Pulse Front Research Articles

1.4‐mJ High Energy Terahertz Radiation from Lithium Niobates

AbstractFree‐space super‐strong terahertz (THz) electromagnetic fields offer multifaceted capabilities for reaching extreme nonlinear THz optics. However, the lack of powerful solid‐state THz sources with single pulse energy >1 mJ is impeding the proliferation of extreme THz applications. The fundamental challenge lies in hard to achieve high efficiency due to high intensity pumping caused crystal damage, linear absorption, and nonlinear distortion induced short effective interaction length, and so on. Here, through cryogenically cooling the crystals, tailoring the pump laser spectra, chirping the pump pulses, and magnifying the laser energies, 1.4‐mJ THz pulses are successfully realized in lithium niobates under the excitation of 214‐mJ femtosecond laser pulses via tilted pulse front technique. The 800 nm‐to‐THz energy conversion efficiency reaches 0.7%, and a free‐space THz peak electric and magnetic field reaches 6.3 MV cm−1 and 2.1 Tesla. Numerical simulations reproduce the experimental optimization processes. To show the capability of this super‐strong THz source, nonlinear absorption in high conductive silicon induced by strong THz electric field is demonstrated. Such a high‐energy THz source with a relatively low peak frequency is very appropriate not only for electron acceleration toward table‐top X‐ray sources but also for extreme THz science and nonlinear applications.

Ripple period adjustment on SiC surface based on electron dynamics control and its polarization anisotropy

In this paper, the Mach Zehnder interferometer is utilized to generate a collinear dual optical path with 800-nm center wavelength, 1 kHz repetition rate, 120-fs pulse duration and an energy ratio of 1:1 to scan 6H-SiC crystal at a scanning speed of 500 μm/s, resulting in laser-induced periodic surface structure (LIPSS). From the perspective of instantaneous electron density level, variation of the period of low spatial frequency LIPSS (LSFL) with interpulse delay time and polarization angle is studied. The scanning electron microscope (SEM) characterization of the line-scanned ablation zone combined with fast Fourier transformation (FFT) spectrum analysis shows that the period of LSFL decreases with the increase of delay time, and remains stable when the delay exceeds 240 fs. Meanwhile, the period of LSFL increases with the increase of polarization angle under the same delay time, showing an anisotropy that dependent on the polarization angle. The variation trend of the maximum electron density level with delay time calculated by electron rate equation is roughly consistent with the periodic variation trend. Interaction between incident light and transient metal-like SiC surface is simulated based on finite-difference time-domain method (FDTD). The simulation results show that the surface of the sample has a periodic light field enhancement structure controlled by the transient electron density, which explains the phenomenon that the period decreases with increasing delay time. It is further confirmed that the formation of LSFL is due to the interference of incident light and surface plasmon, and the period of LSFL can be controlled by adjusting the electron density level by delay time. The periodic polarization dependence of LSFL may be related to the relative orientation change of the laser pulse front tilt (PFT) and laser polarization.

Innovative single-shot 2D pulse front tilt diagnostic

Abstract The presence of pulse front tilt (PFT), caused by angular dispersion (AD) in femtosecond laser pulses, could degrade the performance of the laser system and/or impact the experimental yields. We present a single-shot diagnostic capable of measuring the AD in the x–y plane by adopting an intensity mask. It can be applied to stretched pulses, making it ideal for diagnosing the AD along the amplification chain of a high-power laser system, and to ultrashort pulses exiting from an optical compressor. In this way, it can help in properly characterizing a laser pulse before it is delivered to the target area. In this Letter, we present experimental evidence of AD retrieval for different compression configurations, supported by theoretical analysis.

Analysis of angular dispersion induced by wavefront rotation in nanosecond optical parametric chirped pulse amplification.

Angular dispersion observed in a nanosecond optical parametric chirped-pulse amplification (ns-OPCPA) amplifier adopted in the frontend of a multi-PW laser was analyzed. The theory on the angular dispersion, extended by including the wavefront rotation and the pulse front tilt of a strongly chirped laser pulse, revealed that the wavefront rotation is a major contributor to the angular dispersion, as compared to the pulse front tilt, in a ns-OPCPA amplifier. It was also shown that the wavefront rotation could be introduced by the phase mismatch and the noncollinear propagation angle in the noncollinear ns-OPCPA amplifier. The theoretical prediction was experimentally verified by measuring the angular dispersion of the ns-OPCPA frontend installed in the 20-fs, 4-PW Ti:Sapphire laser. We emphasize the importance of the proper characterization and control of the angular dispersion in the ns-OPCPA amplifier since the focus intensity of an ultrahigh power laser could be significantly reduced due to the spatiotemporal effect even for small induced angular dispersion.

Directly Measuring the Pulse Front Distortion of High-Peak-Power Femtosecond Lasers

Pulse front distortion occurring in lenses can broaden the temporal profile of the pulse at focus and therefore decrease the focused intensity, especially for large-aperture femtosecond lasers. A previously proposed self-reference cross correlator was improved to directly measure the pulse front distortion of high-peak-power femtosecond lasers. The measured results of a 200 TW/27 fs laser are in good accordance with the calculated value. Moreover, the temporal intensity distribution of the pulse in the focal region was also investigated, in order to better guide and further promote the strong laser-matter interaction investigations. According to the measured PFD, the effective pulse duration at far field of this 200 TW laser was theoretically simulated to be ≈49 fs, which is almost two times the generally regarded 27 fs. As a result, the actually available focused intensity of this laser is only 55% of the case without pulse front distortion.

Energy deposition parameters revealed in the transition from 3D to 1D femtosecond laser ablation of fluorite at high-NA focusing

Ultrashort-pulse laser surface and bulk nano- and micromachining of dielectrics have multiple promising applications in micro-optics, microfluidics, and memory storage. The fundamental principles relate intrinsic inter-band multi-photon (MPA) and laser-induced intra-band free-carrier absorption (FCA) to particular ablation mechanisms and features. These principles are yet to be quantified into a complete set of basic experimental laser-matter interaction parameters, describing photoexcitation, relaxation, and final ablation. In this study, we considered the characteristic double-crater structure of single-shot ablation spots on dielectric surfaces and single-shot transmission spectra to extract crucial information about the underlying basic processes of ultrafast photoexcitation and laser energy deposition. Specifically, energy-dependent crater profiles and accompanying prompt self-phase modulation (SPM) spectral broadening were studied in single-shot surface ablation experiments on fluorite (CaF2) surface photo-excited by tightly focused 515- or 1030-nm, 300-fs laser pulses. Crater size dependence demonstrated two slopes, scaling proportionally to the squared focal 1/e-radius at higher energies (intensities) for larger ablated spots, and a much smaller squared 1/e-radius at lower energies (intensities) for (sub) micron-wide ablated spots, indicating a transition from 1D to 3D-ablation. As a result, these slopes were related to lower-intensity wavelength-dependent multi-photon inter-band transitions and wavelength-independent higher-intensity linear absorption in the emerging near-critical electron-hole plasma (EHP), respectively. Crater depth dependences on the local laser intensity fitted in the corresponding ranges by multi- and one-photon absorption provided the corresponding absorption coefficients. Spectral broadening measurements indicated even values for the red and blue shoulders of the laser pulse spectrum, representing the SPM effect in the weakly excited fluorite at the leading pulse front and providing the corresponding Kerr coefficient. In the second regime, the blue-shoulder broadening value saturated, indicating the appearance of near-critical plasma screening at the trailing pulse front, which is consistent with our calculations. These complementary experiments and related analysis provided an important set of key basic parameters, characterizing not only surface ablation, but also propagation of high-intensity ultrashort laser pulses in bulk fluorite, and enabling precise forecasting of optimal energy deposition for high-efficiency ultrashort-laser micro-structuring of this dielectric material.

Terahertz photoconductive waveguide emitter with excitation by a tilted optical pulse front.

We explore the tilted-pulse-front excitation technique to control the superradiant emission of terahertz (THz) pulses from large-area photonconductive semiconductor switches. Two cases are studied. First, a photoconductive antenna emitting into free space, where the propagation direction of the optically generated THz beam is controlled by the choice of the tilt angle of the pump pulse front. Second, a THz waveguide structure with an integrated photoconductive window for the generation of THz radiation, where the injection of the THz radiation into a waveguide mode is optimized by the pulse front tilt. By providing long interaction lengths, such a waveguide-based optical-pump/THz-probe set-up may provide a new platform for the study of diverse short-lived optically induced excitations.

Long propagating velocity-controlled Einstein's mirror for terahertz light conversion.

We show that Einstein's relativistic mirror with long (hundreds of µm) propagation distance and controllable propagation velocity can be implemented in the form of a dense free carrier front generated by multiphoton absorption of tilted-pulse-front femtosecond laser pulses in a dielectric or semiconductor medium. The velocity control is achieved by varying the pulse front tilt angle. Simulations demonstrate that such fronts can serve as efficient Doppler-type converters of terahertz pulses. In particular, the pulse reflected from a front, generated by three-photon absorption of a Ti:sapphire laser in ZnS, can exhibit strong (up to more than an order of magnitude) pulse compression and spectrum broadening without a noticeable amplitude change. The proposed technique may be used to convert strong low-frequency terahertz pulses, generated by optical rectification of tilted-pulse-front laser pulses, to desirable temporal and spectral characteristics for a variety of applications.

Numerical study of sum frequency ultrashort pulse compression in borate crystals

Second harmonic generation (SHG) of picosecond pulses in type II phase-matched nonlinear optical crystals is not widely employed because of the lower efficiencies compared to the type I phase-matching scheme. The limited efficiencies come from the difference between group velocities (GV difference) of the ordinary and extraordinary polarized input pulses. However, if the input pulses are delayed before the nonlinear crystal, a short second harmonic pulse can be generated with a slowly widening temporal overlap. Furthermore, this GV difference can be controlled by the tilting of the pulse fronts, and optimal GV difference can be obtained to achieve powerful output pulses with durations an order of magnitude lower than those of the input pulses. In this work, we present numerical results of SHG pulse compression in a beta barium borate (BBO) nonlinear crystal, which is ideal for SHG of high-power 1030 nm thin-disk lasers. The pulse compression is controlled by predelay and tilting of the pulse fronts. We find optimal parameters to achieve five-fold increase in output power and 20-fold pulse compression of 1.7 ps input pulses. Finally, we consider the experimental aspects of the group velocity control.

The effect of negative feedback in multipoint nanosecond corona discharge

The results of studies on the use of low-temperature non-equilibrium plasma for the generation of ozone (O3) in air and oxygen are presented. The results were obtained at facilities called plasma ozonators (PO), in which O3 was generated by means of a nanosecond pulsed streamer corona discharge (NCD). The NCD was created in reactor chambers consisting of coaxially arranged high-voltage multi-pointed and grounded tubular electrodes. The high-voltage electrode was supplied with a pulse voltage generated by a three-stage Fitch frequency generator. The experiments used three types of PO with a capacity of 1–6 kW. The range of pulse amplitude was 50–75 kV, of pulse front duration was 150–250 ns, of pulse duration was 300–500 ns and of pulse repetition rate was 100–1000 Hz. The air flow through the PO varied from 10 to 1500 m3 h−1. It has been established that the NCD is a system with negative feedback (NFE). The effect of NFE is that O3 production with the help of NCD leads to a sharp decrease in corona streamer currents and energy introduced into the gas. Due to the effect of NFE with increasing O3 concentration, the efficiency of its operating time in PO decreases by 3–4 times. A possible mechanism of the NFE effect, which is uniquely related to the structure of the nanosecond streamer corona, is discussed.

Development of a five-stage solid-state linear transformer driver.

In this paper, the development of a five-stage solid-state linear transformer driver (LTD) is described. Each stage consists of eight compact pulse generating modules and a magnetic core. The pulse generating modules contain a multilayer-ceramic-capacitor-based pulse-forming network (PFN) and an insulated-gate bipolar transistor (IGBT) switch array, as well as magnetic switches, which are used to speed up the pulse front. To prevent damage from the reverse voltage to the IGBT switch, a reverse voltage absorption circuit was added to the PFN. For this study, a larger cross-sectional core with improved output characteristics was adopted. The developed five-stage LTD has the advantages of long life, low jitter, fast rising edge, and so on. The device can provide a 35 kV, 119 ns, 4.3 kA square pulse train with a maximum frequency of 50 Hz. On this basis, a 50-stage LTD of output 500 kV, which would serve as a high-power microwave driver source, is under development.

Propagation characteristics of a spatially chirped Gaussian laser beam propagating through multiple lenses

Variation of curvature of laser beam changes characteristics of spatially chirped pulsed Gaussian (SCPG) laser beam primarily due to varying spectral divergence. Parametric dependence of different pulse parameters, e.g. angular chirp, pulse front tilt, pulse width, beam radius, radius of curvature etc., is presented for a SCPG laser beam propagating through single and pair of reflective or refractive optical system. Effect of chromatic aberration on characteristic of SCPG laser beam have also been presented under different propagation conditions. Different expressions for various parameters of pulsed Gaussian beam are extended using recursive relation for a sequence of multiple chromatic lenses generally used in large scale high energy high power laser system. Discussion is supported with few examples of lens system.

A methodology of evaluation of metal surface vibration amplitude at current pulse fronts at electropulse impact

A methodology of evaluation of metal surface vibration amplitude at current pulse fronts at electropulse impact

Optimization of Electric Thrust Based on Pulse Arc Plasma Using Pulsed Magnetic Field

Based on the results of a numerical simulation, a possibility in principle is shown to achieve an effective magneto-induction correction of high-gradient plasma expansion from a localized arc source and a respective severalfold increase in the thrust pulse with a steepness of the induction rise in the accelerator on the order of 104 T/s. In these conditions, a pulse-periodic mode of the device operation is required with a delay of the current pulse front in the magnetic field source relative to the ignition voltage pulse in the plasma source, which is determined by the expansion velocity of the plasma cloud within the device.

Enabling high repetition rate nonlinear THz science with a kilowatt-class sub-100 fs laser source.

Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical phenomena in solid state and atomic physics. Recent upgrades of x-ray FEL facilities are pushing to much higher repetition rates, enabling unprecedented signal-to-noise ratio for pump probe experiments. This requires the development of suitable THz pump sources that are able to deliver intense pulses at compatible repetition rates. Here we present a high-power laser-driven THz source based on optical rectification in LiNbO3 using tilted pulse front pumping. Our source is driven by a kilowatt-level Yb:YAG amplifier system operating at 100 kHz repetition rate and employing nonlinear spectral broadening and recompression to achieve sub-100 fs pulses with pulse energies up to 7 mJ that are necessary for high THz conversion efficiency and peak field strength. We demonstrate a maximum of 144 mW average THz power (1.44 μJ pulse energy), consisting of single-cycle pulses centered at 0.6 THz with a peak electric field strength exceeding 150 kV/cm. These high field pulses open up a range of possibilities for nonlinear time-resolved THz experiments at unprecedented rates.

High-power picosecond deep-UV source via group velocity matched frequency conversion

Powerful ultrashort pulses in the deep-ultraviolet (deep-UV) are beneficial for diverse applications from fundamental science to industrial materials processing. However, reaching high powers via conventional approaches is challenging due to three central issues: dispersion, multiphoton absorption, and optical damage. Here, we simultaneously overcome these issues with a novel fifth-harmonic generation architecture optimized for group velocity matching. We use tilted pulse fronts, including a noncollinear geometry in the final sum-frequency generation stage. This enables lower intensities and longer crystals, thereby favoring the birefringently phase matched χ ( 2 ) process over higher-order multiphoton absorption processes. Moreover, we demonstrate low-loss cascaded χ ( 2 ) -based spatiotemporal flattening of the input pulses, which enhances the uniformity of the conversion efficiency throughout the beam profile. Through these techniques, we realize a picosecond deep-UV generation source at 206 nm with record-high 2.5 W average output power and a repetition rate of 100 kHz. This result paves the way for a new era of high-power ultrafast deep-UV lasers.

Single-cycle, MHz repetition rate THz source with 66 mW of average power.

We demonstrate terahertz (THz) generation using the tilted pulse front method in lithium niobate, driven at an unprecedented high average power of more than 100 W and at a 13.3 MHz repetition rate, provided by a compact amplifier-free mode-locked thin-disk oscillator. The conversion efficiency was optimized with respect to the pump spot size and pump pulse duration, enabling us to generate a maximum THz average power of 66 mW, which is, to the best of our knowledge, the highest reported to date from a laser-driven, few-cycle THz source. Furthermore, we identify beam walk-off as the main obstacle that currently limits the conversion efficiency in this excitation regime (with moderate pulse energies and small spot sizes). Further upscaling to the watt level and beyond is within reach, paving the way for linear and nonlinear high average power THz spectroscopy experiments with an exceptional signal-to-noise ratio at megahertz repetition rates.

Design of an amplitude-splitting hard x-ray delay line with subnanoradian stability.

We present the design and analysis of a hard x-ray split-delay optical arrangement that combines diffractive and crystal optics. Transmission gratings are employed to achieve the much-desired amplitude splitting and recombination of the beam. Asymmetric channel-cut crystals are utilized to tune the relative delay time. The use of a dispersion-compensation arrangement of the crystals allows the system to achieve subnanoradian pointing stability during a delay scan. It also minimizes wavefront distortion and preserves the pulse front and pulse duration. We analyze the performance of a prototype design that can cover a delay time range of 15 ps with a sub-20 fs time resolution at 10 keV. We anticipate that this system can fully satisfy the very demanding stability requirements for performing split-pulse x-ray photon correlation spectroscopy measurements for the investigation of fast atomic scale dynamics in complex disordered matter.

Absorption and opacity threshold for a thin foil in a strong circularly polarized laser field.

We show that a commonly accepted transparency threshold for a thin foil in a strong circularly polarized normally incident laser pulse needs a refinement. We present an analytical model that correctly accounts for laser absorption. The refined threshold is determined not solely by the laser amplitude, but by other parameters that are equally or even more important. Our predictions are in perfect agreement with particle-in-cell simulations. The refined criterion is crucial for configuring laser plasma experiments in the high-field domain. In addition, an opaque foil steepens the pulse front, which can be important for numerous applications.

Investigation of the possibility to use GaAs Hall-effect sensors in active magnetic positioning systems

The paper focuses on the investigation of the possibility to use GaAs Hall-effect sensors (detectors) in active magnetic positioning systems. On the basis of the avalanche S-diode a pulsed magnetic field generator with the pulse front width of 0.3 ns and the current of 10–300 A has been developed. The work studies Hall-effect sensor transient fenomena which transient time is equal to 0.4 ns. The Hall-effect sensor noise in ultra-wide frequency band is estimated. The investigation shows that it is possible to use Hall-effect sensors in active magnetic positioning systems with the operational range of up to 1 m and a few-centimeter spatial resolution.