Radiation Yield Research Articles

Simulation of the generation of the characteristic X-ray emission by hot electrons in a foil

We have developed a model to calculate the yield of the characteristic X-ray radiation from a foil, taking into account the dependence of the average energy and the number of hot electrons on the intensity of the laser pulse, the self-absorption of X-rays and the effect of refluxing of hot electrons. The yield of Kα radiation from a silver foil is optimised at relativistic intensities. A method is proposed for diagnosing the effect of electron refluxing, which greatly increases the yield of Kα radiation.

Increasing the K-shell yield of line radiation in Z-pinch implosions using alloyed Al/Mg wire-arrays

The variation of the K-shell yield of pure aluminum wire-array Z-pinch implosions with load parameters is discussed. The mechanism and the efficiency of increasing the K-shell yield using alloyed Al/Mg wire-arrays are numerically investigated. It has been shown that the maximum K-shell yield from a pure aluminum wire-array Z-pinch implosion can be obtained at an optimal load mass for a given generator and at a fixed initial wire-array radius. This optimal load mass is determined by the load energy coupling with the generator, the capability of Z-pinch plasmas to emit the K-shell radiation, and the self absorption of K-shell lines. For different generators, the optimal load mass increases as the drive current increases, and the line absorption limits the further increase of K-shell radiation. The coupled energy per ion is likely decreasing with increased mass, so the plasma might not be able to ionize into the K-shell. Also, the ability of the plasma to radiatively cool can increase with mass, thus, making it difficult for the plasma to ionize into and remain in the K-shell during the stagnation phase of the implosion. Alloyed Al/Mg wire-arrays were thus suggested to be used to decrease the opacity of K-shell lines and to increase the overall K-shell yield. In this paper, we show that using alloyed Al/Mg wire-arrays will decrease the opacity and increase the K-shell yield remarkably if the plasma is optically thick. We will also show that the efficiency of increasing the K-shell yield with alloyed Al/Mg wire-arrays cannot increase indefinitely. The ratio of K-shell yield from an alloyed Al/Mg wire-array to that from a pure aluminum wire-array reaches a limit. For example, we show that when the mass share of magnesium is 10% then this limit is 1.2, and for a 50% mass share, the limit is 1.3.

Characteristics of implosion and radiation for aluminum planar wire array z-pinch at 1.5 MA

Planar wire arrays Z pinches were carried out on Qiangguang generator (1.5 MA, 100 ns). Loads with varied row widths (6–24 mm) and wire numbers (10–34) were employed in the experiments. The implosion dynamics of planar wire arrays has been studied. Meanwhile, the changes of the implosion time, radiation yield and power with array mass, inter-wire gap, and array width were investigated. The images of a soft X-ray camera exhibit that the trailing mass, precursor column, and R-T instability exist during the implosion phase, and when m = 0 maybe accompanied with m = 1, instability will rapidly develop after stagnation. The implosion trajectories show that loads will implode by the snowplow mode and about 50% of total initial array mass will participate in the final implosion. The maximum total X-ray energy is 22 kJ with a power of 630 GW, while the maximum K-shell yield is 3.9 kJ with a power of 158 GW. Experiments with different planar wire arrays show that the value of mPD02 (the product of line mass and squared width) is the critical factor which affects the implosion time and the X-ray products of the wire arrays. The optimum value of mPD02 should be in the range of 200–400 μgcm and the inter-wire gap should be less than 1 mm.

Experimental characterization of bi-directional terahertz emission from gold-coated nanogratings

The THz radiation emission of Au-coated nanogratings (fused silica substrate, 30 nm Au layer thickness, 500 nm grating constant) upon fs laser irradiation (785 nm, 150 fs, 1 kHz, ≤1 mJ/pulse) is observed in both directions along the laser beam axis (forward and backward) and for both, illumination of the Au/air or the Au/silica interface. THz radiation along the laser beam propagation is emitted in a narrow solid angle of about 15° fwhm independent on the laser pulse fluence, the angle of incidence and the nanograting profile. The bar width and groove depth of the nanograting as well as the angle of laser beam incidence strongly affect the THz radiation yield. The energy of single THz light pulses is measured absolutely (2 fJ in the 0.3–0.38 THz range) using a highly sensitive and fast superconducting transition edge sensor. The bi-directional emission of THz radiation is in agreement with the model assumption of surface plasmon polaritons propagating simultaneously on both Au layer interfaces (Au/air and Au/silica).

Off-Axis Phase-Matched Terahertz Emission from Two-Color Laser-Induced Plasma Filaments

We observe off-axis phase-matched terahertz generation in long air-plasma filaments produced by femtosecond two-color laser focusing. Here, phase matching naturally occurs due to off-axis constructive interference between locally generated terahertz waves, and this determines the far-field terahertz radiation profiles and yields. For a filament longer than the characteristic two-color dephasing length, it emits conical terahertz radiation in the off-axis direction, peaked at 4-7° depending on the radiation frequencies. The total terahertz yield continuously increases with the filament length, well beyond the dephasing length. The phase-matching condition observed here provides a simple method for scalable terahertz generation in elongated plasmas.

Study of the radiation spectra of fast Z-pinches formed during the implosion of wire arrays in the Angara-5-1 facility

Results are presented from measurements of the radiation spectra of the Z-pinch tungsten plasma produced during the implosion of cylindrical wire arrays with a linear mass of 200–400 μg/cm and an initial diameter of 12–20 mm at a current of ∼3 MA in the experiments performed at the Angara-5-1 facility. The radiation spectra in the photon energy range of 50–900 eV were recorded on a UF-4 X-ray film by using a spectrograph with a transmission grating. The radiation spectrum in the photon energy range of 1–3 keV was recorded using a crystalline panoramic spectrograph. A curtain shutter was used to protect the transmission grating from fast microparticles produced due to the erosion of high-voltage electrodes. The total radiation yield was measured with a thermocouple calorimeter. It is shown that most of the tungsten plasma radiation energy is emitted in the photon energy range of 80–300 eV. Measurements of the spectral intensity of pinch radiation with a spatial resolution along the pinch radius showed that the effective transverse diameter of the pinch did not exceed 2 mm, which agrees with independent current measurements of the pinch size. The results of measurements of the spectral intensity of pinch radiation were compared with calculations per-formed under the assumption of a stationary homogeneous plasma.

The influence of crystallinity on radiation stability of UHMWPE

The influence of ionizing radiation on ultra high molecular weight polyethylene (UHMWPE) was studied using EPR spectroscopy and GC. Two samples of various degree of crystallinity, 85% and 53%, were investigated upon exposure to electron beam. In this study it was found that radicals generated following irradiation decay much faster in amorphous than in crystalline phase. The primary product generated in both phases is second ordered alkyl radical. EPR spectra detected for the sample containing 85% crystalline regions revealed a quintet of hyperfine splitting about 2.28mT and the signal was tentatively assigned to the product of β-fragmentation. The radiation yield of hydrogen for two studied samples of various crystallinity was similar.

Application of a mode-locked fiber laser for highly time resolved broadband absorption spectroscopy and laser-assisted breakdown on micro-plasmas

Absorption spectroscopy is known to be a powerful tool to gain spatially and temporally resolved information on excited and reactive species in a plasma discharge. Furthermore, the interaction of the discharge with short intense laser pulses can trigger the ignition and the transition into other transient states of the plasma. In this context laser-assisted ‘pump-probe’ experiments involving simultaneously generated supercontinuum radiation yield highly temporally resolved and spatially well-defined information on the transient phenomena. In this paper we demonstrate the possibility for ‘pump–probe’ experiments by initiating breakdown on a picosecond time scale (‘pump’) with a high-power beam and measuring the broadband absorption with the simultaneously provided supercontinuum (‘probe’). Since both pulses are generated from the same mode-locked master oscillator, they have a strong level of synchronization.

Coherent X-ray radiation generated by a relativistic electron in an artificial periodic structure

A theory of coherent X-ray radiation from a relativistic electron crossing an artificial periodic layered structure in the Laue scattering geometry is constructed. The expressions describing the spectral-angular radiation parameters are obtained. It is shown that the radiation yield in such a medium may substantially exceed the radiation yield in a crystal under analogous conditions.

Diffracted transition radiation of relativistic electrons in an artificial periodic structure

A theory concerning the coherent X-ray radiation of relativistic electrons crossing an artificial periodic medium in Laue scattering geometry has been constructed. Expressions describing the spectralangular characteristics of radiation in the Bragg scattering direction have been obtained and studied. Radiation is considered in analogy with that in the crystal medium as a result of the coherent summation of the contributions of two radiation mechanisms, in particular, parametric X-ray radiation (PXR) and diffracted transition radiation (DTR). It is shown that the DTR yield from a layered target can exceed the particle radiation yield in a single-crystal radiator by one order or more under similar conditions.

Spectroscopic analysis of Cu wire array implosions on the refurbished Z generator

Experimental investigations of pinches on the refurbished Z (ZR) generator using Cu arrays have been initiated and more are planned for the near future. Significant X-ray emissions in the K-shell from moderately high atomic number plasmas such as Cu generate extreme interest. However, the production of these hard photons from high Z materials comes with a price. There is substantial loss of radiative yield due to stripping through many electrons present in high Z materials to reach to the H- or He-like ionization stages. Production of hard X-rays for materials with atomic number higher than Cu such as Kr is very difficult and theoretical predictions are even more uncertain. Previous experimental efforts using Cu as a plasma pinch load are encouraging and promote further investigations of this element on the refurbished Z machine for achieving photon energies higher than 5 keV and obtaining sufficient radiative yield. We will analyze the ionization dynamics and generate Cu spectrum using the temperature and density conditions obtained from 1-D non-LTE radiation hydrodynamics simulations of Cu wire array implosions on ZR. These results will be compared with K- and L-shell experimental spectrum of shot Z 1975. Theoretical K- and L-shell spectroscopy provides validation of atomic and plasma modeling when compared to available experimental data and also provides useful diagnostics for the plasma parameters. Our self-consistently generated non-LTE collisional-radiative model employs an extensive atomic level structure and data for all dominant atomic processes that are necessary to model accurately the pinch dynamics and the spectroscopic details of the emitted radiation.

Spontaneous emission control of single quantum dots in bottom-up nanowire waveguides

Nanowire waveguides with controlled shape are promising for engineering the collection efficiency of quantum light sources. We investigate the exciton lifetime in individual InAsP quantum dots, perfectly positioned on-axis of InP nanowire waveguides. We demonstrate control over the quantum dot spontaneous emission by varying the nanowire diameter in e-beam patterned arrays, which modifies the coupling efficiency of the emitter to the fundamental waveguide mode. The spontaneous emission rate is inhibited by a factor of 12 in thin nanowires compared to nanowires with optimized waveguide diameter. From the measured inhibition factor, we determine a high radiative yield exceeding 92% in bottom-up grown nanowires.

Optical characterization of Er3+and Yb3+ co-doped barium fluorotellurite glass

Spectroscopic studies of Er3+/Yb3+ co-doped (Ba,La)-fluorotellurite glass composition have been carried out using standard experimental and theoretical methods. Quantitative analyses of the room temperature absorption and emission spectra as well as the emission lifetimes yield various important spectroscopic parameters such as the radiative decay rates, fluorescence branching ratios, and emission/absorption cross sections. In addition, internal radiative quantum yields have been determined for the infrared emission at 1571nm and for the upconversion emission at 547nm. The influence of various non-radiative properties such as multiphonon relaxation, concentration quenching, and quenching by hydroxyl radicals have also been quantitatively estimated and correlated with the observed spectral properties. The comparative studies with the other composition of tellurite and different glasses showed that present glass composition could be a potential candidate for the broadband amplifier.

STRATEGIES FOR THE OPTIMUM SEPARATION OF GAMMA RADIOLYTIC DEGRADATION PRODUCTS OF METHOXYCHLOR USING RP-HPLC

Different types of reversed phase (RP) columns have been incorporated for the separation of gamma radiolytic degradation products (DPs) of methoxychlor. The effect of carbon chain length, carbon content, surface area, pore size, pore volume, and column dimensions of RP columns on DPs separation has also been investigated. The separation of DPs has been optimized employing methanol-water mobile phase and UV-DAD. In methanol media two major and five minor DPs were detected in gamma irradiated MXC by RP-HPLC. The peaks eluting before the parent peak on reversed phase column are expected to be relatively polar compounds while peaks after MXC are assumed to be non-polar in nature corresponding to general RP behavior. From HPLC analysis it is inferred that at gamma radiation dose of 5 kGy ≥95% MXC has been degraded for a dose rate of 200 Gyh−1. The chemical radiation yield (G-value) along with effect of MXC concentration on degradation has also been explored. The physico-chemical parameters of RP columns have been compared under the optimum separation conditions. It may be concluded that HPLC is an excellent tool to investigate radiolytic degradation of persistent organic pollutants.

A study on size effect of carboxymethyl starch nanogel crosslinked by electron beam radiation

The formation of carboxymethyl starch (CMS) nanogel with 50nm less particle size was carried out through a radiation crosslinked process on the electron beam (EB) linear accelerator. Changes of intrinsic viscosities and weight averaged molecular weight in the CMS concentration, which ranged from 3 to 10mgml−1 in absorbed doses were investigated. There were some new peaks in the 1H NMR spectra of CMS nanogel compared with those of CMS polymer. These results were anticipated that the predominant intramolecular crosslinking of dilute CMS aqueous solution occurred while being exposed to a short intense pulse of ionizing radiation. Hydrodynamic radius (often called particle size, Rh) and distribution of particle size were measured by a dynamic light scattering technique. The radiation yield of intermolecular crosslinking of CMS solution was calculated from the expression of Gx (Charlesby, 1960; Jung-Chul, 2010). The influence of the “size effect” was demonstrated by testing culture of Lactobacillus bacteria on MRS agar culture medium containing CMS nanogel and polymer. Results showed that the number of Lactobacillus bacteria growing on nanogel containing culture medium is about 170cfu/ml and on polymer containing culture medium is only 6cfu/ml.

Doping Location-Dependent Energy Transfer Dynamics in Mn-Doped CdS/ZnS Nanocrystals

Dynamics of energy transfer and charge carrier localization in Mn-doped CdS/ZnS core/shell nanocrystals correlated with doping location and concentration are studied via transient absorption measurement of exciton relaxation dynamics. The strong dependence of exciton-Mn energy transfer rate on doping location was directly resolved in the transient bleach recovery and electron intraband absorption data by using layer-by-layer synthesized Mn-doped nanocrystals. With 1.2 nm decrease in doping radius in the ZnS shell, energy transfer rate increases by 6 fold. We identified that hole trapping is the major competing process that inhibits the energy transfer in Mn-doped CdS/ZnS nanocrystals. From the branching ratio of the energy transfer and hole trapping, combined with luminescence quantum yield measurement, we also obtained doping location-dependent radiative relaxation quantum yield of Mn(2+) ions that is as high as 0.95.

Directly suspended droplet microextraction combined with energy-dispersive X-ray fluorescence spectrometry to determine nano levels of phosphate in surface water

Directly suspended droplet microextraction (DSDME) for determination of phosphate by energy-dispersive X-ray fluorescence spectrometry (EDXRF) is proposed. The method is based on the determination of phosphate, through molybdenum in the phosphomolybdenum blue complex. Because phosphorus is determined indirectly via molybdenum fluorescent radiation the difficulties of low fluorescent yield and low energy of phosphorus radiation are successfully overcome. A good ratio of phosphorus to molybdenum (1 to 37) and a sensitive Kα line of molybdenum give the possibility to determine a low concentration of phosphorus. Under the optimized conditions, good linearity, up to 20 μg of phosphorus (r = 0.9995), and the detection limit (2.8 ng mL−1) for the sample of 1.5 mL were achieved. The total RSD for the EDXRF determination of phosphorus followed by DSDME was 2.6% and taking into account all steps preceding the determination and the uncertainty of EDXRF measurements, the proposed method can be recognized as highly precise. The enrichment factor was equal to 56.8. The developed method was used to determine the total phosphorus content in surface waters. The accuracy and repeatability of the proposed procedure were checked by the standard addition method. The recovery in the range 93.5–97% was satisfactory and indicated the usefulness of the developed procedure.

Effect of Irrigation to Winter Wheat on the Radiation Use Efficiency and Yield of Summer Maize in a Double Cropping System

In north China, double cropping of winter wheat and summer maize is a widely adopted agricultural practice, and irrigation is required to obtain a high yield from winter wheat, which results in rapid aquifer depletion. In this experiment conducted in 2001-2002, 2002-2003, and 2004-2005, we studied the effects of irrigation regimes during specific winter wheat growing stage with winter wheat and summer maize double cropping systems; we measured soil moisture before sowing (SMBS), the photosynthetic active radiation (PAR) capture ratio, grain yield, and the radiation use efficiency (RUE) of summer maize. During the winter wheat growing season, irrigation was applied at the jointing, heading, or milking stage, respectively. The results showed that increased amounts of irrigation and irrigation later in the winter wheat growing season improved SMBS for summer maize. The PAR capture ratio significantly (LSD, P < 0.05) increased with increased SMBS, primarily in the 3 spikes leaves. With improved SMBS, both the grain yield and RUE increased in all the treatments. These results indicate that winter wheat should be irrigated in later stages to achieve reasonable grain yield for both crops.

Preparation of inorganic crystalline compounds induced by ionizing, UV and laser radiations

Results on preparation of nickel, zinc, yttrium, aluminum and cobalt oxides, zinc peroxide and hydroxide, yttrium and lutetium aluminum garnets and cobalt(II) aluminate via irradiation of aqueous solutions containing soluble metal salts and radical scavengers (formate anion or propan-2-ol) are summarized in this paper. Various physico-chemical and structural properties of prepared compounds (e.g. crystallinity, specific surface area, particle size) are also reported.All used variants of radiation method are rather convenient and simple, and yield nano-scale powder materials with interesting characteristics. Prepared materials generally have high chemical purity, high specific surface area and narrow distribution of particle size (ranging in tens of nm).Generally, accelerated electrons, gamma, and UV radiation yield materials with comparable properties and structural characteristics, but UV-radiation seems to be the most convenient for preparation of intricate compounds such as synthetic garnets and spinels, while ionizing radiation is better for preparation of compounds doped with foreign ions.Among discussed compounds, only zinc oxide, peroxide and hydroxide were prepared directly via irradiation. For preparation of other crystalline oxidic compounds, mild heat treatment of amorphous or weakly crystalline solid phase was necessary.

Radiation Yield and Radicals Produced in Irradiated Poly (Butylene Succinate)

Normal 0 false false false EN-US X-NONE X-NONE MicrosoftInternetExplorer4 The main chemical effects of ionizing irradiation on polymers are crosslinking and chain scission. Both processes occur simultaneously and their yields determine the final results of processing. The radiation yield of crosslinking could be determined by several methods depending on the characteristics of the material and properties of the gel. Radiation parameters of gelation, such as gelation dose and ratio of scission yield to crosslinking yield, as well as their values were estimated. In this study, those parameters depend on the amount of Trimethallyl isocyanurate (TMAIC) in Poly(butylene succinate) (PBS), molecular weight of PBS, and irradiation condition. In the absence of TMAIC, higher molecular weight of PBS required less energy to start gelation process compare to lower molecular weight of PBS. While in the presence of TMAIC all of the PBS samples require similar energy to start gelation process. The existence of macroradicals were observed by Electron Spin Resonance measurements. The result showed that the spectra consisted of signals derived from radicals on carbon nearby carbonyl, and signals derived from radicals on carbon reside between two similar carbon on polymer, both of radicals lead to crosslinking.