Plasma Amplifier Research Articles

Relativistic Eulerian Vlasov simulations of the amplification of seed pulses by Brillouin backscattering in plasmas

We apply an Eulerian Vlasov code to study the amplification by Brillouin scattering of a short seed laser pulse by a long pump laser pulse in an underdense plasma. The stimulated Brillouin backscattering interaction is the coupling of the pump and seed electromagnetic waves propagating in opposite directions, and the ion plasma wave. The code solves the one-dimensional relativistic Vlasov-Maxwell set of equations. Large amplitude ion waves are generated. In the simulations we present, the density plateau of the plasma is ne=0.3 nc (nc is the critical density), which excludes spurious stimulated Raman scattering amplification (which can occur only if ne<nc/4). We also varied the duration and/or amplitude of the short input seed pulse to study how these influence its subsequent behaviour. An initially broad pulse grows more rapidly than an initially narrow pulse. Furthermore, for an initially broader seed pulse, towards the end of the simulation, it is seen to become narrower and to gradually detach from the trailing signal. On the contrary, initially very narrow seed pulses are seen to broaden. The absence of noise in the Vlasov simulations allows to simulate long plasma amplifier lengths, and to follow the evolution of the system with a fully kinetic description and with an accurate representation of the phase-space structures of distribution function.

Backward Lasing of Air plasma pumped by Circularly polarized femtosecond pulses for the saKe of remote sensing (BLACK).

Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward Amplified Spontaneous Emission (ASE) at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt. Express, 22, 12750 (2014)). Here, we report that a seed pulse injected in the backward direction can be amplified by ~200 times inside this plasma amplifier. The amplified 337 nm radiation can be either linearly or circularly polarized, dictated by the seeding pulse, which is distinct from the non-polarized nature of the ASE. We performed comprehensive measurements of the spatial profile, optical gain dynamics, and seed pulse energy dependence of this amplification process. These measurements allow us to deduce the pulse duration of the ASE and the amplified 337 nm radiation as well as the corresponding laser intensity inside the plasma amplifier. It indicates that the amplification is largely in the unsaturated regime and that further improvement of laser energy is possible. Moreover, we observed optical gain in plasma created in ambient air. This represents an important step towards future applications exploiting backward lasing for remote atmospheric sensing.

X-ray laser plasma amplifiers

The realization of an X-ray laser plasma amplifier using a stretched X-ray pulse leads to higher intensity and better quality X-ray laser pulses.

Gain dynamics in a soft-X-ray laser amplifier perturbed by a strong injected X-ray field

Seeding soft-X-ray plasma amplifiers with high harmonics has been demonstrated to generate high-brightness soft-X-ray laser pulses with full spatial and temporal coherence. The interaction between the injected coherent field and the swept-gain medium has been modelled. However, no experiment has been conducted to probe the gain dynamics when perturbed by a strong external seed field. Here, we report the first X-ray pump–X-ray probe measurement of the nonlinear response of a plasma amplifier perturbed by a strong soft-X-ray ultra-short pulse. We injected a sequence of two time-delayed high-harmonic pulses (λ = 18.9 nm) into a collisionally excited nickel-like molybdenum plasma to measure with femtosecond resolution the gain depletion induced by the saturated amplification of the high-harmonic pump and its subsequent recovery. The measured fast gain recovery in 1.5–1.75 ps confirms the possibility to generate ultra-intense, fully phase-coherent soft-X-ray lasers by chirped pulse amplification in plasma amplifiers.

Wavefront improvement in an injection-seeded soft x-ray laser based on a solid-target plasma amplifier

The wavefront of an injection-seeded soft x-ray laser beam generated by amplification of high-harmonic pulses in a λ=18.9 nm molybdenum plasma amplifier was measured by a Hartmann wavefront sensor with an accuracy of λ/32 root mean square (rms). A significant improvement in wavefront aberrations of 0.51±0.03λ rms to 0.23±0.01λ rms was observed as a function of plasma column length. The variation of wavefront characteristic as a function time delay between the injection of the seed and peak of soft x-ray amplifier pump was studied. The measurements were used to reconstruct the soft x-ray source and confirm its high peak brightness.

Spectral characteristics of ultra-short laser pulses in plasma amplifiers

Amplification of laser pulses based on the backscattering process in plasmas can be performed using either the response of an electron plasma wave or an ion-acoustic wave. However, if the pulse durations become very short and the natural spread in frequency a substantial amount of the frequency itself, the Raman and Brillouin processes start to mix. Kinetic simulations show the transition from a pure amplification regime, in this case strong-coupling Brillouin, to a regime where a considerable downshift of the frequency of the amplified pulse takes place. It is conjectured that in the case of very short pulses, multi-modes are excited which contribute to the amplification process.

Observation and theory of X-ray mirages

The advent of X-ray lasers allowed the realization of compact coherent soft X-ray sources, thus opening the way to a wide range of applications. Here we report the observation of unexpected concentric rings in the far-field beam profile at the output of a two-stage plasma-based X-ray laser, which can be considered as the first manifestation of a mirage phenomenon in X-rays. We have developed a method of solving the Maxwell–Bloch equations for this problem, and find that the experimentally observed phenomenon is due to the emergence of X-ray mirages in the plasma amplifier, appearing as phase-matched coherent virtual point sources. The obtained results bring a new insight into the physical nature of amplification of X-ray radiation in laser-induced plasma amplifiers and open additional opportunities for X-ray plasma diagnostics and extreme ultraviolet lithography.

Soft x-ray plasma-based seeded multistage amplification chain

To date, plasma-based soft x-ray lasers have demonstrated experimentally 1 μJ, 1 ps (1 MW) pulses. This Letter reports extensive study using time-dependant Maxwell-Bloch code of seeding millimeter scale plasmas that store more than 100 mJ in population inversion. Direct seeding of these plasmas has to overcome very strong amplified spontaneous emission (ASE) as well as prevent wake-field amplification. Below 100 nJ injected energy, seed produces pulses with picosecond duration. To overcome this limitation, a new scheme has been studied, taking advantage of a plasma preamplifier that dramatically increases the seed energy prior to entering the main plasma amplifier leading to ASE and wake-free, fully coherent 21.6 μJ, 80 fs pulses (0.27 GW).

Simultaneous stimulated Raman, Brillouin, and electron-acoustic scattering reveals a potential saturation mechanism in Raman plasma amplifiers

In a Raman plasma amplifier, the aim is to create plasma conditions in which Raman backscattering is the fastest growing instability, outrunning all competing effects so that it is possible to amplify and compress a laser beam to unprecedented unfocused intensities by utilizing that instability. However, achieving high efficiencies via this scheme has proven very difficult experimentally. Recent data show the simultaneous occurrence of stimulated Raman scattering (SRS), stimulated Brillouin scattering (SBS), and stimulated electron-acoustic scattering (SEAS). The appearance of SEAS is indicative of strong particle trapping, the existence of which is hard to justify without highlighting the interplay between SRS and SBS.

On the theory of a Cherenkov relativistic plasma emitter with a coaxial electrodynamic system

A plasma microwave amplifier based on a relativistic electron beam in an electrodynamic system in the form of a coaxial waveguide with a thin tubular plasma in a strong external magnetic field has been considered. Dispersion relations for determining the spectra of plasma and beam waves in the coaxial waveguide, as well as the general dispersion relation describing beam-plasma interaction, have been obtained in the linear approximation. The frequency dependences of the spatial growth rates for different plasma radii and different plasma frequencies, as well as the characteristic frequencies of the plasma amplifier, have been obtained by numerically and analytically solving the dispersion relations. The parameters of the plasma amplifier and generator with the coaxial electrodynamic system have been estimated for their experimental implementation.

Possible origins of a time-resolved frequency shift in Raman plasma amplifiers

Raman amplification is a resonant process in which the energy of a long pump pulse is transferred to a short seed pulse by a plasma wave. There has been a significant effort to identify a window in parameter space within which the interaction is expected to be highly efficient and not degraded by competing instabilities or excessive damping. However, experimental results have thus far failed to approach the theoretical limits. Recent amplified signal spectra display a characteristic blue shift, which evolves within the seed pulse duration and suggests that the mechanism responsible for this shift is also limiting amplification in these experiments. We present the evidence and explore different hypotheses for the origins of the shift—namely localization in density minima along the axis of laser propagation induced by an ion acoustic wave that could arise from the Langmuir decay instability, filamentation which could also modulate the plasma density but in the plane transverse to laser propagation, particle trapping, and additional ionization induced by the amplified seed field.

Poster #10 MAGNETIC RESONANCE IMAGING CHARACTERIZATION OF EARLY POSTNATAL PHENCYCLIDINE TREATMENT AS A RAT MODEL OF SCHIZOPHRENIA

We have studied the effect of prepulses in enhancing the efficiency of generating ASE beams in soft X-ray laser plasma amplifiers based on pumping Ne-like ions. Slab targets were irradiated with a weak prepulse followed by a main plasma heating pulse of nanosecond duration. Time-integrated: time and spectrally resolved and time and angularly resolved lasing emissions on the 3p-3s (J = 0–1) XUV lasing lines of Ne-like Ni, Cu and Zn at wavelengths 232 Å, 221 Å and 212 Å respectively have been monitored. Measurements were made for pre-pulse/main-pulse intensity ratios from 10−5–10−1 and for pump delay times of 2 ns and 4.5 ns. Zinc is shown to exhibit a peak in output intensity at ∼ 2 × 10−3 pre-pulse fraction for a 4.5 ns pump delay, with a main pulse pump intensity of ∼ 1.3 × 1013W cm−2 on a 20 mm target. The Zn lasing emission had a duration of ∼ 240 ps and this was insensitive to prepulse fraction. The J = 0–1 XUV laser output for nickel and copper increased monotonically with prepulse fraction, with copper targets showing least sensitivity to either prepulse level or prepulse to main pulse delay. Under the conditions of the study, the pre-pulse level was observed to have no significant influence on the output intensity of the 3p-3s (J = 2−1) lines of any of the elements investigated.

Radiative properties for warm and hot dense matter

We will present calculations of opacities for matter under LTE conditions. Opacities are needed in radiation transport codes to study processes like Inertial Confinement Fusion and plasma amplifiers in X-ray secondary sources. For the calculations we use the code BiGBART, with either a hydrogenic approximation with j-splitting or self-consistent data generated with the atomic physics code FAC. We calculate the atomic structure, oscillator strengths, radiative transition energies, including UTA computations, and photoionization cross-sections. A DCA model determines the configurations considered in the computation of the opacities. The opacities obtained with these two models are compared with experimental measurements.

Bessel spatial profile of a soft x-ray laser beam

We report far-field profile measurements of an optical-field-ionized high-order harmonic-seeded soft x-ray laser. We show that the beam transverse profile can be controlled between a regular Gaussian shape and a Bessel profile exhibiting several rings via the infrared laser pump intensity. These experimental data are supported by a complete numerical modeling including a two-dimensional plasma amplifier simulation and a two-level soft x-ray amplification using a Maxwell–Bloch treatment. This model takes into account the experimental high-order harmonic wavefront and intensity before it is numerically amplified.

Hydrodynamic study of plasma amplifiers for soft-x-ray lasers: A transition in hydrodynamic behavior for plasma columns with widths ranging from20 μmto 2 mm

Plasma-based seeded soft-x-ray lasers have the potential to generate high energy and highly coherent short pulse beams. Due to their high density, plasmas created by the interaction of an intense laser with a solid target should store the highest amount of energy density among all plasma amplifiers. Our previous numerical work with a two-dimensional (2D) adaptive mesh refinement hydrodynamic code demonstrated that careful tailoring of plasma shapes leads to a dramatic enhancement of both soft-x-ray laser output energy and pumping efficiency. Benchmarking of our 2D hydrodynamic code in previous experiments demonstrated a high level of confidence, allowing us to perform a full study with the aim of the way for 10-100 μJ seeded soft-x-ray lasers. In this paper, we describe in detail the mechanisms that drive the hydrodynamics of plasma columns. We observed transitions between narrow plasmas, where very strong bidimensional flow prevents them from storing energy, to large plasmas that store a high amount of energy. Millimeter-sized plasmas are outstanding amplifiers, but they have the limitation of transverse lasing. In this paper, we provide a preliminary solution to this problem.

Observation of spectral gain narrowing in a high-order harmonic seeded soft-x-ray amplifier

We report an observation of spectral gain narrowing of a high-order harmonic amplified by a soft-x-ray optical-field-ionized plasma. The temporal coherence and spectral linewidth of both the seeded and unseeded soft-x-ray lasers were experimentally measured using a varying-path-difference interferometer. The results showed that the high-order harmonic is subject to a strong spectral narrowing during its propagation in the plasma amplifier without rebroadening at saturation. This is in good agreement with a radiative transfer calculation including gain narrowing and saturation rebroadening.

Optimization of soft x-ray amplifier by tailoring plasma hydrodynamics

Plasma-based seeded soft x-ray lasers have the potential to generate a high-energy, highly coherent, short pulse beam. Owing to their high density, plasmas created by interaction of an intense laser with a solid target should store the highest amount of energy among all plasma amplifiers. However, to date output energy from seeded solid amplifiers remains as low as 60 nJ. We demonstrated that careful tailoring of the plasma shape is crucial for extracting energy stored in the plasma. With 1-mm-wide plasma, energy as high as 20 microJ in sub-ps pulses is achievable. With such tailored plasma, gain and pumping efficiency have been increased by nearly a factor of 10 as compared to the narrower plasma amplifiers studied here.

Aberration-free laser beam in the soft x-ray range

By seeding an optical-field-ionized population-inverted plasma amplifier with the 25th harmonic of an IR laser, we have achieved what we believe to be the first aberration-free laser beam in the soft x-ray spectral range. This laser emits within a cone of 1.34 mrad(1/e(2)) at a repetition rate of 10 Hz at a central wavelength of 32.8 nm. The beam exhibits a circular profile and wavefront distortions as low as lambda/17. A theoretical analysis of these results shows that this high beam quality is due to spatial filtering of the seed beam by the plasma amplifier aperture.

Measurement of1−pssoft-x-ray laser pulses from an injection-seeded plasma amplifier

We report on a pulsewidth measurement of phase-coherent soft x-ray laser pulses generated by injection seeding a solid-target plasma amplifier with high harmonic pulses. A pulse duration of $1.13\ifmmode\pm\else\textpm\fi{}0.47\phantom{\rule{0.3em}{0ex}}\mathrm{ps}$ was measured for a seeded Ne-like Ti plasma amplifier operating at $32.6\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ using an ultrafast streak camera. This is the shortest pulse duration reported to date from a table-top soft x-ray laser amplifier. The result agrees with model simulations which suggest that intense femtosecond soft x-ray laser pulses could be obtained by injection seeding a tailored plasma amplifier in which the gain is confined to a high density region.

An optical-field-induced plasma amplifier for short-pulse vacuum UV radiation

Practical short-wavelength lasers in the vacuum-UV (VUV) spectral region are in high demand in fields such as photolithography and photochemical science because of their fine spatial resolution and ease in triggering reactions. In addition, because VUV emissions do not exist in the atmosphere, they may lead to interesting new phenomena.1, 2 However, few laser media can access this spectral region. Indeed, gas lasers still dominate, especially in the deep VUV (<160nm), where they produce emissions directly. Solid-state laser media, on the other hand, must employ nonlinear wavelength conversion, with a concomitant lowering of efficiency and output. Development of gaseous lasers is further encouraged by the transparent optics at wavelengths down to 105nm. However, the availability of such lasers is limited by our lack of knowledge about their operation. Among existing gaseous lasers, discharge-pumped argon fluoride (ArF) (193nm) and fluorine (F2) (157nm) enjoy the most widespread use. We have been investigating efficient emission sources using rare-gas excimer molecules, such as Ar2* at 126nm and Kr2* (krypton) at 147nm. These deep-VUV lasers are assumed to have unique characteristics in terms of laser-material interactions. The emission wavelength is so short that the penetration depth into materials is also short, usually in the nanometer range. For most materials, the VUV emission energy should thus be absorbed in a very shallow nanorange-thin layer. We have realized nanorange surface alteration of transparent materials such as silicon dioxide (SiO2) using Ar2* excimer lamp emission at 126nm.1 High-quality silicon nitride thin films were produced by irradiating Ar2* excimer emission in silane and ammonia.2 Figure 1. Laser intensity dependence of the harmonic (integer frequency multiple) intensity (I) and ion signal. Xe: Xenon.