Use Of Pulses Research Articles

Single-shot ultrafast imaging of plasma dynamics induced by dual-angle ultrashort laser pulses with subpicosecond delay

Spatiotemporal manipulation of ultrashort laser pulses is crucial for enhancing laser processing and phonon generation. Optimization of these applications requires ultrafast visualization of the underlying processes. In this study, we induced laser ablation using spatiotemporally manipulated double pulses focused from two angles onto a glass surface with a 0.7 ps interval, and captured the images of its dynamics with 5 sequential frames at a frame interval of 0.8 ps. The observed dynamics suggest that the laser profile reflected on the glass surface is influenced by its topography, which in turn affects the behavior of air breakdown plasmas.

Tabletop Tunable Chiral Photonic Emitter.

The increasing interest in chiral light stems from its spiral trajectory along the propagation direction, facilitating the interaction between different polarization states of light and matter. Despite tremendous achievements in chiral light-related research, the generation and control of chiral pulses have presented enduring challenges, especially at the terahertz and ultraviolet spectral ranges, due to the lack of suitable optical elements for effective pulse manipulation. Conventionally, chiral light can be obtained from intricate optical systems, by an external magnetic field, or by metamaterials, which necessitate sophisticated optical configurations. Here, leveraging the high harmonic generation process, we propose a versatile tunable chiral emitter, composed of only two planar Weyl semimetals slabs, addressing the challenges in both spectral ranges. Our results open the way to a compact tunable chiral emitter platform in both terahertz and ultra-violet frequency ranges. This advancement holds the potential to serve as the cornerstone for integrated chiral photonics.

Optical manipulation of ultrashort laser pulses for applications in challenging environments

Over the last few years, high throughput ultrashort-pulse laser sources have become increasingly affordable. This facilitated the emergence of many applications that require sub-micron precision material modification. Processes have been demonstrated in applications including micro-structuring semiconductor chips, manufacturing complex 3D parts or inscribing optical materials for data storage. Furthermore, recent progress in techniques for the optical manipulation of ultrashort laser pulses opened up new avenues in applications for challenging environments such as those involving high energy physics or particle beam radiotherapy. These applications require high-resolution 3D structures to be produced in radiation tolerant materials, to make particle sensors with the required sensitivity and resolution. For such processes, accurate spatial and temporal structuring and manipulating of optical parameters such as polarization, wavefront and intensity of laser beams, is essential. This paper presents recent results in advanced optical manipulation including the induction of helical or longitudinal fields at the focus. The resulting laser material coupling interactions are characterized and their suitability for making particle sensors from radiation hard materials considered.

Synthesis and analysis of an ensemble of SAR signals

Due to the development of digital technologies for receiving and transmitting radio location signals, the development of modern radars with a synthesized aperture has made it possible to widely use an ensemble of probing signals with periodic sequences of identical pulses. The manipulation of probing pulses in transmission opens up opportunities to reduce the level of interference of ambiguity in range, expand the capture bands, improve azimuth resolution, and reduce interference from the background surrounding the target. However, the literature currently does not sufficiently address the issues of synthesis and analysis of ensembles of probing signals for a synthetic aperture radar (RSA) placed on board an unmanned aerial vehicle. Several variants of the implementation of ensembles of probing signals in the RSA are considered, mathematical modeling and experimental testing are carried out on the basis of the RSA operating in the VHF frequency range, placed on board an unmanned aerial vehicle (UAV). The conducted modeling allows us to draw the following conclusions. The best characteristics are possessed by an ensemble of signals encoded by Huffman codes, where M-sequences were used to "scatter" the roots. In second place is an ensemble of signals encoded by composite M-sequences. However, with an increase in the base of probing signals (N>64), the best results are shown by an ensemble of signals based on composite M-sequences.

Multidimensional ultrashort optical pulse manipulation using spatial light modulation.

Ultrashort optical pulse manipulation is one of the key techniques for applications such as high-speed imaging and high-precision laser processing. In this study, we demonstrate the multidimensional manipulation of ultrashort optical pulses by integrating spatial dispersion and spatial light modulation. Specifically, by modulating the phase of each wavelength, we achieve arbitrary adjustments in multiple dimensions, including number of sub pulses, time interval, intensity, and pulse width simultaneously and independently with a simple setup and few calculations. The performance of the optical pulse manipulation method is verified through both numerical simulations and experiments.

Generation of sub-10-fs deep and extreme ultraviolet pulses for time-resolved photoemission spectroscopy.

We present a light source capable of generating sub-10-fs deep UV (DUV) and extreme UV (EUV) pulses for use in time-resolved photoemission spectroscopy. The fundamental output of a Ti:sapphire laser was compressed using the multi-plate method and mixed with the uncompressed second harmonic in a filamentation four-wave mixing process to generate sub-10-fs DUV pulses. Sub-10-fs EUV pulses were generated via high-order harmonic generation driven by the second harmonic pulses that were compressed using Ar gas and chirped mirrors. The minimum cross correlation time between 267 and 57 nm (corresponding to 21.7 eV) was measured to be 10.6 ± 0.4 fs.

Underwater Wavelength Attack on Discrete Modulated Continuous-Variable Quantum Key Distribution.

The wavelength attack utilizes the dependence of beam splitters (BSs) on wavelength to cause legitimate users Alice and Bob to underestimate their excess noise so that Eve can steal more secret keys without being detected. Recently, the wavelength attack on Gaussian-modulated continuous-variable quantum key distribution (CV-QKD) has been researched in both fiber and atmospheric channels. However, the wavelength attack may also pose a threat to the case of ocean turbulent channels, which are vital for the secure communication of both ocean sensor networks and submarines. In this work, we propose two wavelength attack schemes on underwater discrete modulated (DM) CV-QKD protocol, which is effective for the case with and without local oscillator (LO) intensity monitor, respectively. In terms of the transmittance properties of the fused biconical taper (FBT) BS, two sets of wavelengths are determined for Eve's pulse manipulation, which are all located in the so-called blue-green band. The derived successful criterion shows that both attack schemes can control the estimated excess noise of Alice and Bob close to zero by selecting the corresponding condition parameters based on channel transmittance. Additionally, our numerical analysis shows that Eve can steal more bits when the wavelength attack controls the value of the estimated excess noise closer to zero.

Field-resolved space–time characterization of few-cycle structured light pulses

Accompanied by the rapid development of ultrafast laser platforms in recent decades, the spatiotemporal manipulation of ultrashort laser pulses has attracted much attention due to the potential for cutting-edge applications of structured light, including optical tweezers, optical communications, super-resolution imaging, time-resolved spectroscopy in molecules and quantum materials, and strong-field physics. Today, techniques capable of characterizing the full spatial, temporal, and polarization state properties of structured light are strongly desired. Here, we demonstrate a technique, termed 3D TIPTOE, for characterizing structured mid-infrared waveforms, which uses only a two-dimensional silicon-based image sensor as both the detector and the nonlinear medium. By combining the advantages of the sub-cycle time resolution afforded by nonlinear excitation and the spatial resolution inherent to the two-dimensional sensor, the 3D TIPTOE technique allows full characterization of structured electric fields, significantly reducing the complexity of detection compared to other techniques. The validity of the technique is established by measuring both few-cycle Bessel–Gaussian pulses and radially polarized femtosecond vector beams.

Precise mode control of laser-written waveguides for broadband, low-dispersion 3D integrated optics

Three-dimensional (3D) glass chips are promising waveguide platforms for building hybrid 3D photonic circuits due to their 3D topological capabilities, large transparent windows, and low coupling dispersion. At present, the key challenge in scaling down a benchtop optical system to a glass chip is the lack of precise methods for controlling the mode field and optical coupling of 3D waveguide circuits. Here, we propose an overlap-controlled multi-scan (OCMS) method based on laser-direct lithography that allows customizing the refractive index profile of 3D waveguides with high spatial precision in a variety of glasses. On the basis of this method, we achieve variable mode-field distribution, robust and broadband coupling, and thereby demonstrate dispersionless LP21-mode conversion of supercontinuum pulses with the largest deviation of <0.1 dB in coupling ratios on 210 nm broadband. This approach provides a route to achieve ultra-broadband and low-dispersion coupling in 3D photonic circuits, with overwhelming advantages over conventional planar waveguide-optic platforms for on-chip transmission and manipulation of ultrashort laser pulses and broadband supercontinuum.

UV-induced resonant excitations of electrons near the Brillouin zone boundary in solid high harmonic generation

Abstract We propose a novel mechanism to manipulate the electron dynamics at the boundary of the Brillouin zone (BZ) through resonant excitation induced by ultraviolet (UV) laser pulses in solid high harmonic generation (HHG). When adding weak UV pulses to a stronger mid-infrared (MIR) driving field, we show that UV pulses with specific wavelengths generate a resonant excitation zone around the Γ point in k − space, which facilitates the interband transition of electrons in the BZ boundary region. The scheme is not only significant for achieving higher harmonic yield, but also exhibits strong robustness at a relatively low MIR driving intensity due to the inherent manipulation of UV pulses for interband dynamics of BZ boundary electrons. The semiclassical four-step model is adopted to elucidate underlying physics.

Gigahertz streaking and compression of low-energy electron pulses.

Although radio frequency (RF) technology is routinely employed for controlling high-energy pulses of electrons, corresponding technology has not been developed at beam energies below several kiloelectronvolts. In this work, we demonstrate transverse and longitudinal phase-space manipulation of low-energy electron pulses using RF fields. A millimeter-sized photoelectron gun is combined with synchronized streaking and compression cavities driven at frequencies of and , respectively. The phase-controlled acceleration and deceleration of photoelectron pulses is characterized in the energy range of -. Deflection from a transient space-charge cloud at a metal grid is used to measure a fourfold compression of electron pulses, from to pulse duration.

Generation of ultra-intense vortex laser from a binary phase square spiral zone plate.

With the development of ultra-intense laser technology, the manipulation of relativistic laser pulses has become progressively challenging due to the limitations of damage thresholds for traditional optical devices. In recent years, the generation and manipulation of ultra-intense vortex laser pulses by plasma has attracted a great deal of attention. Here, we propose a new scheme to produce a relativistic vortex laser. This is achieved by using a relativistic Gaussian drive laser to irradiate a plasma binary phase square spiral zone plate (BPSSZP). Based on three-dimensional particle-in-cell (3D-PIC) simulations, we find that the drive laser has a phase difference of π after passing through the BPSSZP, ultimately generating the vortex laser with unique square symmetry. Quantitatively, by employing a drive laser pulse with intensity of 1.3 × 1018~W/cm2, a vortex laser with intensity up to 1.8 × 1019~W/cm2, and energy conversion efficiency of 18.61% can be obtained. The vortex lasers generated using the BPSSZP follow the modulo-4 transmutation rule when varying the topological charge of BPSSZP. Furthermore, the plasma-based BPSSZP has exhibited robustness and the ability to withstand multiple ultra-intense laser pulses. As the vortex laser generated via the BPSSZP has high intensity and large energy conversion efficiency, our scheme may hold potential applications in the community of laser-plasma, such as particles acceleration, intense high-order vortex harmonic generation, and vortex X/γ-ray sources.

Thermo-optical liquid-crystal phase modulator for ultrafast optics, driven by neural network

We propose a new spatial light modulator (SLM) concept, relying on a local thermal modification of a thick liquid crystal layer, that is optically-induced through the absorption of a control beam. This innovative thermo-optically addressed SLM, coined TOA-SLM, has shown dynamic phase control capabilities over multi-octave light spectrum, as a promising candidate for spatial or temporal manipulation of ultrafast pulses. In addition to being ultra-broadband and programmable, such a device is low-cost, large-aperture and un-segmented with a high number of control points. The construction and training of a neural network-based statistical model provides configurable design of a prototype TOA-SLM. This step, together with the ultra-broadband acceptance of the device and its ability to introduce continuous and deep phase modulation over a large aperture, opens the way for ultrafast laser aberration compensation using this new technology.

Ultrashort Ne+ ion pulses for use in pump–probe experiments: numerical simulations

A time resolved experiment to investigate the ultrafast dynamics following an ion impact onto a solid surface requires an ultrashort ion pump pulse in combination with a properly synchronized and time resolved probe. In order to realize such an experiment, we have investigated a strategy to use femtosecond laser photoionization of atoms entrained in a pulsed supersonic jet for the production of sufficiently short ion pulses. While the generation of Arq+ ions was targeted in previous work, it has in the meantime been demonstrated that argon is not suitable due to extensive cluster formation in the supersonic expansion. Here, we therefore present numerical simulations investigating the use of neon as a precursor gas and show the feasibility of pulses containing up to ∼1000 Ne+ ions at keV energies and picosecond duration. In the process, we demonstrate that space charge broadening can be significantly reduced by detuning the flight time focusing conditions of an ion bunching system. Moreover, the results show that a controlled variation of the buncher geometry and potentials permits the generation of picosecond pulses at variable ion energy between 1 and 5 keV.

All-optical generation, detection, and manipulation of picosecond acoustic pulses in 2D semiconductor/dielectric heterostructures

Launching, tracking, and controlling picosecond acoustic (PA) pulses are fundamentally important for the construction of ultrafast hypersonic wave sources, ultrafast manipulation of matter, and spatiotemporal imaging of interfaces. Here, we show that GHz PA pulses can be all-optically generated, detected, and manipulated in a 2D layered MoS2/glass heterostructure using femtosecond laser pump–probe. Based on an interferometric model, PA pulse signals in glass are successfully decoupled from the coexisting temperature and photocarrier relaxation and coherent acoustic phonon (CAP) oscillation signals of MoS2 lattice in both time and frequency domains. Under selective interface excitations, temperature-mediated interfacial phonon scatterings can compress PA pulse widths by about 50%. By increasing the pump fluences, anharmonic CAP oscillations of MoS2 lattice are initiated. As a result, the increased interatomic distance at the MoS2/glass interface that reduces interfacial energy couplings can markedly broaden the PA pulse widths by about 150%. Our results open new avenues to obtain controllable PA pulses in 2D semiconductor/dielectric heterostructures with femtosecond laser pump–probe, which will enable many investigations and applications.

Reduced Scaling Real-Time Coupled Cluster Theory.

Real-time coupled cluster (CC) methods have several advantages over their frequency-domain counterparts, namely, response and equation of motion CC theories. Broadband spectra, strong fields, and pulse manipulation allow for the simulation of complex spectroscopies that are unreachable using frequency-domain approaches. Due to the high-order polynomial scaling, the required numerical time propagation of the CC residual expressions is a computationally demanding process. This scaling may be reduced by local correlation schemes, which aim to reduce the size of the (virtual) orbital space by truncation according to user-defined parameters. We present the first application of local correlation to real-time CC. As in previous studies of locally correlated frequency-domain CC, traditional local correlation schemes are of limited utility for field-dependent properties; however, a perturbation-aware scheme proves promising. A detailed analysis of the amplitude dynamics suggests that the main challenge is a strong time dependence of the wave function sparsity.

Supercontinuum Generation from Airy-Gaussian Pulses in Photonic Crystal Fiber with Three Zero-Dispersion Points

The supercontinuum generation and manipulation of Airy-Gaussian pulses in a photonic crystal fiber with three zero-dispersion points are studied using the split-step Fourier method. Firstly, the spectral evolution of Airy-Gaussian pulses in four photonic crystal fibers with different barrier widths was discussed, and the optimal fiber was determined after considering the factors of width and flatness. By analyzing the mechanism of supercontinuum generation in photonic crystal fibers with single, double and three zero-dispersion points, it is found that the photonic crystal fiber with three zero-dispersion points have a larger spectral width due to the component of tunneling solitons. Then, the effects of four characteristic parameters (truncation factor a, distribution factor χ0, initial chirp C and central wavelength λ) on forming the supercontinuum spectrum of Airy-Gaussian pulses are analyzed in detail. The results show that the spectral width and energy intensity of the dispersive wave and tunneling soliton generation can be well controlled by adjusting the barrier width and initial parameters of the pulse. These research results provide a theoretical basis for generating and manipulating high-power mid-infrared supercontinuum sources.

Control and stabilization of Kerr cavity solitons and breathers driven by chirped optical pulses

We investigate the impact of chirped driving fields on the dynamics and generation of Kerr cavity breathers and solitons. Synchronous phase and amplitude modulation of the pumping field can be exploited in order to control soliton dynamics. Here we show that using a phase-modulated super-Gaussian pump permits to stabilize the oscillations of breathing solitons. Moreover, our scheme permits to obtain new dynamical attractors, with a prescribed temporal intra-cavity pattern. Straightforward applications are the deterministic generation of optical frequency soliton combs, optical tweezers, and more generally, all-optical manipulation of light pulses.

Coherent Manipulation of Ultrashort Free Electrons Pulses via Quantized Electron-Photon Interaction Mediated by Transversely- and Longitudinally-Shaped Optical Fields.

Coherent Manipulation of Ultrashort Free Electrons Pulses via Quantized Electron-Photon Interaction Mediated by Transversely- and Longitudinally-Shaped Optical Fields.

Observation of Generalized Dynamic Localizations in Arbitrary‐Wave Driven Synthetic Temporal Lattices

AbstractDynamic localization (DL) refers to a wavefunction confinement effect of electrons in periodic lattices under an ac electric field driving. Recent studies have transplanted DLs from electronic to photonic systems using periodically curved waveguide lattices, where the ac electric field is mimicked by the waveguide's bending curvature. However, due to the severe limitations of bending losses and poor tunability for highly curved, arbitrarily shaped waveguides, present studies mainly focus on DL under the simplest sinusoidal‐wave driving; its extension to an arbitrary‐wave driving remains challenging. Here, by constructing a synthetic temporal lattice with a coupled fiber‐loop circuit, the limitations of spatially curved waveguides are circumvented and generalized DLs are experimentally demonstrated under arbitrary‐wave driving. First, by applying band‐collapse criteria, the general conditions for the driving field's symmetry to achieve DLs are revealed. Then, two representative even‐function driving fields of square‐ and triangle‐waveforms are chosen, and wave‐packet revivals are observed as signatures of DLs. As a counter‐example, the breakdown of DL is also verified using odd‐function driving field of sawtooth‐waveform. The work reveals the conditions for realizing generalized DLs and experimentally verifies them using synthetic lattice schemes. This paradigm may find potential applications in versatile temporal‐waveform reshaping, pulse manipulations for optical communications, and signal processing.