Pulses Of Extreme Ultraviolet Radiation Research Articles

Ultrafast opto-magnetic effects in the extreme ultraviolet spectral range

Coherent light-matter interactions mediated by opto-magnetic phenomena like the inverse Faraday effect (IFE) are expected to provide a non-thermal pathway for ultrafast manipulation of magnetism on timescales as short as the excitation pulse itself. As the IFE scales with the spin-orbit coupling strength of the involved electronic states, photo-exciting the strongly spin-orbit coupled core-level electrons in magnetic materials appears as an appealing method to transiently generate large opto-magnetic moments. Here, we investigate this scenario in a ferrimagnetic GdFeCo alloy by using intense and circularly polarized pulses of extreme ultraviolet radiation. Our results reveal ultrafast and strong helicity-dependent magnetic effects which are in line with the characteristic fingerprints of an IFE, corroborated by ab initio opto-magnetic IFE theory and atomistic spin dynamics simulations.

Time-resolved spectral investigation of low-temperature plasma induced in gas mixtures by laser-produced plasma or nanosecond pulses of extreme ultraviolet radiation

Time-resolved spectral investigation of low-temperature plasma induced in gas mixtures by laser-produced plasma or nanosecond pulses of extreme ultraviolet radiation

Quantitative Ultrafast Electron-Temperature Dynamics in Photo-Excited Au Nanoparticles.

The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measured, by means of ultrafast time-resolved photoemission spectroscopy induced by extreme-ultraviolet radiation pulses. The temperature of the electron gas is deduced by recording and fitting high-resolution photo emission spectra around the Fermi edge of gold nanoparticles providing a direct, unambiguous picture of the ultrafast electron-gas dynamics. These results will be instrumental to the refinement of existing models of femtosecond processes in laterally-confined and bulk condensed-matter systems, and for understanding more deeply the role of hot electrons in technologicalapplications.

Physico-Chemical Surface Modifications of Polyetheretherketone (PEEK) Using Extreme Ultraviolet (EUV) Radiation and EUV-Induced Nitrogen Plasma.

In this work, the effect of extreme ultraviolet (EUV) radiation and the combination of EUV radiation and low-temperature nitrogen plasma on the physico-chemical properties of polyetheretherketone (PEEK) surfaces were presented. The laser-plasma EUV source based on a double gas puff target was used in this experiment to irradiate PEEK surfaces with nanosecond pulses of EUV radiation and to produce low-temperature plasma through the photoionization of nitrogen with EUV photons. The changes in surface morphology on irradiated polymer samples were examined using atomic force microscopy (AFM) and scanning electron microscopy (SEM). Chemical changes of the PEEK surfaces were analysed using X-ray photoelectron spectroscopy (XPS). EUV radiation and nitrogen plasma treatment caused significant changes in the topography of modified PEEK’s surfaces and an increase in their average roughness. Strong chemical decomposition, appearance of new functional groups as well as incorporation of nitrogen atoms up to ~17 at.% on the PEEK’s surface were observed.

Response of fusion plasma-facing materials to nanosecond pulses of extreme ultraviolet radiation

AbstractThe experimental study of damage to tungsten (W), molybdenum (Mo), and silicon carbide (SiC) surfaces induced by focused extreme ultraviolet laser radiation (λ ~ 47 nm/~1.5 ns/21–40 µJ) is presented. It was found that W and Mo behaved similarly: during the first shot, the damaged area is covered by melted and re-solidified material, in which circular holes appear – residua of just opened pores/bubbles, from which pressurized gas/vapors escaped. Next cracks and ruptures appear and the W has a tendency to delaminate its surface layer. Contrary, single-crystalline SiC has negligible porosity and sublimates; therefore, no escape of “pressurized” gas and no accompanying effects take place. Moreover, SiC at sublimating temperature decomposes to elements; therefore, the smooth crater morphology can be related to local laser energy density above ablation threshold. When more shots are accumulated, in all three investigated materials, the crater depth increases non-linearly with number of these shots. The surface morphology was investigated by an atomic force microscope, the surface structure was imaged by a scanning electron microscope (SEM), and the structure below the surface was visualized by SEM directed into a trench that is milled by focused ion beam. Additionally, structural changes in SiC were revealed by Raman spectroscopy.

Dose-Rate Effects in Breaking DNA Strands by Short Pulses of Extreme Ultraviolet Radiation.

In this study, we examined dose-rate effects on strand break formation in plasmid DNA induced by pulsed extreme ultraviolet (XUV) radiation. Dose delivered to the target molecule was controlled by attenuating the incident photon flux using aluminum filters as well as by changing the DNA/buffer-salt ratio in the irradiated sample. Irradiated samples were examined using agarose gel electrophoresis. Yields of single- and double-strand breaks (SSBs and DSBs) were determined as a function of the incident photon fluence. In addition, electrophoresis also revealed DNA cross-linking. Damaged DNA was inspected by means of atomic force microscopy (AFM). Both SSB and DSB yields decreased with dose rate increase. Quantum yields of SSBs at the highest photon fluence were comparable to yields of DSBs found after synchrotron irradiation. The average SSB/DSB ratio decreased only slightly at elevated dose rates. In conclusion, complex and/or clustered damages other than cross-links do not appear to be induced under the radiation conditions applied in this study.

Ion energy distributions in highly transient EUV induced plasma in hydrogen

This work reports on the measurements of ion flux composition and ion energy distribution functions (IEDFs) at surfaces in contact with hydrogen plasmas induced by extreme ultraviolet (EUV) radiation. This special type of plasma is gaining interest from industries because of its appearance in extreme ultraviolet lithography tools, where it affects exposed surfaces. The studied plasma is induced in 5 Pa hydrogen gas by irradiating the gas with short (30 ns) pulses of EUV radiation (λ= 10–20 nm). Due to the low duty cycle (10–4), the plasma is highly transient. The composition and IEDF are measured using an energy resolved ion mass spectrometer. The total ion flux consists of H+, H2+, and H3+. H3+ is the dominant ion as a result of the efficient conversion of H2+ to H3+ upon collision with background hydrogen molecules. The IEDFs of H2+ and H3+ appear similar, showing a broad distribution with a cut-off energy at approximately 8 eV. In contrast, the IEDF of H+ shows an energetic tail up to 18 eV. Most probably, the ions in this tail gain their energy during their creation process by photoionization and dissociative electron impact ionization.

Extreme ultraviolet transient absorption of solids from femtosecond to attosecond timescales

High-harmonic generation (HHG) produces ultrashort pulses of extreme ultraviolet radiation (XUV), which can be used for pump–probe transient absorption spectroscopy in metal oxides, semiconductors, and dielectrics. Femtosecond transient absorption on iron and cobalt oxides identifies ligand-to-metal charge transfer as the main spectroscopic transition, rather than metal-to-metal charge transfer or d–d transitions, upon photoexcitation in the visible. In silicon, attosecond transient absorption reveals that electrons tunnel into the conduction band from the valence band under strong-field excitation, to energies as high as 6 eV above the conduction band minimum. Extensions of these experiments to other semiconductors, such as germanium, and other transition metal oxides, such as vanadium dioxide, are discussed. Germanium is of particular interest because it should be possible to follow both electron and hole dynamics in a single measurement using transient XUV absorption.

Kr photoionized plasma induced by intense extreme ultraviolet pulses

Irradiation of any gas with an intense EUV (extreme ultraviolet) radiation beam can result in creation of photoionized plasmas. The parameters of such plasmas can be significantly different when compared with those of the laser produced plasmas (LPP) or discharge plasmas. In this work, the photoionized plasmas were created in a krypton gas irradiated using an LPP EUV source operating at a 10 Hz repetition rate. The Kr gas was injected into the vacuum chamber synchronously with the EUV radiation pulses. The EUV beam was focused onto a Kr gas stream using an axisymmetrical ellipsoidal collector. The resulting low temperature Kr plasmas emitted electromagnetic radiation in the wide spectral range. The emission spectra were measured either in the EUV or an optical range. The EUV spectrum was dominated by emission lines originating from Kr III and Kr IV ions, and the UV/VIS spectra were composed from Kr II and Kr I lines. The spectral lines recorded in EUV, UV, and VIS ranges were used for the construction of Boltzmann plots to be used for the estimation of the electron temperature. It was shown that for the lowest Kr III and Kr IV levels, the local thermodynamic equilibrium (LTE) conditions were not fulfilled. The electron temperature was thus estimated based on Kr II and Kr I species where the partial LTE conditions could be expected.

Double electric layer influence on dynamic of EUV radiation from plasma of high-current pulse diode in tin vapor

Generation of high-power pulses of extreme ultraviolet radiation from multi-charged tin plasma is of great interest to many applications. We studied the electric potential distribution in the discharge gap in kind of the electric double layer and its effect on the extreme ultraviolet generation. The local plasma heating by electron beam, formed in the double layer, leads to generation of peak radiation pulses and as a result to an increase in the radiation power.

Experimental observations in compact capillary discharges

We present experimental results on the characterization of a non-ablating fast pulsed capillary discharge, with a hollow cathode (HC) geometry, operating in argon below 1 Torr. Both the pre-breakdown and breakdown phase of the discharge are investigated with several diagnostics, which include electron beam monitoring, capacitive probe array and extreme ultraviolet (EUV) detector array. The pre-breakdown phase is found to be characterized by the emission of HC electron beams, which assist the propagation of a high speed ionization wave, with typical velocity in the 106–107 m s−1. Coinciding with electric breakdown a fast EUV radiation pulse is emitted. The leading edge of the radiation pulse is due to beam target emission by the HC electron beams. At the breakdown the radiation emission is mainly centered in the 5–15 nm spectral window, and is emitted from a capillary plasma which is being heated by a kiloampere level, 10 ns half-width current pulse.

Behavior of SiO2 nanostructures under intense extreme ultraviolet illumination

The stability of conducting atomic force microscope (C-AFM)-induced surface modifications of thermally grown SiO2 under intense illumination in the extreme ultraviolet (EUV) is investigated with low-energy electron microscopy (LEEM) and x-ray photoemission electron microscopy (XPEEM). With LEEM we find that the protrusions are heavily charged after their formation, but this charge is annihilated after exposure of the sample to short pulses of EUV radiation. The spectra obtained from XPEEM reveal that the stripes formed by C-AFM consist of SiO2. After extended EUV exposure, a radiation-induced desorption of the stripes as well as a desorption of the thermal oxide is observed.

Superfluorescence with cold trapped neon atoms

A method for observation of superfluorescence in a cloud of cold metastable Ne atoms is proposed. Means of achieving a cold sample of trapped metastable atoms are discussed. The feasibility of obtaining conditions for a superfluorescence pulse is studied. The paper also discusses the prospects for obtaining intense pulses of extreme ultraviolet radiation.