay-line readout technique (DLPPAC). We will also discuss problems that arise due to electric discharges at high rates and briefly describe ongoing developments at FRIB. Published by the American Physical Society 2024

Proton Shell Gaps in N=28 Nuclei from the First Complete Spectroscopy Study with FRIB Decay Station Initiator.

The first complete measurement of the β-decay strength distribution of _{17}^{45}Cl_{28} was performed at the Facility for Rare Isotope Beams (FRIB) with the FRIB Decay Station Initiator during the second FRIB experiment. The measurement involved the detection of neutrons and γ rays in two focal planes of the FRIB Decay Station Initiator in a single experiment for the first time. This enabled an analytical consistency in extracting the β-decay strength distribution over the large range of excitation energies, including neutron unbound states. We observe a rapid increase in the β-decay strength distribution above the neutron separation energy in _{18}^{45}Ar_{27}. This was interpreted to be caused by the transitioning of neutrons into protons excited across the Z=20 shell gap. The SDPF-MU interaction with reduced shell gap best reproduced the data. The measurement demonstrates a new approach that is sensitive to the proton shell gap in neutron rich nuclei according to SDPF-MU calculations.

Precision Mass Measurement of the Proton Dripline Halo Candidate ^{22}Al.

We report the first mass measurement of the proton-halo candidate ^{22}Al performed with the low energy beam ion trap facility's 9.4T Penning trap mass spectrometer at facility for rare isotope beams. This measurement completes the mass information for the lightest remaining proton-dripline nucleus achievable with Penning traps. ^{22}Al has been the subject of recent interest regarding a possible halo structure from the observation of an exceptionally large isospin asymmetry [J. Lee et al., Large isospin asymmetry in Si22/O22 Mirror Gamow-Teller transitions reveals the halo structure of ^{22}Al, Phys. Rev. Lett. 125, 192503 (2020).PRLTAO0031-900710.1103/PhysRevLett.125.192503]. The measured mass excess value of ME=18 092.5(3) keV, corresponding to an exceptionally small proton separation energy of S_{p}=100.4(8) keV, is compatible with the suggested halo structure. Our result agrees well with predictions from sd-shell USD Hamiltonians. While USD Hamiltonians predict deformation in the ^{22}Al ground state with minimal 1s_{1/2} occupation in the proton shell, a particle-plus-rotor model in the continuum suggests that a proton halo could form at large quadrupole deformation. These results emphasize the need for a charge radius measurement to conclusively determine the halo nature.

Rf chopper for prebunched radioactive ion beams

An rf chopper system is being designed for the ReAccelerator (ReA) linac at the Facility for Rare Isotope Beams at Michigan State University. The 80.5 MHz ReA radio-frequency quadrupole accelerates prebunched 16.1 MHz beams, producing four satellite bunches for every main bunch. The chopper system includes an rf deflector that kicks every bunch vertically to spatially separate main and satellite bunches. A constant magnetic field superimposed with the chopper electric field biases the beam trajectory to ensure the high-intensity bunches do not experience a net deflection and are injected straight to the ReA6 cryomodule or sent for experiments. The kicked bunches are low in intensity and will be sent to a beam dump, resulting in a clean 16.1 MHz beam structure, which allows for a reliable time-of-flight separation of the isotopes. Published by the American Physical Society 2024

Observation of New Isotopes in the Fragmentation of ^{198}Pt at FRIB.

Five previously unknown isotopes (^{182,183}Tm, ^{186,187}Yb, ^{190}Lu) were produced, separated, and identified for the first time at the Facility for Rare Isotope Beams (FRIB) using the Advanced Rare Isotope Separator (ARIS). The new isotopes were formed through the interaction of a ^{198}Pt beam with a carbon target at an energy of 186 MeV/u and with a primary beam power of 1.5kW. Event-by-event particle identification of A, Z, and q for the reaction products was performed by combining measurements of the energy loss, time of flight, magnetic rigidity Bρ, and total kinetic energy. The ARIS separator has a novel two-stage design with high resolving power to strongly suppress contaminant beams. This successful new isotope search was performed less than one year after FRIB operations began and demonstrates the discovery potential of the facility which will ultimately provide 400kW of primary beam power.

Accelerator and beam physics challenges in support of FRIB experiments

The Facility for Rare Isotope Beams (FRIB), a major nuclear physics facility for research with fast, stopped and reaccelerated rare isotope beams, started operation in May 2022. Since then, a dozen nuclear physics experiments have been successfully accomplished. Typically, the experiments with rare isotope beams last a week or two. Each experiment requires a different primary beam species and energies. Shortening the accelerator and fragment separator setup time is critical to meet the demands of the FRIB Users community. Currently, the primary focus in the linac is reducing the accelerator setup time and beam power ramp-up. Many physics applications have been developed and used to set up the accelerator and beamlines. The simultaneous acceleration of multiple charge states of heavy ion beams is routinely used to minimize the beam power deposition on the charge selector slits after the stripper. This paper discusses the challenges of linac tune development for the acceleration of various ion species.

Pre-experiment of 70 MeV H - cyclotron for producing ISOL RI beam.

The Rare Isotope Science Project (RISP) is currently constructing equipment and facilities for the Rare Isotope Accelerator complex for ON-line experiments (RAON). The first experiment being conducted involves the acceleration of a proton to 70MeV using a cyclotron, which is then delivered to a SiC target to generate a radioactive isotope beam in the ISOL system. However, before conducting this experiment, a preliminary experiment was performed to confirm the exact location and shape of the proton beam to prevent loss of the proton beam. The pre-experiment involved configuring a faraday cup, wire grid scanner, collimator, and slit inside the proton beam diagnostic module to understand the characteristics of the proton beam at the target position. The beam current ranged from 1 μA to 1.5 μA, and the beam size was confirmed to be within the 2×2cm 2 slit size.

Quantification and purification of isotopic contamination at the ReAccelerator of the Facility for Rare Isotope Beams.

At the ReAccelerator within the Facility for Rare Isotope Beams, a combination of an interchangeable aluminum foil and a silicon detector was developed to quantify isobaric contamination in rare isotope beams. The device is simple to operate and is now used routinely. In this article, we describe the system and show an application of the device to determine the level of contamination of an Si-32 rare isotope beam by stable S-32. In addition, we describe how the new diagnostic device helped confirm an enhancement of the beam purity prior to beam delivery to experiments.

Applications of Machine Learning and Neural Networks for FT-ICR Mass Measurements with SIPT

The single-ion Penning trap (SIPT) at the Low-Energy Beam Ion Trapping Facility has been developed to perform precision Penning trap mass measurements of single ions, ideal for the study of exotic nuclei available only at low rates at the Facility for Rare Isotope Beams (FRIB). Single-ion signals are very weak—especially if the ion is singly charged—and the few meaningful ion signals must be disentangled from an often larger noise background. A useful approach for simulating Fourier transform ion cyclotron resonance signals is outlined and shown to be equivalent to the established yet computationally intense method. Applications of supervised machine learning algorithms for classifying background signals are discussed, and their accuracies are shown to be ≈65% for the weakest signals of interest to SIPT. Additionally, a deep neural network capable of accurately predicting important characteristics of the ions observed by their image charge signal is discussed. Signal classification on an experimental noise dataset was shown to have a false-positive classification rate of 10.5%, and 3.5% following additional filtering. The application of the deep neural network to an experimental 85Rb+ dataset is presented, suggesting that SIPT is sensitive to single-ion signals. Lastly, the implications for future experiments are discussed.