Urban park waterfront green spaces provide positive mental health benefits to the public. In order to further explore the specific influence mechanism between landscape elements and public psychological response, 36 typical waterfront green areas in Xihu Park and Zuohai Park in Gulou District, Fuzhou City, Fujian Province, China, were selected for this study. We used semantic segmentation technology to quantitatively decompose the 36 scenes of landscape elements and obtained a public psychological response evaluation using virtual reality technology combined with questionnaire interviews. The main results showed that: (1) the Pyramid Scene Parsing Network (PSPNet) is a model suitable for quantitative decomposition of landscape elements of urban park waterfront green space; (2) the public’s overall evaluation of psychological responses to the 36 scenes was relatively high, with the psychological dimension scoring the highest; (3) different landscape elements showed significant differences in four dimensions. Among the elements, plant layer, pavement proportion, and commercial facilities all have an impact on the four dimensions; and (4) the contribution rate of the four element types to the public’s psychological response is shown as spatial element (37.9%) > facility element (35.1%) > natural element (25.0%) > construction element (2.0%). The obtained results reveal the influence of different landscape elements in urban park waterfront green spaces on public psychology and behavior. Meanwhile, it provides links and methods that can be involved in the planning and design of urban park waterfront green space, and also provides emerging technical support and objective data reference for subsequent research.
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