Polariton Field Research Articles

Spatial and polarization-resolved exciton–photon coupling in quasi-whispering-gallery mode ZnO microrod cavity

Whisper gallery mode (WGM) resonances and the coupling of excitons and WGMs are measured from ZnO microrod cavity in the visible and ultraviolet spectral ranges. The coupling of excitons and WGMs leads to split modes which exhibit a clear spatial dependence due to the uneven field distribution of WGM on ZnO microrod surface. Polarization dependent behavior together with a blueshift of the upper polariton branch mode are observed owing to the transition polarization of different types of excitons in the ZnO microcavity. Numerical simulations are carried out using finite element method to support the experimental results. This work reveals the spatial and polarization dependent exciton–photon coupling in a ZnO microrod which implies promising applications in photonic polariton field ranging from ultraviolet lasers, high-sensitivity detectors to optoelectronic devices

Image polaritons in van der Waals crystals

Abstract Polaritonic modes in low-dimensional materials enable strong light–matter interactions and the manipulation of light on nanometer length scales. Very recently, a new class of polaritons has attracted considerable interest in nanophotonics: image polaritons in van der Waals crystals, manifesting when a polaritonic material is in close proximity to a highly conductive metal, so that the polaritonic mode couples with its mirror image. Image modes constitute an appealing nanophotonic platform, providing an unparalleled degree of optical field compression into nanometric volumes while exhibiting lower normalized propagation loss compared to conventional polariton modes in van der Waals crystals on nonmetallic substrates. Moreover, the ultra-compressed image modes provide access to the nonlocal regime of light–matter interaction. In this review, we systematically overview the young, yet rapidly growing, field of image polaritons. More specifically, we discuss the dispersion properties of image modes, showcase the diversity of the available polaritons in various van der Waals materials, and highlight experimental breakthroughs owing to the unique properties of image polaritons.

A topological lattice of plasmonic merons

Topology is an intrinsic property of the orbital symmetry and elemental spin–orbit interaction, but also, intriguingly, designed vectorial optical fields can break existing symmetries, to impose (dress) topology through coherent interactions with trivial materials. Through photonic spin–orbit interaction, light can transiently turn on topological interactions, such as chiral chemistry, or induce non-Abelian physics in matter. Employing electromagnetic simulations and ultrafast, time-resolved photoemission electron microscopy, we describe the geometric transformation of a normally incident plane wave circularly polarized light carrying a defined spin into surface plasmon polariton field carrying orbital angular momentum which converges into an array of plasmonic vortices with defined spin textures. Numerical simulations show how within each vortex domain, the photonic spin–orbit interaction molds the plasmonic orbital angular momentum into quantum chiral spin angular momentum textures resembling those of a magnetic meron quasiparticles. We experimentally examine the dynamics of such meron plasmonic spin texture lattice by recording the ultrafast nanofemto plasmonic field evolution with deep subwavelength resolution and sub-optical cycle time accuracy from which we extract the linear polarization, L-line singularity distribution, that defines the periodic lattice boundaries. Our results reveal how vectorial optical fields can impress their topologically nontrivial spin textures by coherent dressing or chiral excitations of matter.

Polaritonic Vortices with a Half-Integer Charge.

Topological spin textures are field arrangements that cannot be continuously deformed to a fully polarized state. In particular, merons are topological textures characterized by half-integer topological charge ±1/2 and vortex-like swirling patterns at large distances. Merons have been studied previously in the context of cosmology, fluid dynamics, condensed matter physics and plasmonics. Here, we visualized optical spin angular momentum of phonon polaritons that resembles nanoscale meron spin textures. Phonon polaritons, hybrids of infrared photons and phonons in hexagonal boron nitride, were excited by circularly polarized light incident on a ring-shaped antenna and imaged using infrared near-field techniques. The polariton field reveals a half-integer topological charge determined by the handedness of the incident beam. Our phonon polaritonic platform opens up new pathways to create, control, and visualize topological textures.

Drawing structured plasmonic field with on-chip metalens

Abstract The ability to draw a structured surface plasmon polariton (SPP) field is an important step toward many new opportunities for a broad range of nanophotonic applications. Previous methods usually require complex experimental systems or holographic optimization algorithms that limit their practical applications. Here, we propose a simple method for flexible generation of structured SPP field with on-chip plasmonic metalenses. The metalens is composed of multiple plasmonic focusing nanostructures whose focal shape and position can be independently manipulated, and through their superposition, SPP fields with specially designed patterns are obtained. Based on this method, we demonstrate several structured SPP fields including S- and W-shaped SPP focal fields and tunable SPP bottle beams. This work could provide new ideas for on-chip manipulation of optical surface waves, and contribute to applications such as on-chip photonic information processing and integrated photonic circuits.

Vectorial polaritons in the quantum motion of a levitated nanosphere

The strong coupling between elementary excitations of the electromagnetic field (photons) and quantized mechanical vibrations (phonons) produces hybrid quasi-particle states, known as phonon-polaritons. Their typical signature is the avoided crossing between the eigenfrequencies of the coupled system, as paradigmatically illustrated by the Jaynes-Cummings Hamiltonian, and observed in quantum electrodynamics experiments where cavity photons are coupled to atoms, ions, excitons, spin ensambles and superconducting qubits. In this work, we demonstrate the generation of phonon-polaritons in the quantum motion of an optically-levitated nanosphere. The particle is trapped in high vacuum by an optical tweezer and strongly coupled to a single cavity mode by coherent scattering of the tweezer photons. The two-dimensional motion splits into two nearly-degenerate components that, together with the optical cavity mode, define an optomechanical system with three degrees-of-freedom. As such, when entering the strong coupling regime, we observe hybrid light-mechanical states with a dispersion law typical of tripartite quantum systems. Remarkably, the independent components of motion here identify a physical vibration direction on a plane that, similarly to the polarization of light, confers a vectorial nature to the polariton field. Our results pave the way to novel protocols for quantum information transfer between photonic and phononic components and represent a key-step towards the demonstration of optomechanical entangled states at room temperature.

The emerging field of molecular vibrational polaritons in synthetic chemistry

Molecular vibrational polaritons and ultrafast vibrational spectroscopy combine to further studies into synthetic chemistry and quantum technology.

Giant synthetic gauge field for spinless microcavity polaritons in crossed electric and magnetic fields

The artificial gauge field for electrically neutral exciton polaritons devoid from the polarization degree of freedom can be synthesized by means of applying crossed electric and magnetic fields. The appearance of the gauge potential can be ascribed to the motional (magneto-electric) Stark effect which is responsible for the presence of a linear-in-momentum contribution to the exciton kinetic energy. We study the interplay of this phenomenon with the competing effect which arises from the Rabi-splitting renormalization due the reduction of the electron–hole overlap for a moving exciton. Accounting for this mechanism is crucial in the structures with the high ratio of Rabi splitting and the exciton binding energy. Besides, we propose an approach which boosts the gauge field in the considered system. It takes advantage of the crossover from the hydrogen-like exciton to the strongly dipole-polarized exciton state at a specific choice of electric and magnetic fields. The strong sensitivity of the exciton energy to the momentum in this regime leads to the large values of the gauge field. We consider the specific example of a GaAs ring-shape polariton Berry phase interferometer and show that the flux of the effective magnetic field may approach the flux quantum value in the considered crossover regime.

Trapping and rotation of microparticles using a metasurface exciting by linearly polarized beam

We numerically demonstrate trapping and rotation of particles using a metasurface formed by arranging nanocavities as a right-handed Archimedes’ spiral. Excited by a 90° linearly polarized beam, a focused surface plasmon polariton (SPP) field is formed at the center of the spiral, and the particle can be trapped by the field. While excited by −45° linearly polarized beams, a vortex SPP field carrying orbital angular momentum is formed, and the particles can be trapped and rotated in the clockwise direction at the vortex field.

Dynamic tailoring of an optical skyrmion lattice in surface plasmon polaritons: comment.

We comment on a recent paper entitled "Dynamic tailoring of an optical skyrmion lattice in surface plasmon polaritons" [Opt. Express28, 10322 (2020)10.1364/OE.384718] and disprove the assertion that Bloch-type skyrmions exist in the magnetic field of surface plasmon polaritons.

Dynamic tailoring of an optical skyrmion lattice in surface plasmon polaritons: reply.

This is a Reply to the Comment by Meiler, Frank, and Giessen directed to a recent paper "Dynamic tailoring of an optical skyrmion lattice in surface plasmon polaritons" [Opt. Express28, 10320 (2020)10.1364/OE.384718] regarding to the existence of Bloch-type skyrmions in the magnetic field of surface plasmon polaritons.

Polariton condensation and surface enhanced Raman in spherical ZnO microcrystals

Preparation and characterization of polariton Bose–Einstein condensates in micro-cavities of high quality are at the frontier of contemporary solid state physics. Here, we report on three-dimensional polariton condensation and confinement in pseudo-spherical ZnO microcrystals. The boundary of micro-spherical ZnO resembles a stable cavity that enables sufficient coupling of radiation with material response. Exciting under tight focusing at the low frequency side of the bandgap, we detect efficiency and spectral nonlinear dependencies, as well as signatures of spatial delocalization of the excited states which are characteristics of dynamics in polariton droplets. Expansion of the photon component of the condensate boosts the leaky field beyond the boundary of the ZnO microcrystals. Using this, we observe surface polariton field enhanced Raman responses at the interface of ZnO microspheres. The results demonstrate how readily available spherical semiconductor microstructures facilitate engineering of polariton based electronic states and sensing elements for diagnostics at interfaces.

Direct observation of photonic Landau levels and helical edge states in strained honeycomb lattices

We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars. A strong synthetic field is induced in both the s and p orbital bands by engineering a uniaxial hopping gradient in the lattice, giving rise to the formation of Landau levels at the Dirac points. We provide direct evidence of the sublattice symmetry breaking of the lowest-order Landau level wavefunction, a distinctive feature of synthetic magnetic fields. Our realization implements helical edge states in the gap between n = 0 and n = ±1 Landau levels, experimentally demonstrating a novel way of engineering propagating edge states in photonic lattices. In light of recent advances in the enhancement of polariton–polariton nonlinearities, the Landau levels reported here are promising for the study of the interplay between pseudomagnetism and interactions in a photonic system.

Impact of the Energetic Landscape on Polariton Condensates' Propagation along a Coupler

AbstractPolariton condensates' propagation is strongly dependent on the particular energy landscape the particles are moving upon, in which the geometry of the pathway laid for their movement plays a crucial role. Bends in the circuit's trajectories affect the condensates' speed and oblique geometries introduce an additional discretization of the polaritons' momenta due to the mixing of short and long axis wavevectors on the propagating eigenvalues. In this work, the nature of the propagation of condensates along the arms of a polariton coupler is studied by a combination of time‐resolved micro‐tomography measurements and a theoretical model based on a mean field approximation where condensed polaritons are described by an equation for the slow varying amplitude of the polariton field coupled to an equation for the density of incoherent excitons.

An ultrafast and low-power slow light tuning mechanism for compact aperture-coupled disk resonators**Project supported by the National Natural Science Foundation of China (Grant Nos. 11647122 and 61705064) and the Natural Science Foundation of Hubei Province, China (Grant Nos. 2018CFB672 and 2018CFB773).

An ultrafast and low-power slow light tuning mechanism based on plasmon-induced transparency (PIT) for two disk cavities aperture-coupled to a metal-dielectric-metal plasmonic waveguide system is investigated numerically and analytically. The optical Kerr effect is enhanced by the local electromagnetic field of surface plasmon polaritons, slow light, and graphene–Ag composite material structures with a large effective Kerr nonlinear coefficient. Through the dynamic adjustment of the frequency of the disk nanocavity, the group velocity is controlled between c/53.2 and c/15.1 with the pump light intensity increased from 0.41 MW/cm2 to 2.05 MW/cm2. Alternatively, through the dynamic adjustment of the propagation phase of the plasmonic waveguide, the group velocity is controlled between c/2.8 and c/14.8 with the pump light intensity increased from 5.88 MW/cm2 to 11.76 MW/cm2. The phase shift multiplication of the PIT effect is observed. Calculation results indicate that the entire structure is ultracompact and has a footprint of less than 0.8 μm2. An ultrafast responsive time in the order of 1 ps is reached due to the ultrafast carrier relaxation dynamics of graphene. All findings are comprehensively analyzed through finite-difference time-domain simulations and with a coupling-mode equation system. The results can serve as a reference for the design and fabrication of nanoscale integration photonic devices with low power consumption and ultrafast nonlinear responses.

Plasmonic nanojet: an experimental demonstration.

We propose and study a microstructure based on a dielectric cuboid placed on a thin metal film that can act as an efficient plasmonic lens allowing the focusing of surface plasmons at the subwavelength scale. Using numerical simulations of surface plasmon polariton (SPP) field intensity distributions, we observe high-intensity subwavelength spots and formation of the plasmonic nanojet (PJ) at the telecommunication wavelength of 1530 nm. The fabricated microstructure was characterized using amplitude and phase-resolved scattering-type scanning near-field optical microscopy. We show the first experimental observation of the PJ effect for the SPP waves. Such a novel, to the best of our knowledge, and simple platform can provide new pathways for plasmonics, high-resolution imaging, and biophotonics, as well as optical data storage.

Polarization and angle dependent subwavelength coupling and dramatic reflection enhancement/reduction from an ITO–LiNbO3 interface

Two-dimensional electron gases (2DEGs) were demonstrated in indium–tin–oxide (ITO)-coated lithium niobate (LN) slabs by monitoring the very first reflection (VFR). Being dictated by light–matter interaction within the half-a-wavelength range, two-fold enhancement of the VFR was observed at one incidence angle, while two-and-half-fold reduction was obtained at another angle, when illuminating a Z-cut ITO–LN slab with two laser beams at 532 nm from the same side. In terms of exponential gain coefficient, such VFR enhancement/reduction corresponds to a range from −7.416 × 104 cm−1 to +4.68 × 104 cm−1, three orders of magnitude higher than that expected from the conventional photorefractive (PR) theory. The nanometer-thick 2DEG and the coupling role played by the evanescent field of the surface plasmon polaritons (SPPs) impose a much looser coherency requirement for the interacting light beams, which was verified by the solid energy coupling observed while rotating the polarization state of one laser beam. As much as 18.4 mW of the side diffraction mode associated with the light track formed on the slab surface, which sheds some light on the dramatic coupling dynamics. All these findings above were far beyond the reach of conventional PR theory, yet well consistent with the physical picture of 2DEG-supported SPPs and their interactions at the ITO–LN interface, offering a good opportunity to conceive and design future photonic/electronic devices for optical modulators.

A study of two-photon florescence in metallic nanoshells

A theory of the two-photon florescence for a metallic nanoshell in the presence of quantum emitters has been developed. The metallic nanoshell is made of a metallic nanosphere as a core and a dielectric material as a shell. An ensemble of quantum emitters is deposited on the surface of the dielectric shell. A probe field is applied to study the two-photon process in the metallic nanoshell. Surface plasmon polaritons are created at the interface between the core and shell due to coupling between probe photons and surface plasmons present at the surface of the metallic nanosphere. The intensity of the surface plasmon polariton field is huge when the probe photon energy is in resonance with the polariton resonance energy. Induced electric dipoles are created in each quantum emitter due to the surface plasmon polariton field and the probe field. Dipoles in quantum emitters interact with each other via the dipole-dipole interaction. The dipole-dipole interaction is calculated using the many-body theory and mean field approximation. It is found that the dipole-dipole interaction has new term which is induced by the surface plasmon polariton field. An analytical expression of the two-photon florescence is derived in the presence the dipole-dipole interaction. Our theory predicts that the intensity of the two-photon florescence is enhanced in the presence of quantum emitters relative to the florescence of the metallic nanoshell in isolation. Physics behind the enhancement is the presence of the dipole-dipole interaction between the ensemble of quantum emitters. It is also found that as the concentration of quantum emitters increases, the dipole-dipole field also increases. This in turn, increases the two-photon florescence as function of the concentration. Finally, we have compared our theory with experiments of a metallic nanoshell which is made for Au nanosphere core and the SiO2 shell. The metallic nanoshell is surrounded by various concentrations of Cadmium-Selenium quantum dots as quantum emitters. A good agreement between theory and experiment is found.

Molecular polaritons for controlling chemistry with quantum optics.

This is a tutorial-style introduction to the field of molecular polaritons. We describe the basic physical principles and consequences of strong light-matter coupling common to molecular ensembles embedded in UV-visible or infrared cavities. Using a microscopic quantum electrodynamics formulation, we discuss the competition between the collective cooperative dipolar response of a molecular ensemble and local dynamical processes that molecules typically undergo, including chemical reactions. We highlight some of the observable consequences of this competition between local and collective effects in linear transmission spectroscopy, including the formal equivalence between quantum mechanical theory and the classical transfer matrix method, under specific conditions of molecular density and indistinguishability. We also overview recent experimental and theoretical developments on strong and ultrastrong coupling with electronic and vibrational transitions, with a special focus on cavity-modified chemistry and infrared spectroscopy under vibrational strong coupling. We finally suggest several opportunities for further studies that may lead to novel applications in chemical and electromagnetic sensing, energy conversion, optoelectronics, quantum control, and quantum technology.

Mapping the near-field spin angular momenta in the structured surface plasmon polariton field.

Optical spin angular momenta in a confined electromagnetic field exhibit a remarkable difference with their free space counterparts; in particular, the optical transverse spin that is locked with the energy propagating direction lays the foundation for many intriguing physical effects such as unidirectional transportation, quantum spin Hall effects, photonic Skyrmions, etc. In order to investigate the underlying physics behind the spin-orbit interactions as well as to develop the optical spin-based applications, it is crucial to uncover the spin texture in a confined field, yet it faces challenges due to their chiral and near-field vectorial features. Here, we propose a scanning imaging technique which can map the near-field distributions of the optical spin angular momenta with an achiral dielectric nanosphere. The spin angular momentum component normal to the interface can be uncovered experimentally by employing the proposed scanning imaging technique and the three-dimensional spin vector can be reconstructed theoretically with the experimental results. The experiment is demonstrated on the example of surface plasmon polaritons excited with various vector vortex beams under a tight-focusing configuration, where the spin-orbit interaction emerges clearly. The proposed method, which can be utilized to reconstruct the photonic Skyrmion and other photonic topological structures, is straightforward and of high precision, and hence it is expected to be valuable for the study of near-field spin optics and topological photonics.