Carbon fiber reinforced polymer (CFRP) have become gradually important in the aerospace industry due to their outstanding strength-to-weight ratio. However, traditional mechanical surface treatment methods are challenging to apply to CFRP because of their anisotropic and nonhomogeneous properties. Femtosecond laser offers unique advantages for surface treatment, as it allows processing with very low thermal load due to the extremely short interaction time. This study investigates the effect of different surface structures resulting from surface treatment using a femtosecond laser on adhesive properties of CFRP. The experimental results show that: 1) beam shaping can be realized by using the plano-convex cylindrical mirror, which improves the quality of laser processing and greatly improves processing efficiency. It only takes 20 s to complete the laser processing of a 1 cm*1 cm area, which increases the work efficiency by 49 times. 2) pre-bonding surface treatment significantly enhances the tensile shear strength of the single lap joint, and the shear strength of samples with low spatial frequency LIPSS (LSFL) (14.57 ± 1.58 MPa) is 2.96 times higher than that of the untreated sample (US) (4.92 ± 1.34 MPa). 3) LSFL structure exhibits the best results, because the surface of CFRP with LSFL exhibits a relatively higher surface polarity and surface energy. This study provides an efficient, high-precision, and low-damage surface treatment method for preparing CFRP for adhesive bonding, which may promote the application of femtosecond laser technology in difficult-to-process composite materials and provide new methods and technical support for its application in aerospace, vehicle manufacturing, and other fields.
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