Polarization Of Incident Light Research Articles

Room temperature mid-wave infrared guided mode resonance InAsSb photodetectors

We demonstrate room temperature operation of mid-wave infrared photodetectors leveraging a guided mode resonance architecture and bulk alloy InAsSb absorbers. Room temperature operation with low dark current is achieved by using detector structures with ultra-thin (150, 250 nm) absorbers leveraging the strong confinement enabled by the guided mode architecture. Devices with 1D and 2D grating arrays are fabricated and characterized, and compared to unpatterned detector devices. We see enhancement in the detectors’ optical response associated with coupling to both TE- and TM-polarized guided modes and good agreement between experimental and theoretically-predicted behavior. We show strong enhancement for unpolarized light incident on 2D grating arrays, with a broader spectral response than observed for polarized light incident upon 1D grating GMR detectors. The bulk InAsSb detectors presented in this work offer enhanced performance at room temperature for a range of imaging and sensing applications.

High-Performance Planar Broadband Hot-Electron Photodetection through Platinum-Dielectric Triple Junctions.

Recently, planar and broadband hot-electron photodetectors (HE PDs) were established but exhibited degraded performances due to the adoptions of the single-junction configurations and the utilizations of absorbable films with thicknesses larger than the electronic mean free path. In this work, we present a five-layer design for planar HE PDs assisted by triple junctions in which an ultrathin Pt layer dominates the broadband and displays strong optical absorption (>0.9 from 900 nm to 1700 nm). Optical studies reveal that the optical admittance matching between optical admittances of designed device and air at all interested wavelengths is responsible for broadband light-trapping that induces prominent energy depositions in Pt layers. Electrical investigations show that, benefitting from suppressed hot-electron transport losses and increased hot-electron harvesting junctions, the predicted responsivity of the designed HE PD is up to 8.51 mA/W at 900 nm. Moreover, the high average absorption (responsivity) of 0.96 (3.66 mA/W) is substantially sustained over a broad incidence angle regardless of the polarizations of incident light. The comparison studies between five-layer and three-layer devices emphasize the superiority of five-layer design in strong optical absorption in Pt layers and efficient hot-electron extraction.

Mie Magnetic Structural Colors from Short Chains of TiO2 Nanospheres.

We demonstrate distinctive structural colors within a small footprint by using a short chain of nanospheres. Rather than using high-index materials like Si (n ∼ 4), which ensure strong modal confinement, TiO2 is employed. TiO2 has an intermediate index (n ∼ 2), promoting stronger modal coupling between the magnetic dipoles of each particle. This approach enables selective engineering of the magnetic response and yields larger spectral changes compared to that of Si. Despite the lower refractive index, the absence of absorption in TiO2 also produces higher scattering intensities than Si. We develop a quasistatic analytical model that describes the dipolar modal coupling in a trimer and use it to reveal distinct magnetic field strengths in the outer or central particle depending on the polarization of incident light. These results suggest pathways to manipulate the magnetic field in chains of particles and create vibrant structural colors with simple configurations.

A Novel Incident Circular Polarized Light Raman Optical Activity (ICP‐ROA) Spectrometer With Advanced Polarization Control

ABSTRACTThe design and setup of a novel and simple backscatter Raman optical activity (ROA) spectrometer with incident light circular polarization (ICP) is presented, constructed from commercially available components. Incident light polarization is controlled using a combination of waveplates, compensating for unwanted birefringence and beam offsets. Realignment of the spectra in post‐processing reduced artifacts caused by spatial offsets. Spurious signals from achiral solvents like toluene and water are almost completely removed. The setup was validated by measuring references samples, including α‐pinene, carvone, and glucose in aqueous solution. The spectra show very good agreement with previously published results.

Research on sensing characteristics of high Q-factor all-dielectric metasurfaces based on geometric breaking

The bound states in the continuum (BIC) are widely used in designing metamaterials with high quality factor (Q-factor) resonances due to their perfect localization in the continuous spectral range coexisting with expanding waves. In this study, a T-shaped nanohole all-dielectric metasurface structure is proposed based on the unique electromagnetic properties of all-dielectric metasurfaces, and the fundamental reason of its coupled state and the theoretical basis of BIC excitation are deeply investigated based on the theory of group theory, and the geometric symmetry is broken from multiple angles, and the coupling relationship between discrete eigenmodes and the external continuum is specifically analyzed during the change of symmetry, its spectral response and near-field distribution are numerically calculated. In addition, based on the modulation mechanism of the incident light polarization angle, the three-channel resonance tuning with two resonances of the same frequency and one of a different frequency is realized under the condition that the resonance position and the Q-factor are not affected. This study not only provides a theoretical basis for the excitation conditions and evolution regularity of symmetry-protected BIC, but also solves the problem in the traditional analysis of resonance phenomena without taking the high Q-factor and stability into account, which can provide new designing methods for optical metasurface devices with multi-channel resonance.

Enhancing phase modulation and group delay in reflective Huygens metasurfaces via a Fabry-Perot cavity

Huygens metasurfaces exhibit excellent optical properties such as 2π phase modulation and slow light effects. However, they face challenges including wide bandwidth and low group delay due to their high radiation losses. Here, we propose a reflective Huygens metasurface coupled with an F-P cavity. We demonstrate that F-P resonance modes can couple with magnetic-quasi-bound-state (M-QBIC) and electric-quasi-bound-state (E-QBIC) in the Huygens metasurface through constructive interference, significantly enhancing the quality factors of both QBICs. Through structural parameter optimization, our reflective Huygens metasurface achieves 4π phase modulation and a high group delay of up to 166 ps. Compared to the non-coupled Huygens metasurface with the same structural asymmetry, the group delay of the F-P coupled reflective Huygens metasurface is enhanced by up to 30 times. Our design reduces the fabrication precision requirements for Huygens metasurfaces, enabling similar group delays to be achieved in low-symmetry coupling structures as in highly symmetric non-coupling structures. Additionally, the performance of this metasurface shows robustness to changes in incident light polarization. This design highlights the potential for achieving high-quality factors, large phase modulation, and large group delay, offering new avenues for the design of highly sensitive tunable devices, efficient nonlinear optical devices, and narrowband slow light devices.

Design of Compact Dielectric Metalens Visor for Augmented Reality Using Spin-Dependent Supercells

Augmented reality overlays computer-generated virtual information onto real-world scenes, enhancing user interaction and perception. However, traditional augmented reality optical systems are usually large, bulky, and have limited optical performance. In this paper, we propose a novel compact monochrome reflective dielectric metalens visor with see-through properties, engineered using a periodic structure of spin-dependent supercells. The supercell, which is composed of staggered twin nanofins, provides spin-dependent destructive or constructive interference with different circularly polarized incidences. The design combines the principles of interference with the Pancharatnam–Berry phase to enhance reflection at a working wavelength of 650 nm while maintaining good transmission. Right circularly polarized light incident from the substrate side causes destructive interference, enabling the supercell to work in reflection mode, while left circularly polarized light causes constructive interference, enabling the supercell to work in transmission mode. Furthermore, the supercell-constructed metalens can achieve near-diffraction-limited reflective focusing and a broad diagonal field of view of approximately 96°. In addition, compared to transmissive metalens visors, the reflective design eliminates the need for a beam splitter, significantly reducing the size and weight of the system. Our work could facilitate the development of compact and lightweight imaging systems and provide valuable insights for augmented reality near-eye display applications.

Infrared routing and switching with tunable spectral bandwidth using arrays of metallic nanoantennas.

We study infrared routing and switching with tunable spectral bandwidth using in-plane scattering of light by flat Au nanoantenna arrays. The base dimensions of these nanoantennas are approximately 250 by 850 nm, while their heights vary from 20 to 150 nm. Our results show that, with the increase in height, the arrays become more efficient scatterers while their spectra broaden within the 1-1.6 $\mu$m range. Our findings demonstrate that such processes strongly depend on the incident light polarization. For a given polarization, the incident light is efficiently scattered in only two opposite directions along the plane of the arrays, with insignificant transmission. Switching such a polarization by 90$^\circ$, however, suppresses this process, allowing the light to mostly pass through the arrays with minimal scattering. These unique characteristics suggest a tunable beam splitter application in the 1-1.6 $\mu$m range and even longer wavelengths.

Dark-field microscopy studies of single silicon nanoparticles fabricated by e-beam evaporation technique: effect of thermal annealing, polarization of light and deposition parameters.

Herein, we report the dark-field microscopic studies on single silicon nanoparticles (SiNPs) fabricated using different deposition parameters in the electron beam (e-beam) evaporation technique. The morphology of the fabricated SiNPs is studied using the Atomic Force Microscope. Later, for the first time, the effect of thermal annealing and deposition parameters (i.e., beam current and deposition time) on the far-field scattering images and spectra of single SiNPs is studied using a transmission-mode dark-field optical microscope to estimate the wavelength locations and full-width at half maxima of the optical resonances of single SiNPs. Finally, the role of polarization of incident light on the optical resonances of single SiNPs is also studied by recording their scattering images and spectra.&#xD.

Distribution of Single-Particle Resonances Determines the Plasmonic Response of Disordered Nanoparticle Ensembles.

Understanding how colloidal soft materials interact with light is crucial to the rational design of optical metamaterials. Electromagnetic simulations are computationally expensive and have primarily been limited to model systems described by a small number of particles-dimers, small clusters, and small periodic unit cells of superlattices. In this work we study the optical properties of bulk, disordered materials comprising a large number of plasmonic colloidal nanoparticles using Brownian dynamics simulations and the mutual polarization method. We investigate the far-field and near-field optical properties of both colloidal fluids and gels, which require thousands of nanoparticles to describe statistically. We show that these disordered materials exhibit a distribution of particle-level plasmonic resonance frequencies that determines their ensemble optical response. Nanoparticles with similar resonant frequencies form anisotropic and oriented clusters embedded within the otherwise isotropic and disordered microstructures. These collectively resonating morphologies can be tuned with the frequency and polarization of incident light. Knowledge of particle resonant distributions may help to interpret and compare the optical responses of different colloidal structures, correlate and predict optical properties, and rationally design soft materials for applications harnessing light.

Axion‐Like Interactions and CFT in Topological Matter, Anomaly Sum Rules and the Faraday Effect

AbstractFundamental aspects of chiral anomaly‐driven interactions in conformal field theory (CFT) in four spacetime dimensions are discussed. These interactions find application in very general contexts, from early universe plasma to topological condensed matter. The key shared characteristics of these interactions are outlined, specifically addressing the case of chiral anomalies, both for vector currents and gravitons. In the case of topological materials, the gravitational chiral anomaly is generated by thermal gradients via the (Tolman–Ehrenfest) Luttinger relation. In the CFT framework, a nonlocal effective action, derived through perturbation theory, indicates that the interaction is mediated by excitation in the form of an anomaly pole, which appears in the conformal limit of the vertex. To illustrate this, it is demonstrated how conformal Ward identities (CWIs) in momentum space allow to reconstruct the entire chiral anomaly interaction in its longitudinal and transverse sectors just by inclusion of a pole in the longitudinal sector. Both sectors are coupled in amplitudes with an intermediate chiral fermion or a bilinear Chern–Simons current with intermediate photons. In the presence of fermion mass corrections, the pole transforms into a cut, but the absorption amplitude in the axial‐vector channel satisfies mass‐independent sum rules related to the anomaly in any chiral interaction. The detection of an axion‐like/quasiparticle in these materials may rely on a combined investigation of these sum rules, along with the measurement of the angle of rotation of the plane of polarization of incident light when subjected to a chiral perturbation. This phenomenon serves as an analog of a similar one in ordinary axion physics, in the presence of an axion‐like condensate, which is rederived using axion electrodynamics.

Absorption and Reflection of Switchable Multifunctional Metamaterial Absorber Based on Vanadium Dioxide

A dynamically tunable terahertz broadband absorber based on the metamaterial structure of vanadium dioxide (VO2) is proposed and analyzed. The absorber consists of two patterned VO2 layers and a metal bottom layer separated by two polytetrafluoroethylene (PTFE) dielectric layers. Simulation results show that the absorption exceeds 90% in the frequency range of 2.4–11 THz with a relative bandwidth of 128.4% under normal incidence. When VO2 is in the metal phase, the designed absorber functions as an ideal absorber. The absorption rate can be flexibly adjusted from 2% to 99% as vanadium dioxide transitions from the insulator phase to the metal phase. Therefore, the newly developed broad structure has the capability to seamlessly transition between functioning as an absorber or reflector through modifications in the conductivity of VO2 from the insulator phase to the metal phase. Moreover, further insight into the underlying physical processes can be gained by studying the insensitivity of the proposed absorber to the polarization of incident light and its ability to achieve high absorption across a wide range of incident angles. Impedance matching theory and electric field distribution of the absorber are investigated. The THz absorber has many potential applications in fields such as THz sensors, modulation, and switches.

Investigation of growth and polarized spectra of Ho3+ ions heavily doped BaY2F8 crystal

A BaY2F8 (BYF) single crystal heavily doped with Ho3+ ion was grown successfully using the Czochralski (Cz) method. The infrared fluorescence spectra (2–4 μm) and fluorescence lifetime at 3.9 μm were investigated. The detailed polarization absorption properties of Ho:BYF, especially the absorption spectrum in 850–950 nm range, were reported for the first time. The maximum absorption cross-section was at 888.15 nm, σabs = 1.26✕10−21 cm2 (E//c). In comparison, the peak positions of the absorption cross sections in the other two polarization directions were at 885.80 nm and 890.45 nm, respectively, indicating that incident light's polarization direction greatly influences absorption. The spectroscopic parameters were calculated based on the Judd–Ofelt theory.

First-principles simulations of high-order harmonics generation in thin films of wide bandgap materials [Invited

High-order harmonics generation (HHG) is the only process that enables tabletop-sized sources of extreme ultraviolet (XUV) light. The HHG process typically involves light interactions with gases or plasma––material phases that hinder wider adoption of such sources. This motivates the research in HHG from nanostructured solids. Here, we employ the time-dependent density function theory (TDDFT) to investigate material platforms for HHG at the nanoscale using first-principles supercomputer simulations. We reveal that wide bandgap semiconductors, aluminum nitride (AlN) and silicon nitride (Si3N4), are highly promising for XUV light generation when compared to silicon, one of the most common nonlinear nanophotonic materials. In our calculations, we assume excitation with a 100 fs pulse duration, 1×1013W/cm2 peak power, and 800 nm central wavelength. We demonstrate that in AlN material the interplay between the crystal symmetry and the incident light direction and polarization can enable the generation of both even and odd harmonics. Our results should advance the development of high-harmonics generation of XUV light from nanostructured solids.

Reconfigurable and polarization-dependent optical filtering for transflective full-color generation utilizing low-loss phase-change materials

All-dielectric metasurface, which features low optical absorptance and high resolution, is becoming a promising candidate for full-color generation. However, the optical response of current metamaterials is fixed and lacks active tuning. In this work, we demonstrate a reconfigurable and polarization-dependent active color generation technique by incorporating low-loss phase change materials (PCMs) and CaF2 all-dielectric substrate. Based on the strong Mie resonance effect and low optical absorption structure, a transflective, full-color with high color purity and gamut value is achieved. The spectrum can be dynamically manipulated by changing either the polarization of incident light or the PCM state. High transmittance and reflectance can be simultaneously achieved by using low-loss PCMs and substrate. The novel active metasurfaces can bring new inspiration in the areas of optical encryption, anti-counterfeiting, and display technologies.

DFT formalism studies on the structural and electronic properties of hexagonal graphene quantum dot with B, N and Si substitutional impurities

The study of carbon-based nanostructured materials is a highly active research field, that has made significant progress in the study of twodimensional materials and nanotechnology. The interest in these materials is mainly attributed to the fascinating properties they exhibit, as seen in the case of graphene as a 2D material, as well as emergence on numerous novel 2D materials and their heterostructures. Additionally, there is important interest in systems such as 2D quantum dots. Therefore, this work focuses on the systematic study of graphene quantum dots of various sizes, all within the framework of first-principles density functional theory. We started with the simplest graphene quantum dot (GQD) structure, benzene (C6H6), which consist of six carbon atoms passivated with hydrogen atoms. We then increased its size by adding more aromatic rings, resulting in the following GQD configurations: C24H12, C54H18, C96H24, C150H30 and C216H36. We report the density of states (DOS) and the imaginary part of the dielectric function (ε2) for the system, analyzing both the pristine configuration and the effect of both single and double (boron, nitrogen and silicon, denoted as Sa). The double substitutional atom study was done considering random, ortho-, meta-, and para-director positions just for the C94H24Sa2 GQD. In general, we can conclude that as the GQD increases in size, the HOMO-LUMO energy decreases. Furthermore, it is observed that boron and nitrogen exhibit their expected n-, and p-type doping characteristics, but this differs between single and double Sa substitutions. Additionally, the imaginary part of the dielectric function is highly sensitive to the positions of single and double substitutional atoms, as well as the polarization of incident light. Therefore, we suggest that these differences can be used to clearly determinate the type of substitutional atoms and their positions from optical measurements.

VO2-Based metasurface for dynamically tunable terahertz surface plasmonic waves

Surface plasmonic waves (SPWs), which propagate along metal-dielectric interfaces, play a pivotal role in various photonic applications such as highly integrated photonic devices, super-resolution imaging, high-sensitivity sensing, on-chip integrated systems, etc. The ability to control the excitation direction of the SPWs is of great importance in these applications. In this work, we propose a terahertz on-chip metasurface device whose SPWs propagation direction can be dynamically tuned at the excitation source by exploiting the vanadium dioxide (VO2). Under circularly polarized light incidence, destructive or constructive interference formed in the subwavelength square ring slit resonators (SRSRs) arrays, resulting in the unidirectional propagation of terahertz SPWs. By adjusting the conductivity of VO2, the flexible control over the propagation direction of SPWs is realized. This approach significantly enhances the level of control compared to previous traditional polarization control method which can only be modulated by the polarization state, marking a notable advancement in the development of functional devices that harness the power of SPWs.

Controllable optical tweezer and spanner in evanescent fields via a single plasmonic metasurface

A dual-functional plasmonic metasurface is proposed to realize trapping and rotation of microparticles in evanescent fields by simply changing the polarization of incident light. The metasurface is constituted with subwavelength rectangular nanoslit that is perforated in an Au film on the glass substrate. Simulated near-field intensity distributions show that surface plasmon vortex with designed topological charge and focused point with enhanced intensity can be controllably generated in the center region of the designed metasurface by different circularly polarized lights. Calculated optical force and optical potential on a polystyrene sphere further demonstrate the good performances of rotating and trapping a microparticle with the generated vortex and focused surface plasmon polaritons. Moreover, two examples designed with different topological charges demonstrate the flexibility of these metasurfaces in tuning the rotation radius of microparticles. The advantages of the proposed metasurface in design flexibility, multifunctionality, and small size may provide new possibilities for applications of integrated optical manipulation devices and systems.

Tunable third harmonic generation based on high-Q polarization-controlled hybrid phase-change metasurface

Abstract Dielectric metasurfaces have made significant advancements in the past decade for enhancing light–matter interaction at the nanoscale. Particularly, bound states in the continuum (BICs) based on dielectric metasurfaces have been employed to enhance nonlinear harmonic generation. However, conventional nonlinear metasurfaces are typically fixed in their operating wavelength after fabrication. In this work, we numerically demonstrate tunable third harmonic generation (THG) by integrating a dielectric metasurface with the phase-change material Ge2Sb2Te5 (GST). The hybrid phase-change metasurface can support two BICs with different electromagnetic origins, which are transformed into two high-Q quasi-BICs through the introduction of structural asymmetry. The two quasi-BICs are selectively excited by controlling the polarization of incident light, and their wavelengths are tunable due to the phase transition of GST. Notably, the efficiency of THG is significantly enhanced at the fundamental wavelengths corresponding to the two quasi-BICs, and the operating wavelength for THG enhancement can be dynamically tuned through the GST phase transition. Furthermore, the wavelength of THG enhancement can be further tuned by manipulating the polarization of pump light. Additionally, a high-Q analog of electromagnetically induced transparency is numerically achieved through the interaction between a low-Q Mie resonance and a quasi-BIC mode, which also improves the THG efficiency. The high-Q polarization-controlled hybrid phase-change metasurface holds promise for applications in dynamically tunable nonlinear optical devices.

Graphene-based tunable tri-band terahertz refractive index sensor

A tunable tri-band terahertz refractive index sensor based on graphene is proposed and designed. The structure of the sensor comprises a gold (Au) substrate layer, a dielectric layer (Topas), and a graphene pattern layer. The numerical simulation results demonstrate that the sensor exhibits three narrowband absorption peaks at 1.68, 3.82, and 4.78 THz, and the corresponding absorption rate can reach 99.9%, 98.0%, and 97.9%, respectively. By adjusting the Fermi level of graphene, the resonant frequency of the sensor can be effectively tuned. Notably, due to the rotational symmetry of the structure, the sensor shows insensitivity to transverse magnetic and transverse electric polarizations of incident light. By varying the refractive index of surrounding analytes, the sensor’s sensitivity and Figure of Merit (FOM) are studied. The sensitivities of the three resonance peaks are 0.59, 1.19, and 1.38 THz/RIU, with corresponding FOM values of 2.57, 3.40, and 6.58, respectively. Furthermore, the feasibility and effectiveness of the designed sensor in practical applications are verified by testing five types of samples. These findings indicate that the proposed sensor has superior performance in sensitivity and selectivity, which makes it have a great potential for applications in the fields of material characterization, environmental monitoring, and biomedicine detection in the terahertz band.