Applications In Quantum Optics Research Articles

Pancharatnam phase control of atomic ensembles based on quantum memory effects in photonic cavities

In this paper, we explore the manipulation and control of the Pancharatnam phase in atomic ensembles through the utilization of quantum memory effects. By analyzing the time evolution of the excited state population of [Formula: see text]-atoms within a single photonic cavity, we gain insights into the behavior and manipulation of this phase. Numerical simulations of the system exact solution yield density plots illustrating the time evolution of the excited state population and Pancharatnam phase. Our findings demonstrate the potential to control the system dynamics using the Pancharatnam phase in atomic ensembles through quantum memory effects. The observed behaviors and characteristics contribute to our understanding of quantum systems and hold promise for crucial applications in quantum information processing and communication. These results provide valuable insights into the fundamental aspects of the Pancharatnam phase and its control, paving the way for further investigations and applications in quantum optics and information science.

Tunable GaAsxP1-x Quantum-Dot Emission in Wurtzite GaP Nanowires.

We present a fairly understudied material system suitable for the realization of tunable quantum-dot (QD) emission within the visible-to-near-infrared spectrum (in particular, in the 650-720 nm wavelength range). Specifically, crystal-pure wurtzite gallium phosphide (GaP) nanowires (NWs) are synthesized, incorporating single gallium arsenide phosphide (GaAsxP1-x) QDs of various compositions. Detailed growth procedures are outlined, accompanied by an analysis of the synthesis challenges encountered during the realization of these nanostructures and the strategies to solve them. Notably, a great degree of control over the shape and composition of the ternary alloy QD is achieved, enabling a well-defined confinement and the tunability of the emission wavelength. This is confirmed by low-temperature microphotoluminescence (μ-PL) investigation showing that the NW emission is dominated by a narrow peak whose energy shifts according to the As content of the QD: from ∼650 nm (As = 70%) to ∼720 nm (As = 90%). Moreover, a localized and efficient carrier recombination mechanism is found by single-NW μ-PL mapping, confirming that this emission arises from the QD. Finally, a power and temperature μ-PL study is presented and used to characterize the QD excitonic properties and the nature of the involved energy levels. Our findings underscore the potential for these QDs in NWs with tailored compositions to achieve the desired light emission characteristics, thereby advancing applications in quantum optics and nanophotonics.

Universal analyzer for measuring the orbital angular momentum spectrum of a randomly fluctuated beam.

The orbital angular momentum (OAM) of beams provides an additional degree of freedom and has been applied in various scientific and technological fields. Accurate and quantitative measurement of intensity distributions across different OAM modes, referred to as the OAM spectrum of a beam, is crucial. Here, we propose a straightforward and efficient experimental setup for measuring the OAM spectrum of a randomly fluctuating beam. By employing a modal decomposition analyzer, a randomly fluctuating light field can be decomposed into an incoherent superposition of a series of modes, followed by a coordinate transformation to calculate the OAM spectrum. This method is suitable for measuring the OAM spectrum of partially coherent beams and superposition of vortex beams. The experimental results are in good agreement with the theoretical predictions. Precise measurement of the OAM spectrum is critical for various applications in optical communications, quantum optics, and digital imaging.

Sympathetic Mechanism for Vibrational Condensation Enabled by Polariton Optomechanical Interaction.

We demonstrate a macrocoherent regime in exciton-polariton systems, where nonequilibrium polariton Bose-Einstein condensation coexists with macroscopically occupied vibrational states. Strong exciton-vibration coupling induces an effective optomechanical interaction between cavity polaritons and vibrational degrees of freedom of molecules, leading to vibrational amplification in a resonant blue-detuned configuration. This interaction provides a sympathetic mechanism to achieve vibrational condensation with potential applications in cavity-controlled chemistry, nonlinear, and quantum optics.

Vortex bifocusing of extreme ultraviolet using modified Fermat-spiral photon-sieve splitter.

Structured beams carrying orbital angular momentum (OAM) provide powerful capabilities for applications in optical tweezers, super-resolution imaging, quantum optics, and ad-vanced microparticle manipulation. However, it is challenging for generate and control the OAM beams at the extreme ultraviolet (EUV) region due to the lack of suitable wave front shaping optics arise from being limited to the strong absorption of most materials. Here, we use a modified Fermat-spiral photon-sieve splitter to simultaneously generate two focused doughnut beams with opposite helical phase. Our technique enables us to produce splitting focused vortex beams with different rotation directions at EUV wavelengths. Additionally, we provide experimental evidence showcasing the capabilities of our method and further detect the helical phase by self-reference interferometry. This work not only opens a route for OAM-driven applications in EUV radiation, but also paves the way to studies of holographic technique by EUV splitter.

Wide‐Bandgap RBa3(B3O6)3 (R = Nd, Sm, Tb, Dy, and Er) Single Crystals for Ultraviolet Nonlinear Optics

AbstractDiscovery of new materials with enhanced optical properties in the visible and UV‐C range can impact applications in lasers, nonlinear optics, and quantum optics. Here, the optical floating zone growth of a family of rare earth borates, RBa3(B3O6)3 (R = Nd, Sm, Tb, Dy, and Er), with promising linear and nonlinear optical (NLO) properties is reported. Although previously identified to be centrosymmetric, the X‐ray analysis combined with optical second harmonic generation (SHG) assigns the noncentrosymmetric P space group to these crystals. Characterization of linear optical properties reveals a direct bandgap of ≈5.61–5.72 eV and strong photoluminescence in both the visible and mid‐IR regions. Anisotropic linear and nonlinear optical characterization reveals both Type‐I and Type‐II SHG phase matchability, with the highest effective phase‐matched SHG coefficient of 1.2 pm V−1 at 800‐nm fundamental wavelength (for DyBa3(B3O6)3), comparable to β‐BaB2O4 (phase‐matched d22 ≈ 1.9 pm V−1). Laser‐induced surface damage threshold for these environmentally stable crystals is 650–900 GW cm−2, which is four to five times higher than that of β‐BaB2O4, thus providing an opportunity to pump with significantly higher power to generate about six to seven times stronger SHG light. Since the SHG arises from disorder on the Ba‐site, significantly larger SHG coefficients may be realized by “poling” the crystals to align the Ba displacements. These properties motivate further development of this crystal family for laser and wide bandgap NLO applications.

Virtual reality for understanding artificial-intelligence-driven scientific discovery with an application in quantum optics

Virtual reality for understanding artificial-intelligence-driven scientific discovery with an application in quantum optics

Reaching the efficiency limit of arbitrary polarization transformation with non-orthogonal metasurfaces

Polarization transformation is at the foundation of modern applications in photonics and quantum optics. Notwithstanding their applicative interests, basic theoretical and experimental efforts are still needed to exploit the full potential of polarization optics. Here, we reveal that the coherent superposition of two non-orthogonal eigen-states of Jones matrix can improve drastically the efficiency of arbitrary polarization transformation with respect to classical orthogonal polarization optics. By exploiting metasurface with stacking and twisted configuration, we have implemented a powerful configuration, termed “non-orthogonal metasurfaces”, and have experimentally demonstrated arbitrary input-output polarization modulation reaching nearly 100% transmission efficiency in a broadband and angle-insensitive manner. Additionally, we have proposed a routing methodology to project independent phase holograms with quadruplex circular polarization components. Our results outline a powerful paradigm to achieve extremely efficient polarization optics, and polarization multiplexing for communication and information encryption at microwave and optical frequencies.

The three-dimensional harmonic oscillator and solid harmonics in Bargmann space

The three-dimensional harmonic oscillator is solved in Bargmann space. The treatment is pedagogically more transparent than the standard ones, at the price of introducing the Bargmann transform in the context of the one-dimensional oscillator. The standard solid harmonics are similarly derived with minimal technical effort, amounting to a complete self-contained exposition suitable for introductory courses in quantum mechanics or mathematical methods of physics. It provides an early exposure to wavelets, with important contemporary applications in signal analysis and quantum optics.

Few-mode squeezing in type-I parametric downconversion by complete group velocity matching.

Frequency-degenerate pulsed type-I parametric downconversion is a widely used source of squeezed light for numerous quantum optical applications. However, this source is typically spectrally multimode, and the generated squeezing is distributed between many spectral modes with a limited degree of squeezing per mode. We show that in a nonlinear crystal, where the condition of complete group velocity matching (GVM) for the pump and the signal is satisfied, the number of generated modes may be as low as two or three modes. We illustrate the general theory with the example of the MgO-doped lithium niobate crystal pumped at 775 nm and generating squeezed light at 1.55 µm. Our model includes the derivation of the degree of squeezing from the properties of the pump and the crystal and shows that 12 dB of squeezing can be obtained in a periodically poled crystal ata length of 80 mm.

Second Harmonic Generation of Twisted Vector Vortex Beams Using aβ-BaB2O4 Crystal

In this study, we demonstrate both theoretically and experimentally second harmonic generation (SHG) of a twisted vector vortex optical field (TVVOF) using a nonlinear type-II phase-matched β-BaB2O4 (BBO) crystal. Our study introduces a novel method to manipulate SHG by independently modulating the two orthogonal polarization components of a TVVOF. This flexibility in controlling SHG can be achieved through accurate experimental adjustments of the polarization components. Furthermore, we reveal that the SHG can be dynamically tuned by varying the angle between the polarization direction of the optical field and the principal axis of the BBO crystal via rotation. These findings provide a new approach for the flexible manipulation of SHG in structured vector optical fields, which have potential applications in optical communication, quantum optics, and photonic device engineering.

Circularly Polarized Luminescence Without External Magnetic Fields from Individual CsPbBr3 Perovskite Quantum Dots.

Lead halide perovskite quantum dots (QDs), the latest generation of the colloidal QD family, exhibit outstanding optical properties, which are now exploited as both classical and quantum light sources. Most of their rather exceptional properties are related to the peculiar exciton fine-structure of band-edge states, which can support unique bright triplet excitons. The degeneracy of the bright triplet excitons is lifted with energetic splitting in the order of millielectronvolts, which can be resolved by the photoluminescence (PL) measurements of single QDs at cryogenic temperatures. Each bright exciton fine-structure-state (FSS) exhibits a dominantly linear polarization, in line with several theoretical models based on the sole crystal field, exchange interaction, and shape anisotropy. Here, we show that in addition to a high degree of linear polarization, the individual exciton FSS can exhibit a non-negligible degree of circular polarization even without external magnetic fields by investigating the four Stokes parameters of the exciton fine-structure in individual CsPbBr3 QDs through Stokes polarimetric measurements. We observe a degree of circular polarization up to ∼38%, which could not be detected by using the conventional polarimetric technique. In addition, we found a consistent transition from left- to right-hand circular polarization within the fine-structure triplet manifold, which was observed in magnetic-field-dependent experiments. Our optical investigation provides deeper insights into the nature of the exciton fine structures and thereby drives the yet-incomplete understanding of the unique photophysical properties of this class of QDs for the benefit of future applications in chiral quantum optics.

Multifold enhancement of quantum SNR by using an EMCCD as a photon number resolving device

Electron multiplying charge-coupled devices (EMCCDs), owing to their high quantum efficiency and spatial resolution, are widely used to study typical quantum optical phenomena and related applications. Researchers have already developed a procedure that enables one to statistically determine whether a pixel detects a single photon, based on whether its output is higher or lower than the estimated noise level. However, these techniques are feasible at extremely low photon numbers (≈0.15 mean number of photons per pixel per exposure), allowing for at most one photon per pixel. This limitation necessitates a very large number of frames required for any study. In this work, we present a method to estimate the mean rate of photons per pixel per frame for arbitrary exposure time. Subsequently, we make a statistical estimate of the number of photons (≥ 1) incident on each pixel. This allows us to effectively use the EMCCD as a photon number resolving device. This immediately augments the acceptable light levels in the experiments, leading to significant reduction in the required experimentation time. As evidence of our approach, we quantify contrast in quantum correlation exhibited by a pair of spatially entangled photons generated by a spontaneous parametric down conversion process. In comparison with conventional methods, our method realizes an enhancement in the signal-to-noise ratio (SNR) by approximately a factor of 3 for half the data collection time. This SNR can be easily enhanced by minor modifications in experimental parameters such as exposure time, etc.

Research Progress of Single-Photon Emitters Based on Two-Dimensional Materials.

From quantum communications to quantum computing, single-photon emitters (SPEs) are essential components of numerous quantum technologies. Two-dimensional (2D) materials have especially been found to be highly attractive for the research into nanoscale light-matter interactions. In particular, localized photonic states at their surfaces have attracted great attention due to their enormous potential applications in quantum optics. Recently, SPEs have been achieved in various 2D materials, while the challenges still remain. This paper reviews the recent research progress on these SPEs based on various 2D materials, such as transition metal dichalcogenides (TMDs), hexagonal boron nitride (hBN), and twisted-angle 2D materials. Additionally, we summarized the strategies to create, position, enhance, and tune the emission wavelength of these emitters by introducing external fields into these 2D system. For example, pronounced enhancement of the SPEs' properties can be achieved by coupling with external fields, such as the plasmonic field, and by locating in optical microcavities. Finally, this paper also discusses current challenges and offers perspectives that could further stimulate scientific research in this field. These emitters, due to their unique physical properties and integration potential, are highly appealing for applications in quantum information and communication, as well as other physical and technological fields.

Photon-pair generation using inverse-designed thin-film lithium niobate mode converters

Spontaneous parametric down-conversion (SPDC) has become a key method for generating entangled photon pairs. Periodically poled thin-film lithium niobate (TFLN) waveguides induce strong SPDC but require complex fabrication processes. In this work, we experimentally demonstrate efficient SPDC and second harmonic generation using modal phase matching methods. This is achieved with inverse-designed optical mode converters and low-loss optical waveguides in a single nanofabrication process. Inverse design methods provide enhanced functionalities and compact footprints for the converter. Despite the extensive achievements in inverse-designed photonic integrated circuits, the potential of inverse-designed TFLN quantum photonic devices has been seldom explored. The device shows an on-chip conversion efficiency of 3.95% W−1 cm−2 in second harmonic generation measurements and a coincidence count rate up to 21.2 kHz in SPDC experiments. This work highlights the potential of the inverse-designed TFLN photonic devices and paves the way for their applications in on-chip nonlinear or quantum optics.

Coherent radiation at visible wavelengths from sub-keV electron beams.

The Smith-Purcell effect allows for coherent free-electron-driven compact light sources over the entire electromagnetic spectrum. Intriguing interaction regimes, with prospects for quantum optical applications, are expected when the driving free electron enters the sub-keV range, though this has until now remained an experimental challenge. Here, we demonstrate the Smith-Purcell light emission from UV to visible using engineerable, fabricated gratings with periodicities as low as 19 nm and with electron energies as low as 300 eV. Our findings constitute a major step toward broadband, highly tunable, on-chip light sources, observation of quantum recoil effects, and tunable EUV and x ray sources from swift electrons.

Photon number resolving detection with a single-photon detector and adaptive storage loop

Photon number resolving (PNR) measurements are beneficial or even necessary for many applications in quantum optics. Unfortunately, PNR detectors are usually large, slow, expensive, and difficult to operate. However, if the input signal is multiplexed, photon ‘click’ detectors, that lack an intrinsic PNR capability, can still be used to realize photon number resolution. Here, we investigate the operation of a single click detector, together with a storage line with tunable outcoupling. Using adaptive feedback to adjust the storage outcoupling rate, the dynamic range of the detector can in certain situations be extended by up to an order of magnitude relative to a purely passive setup. An adaptive approach can thus allow for photon number variance below the quantum shot noise limit under a wider range of conditions than using a passive multiplexing approach. This can enable applications in quantum enhanced metrology and quantum computing.

Near-resonant light scattering by an atom in a state-dependent trap

Abstract There are an increasing number of experimental scenarios where near-resonant light is applied to atoms tightly trapped in far off-resonant optical fields, such as for quantum optics applications or for atom imaging. Oftentimes, the electronic ground and excited states involved in the optical transition experience unequal trapping potentials. Here, we systematically analyze the effects of unequal trapping on near-resonant atom–light interactions. In particular, we identify regimes where such trapping can lead to significant excess heating compared to atoms in state-independent potentials, and a reduction of total and elastic scattering cross sections associated with a decreased atom–photon interaction efficiency. Understanding these effects can be valuable for achieving maximum efficiency in quantum optics experiments or atom imaging setups, where efficient atom–light interactions on resonance are desired, but achieving equal trapping is not feasible.

Wavelength-polarization-multiplexed multichannel perfect vortex array generator based on dielectric metasurface

The multi-channel perfect vortex (PV) array based on metasurface has important applications in optical communication, particle manipulation, quantum optics, and other fields due to its ultra-thin structure and excellent wavefront control ability. However, it is very challenging to utilize a single metasurface to simultaneously achieve independent channel PV arrays at different wavelengths with low crosstalk and low structural complexity. Here, we propose and design a single rectangular structured metasurface based on TiO2, achieving a multi-channel PV beam array with dual-wavelength and dual-polarization multiplexing. Simulation and experimental results show that when two orthogonal linearly polarized beams with wavelengths of 532 nm and 633 nm are incident on the metasurface, clear PV arrays with corresponding topological charge arrangements can be obtained in different diffraction regions of the same observation plane. The metasurface proposed in this article can enhance the channel capacity of a PV beam array through wavelength-polarization-multiplexing, thus having important application potential in spatial information transmission, high-dimensional information storage, and secure information encryption.

Longitudinally continuous varying high-order cylindrical vector fields enabled by spin-decoupled metasurfaces.

The manipulation of vector optical fields in three-dimensional (3D) space plays a vital role in both fundamental research and practical implementations of polarization optics. However, existing studies mostly focus on 3D vector optical fields with limited modes. Here, an approach of spin-decoupled spatial partitioning is proposed to generate complex 3D vector optical fields with a customizable number of modes on demand. The crosstalk among different modes is effectively suppressed by the decoupling capability of asymmetric photonic spin-orbit interactions (PSOIs) and the design of region displacement for opposite spin states. As a proof-of-concept demonstration, a metasurface is designed to generate longitudinally varying high-order cylindrical vector fields, ranging from the 2nd to the 10th order in even sequences along the propagation direction. The experimental results demonstrate the effectiveness and potential of our approach to enabling precise control of 3D vector optical fields with arbitrary mode combinations. This work holds promising applications in biophotonics, quantum optics, and communications.