Intense electromagnetic pulses are electromagnetic waves with sharp rise time, high field strength and short duration. They have attracted more and more attention in recent years because they can cause destructions or malfunctions of some key national core infrastructures, such as power grids, communication and financial networks, etc. Hence, it is important to harden these facilities to ensure that they can survive in the face of electromagnetic pulse attacks. A direct way to investigate the vulnerabilities of these facilities is placing them in the electromagnetic environments generated by EMP simulators. However, the scale of facilities under test are limited by the working volumes of simulators. With the increase in working volumes and field strength, the price and technical difficulty of simulators are increased. Therefore, low cost and sustainable test methods to investigate vulnerabilities of large-scale systems against EMP are proposed in this study. The study takes advantage of continuous wave immersion (CWI) test and pulse current injection (PCI) test methods, which are low cost and sustainable to predict the pulse responses and assess the nonlinear effect of large-scale facilities under EMP attacks. In a CWI test, the magnitude of the transfer function of large-scale systems or facilities can be measured, and the corresponding phase information of the transfer function can be reconstructed by minimum phase algorithm (MPA) if the systems meet the minimum phase condition. After acquiring the entire information of the transfer function, we can predict the responses of a system under threat-level EMP attacks. However, these responses are obtained under the assumption that the system does not have nonlinear effects. Because the CWI is a low-level test, it cannot simulate the threat-level EMP attacks. In the PCI test proposed here, a bulky pulse current is coupled into the system to stimulate enough current intensity, just as the system was attacked by threat-level EMPs. In this situation, the system would be destroyed, or any other nonlinear effect would occur in the system. After that, the problem is to determine the quantities of the injected current, and a few kinds of norms are introduced in this paper to define the quantities. The method proposed here innovatively takes the experimental results of CWI as reference inputs of PCI tests. In this paper, the accuracy of the response prediction is validated by means of simulations and experiments. Results show that as a low-level test method in the frequency domain, the CWI test method can not only analyze couplings of external electromagnetic energy from frequency domain but also predict responses of the facilities under high amplitude electromagnetic pulses. The nonlinear effect of large-scale facilities can be assessed by applying the PCI test method with the results from CWI prediction. Therefore, if infrastructures or facilities are too large to be tested under EMP simulators, an alternative approach is to carry out the CWI and PCI experiments.