Finite Pulse Research Articles

Experimental coherent-state quantum secret sharing with finite pulses

Experimental coherent-state quantum secret sharing with finite pulses

Modeling resonant energy absorption of finite laser pulses in a doped porous dielectric slab

Modeling resonant energy absorption of finite laser pulses in a doped porous dielectric slab

Nutation-based longitudinal-sensing protocols for high-field NMR with nitrogen-vacancy centers in diamond

Nitrogen-vacancy (N-V) centers in diamond enable nuclear magnetic resonance (NMR) spectroscopy of samples at the nano- and microscale. However, at typical tesla-scale NMR magnetic field strengths, N-V–NMR protocols become difficult to implement due to the challenge of driving fast N-V pulse sequences sensitive to nuclear Larmor frequencies above a few megahertz. We perform simulations and theoretical analysis of the experimental viability of N-V NMR at tesla-scale magnetic fields using a measurement protocol called DRACAERIS (Double Rewound ACquisition Amplitude Encoded Radio Induced Signal). DRACAERIS detects the longitudinal magnetization of the NMR sample at a much lower driven Rabi frequency, more suitable technically for N-V detection. We discuss how pulse errors, finite pulse lengths, and nuclear spin-spin couplings affect the resulting NMR spectra. We find that DRACAERIS is less susceptible to pulse imperfections and off-resonance effects than previous protocols for longitudinal magnetization detection. We also identify reasonable parameters for experimental implementation. Published by the American Physical Society 2024

Formation of CBOC signals with a reduced level of out-of-band radiation

Formulation of the problem. The article considers the issues of choosing low-pass filters with finite and infinite pulse characteristics used to generate CBOC signals with phase manipulation with a reduced level of out-of-band radiation. Purpose. The influence of the filter frequency band on the distortion of CBOC signals in the frequency and time domain is estimated by mathematical modeling. Results. The following filter parameters, peak factor and ACPR (Adjacent Channel Power Ratio) were studied and calculated. Practical significance. The results obtained can be used by developers of local navigation systems.

Controllable multi-soliton spectral tunneling by airy pulses in photonic crystal fiber

A straightforward method to induce tunable multi-soliton spectral tunneling (SST) using a finite energy Airy pulse in a photonic crystal fiber (PCF) featuring three zero-dispersion wavelengths is proposed numerically in the paper. The study reveals that the distinctive multi-envelope structure of the Airy pulse enables the control of tunneling distances, properties, and soliton numbers through modulation of its attenuation factor and peak intensity. Notably, the SST process involving the Airy pulse generates multiple blue-shifted and red-shifted dispersion waves, along with associated trapping waves, contributing to the formation of an ultra-flat and ultra-wide supercontinuum. Furthermore, the velocity and efficiency of multi-SST can be manipulated to enhance the overall tunability of the phenomenon. The findings underscore the potential application of Airy pulse-driven SST in secure multi-frequency signal transmission and controlled supercontinuum generation, with the tunability of these processes being governed by the specific attenuation factor and peak power settings of the input Airy pulse. This work advances the understanding of multi-SST dynamics in PCFs and provides a theoretical framework for exploiting these dynamics in practical information security and optical spectrum management contexts.

Breakdown of argon by a train of high-repetition long-wave-infrared pulses from a free-electron laser oscillator

This study presents an experimental demonstration of laser-induced breakdown in argon, employing a free-electron laser with a wavelength of 10 μm and a repetition rate of 2.856 GHz. Despite the fluence of individual laser pulses being an order of magnitude smaller than the breakdown threshold, cascade ionization developed in the pulse train, leading to breakdown. The breakdown probability within a finite pulse train increases with gas pressure, and it was notably enhanced in a gas chamber with poor cleanliness. Numerical simulations of cascade ionization replicated the experimental results. The simulation revealed that breakdown phenomena are governed by the balance between avalanche multiplication of electrons within laser pulses and electron diffusion during pulse intervals.

Flying-cat parity checks for quantum error correction

Long range, multiqubit parity checks have applications in both quantum error correction and measurement-based entanglement generation. Such parity checks could be performed using qubit-state-dependent phase shifts on propagating pulses of light described by coherent states |α〉 of the electromagnetic field. We consider “flying-cat” parity checks based on an entangling operation that is quantum nondemolition for Schrödinger's cat states |α〉±|−α〉. This operation encodes parity information in the phase of maximally distinguishable coherent states |±α〉, which can be read out using a phase-sensitive measurement of the electromagnetic field. In contrast to many implementations, where single-qubit errors and measurement errors can be treated as independent, photon loss during flying-cat parity checks introduces errors on physical qubits at a rate that is anticorrelated with the probability for measurement errors. We analyze this trade-off for three-qubit parity checks, which are a requirement for universal fault-tolerant quantum computing with the subsystem surface code. We further show how a six-qubit entangled “tetrahedron” state can be prepared using these three-qubit parity checks. The tetrahedron state can be used as a resource for controlled quantum teleportation of a two-qubit state or as a source of shared randomness with potential applications in three-party quantum key distribution. Finally, we provide conditions for performing high-quality flying-cat parity checks in a state-of-the-art circuit QED architecture, accounting for qubit decoherence, internal cavity losses, and finite-duration pulses, in addition to transmission losses. Published by the American Physical Society 2024

Unveiling the interplay of Mollow physics and perturbed free induction decay by nonlinear optical signals of a dynamically driven two-level system

Nonlinear optical signals in optically driven quantum systems can reveal coherences and thereby open up the possibility for manipulation of quantum states. While the limiting cases of ultrafast and continuous-wave excitation have been extensively studied, the time dynamics of finite pulses bear interesting phenomena. In this paper, we explore the nonlinear optical probe signals of a two-level system excited with a laser pulse of finite duration. In addition to the prominent Mollow peaks, the probe spectra feature several smaller peaks for certain time delays. Similar features have been recently observed for resonance fluorescence signals [K. Boos , ]. We discuss that the emergent phenomena can be explained by a combination of Mollow triplet physics and perturbed free induction decay effects, providing an insightful understanding of the underlying physics. Published by the American Physical Society 2024

In situ effective pumping speed measurements as a tool for non-evaporable getter activation and saturation monitoring

We have developed method of in situ effective pumping speed measurements based on injecting finite gas pulse into a vacuum volume and subsequent recording of pressure response using a Residual Gas Analyzer (RGA). The pressure burst caused by injected gas pulse falls exponentially in time and the exponential coefficient of such pressure decay is proportional to total effective pumping speed of all vacuum pumps acting on vacuum chamber volume. The effective pumping speed can be extracted from the dependence of injected gas species pressure vs time recorded by an RGA. Non-Evaporable Getters (NEGs) are widely used in multiple ultra and extremely high vacuum devices and applications during the last several decades. Areas of NEG applications were recently expanded into vacuum devices with relatively high-pressure levels (up to 10−7 Torr) by the invention of high capacity ZAO NEG which can be operated at elevated temperatures. The intrinsic property of all NEG-based vacuum pumps is the reduction of their pumping speed, called “NEG saturation”, after an extended period of operation. Typical time interval for such process can span from about a month and up to a few years depending on NEG type, vacuum level of NEG pump operation, and residual gas content. After that, the NEG pump will require a re-activation cycle to restore its pumping speed close to the initial value. For many applications it is difficult to realize what is the current pumping speed of NEG pump is and when the pump should be re-activated. A method for in situ effective pumping speed measurements developed in this study can be used as a tool for NEG-based pump activation and saturation monitoring. Application of such an approach to monitor pumping status of NEG pumps was utilized and will be continually used at Extended EBIS which was recently developed and commissioned for Relativistic Heavy Ion Collider (RHIC) and future Electron Ion Collider (EIC). The results obtained during commissioning are presented and discussed.

Understanding the Nonlinear Response of SiPMs.

A systematic study of the nonlinear response of Silicon Photomultipliers (SiPMs) was conducted through Monte Carlo (MC) simulations. The MC code was validated against experimental data for two different SiPMs. Nonlinearity mainly depends on the balance between the photon rate and the pixel recovery time. Additionally, nonlinearity has been found to depend on the light pulse shape, the correlated noise, the overvoltage dependence of the photon detection efficiency, and the impedance of the readout circuit. Correlated noise has been shown to have a minor impact on nonlinearity, but it can significantly affect the shape of the SiPM output current. Considering these dependencies and a previous statistical analysis of the nonlinear response of SiPMs, two phenomenological fitting models were proposed for exponential-like and finite light pulses, explaining the roles of their various terms and parameters. These models provide an accurate description of the nonlinear responses of SiPMs at the level of a few percentages for a wide range of situations.

An analysis of double-quantum coherence ESR in an N-spin system: Analytical expressions and predictions.

Electron spin resonance pulsed dipolar spectroscopy (PDS) has become popular in protein 3D structure analysis. PDS studies yield distance distributions between a pair or multiple pairs of spin probes attached to protein molecules, which can be used directly in structural studies or as constraints in theoretical predictions. Double-quantum coherence (DQC) is a highly sensitive and accurate PDS technique to study protein structures in the solid state and under physiologically relevant conditions. In this work, we have derived analytical expressions for the DQC signal for a system with N-dipolar coupled spin-1/2 particles in the solid state. The expressions are integrated over the relevant spatial parameters to obtain closed form DQC signal expressions. These expressions contain the concentration-dependent "instantaneous diffusion" and the background signal. For micromolar and lower concentrations, these effects are negligible. An approximate analysis is provided for cases of finite pulses. The expressions obtained in this work should improve the analysis of DQC experimental data significantly, and the analytical approach could be extended easily to a wide range of magnetic resonance phenomena.

Optoacoustic interferometric characterization system (OPTICS) for the evaluation of fuel quality through speed of sound measurements

Ultrasonic techniques have been applied to assess crucial physical parameters in various types of fuels including the speed of sound (SoS), the bulk modulus and the acoustic attenuation coefficient. Such investigations may have important practical significance as the knowledge of fuel properties is directly related to the analysis of combustion characteristics, engine’s overall performance and exhaust emission in the environment. Nevertheless, typical pulse-echo acoustic methods, require the exact determination of both acoustic source – reflector distance and the time of flight of a finite temporal width ultrasonic pulse, setting thus an upper limit as regards the accuracy of the measurements. To encounter these challenges, we present a novel technology implemented through a low-cost and potentially portable optoacoustic interferometric characterization system (OPTICS) for the investigation of SoS variations in common fuels including automotive diesel, hydrous ethanol and gasoline. At 25 °C, diesel/kerosene blends demonstrated a SoS variation ranging from 1322.91 m/s (0.6 diesel volume fraction) to 1349.79 m/s (diesel fuel only), whereas hydrous ethanol samples varied between 1199.92 m/s (0.95 ethanol volume fraction) to 1149.39 m/s (pure ethanol only). Finally, assessments for 95 and 100 research octane number (RON) gasoline blends showed a SoS range from 1134.42 m/s (RON 95) to 1159.86 m/s (RON 100). The high precision and repeatability (relative uncertainty: ∼10-4) of the performed SoS measurements in controlled samples, has demonstrated the promising potential of OPTICS for the evaluation of fuel physical properties as well as the potential detection of contamination with adulterants.

Signatures of Dynamically Dressed States.

The interaction of a resonant light field with a quantum two-level system is of key interest both for fundamental quantum optics and quantum technological applications employing resonant excitation. While emission under resonant continuous-wave excitation has been well studied, the more complex emission spectrum of dynamically dressed states-a quantum two-level system driven by resonant pulsed excitation-has so far been investigated in detail only theoretically. Here, we present the first experimental observation of the complete resonance fluorescence emission spectrum of a single quantum two-level system, in the form of an excitonic transition in a semiconductor quantum dot, driven by finite Gaussian pulses. We observe multiple emerging sidebands as predicted by theory, with an increase of their number and spectral detuning with excitation pulse intensity and a dependence of their spectral shape and intensity on the pulse length. Detuning-dependent measurements provide additional insights into the emission features. The experimental results are in excellent agreement with theoretical calculations of the emission spectra, corroborating our findings.

Vortex γ photon generation via spin-to-orbital angular momentum transfer in nonlinear Compton scattering

Vortex γ photons with intrinsic orbital angular momenta possess a wealth of applications in various fields—e.g., strong-laser physics, nuclear physics, particle physics, and astrophysics—yet their generation remains unsettled. In this work, we investigate the generation of vortex γ photons via nonlinear Compton scattering of ultrarelativistic electrons in a circularly polarized laser pulse. We develop a quantum electrodynamics scattering theory that explicitly addresses the multiphoton absorption and the angular momentum transfer mechanism. In pulsed laser fields, we unveil the vortex phase structure of the scattering matrix element, discuss how the vortex phase could be transferred to the radiated photon, and derive the radiation rate of the vortex γ photon. We numerically examine the energy spectra and beam characteristics of the radiation, while also investigating the influence of finite laser pulses on the angular momentum and energy distribution of the emitted vortex γ photons. Published by the American Physical Society 2024

LIDAR Point Cloud Augmentation for Dusty Weather Based on a Physical Simulation

LIDAR is central to the perception systems of autonomous vehicles, but its performance is sensitive to adverse weather. An object detector trained by deep learning with the LIDAR point clouds in clear weather is not able to achieve satisfactory accuracy in adverse weather. Considering the fact that collecting LIDAR data in adverse weather like dusty storms is a formidable task, we propose a novel data augmentation framework based on physical simulation. Our model takes into account finite laser pulse width and beam divergence. The discrete dusty particles are distributed randomly in the surrounding of LIDAR sensors. The attenuation effects of scatters are represented implicitly with extinction coefficients. The coincidentally returned echoes from multiple particles are evaluated by explicitly superimposing their power reflected from each particle. Based on the above model, the position and intensity of real point clouds collected from dusty weather can be modified. Numerical experiments are provided to demonstrate the effectiveness of the method.

The Interplay of Common Noise and Finite Pulses on Biological Neurons

The response of neurons is highly sensitive to the stimulus. The stimulus can be associated with a direct injection in vitro experimentation (e.g., time dependent and independent inputs); or post-synaptic potentials resulting from the interaction of many neurons. A typical incoming stimulus resembles a noise which in principle can be described as a random variable. In computational neuroscience, the noise has been extensively studied for different setups. In this study, we investigate the effect of noisy inputs in a minimal network of two identical leaky integrate-and-fire (LIF) neurons interacting with finite pulses. In particular, we consider a Gaussian white noise as a standard function for stochastic modelling of neurons, while taking into account the pulse width as an elementary component for the signal transmission. By exploring the role of noise and finite pulses, the two neurons show a synchronous spiking behaviour characterized by fluctuations in the interspike intervals. Above some critical values the synchronous regime collapses onto asynchronous dynamics. The abrupt change in such dynamics is accompanied by a hysteresis, i.e., the coexistence of synchronous and asynchronous firing behaviour.

Pulse-controlled qubit in semiconductor double quantum dots

We present a numerically-optimized multipulse framework for the quantum control of a single-electron double quantum dot qubit. Our framework defines a set of pulse sequences, necessary for the manipulation of the ideal qubit basis, that avoids errors associated with excitations outside the computational subspace. A novel control scheme manipulates the qubit adiabatically, while also retaining high speed and ability to perform a general single-qubit rotation. This basis generates spatially localized logical qubit states, making readout straightforward. We consider experimentally realistic semiconductor qubits with finite pulse rise and fall times and determine the fastest pulse sequence yielding the highest fidelity. We show that our protocol leads to improved control of a qubit. We present simulations of a double quantum dot in a semiconductor device to visualize and verify our protocol. These results can be generalized to other physical systems since they depend only on pulse rise and fall times and the energy gap between the two lowest eigenstates.

Freestream Temperature Effects on the Receptivity of Hypersonic Boundary Layer Induced by Finite-Amplitude Pulse Entropy Waves

The unsteady hypersonic flow under finite amplitude pulse entropy perturbation at different freestream temperatures was calculated by direct numerical simulation. The flow response characteristics under the perturbation of entropy waves in freestreaming are analyzed. The temperature effect of freestreaming is studied based on the sensitivity of the boundary layer caused by pulse entropy perturbation. The results show that the higher freestream temperature promotes the first growth of the above third-order modes after leaving the head region, and strongly inhibits the first attenuation. The influence of the freestream temperature on the evolution of the induced disturbance wave is more significant than that on the development of the main flow disturbance waves. Low freestream temperature can suppress the attenuation of the modes below the second order. As the disturbance wave evolves downstream, the frequency band of the finite frequency disturbance wave gradually narrows, and the frequency band narrows faster when the temperature of freestreaming is low than when the temperature of freestreaming is high.

Multimode vibrational dynamics and orientational effects in fluorescence-encoded infrared spectroscopy. II. Analysis of early-time signals.

Developing fluorescence-encoded infrared (FEIR) vibrational spectroscopy for single-molecule applications requires a detailed understanding of how the molecular response and external experimental parameters manifest in the detected signals. In Paper I [L. Whaley-Mayda, A. Guha, and A. Tokmakoff, J. Chem. Phys. 159, 194201 (2023)] we introduced a nonlinear response function theory to describe vibrational dynamics, vibronic coupling, and transition dipole orientation in FEIR experiments with ultrashort pulses. In this second paper, we apply the theory to investigate the role of intermode vibrational coherence, the orientation of vibrational and electronic transition dipoles, and the effects of finite pulse durations in experimental measurements. We focus on measurements at early encoding delays-where signal sizes are largest and therefore of most value for single-molecule experiments, but where many of these phenomena are most pronounced and can complicate the appearance of data. We compare experiments on coumarin dyes with finite-pulse response function simulations to explain the time-dependent behavior of FEIR spectra. The role of the orientational response is explored by analyzing polarization-dependent experiments and their ability to resolve relative dipole angles in the molecular frame. This work serves to demonstrate the molecular information content of FEIR experiments, and develop insight and guidelines for their interpretation.

Two-photon double ionization with finite pulses: Application of the virtual sequential model to helium

Two-photon double ionization with finite pulses: Application of the virtual sequential model to helium