AbstractTerahertz (THz) band is expected to satisfy the ever‐increasing demand for high‐capacity wireless data transfer. Multifunctional photonic devices with compactness and low loss are highly pursued for future THz communications. Here, a strategy for planar THz photonics is proposed that enables free wavefront manipulation with submillimeter thin liquid crystal polymer (LCP) films. Such elements work on the spatial geometric phase modulation, which is accomplished by preprogramming the axis orientations of LCP. The LCP monomers follow the guidance of local photoalignment agent and are further polymerized under UV exposure at the existence of a doped photo‐initializer. Thanks to the high resolution and excellent flexibility of the photopatterning technique, THz elements with versatile functions can be realized. As examples, waveplates, polarization gratings, and lenses, which are suitable for the polarization control, beam deflecting, focusing, or collimating, are demonstrated. Due to the intrinsic flexibility of LCP films, an f‐tunable lens enabled by mechanically induced deformation is exhibited. Specific mode generators for vortices and Bessel beams are also presented, which can function as separate channels for the mode division multiplexing in THz communications. This work provides a robust platform for fabricating integrated, low‐loss, and tunable THz elements suitable for the advanced THz apparatuses.
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