Formation Of Polar Stratospheric Clouds Research Articles

Ozone loss rates in the Arctic winter stratosphere during 1994-2000 derived from POAM II/III and ILAS observations: Implications for relationships among ozone loss, PSC occurrence, and temperature

[1] Quantitative chemical ozone loss rates at the 475 K isentropic surface inside the Arctic polar vortex are evaluated for six winters (January through March) using a satellite-based Match technique. Satellite observational data are taken from the Polar Ozone and Aerosol Measurement (POAM) II for 1994–1996, the Improved Limb Atmospheric Spectrometer (ILAS) for 1997, and the POAM III for 1999–2000. The largest ozone loss rates were observed in the end of January 1995 (∼50 ± 20 ppbv d−1), February 1996 (∼40–50 ± 15 ppbv d−1), February 1997 (∼40 ± 8 ppbv d−1), January 2000 (∼60 ± 30 ppbv d−1), and early March 2000 (∼40 ± 10 ppbv d−1). The probability of polar stratospheric cloud (PSC) existence is estimated using aerosol extinction coefficient data from POAM II/III and ILAS. Ozone loss and the PSC probability are strongly correlated and an absolute increase of 10% in the PSC probability is found to amplify the chemical ozone loss rate during Arctic winter by approximately 25 ± 6 ppbv per day or 3.2 ± 0.7 ppbv per sunlit hour. Relationships between average Arctic winter ozone loss rates and various PSC- and temperature-related indices are investigated, including the area of polar vortex that is colder than the threshold temperature for PSC existence (APSC), the PSC formation potential (PFP), and the potential for activation of chlorine (PACl). Of these three, PACl provides the best proxy representation of interannual variability in Arctic ozone loss at the 475 K level. Large ozone loss occurred primarily for air masses that experienced low temperatures between 187 K and 195 K within the previous 10 days and the ozone loss rates clearly increase with decreasing the minimum temperature. The particularly large ozone losses of ∼9 ± 3 ppbv per sunlit hour in February 1996 and January 2000 were associated with low minimum temperatures of 187–189 K, simultaneously with high PSC probabilities.

Volcanic and solar activity, and atmospheric circulation influences on cosmogenic 10Be fallout at Vostok and Concordia (Antarctica) over the last 60 years

The cosmogenic nuclide beryllium-10 ( 10Be), recovered from ice cores, is often used to study solar activity on long timescales. However, the 10Be signal is also influenced by factors other than the Sun. To identify and quantify various contributions to the 10Be signal, two Antarctic snow records from the Vostok and Concordia sites spanning the last 60 years were studied at a sub-annual resolution. Three factors that contribute to the 10Be signal were identified. First, a significant period of approximately 11 yr that can be associated with the modulation of 10Be production by solar activity was detected in both records. The solar imprint constitutes 20–35% of the variance within the total signal. The 11-yr 10Be snow component was attenuated by a factor of ∼0.5 and was delayed by ∼1.4 yr compared to the 10Be production expected within the polar atmosphere. The result could be interpreted as the composite response of a stratospheric 10Be reservoir with an 11-yr modulation that was attenuated and delayed (with respect to 10Be polar production) and to a tropospheric 10Be reservoir with an 11-yr modulation that was not attenuated or delayed. Then, peaks in 10Be concentrations that were ∼66% and ∼35% higher than the average concentration were observed during the stratospheric volcanic eruptions of Agung (in 1963) and Pinatubo (in 1991), respectively. In light of these new results, published 10Be ice core records could be reinterpreted because spikes in 10Be concentration appear at the time of several stratospheric events. The data indicate that stratospheric volcanic eruptions can impact 10Be transport and deposition as a result of the roles played by the sedimentation of sulfate aerosols and the formation and rapid settling of polar stratospheric clouds (PSC). Also, an interannual variability of ∼4 yr was determined in both 10Be records, corresponding to ∼26% of the variance within the signal at Vostok. As with species of marine origin (sodium), this 4-yr variability is interpreted as a tropospheric modulation. The 4-yr variability could be associated with atmospheric circulation associated with the coupled Southern Ocean ocean–atmosphere system. The results presented here, from sites within the high Antarctic plateau, open new possibilities for ice core dating over the last few centuries and for the reconstruction of past solar activity in relation to climate.

Denitrification and polar stratospheric cloud formation during the Arctic winter 2009/2010

Abstract. The sedimentation of HNO3 containing Polar Stratospheric Cloud (PSC) particles leads to a permanent removal of HNO3 and thus to a denitrification of the stratosphere, an effect which plays an important role in stratospheric ozone depletion. The polar vortex in the Arctic winter 2009/2010 was very cold and stable between end of December and end of January. Strong denitrification between 475 to 525 K was observed in the Arctic in mid of January by the Odin Sub Millimetre Radiometer (Odin/SMR). This was the strongest denitrification that had been observed in the entire Odin/SMR measuring period (2001–2010). Lidar measurements of PSCs were performed in the area of Kiruna, Northern Sweden with the IRF (Institutet för Rymdfysik) lidar and with the Esrange lidar in January 2010. The measurements show that PSCs were present over the area of Kiruna during the entire period of observations. The formation of PSCs during the Arctic winter 2009/2010 is investigated using a microphysical box model. Box model simulations are performed along air parcel trajectories calculated six days backward according to the PSC measurements with the ground-based lidar in the Kiruna area. From the temperature history of the backward trajectories and the box model simulations we find two PSC regions, one over Kiruna according to the measurements made in Kiruna and one north of Scandinavia which is much colder, reaching also temperatures below Tice. Using the box model simulations along backward trajectories together with the observations of Odin/SMR, Aura/MLS (Microwave Limb Sounder), CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) and the ground-based lidar we investigate how and by which type of PSC particles the denitrification that was observed during the Arctic winter 2009/2010 was caused. From our analysis we find that due to an unusually strong synoptic cooling event in mid January, ice particle formation on NAT may be a possible formation mechanism during that particular winter that may have caused the denitrification observed in mid January. In contrast, the denitrification that was observed in the beginning of January could have been caused by the sedimentation of NAT particles that formed on mountain wave ice clouds.

The effect of orographic gravity waves on Antarctic polar stratospheric cloud occurrence and composition

[1] A seasonal analysis of the relationship between mesoscale orographic gravity wave activity and polar stratospheric cloud (PSC) composition occurrence around the whole of Antarctica is presented. Gravity wave variances are derived from temperature measurements made with the Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC) Global Positioning System Radio Occultation (GPS-RO) satellites. Data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument onboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite are used to determine the PSC composition class distribution and spatial volume. The results show intermittent large wave activity above the Antarctic Peninsula which is coincident with large volumes of H2O ice PSCs. These ice PSC volumes advect downstream, where increases in nitric acid trihydrate (NAT) PSC volumes occur, supporting the mountain wave seeding hypothesis. During winter 2007 in the latitude range 60°S–70°S, near the edge of the vortex and where temperatures are close to PSC formation thresholds, 30% of all PSCs are attributable to orographic gravity waves. In the separate composition classes, around 50% of both H2O ice PSCs and a high NAT number density liquid–NAT mixture class of PSCs are due to these waves. While we show that planetary waves are the major determinant of PSC presence at temperatures close to the NAT formation threshold, we also demonstrate the important role of mesoscale, intermittent orographic gravity wave activity in accounting for the composition and distribution of PSCs around Antarctica.

Multimodel climate and variability of the stratosphere

[1] The stratospheric climate and variability from simulations of sixteen chemistry-climate models is evaluated. On average the polar night jet is well reproduced though its variability is less well reproduced with a large spread between models. Polar temperature biases are less than 5 K except in the Southern Hemisphere (SH) lower stratosphere in spring. The accumulated area of low temperatures responsible for polar stratospheric cloud formation is accurately reproduced for the Antarctic but underestimated for the Arctic. The shape and position of the polar vortex is well simulated, as is the tropical upwelling in the lower stratosphere. There is a wide model spread in the frequency of major sudden stratospheric warnings (SSWs), late biases in the breakup of the SH vortex, and a weak annual cycle in the zonal wind in the tropical upper stratosphere. Quantitatively, “metrics” indicate a wide spread in model performance for most diagnostics with systematic biases in many, and poorer performance in the SH than in the Northern Hemisphere (NH). Correlations were found in the SH between errors in the final warming, polar temperatures, the leading mode of variability, and jet strength, and in the NH between errors in polar temperatures, frequency of major SSWs, and jet strength. Models with a stronger QBO have stronger tropical upwelling and a colder NH vortex. Both the qualitative and quantitative analysis indicate a number of common and long-standing model problems, particularly related to the simulation of the SH and stratospheric variability.

In situ balloon‐borne measurements of HNO3 and HCl stratospheric vertical profiles influenced by polar stratospheric cloud formation during the 2005–2006 Arctic winter

Within the context of the Envisat satellite validation, the Spectromètre InfraRouge par Absorption de Lasers Embarqués (SPIRALE), balloon‐borne infrared spectrometer was flown in the Arctic stratosphere (Kiruna, Sweden; 67.6°N, 21.6°E) in January 2006. In situ vertical profiles of O3, N2O, HNO3, and HCl were obtained between 13 and 27.3 km. The Stratospheric and Tropospheric Aerosols Counter (STAC) was mounted on board, allowing in situ characterization of the vertical particle distribution at six values of radius between 0.2 and 1.0 μm. Complex structures were observed in both HNO3 and HCl vertical profiles with very low values in the 20.5–22 km layer and simultaneously thin layers of clouds were observed below the HNO3 depleted layer. We used correlations of N2O:HNO3 and O3:HNO3 to characterize these layers and a model approach to investigate the processes involved. It appears that denitrification and renitrification processes have been captured that were linked to the formation of a polar stratospheric cloud. Several tests using different nitric acid trihydrate (NAT) nucleation rates in the model were performed to obtain the best agreement between microphysical and chemical results and measurements. Best results were obtained with a nucleation rate independent of temperature.

Chemistry–Climate Model Simulations of Twenty-First Century Stratospheric Climate and Circulation Changes

Abstract The response of stratospheric climate and circulation to increasing amounts of greenhouse gases (GHGs) and ozone recovery in the twenty-first century is analyzed in simulations of 11 chemistry–climate models using near-identical forcings and experimental setup. In addition to an overall global cooling of the stratosphere in the simulations (0.59 ± 0.07 K decade−1 at 10 hPa), ozone recovery causes a warming of the Southern Hemisphere polar lower stratosphere in summer with enhanced cooling above. The rate of warming correlates with the rate of ozone recovery projected by the models and, on average, changes from 0.8 to 0.48 K decade−1 at 100 hPa as the rate of recovery declines from the first to the second half of the century. In the winter northern polar lower stratosphere the increased radiative cooling from the growing abundance of GHGs is, in most models, balanced by adiabatic warming from stronger polar downwelling. In the Antarctic lower stratosphere the models simulate an increase in low temperature extremes required for polar stratospheric cloud (PSC) formation, but the positive trend is decreasing over the twenty-first century in all models. In the Arctic, none of the models simulates a statistically significant increase in Arctic PSCs throughout the twenty-first century. The subtropical jets accelerate in response to climate change and the ozone recovery produces a westward acceleration of the lower-stratospheric wind over the Antarctic during summer, though this response is sensitive to the rate of recovery projected by the models. There is a strengthening of the Brewer–Dobson circulation throughout the depth of the stratosphere, which reduces the mean age of air nearly everywhere at a rate of about 0.05 yr decade−1 in those models with this diagnostic. On average, the annual mean tropical upwelling in the lower stratosphere (∼70 hPa) increases by almost 2% decade−1, with 59% of this trend forced by the parameterized orographic gravity wave drag in the models. This is a consequence of the eastward acceleration of the subtropical jets, which increases the upward flux of (parameterized) momentum reaching the lower stratosphere in these latitudes.

Cooling of the wintertime Arctic stratosphere induced by the western Pacific teleconnection pattern

A composite analysis for extreme positive events of the Western Pacific (WP) teleconnection pattern with blocking flow configurations observed over the subpolar Far East shows that such an event in winter can trigger a persistent cold period in the polar stratosphere and, if it occurs in fall or early winter, it augments the possibility of the formation of polar stratospheric clouds. The stratospheric cooling occurs in conjunction with the weakening of upper‐tropospheric planetary waves and their upward propagation into the stratosphere soon after the peak time of the WP pattern. Synoptically, this weakening of the upper‐tropospheric planetary waves is manifested as westward evolution of a developing blocking high into the climatological‐mean pressure trough over the subpolar Far East. This study thus presents a unique case where a blocking high can induce cooling in the polar stratosphere rather than warming.

Microphysical properties of Antarctic polar stratospheric clouds and their dependence on tropospheric cloud systems

Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and CloudSat satellite measurements are used to investigate the impact of tropospheric high and deep clouds on the microphysical properties of polar stratospheric clouds (PSCs) over Antarctica during the 2006 and 2007 winters. Based on the attenuated lidar scattering ratio and PSC depolarization ratio (δ′), PSCs are classified into supercooled ternary solution (STS), Mix 1, Mix 2, and ice classes with significantly different microphysical properties in terms of the PSC backscattering coefficient (β532) for 532 nm, the color ratio (β1064/β532), and δ′. In the early stages of the PSC season, STS accounts for more than 50% of the total PSCs, but the Mix 1, Mix 2, and ice classes become more common in the late season. During the late PSC season, close to 70% of PSCs are formed in association with high and deep tropospheric cloud systems, indicating the important role of tropospheric weather systems in Antarctic PSC formation. Tropospheric cloud systems also affect the microphysical properties of PSCs by affecting the relative occurrence of different PSC classes, especially during September and October. Our results also show that there are noticeable differences in color ratio and β532 (at the 0.05 significance level) for the ice class and Mix 2 (late season only) for PSCs associated and not associated with high and deep tropospheric cloud systems. These results indicate that the impact of tropospheric meteorology on PSC formation should be fully considered to better understand interannual variations and recovery of the Antarctic ozone hole.

Chemistry‐climate model simulations of spring Antarctic ozone

Coupled chemistry‐climate model simulations covering the recent past and continuing throughout the 21st century have been completed with a range of different models. Common forcings are used for the halogen amounts and greenhouse gas concentrations, as expected under the Montreal Protocol (with amendments) and Intergovernmental Panel on Climate Change A1b Scenario. The simulations of the Antarctic ozone hole are compared using commonly used diagnostics: the minimum ozone, the maximum area of ozone below 220 DU, and the ozone mass deficit below 220 DU. Despite the fact that the processes responsible for ozone depletion are reasonably well understood, a wide range of results is obtained. Comparisons with observations indicate that one of the reasons for the model underprediction in ozone hole area is the tendency for models to underpredict, by up to 35%, the area of low temperatures responsible for polar stratospheric cloud formation. Models also typically have species gradients that are too weak at the edge of the polar vortex, suggesting that there is too much mixing of air across the vortex edge. Other models show a high bias in total column ozone which restricts the size of the ozone hole (defined by a 220 DU threshold). The results of those models which agree best with observations are examined in more detail. For several models the ozone hole does not disappear this century but a small ozone hole of up to three million square kilometers continues to occur in most springs even after 2070.

Can gravity waves significantly impact PSC occurrence in the Antarctic?

Abstract. A combination of POAM III aerosol extinction and CHAMP RO temperature measurements are used to examine the role of atmospheric gravity waves in the formation of Antarctic Polar Stratospheric Clouds (PSCs). POAM III aerosol extinction observations and quality flag information are used to identify Polar Stratospheric Clouds using an unsupervised clustering algorithm. A PSC proxy, derived by thresholding Met Office temperature analyses with the PSC Type Ia formation temperature (TNAT), shows general agreement with the results of the POAM III analysis. However, in June the POAM III observations of PSC are more abundant than expected from temperature threshold crossings in five out of the eight years examined. In addition, September and October PSC identified using temperature thresholding is often significantly higher than that derived from POAM III; this observation probably being due to dehydration and denitrification. Comparison of the Met Office temperature analyses with corresponding CHAMP observations also suggests a small warm bias in the Met Office data in June. However, this bias cannot fully explain the differences observed. Analysis of CHAMP data indicates that temperature perturbations associated with gravity waves may partially explain the enhanced PSC incidence observed in June (relative to the Met Office analyses). For this month, approximately 40% of the temperature threshold crossings observed using CHAMP RO data are associated with small-scale perturbations. Examination of the distribution of temperatures relative to TNAT shows a large proportion of June data to be close to this threshold, potentially enhancing the importance of gravity wave induced temperature perturbations. Inspection of the longitudinal structure of PSC occurrence in June 2005 also shows that regions of enhancement are geographically associated with the Antarctic Peninsula; a known mountain wave "hotspot". The latitudinal variation of POAM III observations means that we only observe this region in June–July, and thus the true pattern of enhanced PSC production may continue operating into later months. The analysis has shown that early in the Antarctic winter stratospheric background temperatures are close to the TNAT threshold (and PSC formation), and are thus sensitive to temperature perturbations associated with mountain wave activity near the Antarctic peninsula (40% of PSC formation). Later in the season, and at latitudes away from the peninsula, temperature perturbations associated with gravity waves contribute to about 15% of the observed PSC (a value which corresponds well to several previous studies). This lower value is likely to be due to colder background temperatures already achieving the TNAT threshold unaided. Additionally, there is a reduction in the magnitude of gravity waves perturbations observed as POAM III samples poleward of the peninsula.

Global distributions of nitric acid from IASI/MetOP measurements

Abstract. This paper presents the first global distributions of HNO3 total columns acquired by the Infrared Atmospheric Sounding Interferometer (IASI) instrument, launched onboard the MetOp platform in October 2006. IASI is an infrared nadir-looking Fourier transform spectrometer providing atmospheric radiance spectra at 0.5 cm−1 spectral resolution, from which temperature and infrared absorbing gas concentration profiles are retrieved with global Earth coverage twice a day. A first analysis of the IASI measurements in terms of information content demonstrates the possibility of retrieving a total column for HNO3 at all latitudes with a maximal sensitivity in the middle stratosphere. The retrievals are performed from IASI spectra in the atmospheric window using a fast radiative transfer model and inversion software (FORLI) relying on the Optimal Estimation Method. The operational processing of HNO3 total columns is achieved since March 2008. We show that FORLI-HNO3 performs well at all latitudes (RMS of the spectral residuals around 2.3×10−6 W/m2 sr m−1) and provides HNO3 total columns with on average statistical errors of about 12%, reaching the threshold value of 32% at the equatorial belt. The global distributions of the retrieved total columns for one year (from March 2008 to February 2009) are presented and discussed with emphasis given to seasonal and interhemispheric variations. Local seasonal variations at 6 specific locations are also described and discussed in comparison with MLS volume mixing ratios at 46.5 hPa. The seasonal cycle observed in Polar regions is highlighted, with maxima observed in fall-winter and minima during spring-summer. The denitrification inside the Antarctic polar vortex during winter is clearly revealed with unprecedented horizontal resolution: HNO3 columns decreasing down to about 1×1016 molecules cm−2 are observed, which is consistent with the lower values of temperature observed between 50 and 15 hPa (~20–25 km) and the resulting formation and sedimentation of polar stratospheric clouds. During the same period, the collar region of high quantities of HNO3 at the vortex edge is also observed around 65–60° S latitude. Preliminary correlations between IASI derived HNO3 and O3 columns inside the polar vortex are presented and discussed.

Detection of temperatures conducive to Arctic polar stratospheric clouds using CHAMP and SAC‐C radio occultation data

We use global positioning system radio occultation (GPSRO) data from the Challenging Mini‐Satellite Payload for Geophysical Research and Application (CHAMP) and Satélite de Applicaciones Científicas‐C (SAC‐C) low Earth orbiting satellites to investigate the occurrence of air with temperatures cold enough to allow the formation of polar stratospheric clouds (PSCs) during four successive Arctic winters spanning 2001 to 2005. The GPSRO data are validated and compared with analysis data from the European Centre for Medium‐Range Weather Forecasts using a series of criteria designed to eliminate faulty soundings but retain profiles which do not differ too strongly from the model data. We find that GPSRO is able to detect more PSC‐prone temperature profiles during winters with disturbed conditions (in particular during December 2001 and 2003) than the analysis, but that the model fully captures the extent of PSC‐prone air in winters with strong, cold vortices (in particular December 2002 and January 2005). Examination of detailed profiles for December 2001 shows that this difference is due to the ability of GPSRO to detect short‐vertical wavelength features which may represent either localized gravity or global‐scale planetary waves. Since the GPSRO data are now being directly assimilated into operational analysis systems, the benefits of the higher vertical resolution retrievals it provides should become evident in future observational studies of PSC formation and ozone loss, particularly under the disturbed conditions noted in several recent winters.

Variability of the Northern Hemisphere polar stratospheric cloud potential: the role of North Pacific disturbances

AbstractThe potential of the Arctic stratosphere to sustain the formation of Polar Stratospheric Clouds (PSCs) is a key factor in determining the amount of ozone destroyed each winter, and is often measured as a ‘PSC volume’. The latter quantity has been shown to closely follow a near‐linear compact relationship with winter‐averaged column ozone loss, and displays a high variability from monthly to decadal time‐scales. We examine the connection between meteorological conditions in the troposphere and the variability of lower polar stratospheric temperatures over the last four decades, and specifically, conditions leading to a high PSC volume. In addition to the well‐established connection between the North Atlantic Oscillation (NAO) and the polar vortex, we demonstrate the large influence of precursory disturbances over the North Pacific and the Far East, the region of maximum climatological upward wave activity flux. Namely, very high monthly PSC volume (in the top 12%) predominantly follows the development of positive tropospheric height anomalies over the Far East, which lead to a weakening of the background planetary wave trough, and lessened upward wave activity flux into the stratosphere. Precursory anomalies over the Far East are reminiscent of East Asian monsoon amplification episodes. Copyright © 2009 Royal Meteorological Society

The influence of tropical Indian Ocean warming on the Southern Hemispheric stratospheric polar vortex

During the past decades, concurrent with global warming, most of global oceans, particularly the tropical Indian Ocean, have become warmer. Meanwhile, the Southern Hemispheric stratospheric polar vortex (SPV) exhibits a deepening trend. Although previous modeling studies reveal that radiative cooling effect of ozone depletion plays a dominant role in causing the deepening of SPV, the simulated ozone-depletion-induced SPV deepening is stronger than the observed. This suggests that there must be other factors canceling a fraction of the influence of the ozone depletion. Whether the tropical Indian Ocean warming (IOW) is such a factor is unclear. This issue is addressed by conducting ensemble atmospheric general circulation model (AGCM) experiments. And one idealized IOW with the amplitude as the observed is prescribed to force four AGCMs. The results show that the IOW tends to warm the southern polar stratosphere, and thus weakens SPV in austral spring to summer. Hence, it offsets a fraction of the effect of the ozone depletion. This implies that global warming will favor ozone recovery, since a warmer southern polar stratosphere is un-beneficial for the formation of polar stratospheric clouds (PSCs), which is a key factor to ozone depletion chemical reactions.

Past and future conditions for polar stratospheric cloud formation simulated by the Canadian Middle Atmosphere Model

Abstract. We analyze here the polar stratospheric temperatures in an ensemble of three 150-year integrations of the Canadian Middle Atmosphere Model (CMAM), an interactive chemistry-climate model which simulates ozone depletion and recovery, as well as climate change. A key motivation is to understand possible mechanisms for the observed trend in the extent of conditions favourable for polar stratospheric cloud (PSC) formation in the Arctic winter lower stratosphere. We find that in the Antarctic winter lower stratosphere, the low temperature extremes required for PSC formation increase in the model as ozone is depleted, but remain steady through the twenty-first century as the warming from ozone recovery roughly balances the cooling from climate change. Thus, ozone depletion itself plays a major role in the Antarctic trends in low temperature extremes. The model trend in low temperature extremes in the Arctic through the latter half of the twentieth century is weaker and less statistically robust than the observed trend. It is not projected to continue into the future. Ozone depletion in the Arctic is weaker in the CMAM than in observations, which may account for the weak past trend in low temperature extremes. In the future, radiative cooling in the Arctic winter due to climate change is more than compensated by an increase in dynamically driven downwelling over the pole.

Detection of reactive nitrogen containing particles in the tropopause region – evidence for a tropical nitric acid trihydrate (NAT) belt

Abstract. The detection of nitric acid trihydrate (NAT, HNO3×3H2O) particles in the tropical transition layer (TTL) harmonizes our understanding of polar stratospheric cloud formation. Large reactive nitrogen (NOy) containing particles were observed on 8 August 2006 by instruments onboard the high altitude research aircraft M55-Geophysica near and below the tropical tropopause. The particles, most likely NAT, have diameters less than 6 μm and concentrations below 10-4 cm−3. The NAT particle layer was repeatedly detected at altitudes between 15.1 and 17.5 km over extended areas of 9.5 to 17.2° N and 1.5° W to 2.7° E above the African continent. Satellite observations suggest that the NAT particles could have nucleated on ice fed by convective activity. Once nucleated, the NAT particles can slowly grow within the TTL for days, while being transported over long distances. Their in-situ detection combined with global model simulations of the NAT supersaturation near the tropical tropopause indicate the potential for a tropical tropopause NAT particle belt.

Validation of a limited area model over Dome C, Antarctic Plateau, during winter

The limited area model MAR (Modele Atmospherique Regional) is validated over the Antarctic Plateau for the period 2004-2006, focussing on Dome C during the cold season. MAR simulations are made by initializing the model once and by forcing it through its lateral and top boundaries by the ECMWF operational analyses. Model outputs compare favourably with observations from automatic weather station (AWS), radiometers and atmospheric soundings. MAR is able to simulate the succession of cold and warm events which occur at Dome C during winter. Larger longwave downwelling fluxes (LWD) are responsible for higher surface air temperatures and weaker surface inversions during winter. Warm events are better simulated when the small Antarctic precipitating snow particles are taken into account in radiative transfer computations. MAR stratosphere cools during the cold season, with the coldest temperatures occurring in conjunction with warm events at the surface. The decrease of saturation specific humidity associated with these coldest temperatures is responsible for the formation of polar stratospheric clouds (PSCs) especially in August-September. PSCs then contribute to the surface warming by increasing the surface downwelling longwave flux.

Numerical simulations of the three‐dimensional distribution of meteoric dust in the mesosphere and upper stratosphere

Micrometeorites that ablate in the lower thermosphere and upper mesosphere are thought to recondense into nanometer‐sized smoke particles and then coagulate into larger dust particles. Previous studies with one‐dimensional models have determined that the meteoric dust size distribution is sensitive to the background vertical velocity and have speculated on the importance of the mesospheric meridional circulation to the dust spatial distribution. We conduct the first three‐dimensional simulations of meteoric dust using a general circulation model with sectional microphysics to study the distribution and characteristics of meteoric dust in the mesosphere and upper stratosphere. We find that the mesospheric meridional circulation causes a strong seasonal pattern in meteoric dust concentration in which the summer pole is depleted and the winter pole is enhanced. This summer pole depletion of dust particles results in fewer dust condensation nuclei (CN) than has traditionally been assumed in numerical simulations of polar mesospheric clouds (PMCs). However, the total number of dust particles present is still sufficient to account for PMCs if smaller particles can nucleate to form ice than is conventionally assumed. During winter, dust is quickly transported down to the stratosphere in the polar vortex where it may participate in the nucleation of sulfate aerosols, the formation of the polar CN layer, and the formation of polar stratospheric clouds (PSCs). These predictions of the seasonal variation and resulting large gradients in dust concentration should assist the planning of future campaigns to measure meteoric dust.

Association of Antarctic polar stratospheric cloud formation on tropospheric cloud systems

The formation of polar stratospheric clouds (PSCs) is critical to the development of polar ozone loss. However, the mechanisms of PSC formation remain poorly understood, which affects ozone loss models. Here, based on observations by the NASA A‐train satellites, we show that 66% ± 16% and 52% ± 17% of PSCs over west and east Antarctica during the period June–October 2006 were associated with deep tropospheric cloud systems, with maximum depths exceeding 7 km. The development of such deep tropospheric cloud systems should cool the lower stratosphere through adiabatic and radiative processes, favoring PSC development. These deep systems also transport lower tropospheric air into the upper troposphere and lower stratosphere. These new findings suggest that Antarctic PSC formation is closely connected to tropospheric meteorology and thus governed by synoptic scale dynamics, local topography, and large‐scale circulation. More dedicated studies are still needed to better understand Antarctic PSC formation.