Polarization Of Emission Research Articles

Focused polarization hologram with arbitrary polarization to a specified polarization conversion.

Polarization devices play a key role in many optical technologies and applications. However, traditional polarization devices are often large and lack integration, and achieving polarization conversion typically requires combining multiple devices, which makes it challenging to realize integrated optical systems. Following the current trend of optical devices, we propose a method using polarization holographic exposure to prepare polarization conversion devices. This approach allows for the fabrication of devices that can convert arbitrary polarization states into specified polarization states while also incorporating a focusing function. Specifically, two types of polarization conversion holograms are fabricated. One is a linear polarizer with a focusing function, and the other is a circular polarizer with a focusing function. Their polarization extinction ratio is around 35 dB, which has a certain competitiveness in similar devices. This method simplifies the preparation process of multifunctional polarizing devices while ensuring their performance. Our work has potential applications in the fields such as polarization emission, imaging, and sensing. Additionally, this approach broadens the design concept of polarization conversion devices, which may promote the development of optical devices with lower cost and higher integration.

Efficient polarization emission from metasurface-integrated resonant cavity light-emitting diodes

Abstract The pursuit of advanced illumination and display technologies has driven the development of beam manipulation for GaN micro-sized light-emitting diodes (LEDs). To realize an efficient polarization emission light source, we propose metasurface-integrated resonant cavity light-emitting diodes (RCLEDs), incorporating a dual-layer embedded photonic crystal (PhC) within the GaN cavity, and placing a resonant-cavity reflector (RCR) on top of the existing distributed Bragg reflector (denoted as PhC-RCR-RCLED). Numerical simulations reveal a significant enhancement in emission efficiency along with an improved ability to manipulate the emission beams. The averaged transmittance, deflection efficiency, and collection efficiency at the central wavelength for both x- and y-polarizations are 66.9%, 79.6%, and 53.6%, respectively. Compared to the traditional RCLED, our PhC-RCR-RCLED achieves 5.3, 1.2, and 6.3 times enhancements in these three efficiencies. Our scheme paves the way for more efficient and controllable light sources.

Ultrathin BIC Metasurfaces Based on Ultra-Low-Loss Sb2Se3 Phase-Change Material.

Ultrathin and low-loss phase-change materials (PCMs) are highly valued for their fast and effective phase transitions and applications in reconfigurable photonic chips, metasurfaces, optical modulators, sensors, photonic memories, and neuromorphic computing. However, conventional PCMs mostly suffer from high intrinsic losses in the near-infrared (NIR) region, limiting their potential for high quality factor (Q-factor) resonant metasurfaces. Here we present the design and fabrication of tunable bound states in the continuum (BIC) metasurfaces using the ultra-low-loss PCM Sb2Se3. Our BIC metasurfaces, only 25 nm thick, achieve high modulation depth and broad resonance tuning in the NIR with high Q-factors up to 130. Experimentally, we employ these BIC metasurfaces to modulate photoluminescence in rare earth-doped upconversion nanoparticles, reducing the excitation power for multiphoton photoluminescence and enabling emission polarization manipulation. This work offers a promising platform for developing active resonant metasurfaces, with broad applications including optical modulation, ultrafast switches, color filtering, and optical sensing.

Room temperature polarization-resolved Raman and photoluminescence in uniaxially strained layered MoS2

Transition metal dichalcogenides (TMDCs) are one of the material systems of choice toward achieving room temperature quantum coherence. Externally applied strain is used as a more common control mechanism to tune electro-optical properties in TMDCs like molybdenum disulfide (MoS2). However, room temperature electron–phonon interactions in the presence of strain in transition metal dichalcogenides are still not fully explored. In this work, we employ uniaxial strain dependent Raman and photoluminescence (PL) studies on monolayer and bilayer MoS2 to explore electron–phonon physics. Helicity-resolved Raman in MoS2 obeys robust selection rules. Our studies reveal clear modification in these helicity-based selection rules in the presence of moderate uniaxial strain (ϵ = 0.4%–1.2%). The selection rules are restored upon clear symmetry breaking of the in-plane vibrational mode (ϵ > 1.2%). We assign these changes to the onset of Fröhlich interaction in this moderate strain regime. The changes in Raman scattering are accompanied by changes in valley selective relaxation observed through non-resonant photoluminescence (PL). The moderate strain regime also exhibits the onset of PL polarization for indirect excitonic emission under non-resonant excitation. Our experimental observations point toward electron–phonon coupling mechanisms affecting both valley-selective electron relaxation during PL emission as well as polarization-selective Raman scattering of two-dimensional semiconductors at room temperature.

Ultrathin, Dynamically Controllable Circularly Polarized Emission Laser Enabled by Resonant Chiral Metasurfaces.

We demonstrate a simple, low-cost, and ultracompact chiral resonant metasurface design, which, by strong local coupling to a quantum gain medium (quantum emitters), allows to implement an ultrathin metasurface laser, capable of generating tunable circularly polarized coherent lasing output. According to our detailed numerical investigations, the lasing emission can be transformed from linear to circular and switch from right- to left-handed circularly polarized (CP) not only by altering the metasurface chiral response but also by changing the polarization of a linearly polarized pump wave, thus enabling dynamic lasing-polarization control. Given the increasing interest for CP laser emission, our chiral metasurface laser design proves to be a versatile yet straightforward strategy to generate a strong and tailored CP emission laser, promising great potential for future applications in both photonics and materials science.

Influence of resonant plasmonic nanoparticles on optically accessing the valley degree of freedom in 2D semiconductors

The valley degree of freedom in atomically thin transition metal dichalcogenides, coupled with valley-contrasting optical selection rules, holds great potential for future electronic and optoelectronic devices. Resonant optical nanostructures emerge as promising tools for controlling this degree of freedom at the nanoscale. However, their impact on the circular polarization of valley-selective emission remains poorly understood. In our study, we explore a hybrid system where valley-specific emission from a molybdenum disulfide monolayer interacts with a resonant plasmonic nanosphere. Contrary to the simple intuition that a centrosymmetric nanoresonator mostly preserves the degree of circular polarization, our cryogenic experiments reveal significant depolarization of the photoluminescence scattered by the nanoparticle. This striking effect presents an ideal platform for studying the mechanisms governing light-matter interactions in such hybrid systems. Our full-wave numerical analysis provides insights into the key physical mechanisms affecting the polarization response, offering a pathway toward designing novel valleytronic devices.

Spin polarization effect on linear polarization of photon emission following resonant electron capture of lithiumlike ions

Spin polarization effect on linear polarization of photon emission following resonant electron capture of lithiumlike ions

An X-Ray Shell Reveals the Supernova Explosion for Galactic Microquasar SS 433

How black holes are formed remains an open and fundamental question in astrophysics. Despite theoretical predictions, it lacks observations to understand whether the black hole formation experiences a supernova explosion. Here we report the discovery of an X-ray shell north of the Galactic microquasar SS 433 harboring a stellar-mass black hole spatially associated with radio continuum and polarization emissions and an H i cloud. Its spectrum can be reproduced by a 1 keV underionized plasma, from which the shell is inferred to have been created by a supernova explosion 20–30 kyr ago, and its properties constitute evidence for canonical supernova explosions to create some black holes. Our analysis precludes other possible origins including heated by jets or blown by disk winds. According to the lower mass limit of the compact object in SS 433, we roughly deduced that the progenitor should be more massive than 25 M ⊙. The existence of such a young remnant in SS 433 can also lead to new insights into the supercritical accretion in young microquasars and the γ-ray emission of this system. The fallback ejecta may provide accretion materials within tens of thousands of years, while the shock of the supernova remnant may play a crucial role in the cosmic-ray (re)acceleration.

Auroral 3D structure retrieval from the Juno/UVS data

Context. Jovian auroras, the most powerful in the Solar System, result from the interaction between the magnetosphere and atmosphere of Jupiter. While the horizontal morphology of these phenomena has been widely studied, their vertical structure, determined by the penetration depth of the magnetospheric electron into the auroral regions, remains relatively unexplored. Previous observations, including those from the Hubble Space Telescope (HST), have addressed this question to a limited extent. Aims. In this study we aim to map the vertical structure of Jovian auroral emissions. Methods. Using observations from Juno’s UltraViolet Spectrograph (UVS), we examined the vertical structure of the auroral emissions. Building on a recent study of auroral energy mapping based on UVS observations that mapped the average energy of precipitating electrons in the Jovian auroral regions, we find a relationship between this average energy and the volume emission rate (VER) of H2 for two types of electron energy distributions: monoenergetic and a kappa distribution with κ = 2.5. Results. Using brightness maps, we derived the 3D VER structure of Jovian auroras in both northern and southern regions, across multiple spacecraft perijoves (PJs). By considering the example of PJ11, we find that the average altitude of the VER peak in the polar emission region is approximately ~250 km for the monoenergetic distribution case and ~190 km for kappa distribution case. In the main emission region, we find that the average altitude of the VER peak is approximately ~260 km for the case of monoenergetic distribution and ~197 km for kappa distribution case. For the other PJs, we obtained results that are very similar to those of PJ11. Conclusions. Our findings are, on average, consistent with measurements from the Galileo probe and the HST observations. This study contributes to a better understanding of the complexity of Jovian auroras and highlights the importance of using Juno observations when probing their vertical structure. Considering the variability in the κ parameter in the auroral region, we also studied the impact of this variability on the vertical structure of the auroral emission. This sensitivity study reveals that the influence of the κ parameter on our results was very weak. However, the impact of the κ variability on the VER amplitude shows that there is an influence on the thermal structure and chemical composition of the atmosphere in the auroral regions.

Ultralow-frequency Waves in Jupiter’s Magnetopause Boundary Layer

Ultralow-frequency (ULF) waves (∼tens of minutes period) are widely identified in the Jovian system and are believed to be associated with energy dissipation in the magnetosphere and ionosphere. Due to the magnetodisk oscillation related to planetary rotation, it is challenging to identify the periodicities inside the magnetosphere, although remote sensing observations of the polar emissions provide clear evidence of the tens of minutes pulsations. In this study, we take advantage of Juno’s in situ measurements in the magnetopause boundary layer for a long duration, i.e., >4 hr, to directly assess the tens of minutes periodicities of the boundary dynamics caused by the interactions between the internal plasma and external solar wind. Through periodogram analysis on the magnetic field and particle data, we find ULF waves with periodicities of ∼18 minutes, ∼40 minutes, and ∼70–80 minutes, which is generally consistent with pulsations in multiple remote sensing observations. A multiple-harmonic ULF phenomenon was also identified in the observations. The periodicities from in situ measurements provide crucial clues in understanding the origin of pulsating wave/auroral emissions in the Jovian system. The results could also further our understanding of energy transfer and release between the internal plasma of Jupiter and external solar wind.

Using polarization sensitive SMLM to infer the interaction strength of dye-plasmonic nanosphere systems

Single-molecule microscopy is an effective tool for the characterization of fluorophore–plasmonic structure interaction. However, sophisticated evaluation is required as specific information is hidden in the emission. Here, we theoretically and experimentally investigated the emission polarization of rotationally mobile fluorophores near plasmonic Au–Ag alloy nanospheres. We developed an elaborate calculation based on the Mie theory, which considers the rotational mobility of dyes near spherical plasmonic nanoparticles of any size. Furthermore, we have created a simplified model that describes the emission’s degree of polarization within 10% accuracy in the case of small nanoparticles, when dipole approximation is valid. Our results indicate the close relation of the polarization degree of the emission, which can reach up to be ∼0.8 in the resonant case, to fluorescence scattering. DNA-PAINT single-molecule localization microscopy experiments conducted using AF488 and Atto647N dyes revealed that the measured polarization degree distribution followed the tendency predicted by calculations.

Mapping and characterizing magnetic fields in the Rho Ophiuchus-A molecular cloud with SOFIA/HAWC+

Context.Together with gravity, turbulence, and stellar feedback, magnetic fields (B-fields) are thought to play a critical role in the evolution of molecular clouds and star formation processes. The polarization of thermal dust emission is a popular tracer of B-fields in star-forming regions.Aims.We aim to map the morphology and measure the strength of B-fields of the nearby molecular cloud, rho Ophiuchus-A(ρOph-A), to understand the role of B-fields in regulating star formation and in shaping the cloud.Methods.We analyzed the far-infrared (FIR) polarization of thermal dust emission observed by SOFIA/HAWC+ at 89 and 154 μm toward the densest part ofρOph-A, which is irradiated by the nearby B3/4 star, Oph-S1. These FIR polarimetric maps cover an area of ~4.5′ × 4.5′ (corresponding to 0″.18 × 0″.18 pc2) with an angular resolution of 7.8″ and 13.6″ respectively.Results.TheρOph-A cloud exhibits well-ordered B-fields with magnetic orientations that are mainly perpendicular to the ridge of the cloud toward the densest region. We obtained a map of B-field strengths in the range of 0.2–2.5 mG, using the Davis-Chandrasekhar-Fermi (DCF) method. The B-fields are strongest at the densest part of the cloud, which is associated with the starless core SM1, and then decrease toward the outskirts of the cloud. By calculating the map of the mass-to-flux ratio, Alfvén Mach number, and plasmaβparameter inρOph-A, we find that the cloud is predominantly magnetically sub-critical, sub-Alfvénic, which implies that the cloud is supported by strong B-fields that dominate over gravity, turbulence, and thermal gas energy. The measured B-field strengths at the two densest subsregions using other methods that account for the compressible mode are relatively lower than that measured with the DCF method. However, these results do not significantly change our conclusions on the roles of B-fields relative to gravity and turbulence on star formation. Our virial analysis suggests that the cloud is gravitationally unbound, which is consistent with the previous detection of numerous starless cores in the cloud. By comparing the magnetic pressure with the radiation pressure from the Oph-S1 star, we find that B-fields are sufficiently strong to support the cloud against radiative feedback and to regulate the shape of the cloud.

B-fields and Dust in Interstellar Filaments Using Dust Polarization (BALLAD-POL). II. Testing the Radiative Torque Paradigm in Musca and OMC-1

Polarization of starlight and thermal dust emission caused by aligned dust grains is a valuable tool to characterize magnetic fields (B-fields) and constrain dust properties. However, the grain alignment physics is not fully understood. To test the radiative torque (RAT) paradigm, including RAT alignment (RAT-A) and disruption (RAT-D), we use dust polarization observed by Planck and Stratosphere Observatory for Infrared Astronomy/High-resolution Airborne Wideband Camera Plus toward two filaments, Musca and OMC-1, with contrasting physical conditions. Musca, a quiescent filament, is ideal for testing RAT-A, while OMC-1, an active star-forming region OMC-1, is most suitable for testing RAT-D. We found that polarization fraction, P, decreases with increasing polarization angle dispersion function, S , and increasing column density, N(H2), consistent with RAT-A. However, P increases with increasing dust temperature, T d, but decreases when T d reaches a certain high value. We compute the polarization fraction for the ideal models with B-fields in the plane of sky based on the RAT paradigm, accounting for the depolarization effect by B-field tangling. We then compare the realistic polarization model with observations. For Musca with well-ordered B-fields, our numerical model successfully reproduces the decline of P toward the filament spine (aka polarization hole), having higher N(H2) and lower T d, indicating the loss of grain alignment efficiency due to RAT-A. For OMC-1, with stronger B-field variations and higher temperatures, our model can reproduce the observed P–T d and P−N(H2) relations only if the B-field tangling and RAT-D effect are incorporated. Our results provide more robust observational evidence for the RAT paradigm, particularly the recently discovered RAT-D.

Magnetic Field Geometry of the Gamma-Ray Binary PSR B1259–63 Revealed via X-Ray Polarization

Some X-ray binaries containing an energetic pulsar in orbit around a normal star accelerate particles to high energies in the shock cone formed where the pulsar and stellar winds collide. The magnetic field geometry in the acceleration region in such binaries is unknown. We performed the first measurement of the polarization of the X-ray synchrotron emission from a gamma-ray-emitting binary system. We observed PSR B1259–63 with the Imaging X-ray Polarimetry Explorer during an X-ray bright phase following the periastron passage in 2024 June. X-ray polarization is detected with a polarization degree of 8.3% ± 1.5% at a significance of 5.3σ. The X-ray polarization angle is aligned with the axis of the shock cone at the time of the observation. This indicates that the predominant component of the magnetic field in the acceleration region is oriented perpendicular to the shock-cone axis.

Spatiotemporally modulated full-polarized light emission for multiplexed optical encryption

Spatiotemporal control of full freedoms of polarized light emission is crucial in multiplexed optical computing, encryption and communication. Although recent advancements have been made in active emission or passive conversion of polarized light through solution-processed nanomaterials or metasurfaces, these design paths usually encounter limitations, such as small polarization degrees, low light utilization efficiency, limited polarization states, and lack of spatiotemporal control. Here, we addressed these challenges by integrating the spatiotemporal modulation of the LED device, the precise control and efficient polarization emission through nanomaterial assembly, and the programmable patterning/positioning using 3D printing. We achieved an extremely high degree of polarization for both linearly and circularly polarized emission from ultrathin inorganic nanowires and quantum nanorods thanks to the shear-force-induced alignment effect during the protruding of printing filaments. Real-time polarization modulation covering the entire Poincaré sphere can be conveniently obtained through the programming of the on-off state of each LED pixel. Further, the output polarization states can be encoded by an ordered chiral plasmonic film. Our device provides an excellent platform for multiplexing spatiotemporal polarization information, enabling visible light communication with an exceptionally elevated level of physical layer security and multifunctional encrypted displays that can encode both 2D and 3D information.

6-Methoxy-2-Naphthoate as a Standard Chromophore for Chiroptical Studies by Fluorescence-Detected Exciton-Coupled Circular Dichroism.

This study investigated the applicability of fluorescent chromophores for exciton-coupled circular dichroism (ECCD) exploiting fluorescence-detected circular dichroism (FDCD). FDCD had been previously reported useful in allowing the sensitive detection of ECCD in favorable conditions. However, fluorescence detection may prevent applications of the combined method especially when solutions are polarized in emission. Even without polarization of emission, FDCD deviates from circular dichroism (CD) in some cases when the fluorophore of interest interacts with nonfluorescent chromophore. Herein, it was confirmed that employing 6-methoxy-2-naphthoate always yielded interpretable exciton-coupled FDCD spectra even when coupling with nonfluorescent p-substituted benzoates. The 6-methoxy-2-naphthoate chromophore (6-MN) is prescribed in special cases when only a small amount of sample is available for determining the absolute stereochemistry by the CD exciton chirality method observed by FDCD.

Non-thermal outflows of the Milky Way traced by radio polarization and gamma-ray emission

Non-thermal outflows of the Milky Way traced by radio polarization and gamma-ray emission

Off-Normal Polarized Single-Photon Emission with Anisotropic Holography Metasurfaces.

Solid-state quantum emitters (QEs) with arbitrary direction emission and well-defined polarization are critical for scalable single-photon sources and quantum information processing. However, the design strategy for on-chip generation of off-normal photon emission with high-purity polarization characteristics has so far remained elusive. Here, we introduce the anisotropic holography metasurfaces for efficiently manipulating the emission direction and polarization of QE. The proposed method offers a flexible way to realize phase matching in surface plasmon scattering with spatially varying filling factors and provides an efficient route for designing advanced QE-coupled metasurfaces. By nonradiatively coupling nanodiamonds with metasurfaces, we experimentally demonstrate on-chip generation of well-collimated single-photon emission propagating along off-normal directions (i.e., 20° and 30°) featuring a divergence angle lower than 2.5°. The experimental average degree of linear polarization attains up to >0.98, thereby revealing markedly high polarization purity. This study facilitates applications of QEs in the deployment of integrated quantum networks.

Unveiling the spin evolution in van der Waals antiferromagnets via magneto-exciton effects

Among the fascinating phenomena observed in two-dimensional (2D) magnets, the magneto-exciton effect stands out as a pivotal link between optics and magnetism. Although the excitonic effect has been revealed and exhibits a considerable correlation with the spin structures in certain 2D magnets, the underlying mechanism of the magneto-exciton effect remains underexplored, especially under high magnetic fields. Here we perform a systematic investigation of the spin-exciton coupling in 2D antiferromagnetic NiPS3 under high magnetic fields. When an in-plane magnetic field is applied, the exceptional sharp excitonic emission at ~1.4756 eV exhibits a Zeeman-like splitting with g ≈ 2.0, experimentally identifying the exciton as an excitation of dominant triplet-singlet character. By examining the polarization of excitonic emission and simulating the spin evolution, we further verify the correlation between excitonic emission and Néel vector in NiPS3. Our work elucidates the mechanism behind the spin-exciton coupling in NiPS3 and establishes a strategy for optically probing the spin evolutions in 2D magnets.

Sb2S3/AlGaAs-based reconfigurable metasurface for dynamic polarization and directionality control of quantum emitter emission.

In this article, we report, to the best of our knowledge, for the first time, phase change material (PCM)-based reconfigurable metasurfaces for tailoring different degrees of freedom (DoF) of the quantum emitter (QE) emission, namely polarization and directionality, two key controlling factors in applications such as quantum computing, communication, and chiral optics. We have used a hybrid plasmon-QE coupled bullseye grating system utilizing the unexplored concept of composite nano-antennas in quantum photonics as the basic building block of the structures. Carefully engineered azimuthal width profile of the Sb2S3/AlGaAs composite ridge and selectively controlled transition of PCM (Sb2S3) states provide dynamic control over the amplitude and phase of the scattered radiation. Based on this methodology, we have designed five different metasurfaces for on-demand switching of target DoFs of QE emission, ensuring high collection efficiency due to the near-field coupling scheme. The first two metasurfaces switch the majority of the outgoing radiation from radially polarized to circularly polarized, whereas the next two switch the direction of circularly polarized outgoing radiation by a maximum of 9.23° while maintaining the spin state (or polarization chirality) in the simulation environment. The third metasurface category is capable of on-demand generation and separation of opposite spin states of outgoing radiation by 11.48° utilizing the selectively controlled phase transition of Sb2S3. Such reconfigurable multi-dimensional manipulation of QE radiation has not been investigated previously. This work proves the vast potential of active metasurfaces to modify the DoFs of QE emission, paving the way for high-dimensional quantum sources for high-speed quantum communication, higher dimensional quantum processing, and switchable chiral optics.