Quantum Langevin Equation Research Articles

Dynamics of driven Brownian inverted oscillator

In this paper, we derive the quantum Langevin equation for a driven Brownian inverted oscillator in the framework of the Heisenberg picture for the Caldeira-Leggett model. We describe the influence of an arbitrary time-dependent force on an open inverted oscillator dynamics. We take into account environment through the integral operator of relaxation and the force correlation function. The resulting behavior of the system is represented as a combination the time evolution of the position expectation and the variance, being induced simultaneously by spreading the wave packet and the chaotic Brownian motion. We discuss the possibility of stabilization of an open inverted oscillator, when applying external alternating force.

Dynamic Cooling of a Micromechanical Membrane in a Double-cavity Optomechanical System

We theoretically present an optomechanical cooling scheme of a double optical modes which are coupled with the same mechanical resonator by the radiation pressure to analyze the dynamical cooling of a micromechanical membrane. The mean value of the total second-order moments are obtained by solving linearized quantum Langevin equations. We discuss the effect of the significant parameters of the system on the instantaneous-state mean phonon number of the oscillator cooled to the ground state under the resolved sideband regime. Furthermore, the steady-state cooling limit is also studied and the results show that the final mean phonon number splits into two minimum values when the detunings of the two cavity modes are different. Moreover, the minimal value of the final mean phonon number is much less than the case of equal driving detuning. By regulating the detunings of the optical modes from the corresponding driving fields and increasing the coupling strengths, the cooling effect will be optimized obviously.

Electromagnetic field quantization and quantum optical input-output relation for grating

A quantization scheme is developed for the radiation and higher order electromagnetic fields in one dimensional periodic, dispersive and absorbing dielectric medium. For this structure, the Green function is solved based on the plane wave expansion method, thus the photon operators, commutation relations and quantum Langevin equations are given and studied based on the Green function approach, moreover, the input-output relations are also derived. It is proved that this quantum theory can be reduced back to that of the predecessors’ study on the homogenous dielectric. Based on this method, we find that the transformation of the photon state through the lossy grating is non-unitary and that the notable non-unitary transformation can be obtained by tuning the imaginary part of the permittivity, we also discussed the excellent quantum optical properties for the grating which are similar to the classical optical phenomena. We believe our work is very beneficial for the control and regulation of the quantum light based on gratings.

Generalized diffusion of quantum Brownian motion.

This article discusses the numerical result predicted by the quantum Langevin equation of the generalized diffusion function of a Brownian particle immersed in an Ohmic quantum bath of harmonic oscillators. The time dependence of the standard deviation of the reduced Wigner function of the system, obtained by integrating the whole function in the momentum space, is determined as well. The complexity of the equations leads to resort to a much simpler calculation based in the position correlation function. They are done for the three possible regimes of the system, namely, periodic, aperiodic, and overdamped. It is found in the periodic case that the generalized diffusion is a discontinuous function exhibiting negative values during short time periods of time. This counterintuitive result, found theoretically in other systems and waiting for its experimental confirmation, can be perfectly explained in the framework of the quantum Langevin equation. Its oscillatory behavior is primordially due to the response to the external field while its quantum origin contributes only in its magnitude. The results are compared to those of the continuum limit which exhibits similar behavior.

Theory of quantum entanglement of intra-cavity photons produced by a non-degenerate parametric oscillator (NDPO); Semi-classical approach

The von-Neumann entropy (VNE) which is usually expressed in terms of the density operator is the mathematical tool to measure the degree of entanglement of a bi-partite system. Applying the solutions of the quantum Langevin equations, the anti-normally ordered characteristic function of the intra-cavity photons produced by a non-degenerate parametric oscillator is calculated. With the help of the resulting characteristic function, the Q function which is then used to calculate the entanglement of the intra-cavity photons using VNE is determined. Moreover, the photon number distribution of the intra-cavity photons produced by a non-degenerate parametric oscillator coupled to a two-mode squeezed vacuum reservoir is determined.

Magnon heralding in cavity optomagnonics

In the emerging field of cavity optomagnonics, photons are coupled coherently to magnons in solid-state systems. These new systems are promising for implementing hybrid quantum technologies. Being able to prepare Fock states in such platforms is an essential step towards the implementation of quantum information schemes. We propose a magnon-heralding protocol to generate a magnon Fock state by detecting an optical cavity photon. Due to the peculiarities of the optomagnonic coupling, the protocol involves two distinct cavity photon modes. Solving the quantum Langevin equations of the coupled system, we show that the temporal scale of the heralding is governed by the magnon-photon cooperativity and derive the requirements for generating high fidelity magnon Fock states. We show that the nonclassical character of the heralded state, which is imprinted in the autocorrelation of an optical "read" mode, is only limited by the magnon lifetime for small enough temperatures. We address the detrimental effects of nonvacuum initial states, showing that high fidelity Fock states can be achieved by actively cooling the system prior to the protocol.

Generalized self-consistent reservoir model for normal and anomalous heat transport in quantum harmonic chains.

Fictitious stochastic reservoirs incorporate scattering and dephasing mechanisms into the system in contact with these reservoirs. The reservoir-system coupling is described by the related self-energy in terms of the nonequilibrium Green's function formalism or equivalently the quantum Langevin equation formalism. In this study, we investigate thermal transport in a finite segment of an infinitely extended quantum harmonic chain with an equal self-energy at each site by using the self-consistent reservoir approach. In this setup, the entire system is lattice translation invariant so that mismatched boundaries are excluded from the model. Solving the Landauer-Büttiker equations under the self-consistent adiabatic condition, we quantitatively elucidate a thermally induced crossover of ballistic-to-diffusive transport and its scaling relation prescribed by a temperature-dependent mean free path. It is also shown that normal transport emerges in the diffusive limit for a linear self-energy, while nonlinear higher-order ones generically lead to anomalous transport. Physical implications of these observations are discussed in terms of the persistence of a massless Goldstone mode as well as the conservation of total linear momentum.

Non-equilibrium quantum Langevin dynamics of orbital diamagnetic moment

We investigate the time dependent orbital diamagnetic moment of a charged particle in a magnetic field in a viscous medium via the quantum Langevin equation. We study how the interplay between the cyclotron frequency and the viscous damping rate governs the dynamics of the orbital magnetic moment in the high temperature classical domain and the low temperature quantum domain for an Ohmic bath. These predictions can be tested via state of the art cold atom experiments with hybrid traps for ions and neutral atoms. We also study the effect of a confining potential on the dynamics of the magnetic moment. We notice that the rate of approach of the diamagnetic moment to the Bohr–van Leeuwen limit is higher in the presence of a potential compared to a situation where there is no confinement. We obtain the expected Bohr–van Leeuwen limit in the high temperature, asymptotic time (, where is the viscous damping coefficient) limit.

Langevin Approach to Quantum Optics with Molecules

We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross talk between upper and lower polaritons in the strong coupling regime. We also characterize the Förster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.

Axiomatic construction of quantum Langevin equations

A phenomenological construction of quantum Langevin equations, based on the physical criteria of (i) the canonical equal-time commutators, (ii) the Kubo formula, (iii) the virial theorem and (iv) the quantum fluctuation–dissipation theorem is presented. The case of a single harmonic oscillator coupled to a large external bath is analysed in detail. This allows to distinguish a Markovian semi-classical approach, due to Bedeaux and Mazur, from a non-Markovian full quantum approach, due to to Ford, Kac and Mazur. The quantum-fluctuation–dissipation theorem is seen to be incompatible with a Markovian dynamics. Possible applications to the quantum spherical model are discussed.

Enhanced collective Purcell effect of coupled quantum emitter systems

Cavity-embedded quantum emitters show strong modifications of free space radiation properties such as an enhanced decay known as the Purcell effect. The central parameter is the cooperativity $C$, the ratio of the square of the coherent cavity coupling strength over the product of cavity and emitter decay rates. For a single emitter, $C$ is independent of the transition dipole moment and dictated by geometric cavity properties such as finesse and mode waist. In a recent work [Phys. Rev. Lett. 119, 093601 (2017)] we have shown that collective excitations in ensembles of dipole-dipole coupled quantum emitters show a disentanglement between the coherent coupling to the cavity mode and spontaneous free space decay. This leads to a strong enhancement of the cavity cooperativity around certain collective subradiant antiresonances. Here, we present a quantum Langevin equations approach aimed at providing results beyond the classical coupled dipoles model. We show that the subradiantly enhanced cooperativity imprints its effects onto the cavity output field quantum correlations while also strongly increasing the cavity-emitter system's collective Kerr nonlinear effect.

Nonequilibrium phase transition in an open quantum spin system with long-range interaction.

We investigate a nonequilibrium phase transition in a dissipative and coherent quantum spin system using the quantum Langevin equation and mean-field theory. Recently, the quantum contact process (QCP) was theoretically investigated using the Rydberg antiblockade effect, in particular, when the Rydberg atoms were excited in s states so that their interactions were regarded as being between the nearest neighbors. However, when the atoms are excited to d states, the dipole-dipole interactions become effective, and long-range interactions must be considered. Here we consider a quantum spin model with a long-range QCP, where the branching and coagulation processes are allowed not only for the nearest-neighbor pairs but also for long-distance pairs, coherently and incoherently. Using the semiclassical approach, we show that the mean-field phase diagram of our long-range model is similar to that of the nearest-neighbor QCP, where the continuous (discontinuous) transition is found in the weak (strong) quantum regime. However, at the tricritical point, we find a new universality class, which was neither that of the QCP at the tricritical point nor that of the classical directed percolation model with long-range interactions. Implementation of the long-range QCP using interacting cold gases is discussed.

The effective Hamiltonian and propagator of a parabolic confined dissipative electron under a perpendicular magnetic field

We study the model of an electron in an isotropic quantum dot in the presence of a perpendicular magnetic field and dissipation. Starting from the system plus bath approach, the quantum Langevin equations are first obtained and consequently the equation of motion. Then the effective Hamiltonian is derived from the equation of motion. We obtained a new effective Hamiltonian for the case when the magnetic field and dissipation are both present. This effective Hamiltonian is quite different from the one used widely for time-dependent harmonic oscillators under a magnetic field in earlier studies. The corresponding propagator for this new effective Hamiltonian is also calculated. As an example of application, the dissipative dynamics of a Gaussian wavepacket confined in small quantum dots in the presence of a perpendicular magnetic field is studied.

Phononic heat transport in molecular junctions: Quantum effects and vibrational mismatch.

Problems of heat transport are ubiquitous to various technologies such as power generation, cooling, electronics, and thermoelectrics. In this paper, we advocate for the application of the quantum self-consistent reservoir method, which is based on the generalized quantum Langevin equation, to study phononic thermal conduction in molecular junctions. The method emulates phonon-phonon scattering processes while taking into account quantum effects and far-from-equilibrium (large temperature difference) conditions. We test the applicability of the method by simulating the thermal conductance of molecular junctions with one-dimensional molecules sandwiched between solid surfaces. Our results satisfy the expected behavior of the thermal conductance in anharmonic chains as a function of length, phonon scattering rate, and temperature, thus validating the computational scheme. Moreover, we examine the effects of vibrational mismatch between the solids' phonon spectra on the heat transfer characteristics in molecular junctions. Here, we reveal the dual role of vibrational anharmonicity: It raises the resistance of the junction due to multiple scattering processes, yet it promotes energy transport across a vibrational mismatch by enabling phonon recombination and decay processes.

The Quantum analysis of Nondegenerate Three-Level Laser with Spontaneous Emission and Noiseless Vacuum Reservoir

The analysis of quantum properties of the cavity light produced by a coherently driven nondegenerate three-level laser possessing an open cavity and coupled to a two-mode vacuum reservoir is presented. The normal ordering of noise operators associated with the vacuum reservoir is considered. Applying the solutions of the equations of evolution for the expectation values of the atomic operators and the quantum Langevin equations for the cavity mode operators, the squeezing properties, entanglement amplification, and the normalized second-order correlation function of the cavity radiation are described. The three-level laser generates squeezed light under certain conditions, with maximum intracavity squeezing being 50% below the vacuum-state level. Moreover, it is found that the presence of spontaneous emission increases the quadrature squeezing and entanglement and decreses the mean photon number of the two-mode cavity radiation.

Two-Level Atom with Squeezed Light from Optical Parametric Oscillators

The dynamics of a coherently driven two-level atom with parametric amplifier and coupled to a vacuum reservoir is analyzed. The combination of the master equation and the quantum Langevin equation is presented to study the quantum properties of light. By using these equations, we have determined the time evolution of the expectation values of the cavity mode and atomic operators. Moreover, with the aid of these results, the correlation properties of noise operators, and the large-time approximation scheme, we calculate the mean photon number, power spectrum, second-order correlation function, and quadrature variances for the cavity-mode light and fluorescence. It is found that the half-width of the power spectrum for the fluorescent light in the presence of a parametric amplifier increases, while it decreases for the cavity-mode light. Moreover, we have found the probability for the atom to be in the upper level in the presence of a parametric amplifier.

Light propagation through one-dimensional interacting open quantum systems

We apply the quantum Langevin equations approach to study nonlinear light propagation through one-dimensional interacting open quantum lattice models. We write a large set of quantum Langevin equations of lattice operators obtained after integrating out the light fields and use them to derive nonequilibrium features of the lattice models. We first consider a Heisenberg like interacting spin-1/2 chain with nearest-neighbor coupling. The transient and steady-state transport properties of an incoming monochromatic laser light are calculated for this model. We find how the local features of the spin chain and the chain length dependence of light transport coefficient evolve with an increasing power of the incident light. The steady-state light transmission coefficient at a higher power depends non-monotonically on the interaction in a finite chain. While the nonlinear light transmission in our studied model seems to be ballistic in the absence of interaction and for a high interaction, it shows an apparent system-size dependence at intermediate interactions. Later, we extend this method to the long-range interaction between spins of the driven-dissipative lattice model and to incorporate various losses typical in many atomic and solid-state systems.

Capture cross section with quantum diffusion approach

A C++ code for calculating the capture of a projectile by target nucleus is described. The code is based on the quantum diffusion model developed for considering collisions of nuclei at energies below and above the Coulomb barrier. The code provides the capture cross sections and other characteristics of reaction as functions of Ec.m.. The formalism of the model is briefly described. The code contains the Fortran subroutine to calculate the nucleus–nucleus potential. Program summaryProgram title: NuclearCaptureProgram files doi: http://dx.doi.org/10.17632/n66yg8mdzs.1Licensing provisions: GNU General Public License v2Programming language: C++, FortranExternal routines/libraries: GSL-2.2.1 GNU Scientific Library in C++ is required. It is available from https://www.gnu.org/software/gsl .Nature of problem: Capture of colliding nuclei at energies below and above the Coulomb barrierSolution method: Non-Markovian quantum Langevin equations

Theory for Nonlinear Spectroscopy of Vibrational Polaritons.

Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown great promise for exploiting these effects, significant challenges remain in interpreting their spectroscopic signatures. We develop a quantum-mechanical theory of pump-probe spectroscopy for this class of polaritons based on the quantum Langevin equation and the input-output theory. Comparison with recent experimental data shows good agreement upon consideration of the various vibrational anharmonicities that modulate the signals. Finally, a simple and intuitive interpretation of the data based on an effective mode-coupling theory is provided. Our work provides a solid theoretical framework to elucidate nonlinear optical properties of molecular polaritons as well as to analyze further multidimensional spectroscopy experiments on these systems.

Cavity-induced mirror-mirror entanglement in a single-atom Raman laser

We address an experimental scheme to analyze the optical bistability and the entanglement of two movable mirrors coupled to a two-mode laser inside a doubly resonant cavity. With this aim we investigate the master equations of the atom-cavity subsystem in conjunction with the quantum Langevin equations that describe the interaction of the mirror cavity. The parametric amplification-type coupling induced by the two-photon coherence on the optical bistability of the intracavity mean photon numbers is found and investigated. Under this condition, the optical intensities exhibit bistability for all large values of cavity laser detuning. We also provide numerical evidence for the generation of strong entanglement between the movable mirrors and show that it is robust against environmental thermalization.