Prethermal State Research Articles

Anomalous diffusion, prethermalization, and particle binding in an interacting flat band system

We study the broadening of initially localized wave packets in a quasi one-dimensional diamond ladder with interacting, spinless fermions. The lattice possesses a flat band causing localization. We place special focus on the transition away from the flat band many-body localized case by adding very weak dispersion. By doing so, we allow propagation of the wave packet on significantly different timescales which causes anomalous diffusion. Due to the temporal separation of dynamic processes, an interaction-induced, prethermal equilibrium becomes apparent. A physical picture of light and heavy modes for this prethermal behavior can be obtained within Born–Oppenheimer approximation via basis transformation of the original Hamiltonian. This reveals a detachment between light, symmetric and heavy, anti-symmetric particle species. We show that the prethermal state is characterized by heavy particles binding together mediated by the light particles.

Reconstructing effective Hamiltonians from nonequilibrium thermal and prethermal steady states

Reconstructing Hamiltonians from local measurements is key to enabling reliable quantum simulations: both validating the implemented model and identifying any leftover terms with sufficient precision is a problem of increasing importance. Here we propose a deep-learning-assisted variational algorithm for Hamiltonian reconstruction by preprocessing a dataset that is diagnosed to contain thermal measurements of local operators. We demonstrate the efficient and precise reconstruction of local Hamiltonians, while long-range interacting Hamiltonians are reconstructed approximately. Away from equilibrium, for periodically and random multipolar driven systems, we reconstruct the effective Hamiltonian widely used for Floquet engineering of metastable steady states. Moreover, our approach allows us to reconstruct an effective quasilocal Hamiltonian even in the heating regime beyond the validity of the prethermal plateau, where perturbative expansions fail. Published by the American Physical Society 2024

Prethermalization in an open quantum system coupled to a spatially correlated bosonic bath

A nearly-integrable isolated quantum many-body system reaches a quasi-stationary prethermal state before a late thermalization. Here, we revisit a particular example in the settings of an open quantum system (OQS). We consider a collection of non-interacting atoms coupled to a spatially correlated bosonic bath characterized by a bath correlation length. Our result implies that the integrability of the system depends on such a correlation length. If this length is much larger than the distance between the atoms, such a system behaves as a nearly-integrable OQS. We study the properties of the emerging prethermal state for this case, i.e. the state’s lifetime, the extensive number of existing quasi-conserved quantities, the emergence of the generalized Gibbs state, and the scaling of von Neumann entropy, etc. We find that for the prethermal state, the maximum growth of entropy is logarithmic with the number of atoms, whereas such growth is linear for the final steady state, which is the Gibbs state in this case. Finally, we discuss how such prethermal states can have significant applications in quantum entanglement storage devices.

Emergence of prethermal states in a driven dissipative system through cross-correlated dissipation

Periodically driven closed quantum many-body systems are known to exhibit prethermal or quasi-steady-state dynamics. In this work, we theoretically show that such prethermal phases can appear in the dynamics of a dipolar two-spin-1/2 system coupled to a heat bath if the cross terms between the drive and dipolar interactions are taken into consideration. To this end, we use our recently reported fluctuation-regulated quantum master equation (Chakrabarti A. and Bhattacharyya R., Phys. Rev. A 97 (2018) 063837), to show that the predicted dynamics can successfully explain the experimentally observed features of the transient and prethermal regime.

Cascaded dynamics of a periodically driven dissipative dipolar system

Recent experiments show that periodic drives on dipolar systems lead to long-lived prethermal states. These systems are weakly coupled to the environment and reach prethermal states in a timescale much shorter than the timescale for thermalization. Such nearly-closed systems have previously been analyzed using Floquet formalism, which shows the emergence of a prethermal plateau. We use a fluctuation-regulated quantum master equation (FRQME) to describe these systems. In addition to the system-environment coupling, FRQME successfully captures the dissipative effect from the various local interactions in the system. Our investigation reveals a cascaded journey of the system to a final steady state. The cascade involves a set of prethermal or arrested states characterized by a set of quasi-conserved quantities. We show that these prethermal states emerge in a timescale much shorter than the relaxation timescale. We also find and report the existence of a critical limit beyond which the prethermal plateau ceases to exist.

Prethermalization in one-dimensional quantum many-body systems with confinement

Unconventional nonequilibrium phases with restricted correlation spreading and slow entanglement growth have been proposed to emerge in systems with confined excitations, calling their thermalization dynamics into question. Here, we show that in confined systems the thermalization dynamics after a quantum quench instead exhibits multiple stages with well separated time scales. As an example, we consider the confined Ising spin chain, in which domain walls in the ordered phase form bound states reminiscent of mesons. The system first relaxes towards a prethermal state, described by a Gibbs ensemble with conserved meson number. The prethermal state arises from rare events in which mesons are created in close vicinity, leading to an avalanche of scattering events. Only at much later times a true thermal equilibrium is achieved in which the meson number conservation is violated by a mechanism akin to the Schwinger effect. The discussed prethermalization dynamics is directly relevant to generic one-dimensional, many-body systems with confined excitations.

Prethermalization via self driving and external driving of extensive subsystems

We investigate the nonequilibrium states of an interacting multicomponent quantum system when only an extensive subsystem is quantum quenched or driven from the ground state. As a concrete example, we consider a system where two XXZ spin chains are coupled to a transverse field Ising (TFI) chain, and only the transverse field in the TFI chain is quantum quenched or periodically driven in time, starting from an initially ordered state. This system is studied using density matrix renormalization group simulations and various entanglement entropy diagnostics. In the case of quantum quenching, when the transverse field is suddenly switched on to become the largest energy scale, the resulting internal dynamics leads to a prethermal steady state with persistent oscillating magnetization (``self driving'') and emergent conservation laws. Upon applying the time-dependent drive to the TFI chain (``external driving''), sufficiently fast drive gives rise to a prethermal steady state with finite magnetization, whereas a slow drive generates a high-temperature disordered state. We briefly discuss the experimental implementation of our protocol in organic materials with quantum-tunneling hydrogen atoms.

Topological order and entanglement dynamics in the measurement-only XZZX quantum code

We examine the dynamics of a $(1+1)$-dimensional measurement-only circuit defined by the stabilizers of the [[5,1,3]] quantum error correcting code interrupted by single-qubit Pauli measurements. The code corrects arbitrary single-qubit errors and it stabilizes an area law entangled state with a ${D}_{2}={\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}$ symmetry protected topological (SPT) order, as well as a symmetry breaking (SB) order from a twofold bulk degeneracy. The Pauli measurements break the topological order and induce a phase transition into a trivial area law phase. Allowing more than one type of Pauli measurement increases the measurement-induced frustration and the SPT and SB order can be broken either simultaneously or separately at nonzero measurement rate. This yields a rich phase diagram and unanticipated critical behavior at the phase transitions. Although the correlation length exponent $\ensuremath{\nu}=\frac{4}{3}$ and the dynamical critical exponent $z=1$ are consistent with bond percolation, the prefactor of the logarithmic entanglement growth may take noninteger multiples of the percolation value. Remarkably, we identify a robust transient scaling regime for the purification dynamics of $L$ qubits. It reveals a modified dynamical critical exponent ${z}^{*}\ensuremath{\ne}z$, which is observable up to times $t\ensuremath{\sim}{L}^{{z}^{*}}$ and is reminiscent of the relaxation of critical systems into a prethermal state.

Nonequilibrium Prethermal States in a Two-Dimensional Photon Fluid.

We report on the observation of a prethermal state in a nonequilibrium, two-dimensional fluid of light. Direct measurements of the first order coherence function of the fluid reveal the dynamical emergence of algebraic correlations, a quasi-steady-state with properties close to those of thermal superfluids. By a controlled increase of the fluctuations, we observe a crossover from algebraic to short-range (exponential) correlations. We interpret this phenomenon as a nonequilibrium precursor of the Kosterlitz-Thouless transition.

Fractional resonances and prethermal states in Floquet systems

In periodically driven quantum systems, resonances can induce exotic nonequilibrium behavior and new phases of matter without static analog. We report on the emergence of fractional and integer resonances in a broad class of many-body Hamiltonians with a modulated hopping with a frequency that is either a fraction or an integer of the on-site interaction. We contend that there is a fundamental difference between these resonances when interactions bring the system to a Floquet prethermal state. Second-order processes dominate the dynamics in the fractional resonance case, leading to less entanglement and more localized quantum states than in the integer resonance case dominated by first-order processes. We demonstrate the dominating emergence of fractional resonances using the Magnus expansion of the effective Hamiltonian and quantify their effects on the many-body dynamics via quantum states' von Neumann entropy and Loschmidt echo. Our findings reveal novel features of the nonequilibrium quantum many-body system, such as the coexistence of Floquet prethermalization and localization, that may allow to development of quantum memories for quantum technologies and quantum information processing.

Thermal control of the topological edge flow in nonlinear photonic lattices

The chaotic evolution resulting from the interplay between topology and nonlinearity in photonic systems generally forbids the sustainability of optical currents. Here, we systematically explore the nonlinear evolution dynamics in topological photonic lattices within the framework of optical thermodynamics. By considering an archetypical two-dimensional Haldane photonic lattice, we discover several prethermal states beyond the topological phase transition point and a stable global equilibrium response, associated with a specific optical temperature and chemical potential. Along these lines, we provide a consistent thermodynamic methodology for both controlling and maximizing the unidirectional power flow in the topological edge states. This can be achieved by either employing cross-phase interactions between two subsystems or by exploiting self-heating effects in disordered or Floquet topological lattices. Our results indicate that photonic topological systems can in fact support robust photon transport processes even under the extreme complexity introduced by nonlinearity, an important feature for contemporary topological applications in photonics.

Universal scaling at a prethermal dark state

Recent experimental and theoretical progress as well as the prospect of commercially viable quantum technologies have inspired great interest in the study of open quantum systems and their dynamics. Many open quantum systems are well described by an effective non-Hermitian Hamiltonian generating a time evolution that allows eigenstates to decay and dissipate to the environment. In this framework, quantum coherent scaling is traditionally tied to the appearance of dark states, where the effect of dissipation becomes negligible. Here, we discuss the universal dynamical scaling after a sudden quench of the non-Hermitian $O(N)$ model Hamiltonian. While universality is generally spoiled by non-Hermiticity, we find that for a given set of internal parameters short-time scaling behavior is restored with an initial slip exponent profoundly different from that of closed quantum systems. This result is tied to the compensation of dissipation by interaction effects at short times leading to a prethermal dark state, where coherent many-body dynamics can be still observed.

From prethermalization to chaos in periodically driven coupled rotors

Periodically driven (Floquet) systems are said to prethermalize when their energy absorption is very slow for long time. This effect was first discovered in quantum spin models, where the heating rate is exponentially small in the ratio between the driving frequency and the spin bandwidth. Recently, it was shown that prethermalization occurs also in classical systems with an infinite bandwidth. Here, we address the open question of which small parameter controls the lifetime of the prethermal state in these systems. We, first, numerically study the dependence of the lifetime on the initial conditions and on the connectivity in a system of periodically driven coupled rotors. We find that the lifetime is controlled by the temperature of the prethermal state, which is quasi-conserved when the heating is slow. This finding allows us to develop a simple analytical model that describes the crossover from prethermalization to chaos in many-body classical systems.

Absence of Heating in a Uniform Fermi Gas Created by Periodic Driving

Ultracold atomic gas provides a useful tool to explore many-body physics. One of the recent additions to this experimental toolbox is the Floquet engineering, where periodic modulation of the Hamiltonian allows the creation of effective potentials that do not exist otherwise. When subject to external modulations, however, generic interacting many-body systems absorb energy, thus posing a heating problem that may impair the usefulness of this method. For discrete systems with bounded local energy, an exponentially suppressed heating rate with the driving frequency has been observed previously, leaving the system in a prethermal state for exceedingly long durations. But for systems in continuous space, the situation remains unclear. Here we show that Floquet engineering can be employed to a strongly interacting degenerate Fermi gas held in a flat box-like potential without inducing excessive heating on experimentally relevant timescales. The driving eliminates the effect of a spin-dependent potential originating from a simultaneous magnetic levitation of two different spin states. We calculate the heating rate and obtain a power-law suppression with the drive frequency. To further test the many-body behavior of the driven gas, we measure both the pair-condensation fraction at unitarity and the contact parameter across the BEC-BCS crossover. At low driving frequencies, the condensate fraction is reduced by the time-dependent force, but at higher frequencies, it revives and attains an even higher value than without driving. Our results are promising for future exploration of exotic many-body phases of a bulk strongly-interacting Fermi gas with dynamically engineered Hamiltonians.

Floquet Prethermalization with Lifetime Exceeding 90s in a Bulk Hyperpolarized Solid.

We report the observation of long-lived Floquet prethermal states in a bulk solid composed of dipolar-coupled ^{13}C nuclei in diamond at room temperature. For precessing nuclear spins prepared in an initial transverse state, we demonstrate pulsed spin-lock Floquet control that prevents their decay over multiple-minute-long periods. We observe Floquet prethermal lifetimes T_{2}^{'}≈90.9 s, extended >60 000-fold over the nuclear free induction decay times. The spins themselves are continuously interrogated for ∼10 min, corresponding to the application of ≈5.8×10^{6} control pulses. The ^{13}C nuclei are optically hyperpolarized by lattice nitrogen vacancy centers; the combination of hyperpolarization and continuous spin readout yields significant signal-to-noise ratio in the measurements. This allows probing the Floquet thermalization dynamics with unprecedented clarity. We identify four characteristic regimes of the thermalization process, discerning short-time transient processes leading to the prethermal plateau and long-time system heating toward infinite temperature. This Letter points to new opportunities possible via Floquet control in networks of dilute, randomly distributed, low-sensitivity nuclei. In particular, the combination of minutes-long prethermal lifetimes and continuous spin interrogation opens avenues for quantum sensors constructed from hyperpolarized Floquet prethermal nuclei.

Floquet prethermalization and Rabi oscillations in optically excited Hubbard clusters

We study the properties of Floquet prethermal states in two-dimensional Mott-insulating Hubbard clusters under continuous optical excitation. With exact-diagonalization simulations, we show that Floquet prethermal states emerge not only off resonance, but also for resonant excitation, provided a small field amplitude. In the resonant case, the long-lived quasi-stationary Floquet states are characterized by Rabi oscillations of observables such as double occupation and kinetic energy. At stronger fields, thermalization to infinite temperature is observed. We provide explanations to these results by means of time-dependent perturbation theory. The main findings are substantiated by a finite-size analysis.

Rigorous Bounds on the Heating Rate in Thue-Morse Quasiperiodically and Randomly Driven Quantum Many-Body Systems.

The nonequilibrium quantum dynamics of closed many-body systems is a rich yet challenging field. While recent progress for periodically driven (Floquet) systems has yielded a number of rigorous results, our understanding on quantum many-body systems driven by rapidly varying but aperiodic and quasiperiodic driving is still limited. Here, we derive rigorous, nonperturbative, bounds on the heating rate in quantum many-body systems under Thue-Morse quasiperiodic driving and under random multipolar driving, the latter being a tunably randomized variant of the former. In the process, we derive a static effective Hamiltonian that describes the transient prethermal state, including the dynamics of local observables. Our bound for Thue-Morse quasiperiodic driving suggests that the heating time scales like (ω/g)^{-C ln(ω/g)} with a positive constant C and a typical energy scale g of the Hamiltonian, in agreement with our numerical simulations.

Accelerated gap collapse in a Slater antiferromagnet

We study the melting of long-range antiferromagnetic order in the Hubbard model after an interaction quench, using non-equilibrium dynamical mean-field theory. From previous studies, the system is known to quickly relax into a prethermal symmetry-broken state. Using a convergent truncation of the memory integrals in the Kadanoff Baym equations, we unravel the subsequent relaxation dynamics of this state over several orders of magnitude in time. At long times, the prethermal state can be characterized by a single slow variable which is related to the conduction band population. The dynamics of this variable does not follow the paradigmatic steady relaxation of pre-thermal states: It is highly nonlinear, with a pronounced speedup once the gap falls below a certain value. This behavior indicates that non-thermal order can be self-stabilized on some timescale. It is not reproduced using simple Fermi's golden rule estimate for the evolution of the conduction band population.

Topological pumping of a 1D dipolar gas into strongly correlated prethermal states.

Long-lived excited states of interacting quantum systems that retain quantum correlations and evade thermalization are of great fundamental interest. We create nonthermal states in a bosonic one-dimensional (1D) quantum gas of dysprosium by stabilizing a super-Tonks-Girardeau gas against collapse and thermalization with repulsive long-range dipolar interactions. Stiffness and energy-per-particle measurements show that the system is dynamically stable regardless of contact interaction strength. This enables us to cycle contact interactions from weakly to strongly repulsive, then strongly attractive, and finally weakly attractive. We show that this cycle is an energy-space topological pump (caused by a quantum holonomy). Iterating this cycle offers an unexplored topological pumping method to create a hierarchy of increasingly excited prethermal states.

Floquet prethermalization in dipolar spin chains

Periodically driven Floquet quantum systems provide a promising platform to investigate novel physics out of equilibrium. Unfortunately, the drive generically heats up the system to a featureless infinite temperature state. For large driving frequency, the heat absorption rate is predicted to be exponentially small, giving rise to a long-lived prethermal regime which exhibits all the intriguing properties of Floquet systems. Here we experimentally observe Floquet prethermalization using nuclear magnetic resonance techniques. We first show the relaxation of a far-from-equilibrium initial state to a long-lived prethermal state, well described by the time-independent ''prethermal'' Hamiltonian. By measuring the autocorrelation of this prethermal Hamiltonian we can further experimentally confirm the predicted exponentially slow heating rate. More strikingly, we find that in the timescale when the effective Hamiltonian picture breaks down, the Floquet system still possesses other quasi-conservation laws. Our results demonstrate that it is possible to realize robust Floquet engineering, thus enabling the experimental observation of non-trivial Floquet phases of matter.