Planar Laser-induced Fluorescence Measurements Research Articles

Investigation on unsteady formation and evolution of high-temperature zone in a staged swirl combustor

The high-temperature zone of a laboratory staged swirl gas turbine combustor was studied under different Stratification Ratios (SR) based on experimentally validated Large Eddy Simulation (LES). CH4/air mixtures were adopted with a constant global equivalence ratio of 0.5. Three flame conditions with SR = 1, 2 and 3 were chosen for Particle Image Velocimetry (PIV) and OH Planar Laser-Induced Fluorescence (OH-PLIF) measurements. The LES was performed with the Flamelet-Generated Manifold (FGM) combustion model and validated against the experimental velocity fields and flame structures. Then, a detailed analysis of the formation, evolution, and dissipation of the high-temperature zone was conducted. It is observed that a larger SR deteriorates the uniformity of the exit temperature distribution. One major reason is that with increased SR, rich-burn region is observed to be more dominant. This leads to enhanced non-premixed combustion and an extended heat release region towards downstream, which intensively contribute to the high-temperature zone formation. Additionally, vortices along the shear layers are found to enhance the mixing between fluids of different temperatures, which plays a crucial role in dissipating the high-temperature zone. Higher SR leads to a larger Primary Recirculation Zone (PRZ), and the partially dissipated high-temperature fluid can be recirculated into the PRZ, thus increasing the dissipation distance. With lower SR, however, the high-temperature parcels can be broken and even completely dissipated. This accounts for lower temperature gradients and a more uniform exit temperature distribution. The findings from this study offer new perspectives on understanding the effect of temperature in the primary combustion zone on the exit temperature distribution.

Experimental investigation of NO reduction by H2 on Pd using planar laser-induced fluorescence

This study investigates the NO reduction by H2 on a Pd/Al2O3 catalyst in a temperature range of 100–300 °C and NO/H2 ratios from 0.5–2, aiming to gain a deeper understanding of the reaction kinetics and its interaction with mass transfer. Planar laser-induced fluorescence (PLIF) is used to visualize the NO distributions over the catalyst, supplemented by end-of-pipe gas analysis of other components. The reduced Pd-based catalyst undergoes a slow deactivation after exposure to the reactive flow, leading to reduced overall NO conversion and decreased selectivity towards N2. The NO-PLIF measurements are only conducted on the reduced catalyst without considering the temporal evolutions. Despite the overall NO conversion varying only around 50%–65% across all the investigated conditions, the spatially resolved NO distributions reveal three distinct regimes that limit the overall NO conversion: the regime governed by intrinsic reaction rates, the regime constrained by H2 availability, and the regime restricted by NO diffusion. These findings, demonstrating the interaction between reaction kinetics and mass transfer over a heterogeneous catalyst, highlight the significance of analyzing spatially resolved concentration distributions obtained through PLIF measurements. This approach complements the conventional end-of-pipe analysis, offering a more comprehensive understanding of the underlying processes.

Experimental analysis of boron dilution transient flow mixing characteristics based on planar laser induced fluorescence measurement

In Reactor Pressure Vessels (RPV), flow mixing between high and low concentration coolants will cause uneven distribution of boric acid. Severe cases will lead to boron dilution transient and re-criticality safe operation accident. Therefore, accurate measurement of coolant flow mixing characteristics and boron concentration distribution in RPV and study of the mechanism affecting the mixing process are of great significance to improve reactor operation safety. Based on the structural characteristics of large advanced pressurized water reactor pressure vessel, a large-scale visual experimental device was built by 1:6 scale modular design. Optical path correction scheme is used to solve the problem of optical path distortion existing in PLIF technology, and improved ratio calibration method is used to reduce the experimental error of concentration field distribution measurement. Flow mixing process and boron concentration field distribution in pressure vessel under single loop conditions were obtained based on plane laser induced fluorescence technique (PLIF). The influence of Reynolds number on boron diffusion behavior was studied. The experimental results show that during single loop operation, the localized eddy current formed in the left area of the lower head will result in a high concentration retention zone and a V-shaped boric acid concentration distribution in the core. With the increase of the ratio of cold tube flow to injection flow, the time when the high concentration coolant reaches the core hardly changes with the boric acid solution flow rate. The mixing diffusion behavior of boron concentration is the best when the ratio of injection to Reynolds number in the cold tube is at a certain value.

Analyzing 3D fields of refractive index, emission and temperature in spray-flame nanoparticle synthesis via tomographic imaging using multi-simultaneous measurements (TIMes)

Turbulent spray flames issuing from the SpraySyn 2.0 burner were investigated in the present work by means of tomographic imaging using multi-simultaneous measurements (TIMes). This small-scale standard burner is designed to study flame-spray synthesis of tailored nanoparticle systems. The applied measurement technique combined background-oriented schlieren tomography, computed tomography of light emission and two-color tomographic salt emission thermometry to reveal single-shot and time-averaged 3D fields of refractive index (linked to temperature, pressure and species concentration), CH* chemiluminescence (flame front indicator), SrOH emission from synthesized trace amount of Sr(NO3)2 dissolved in the liquid precursor solution (marker of the hot spray-flame products), and temperature of the hot spray-flame products, respectively. The salt emission thermometry technique was extended to tomographic measurements for the first time. Its implementation was based on the voxel-wise intensity ratio of reconstructed thermally-excited SrOH signals at two different regions in the visible spectrum that was converted to temperature using a single calibration curve based on multi-line OH planar laser-induced fluorescence measurements. The cost-effective setup for TIMes was composed of 43 machine-vision cameras equipped with bandpass spectrum filters, an innovative continuous semi-circular background pattern and LED light sources. The combined reconstructed fields provided information on the 3D flame structure in detail, showing the interaction between the flame front and spray stream, and the hot temperature regions. Spray-flame features were quantitatively analyzed, namely temperature, height, width, 3D tilt angle, and spreading half-angle of the flame plume. The temperature measurements proved to be robust against variations in the fuel/oxidizer equivalence ratio for the four investigated operating conditions. The spray flame issuing from the SpraySyn 2.0 burner at the standard operating condition was more stable than that in the previous burner generation, although more asymmetric near the nozzle exit and tilted, which might still cause heterogeneity of the synthesized nanoparticle system.

Active and passive prechamber assisted engine combustion: simultaneous 50kHz formaldehyde PLIF and OH* visualization

Prechamber-assisted internal combustion engines allow lean limit extension by replacing the spark plug with multiple, high-temperature, radical-rich jets that entrain and ignite the main chamber charge. This work reports the first investigation of active ultra-lean, active rich, and passive prechamber assisted prechamber engine operation (with a fixed prechamber geometry) through 50 kHz cycle-resolved measurements of formaldehyde planar laser-induced fluorescence (PLIF) and OH* imaging in a heavy-duty optical engine operating at 1200 rpm. The third harmonic of a burst mode laser (355 nm) provided the excitation source for formaldehyde PLIF, and a high-speed CMOS camera collected the fluorescence signal from the side window of the engine. Bottom-view imaging of OH* chemiluminescence was achieved using an intensified high-speed camera. The high-speed image sequence of the prechamber jet formaldehyde layer and OH* captures the main chamber heat release stages and the interaction between the moving piston and the prechamber jet. The prechamber-assisted combustion process in the main chamber could be segmented into three phases: initial jet, jet wall interaction, and Post Jet Combustion. The first two phases differ between active and passive operations owing to the global lambda, while the last phases mostly remain flame propagation driven. Jet wall interaction leading to mixing and vortical transport across the main chamber is pivotal in main chamber heat release rate shaping. The study reports the dynamics and evolution of main chamber combustion in detailed time-resolved setups.

Simultaneous planar laser-induced fluorescence measurement of reactant NH3, radical NH, and pollutant NO in ammonia-hydrogen flames using a single dye laser

The stability, local extinction, and NOx production of ammonia-hydrogen (NH3-H2) flames are significantly impacted by turbulence-chemistry interactions. A powerful technique to study these interactions is planar laser-induced fluorescence (PLIF). However, multi-scalar PLIF typically requires complex and expensive systems, with multiple laser sources. This study proposes a novel PLIF technique using a single dye laser to perform simultaneous, single-shot imaging of the reactant NH3, radical NH, and pollutant NO in NH3-H2 flames. According to the excitation scans and the emission spectra of NH3, NH, and NO, three wavelength couples can be used to image the three species simultaneously via two-photon excitation of NH3C'−X (2,0), single-photon excitation of NH A3Π−X3Σ− (0,0) near 304 nm, and single-photon excitation of NO A2Σ+−X2Π (0,1) near 237 nm. Wavelengths near 237 nm and 304 nm are obtained simultaneously with only one dye laser by combining outputs of the frequency-doubling and frequency mixing units. NH3-, NH-, and NO-PLIF imaging performance is analyzed by quantifying the signal-to-noise ratios and detection limits. This technique is then used to visualize the structure of premixed and non-premixed flames over wide ranges of NH3 and H2 concentrations in the fuel blend. Results show that the premixed NH3-H2 flames have a compact structure, while the non-premixed flames exhibit a large gap between NH3- and NH-PLIF layers, where ammonia undergoes significant decomposition before reaching the reaction layer. The inner edge of the NO-PLIF layer overlaps well with the reaction layer represented by the NH-PLIF layer in all flames. The fully developed turbulent structure downstream of the NH3-H2 flame causes pinching-off of the premixed flame front and local extinction of the diffusion flame front.

Effect of CO[formula omitted] dilution on structures of premixed syngas/air flames in a gas turbine model combustor

The impact of CO2 dilution on combustion of syngas (a mixture of H2, CO, and CH4) was investigated in a lab-scale gas turbine model combustor at atmospheric pressure conditions. Two mild dilution levels of CO2, corresponding to 15% and 34% of CO2 mole fraction in the syngas/CO2 mixtures, were experimentally investigated to evaluate the effects of CO2 dilution on the flame structures and the emissions of CO and NOx. All experiments were performed at a constant Reynolds number (Re = 10000). High-speed flame luminescence, simultaneous planar laser-induced fluorescence (PLIF) measurements of the OH radicals and particle image velocimetry (PIV) were employed for qualitative and quantitative assessment of the resulting flame and flow structures. The main findings are: (a) the operability range of the syngas flames is significantly affected by the CO2 dilution, with both the lean blowoff (LBO) limit and the flashback limit shifting towards fuel-richer conditions as the CO2 dilution increases; (b) syngas flames exhibit flame-pocket structures with chemical reactions taking place in isolated pockets surrounded by non-reacting fuel/air mixture; (c) the inner recirculation zone tends to move closer to the burner axis at high CO2 dilution, and (d) the NOx emission becomes significantly lower with increasing CO2 dilution while the CO emission exhibits the opposite trend. The flame-pocket structure is more significant with increased CO2 dilution level. The low NOx emissions and high CO emissions are the results of the flame-pocket structures.

Quantifying the dynamical information content of pulsed, planar laser-induced fluorescence measurements.

We have analyzed the effects of the spreads in experimental parameters on the reliability of speeds and angular distributions extracted from a generic surface-scattering experiment based on planar laser-induced fluorescence detection. The numerical model assumes a pulsed beam of projectile molecules is directed at a surface. The spatial distribution of the scattered products is detected by imaging the laser-induced fluorescence excited by a thin, pulsed sheet of laser light. Monte Carlo sampling is used to select from realistic distributions of the experimental parameters. The key parameter is found to be the molecular-beam diameter, expressed as a ratio to the measurement distance from the point of impact. Measured angular distributions are negligibly distorted when this ratio is <∼10%. Measured most-probable speeds are more tolerant, being undistorted when it is <∼20%. In contrast, the spread of speeds or of corresponding arrival times in the incident molecular beam has only very minor systematic effects. The thickness of the laser sheet is also unimportant within realistic practical limits. These conclusions are broadly applicable to experiments of this general type. In addition, we have analyzed the specific set of parameters designed to match the experiments on OH scattering from a liquid perfluoropolyether (PFPE) surface in the Paper I [Roman et al., J. Chem. Phys. 158, 244704 (2023)]. This reveals that the detailed form of the molecular-beam profile is important, particularly on apparent angular distributions, for geometric reasons that we explain. Empirical factors have been derived to correct for these effects.

High-speed planar laser-induced fluorescence investigation of nitric oxide generated by hypersonic Mach reflections for computational fluid dynamics validation

In this article, the authors present an experimental investigation of the thermochemical relaxation regions downstream of symmetric Mach reflections generated in Mach 8.5 flows with stagnation enthalpies from 7 to 10 MJ/kg. The experiment was performed in the Hypervelocity Expansion Tunnel at the National Aerothermochemistry and Hypersonics Laboratory of Texas A&amp;M University. The investigation focused on studying the nitric oxide morphology in the vicinity of a strong normal shock wave and shear layers. Experimental planar laser-induced fluorescence measurements at 250 kHz repetition rate with a quasi-simultaneous natural emission photography demonstrate a sufficient rejection of natural emission and reveal intricate flow structures in the shock vicinity. Steady computational fluid dynamics (CFD) flow solutions obtained with the US3D software were used to simulate laser-induced fluorescence signal levels for quantitative comparison against the experimentally acquired data. The investigation accomplished four objectives: complex flowfield visualization in the vicinity of the Mach stem with 4 μs temporal resolution, evaluation of the level of high-temperature chemistry effects introduced to the freestream by the expansion tunnel, both qualitative and quantitative CFD simulation validation, and cross-checking or introduction of fundamental properties of nitric oxide laser-induced fluorescence including absorption cross section for vibrationally excited states of nitric oxide and a collisional quenching cross section of nitric oxide by atomic nitrogen.

High-speed formaldehyde planar laser-induced fluorescence and schlieren to assess influences of injection pressure and oxygen concentration on Spray A flames

The present study investigates the effect of injection pressure and ambient oxygen concentration variations on the Engine Combustion Network Spray A flame. The two-stage ignition and combustion processes for individual injections are characterized using a high-speed planar laser-induced fluorescence (PLIF) and schlieren imaging diagnostic at high pressure (near 6 MPa). For PLIF measurements, we use a pulse-burst-mode Nd:YAG laser capable of producing a 6 ms long 355-nm pulse-train with 300 pulses at 70 mJ/pulse, separated by 20 µs. The PLIF imaging at high-acquisition rate offers unique insights into understanding the spatiotemporal distribution of formaldehyde (CH2O) and polycyclic aromatic hydrocarbons (PAH). High-speed line-of-sight schlieren with a pulsed infrared light emitting diode (LED) is applied simultaneously with PLIF to visualize the spray penetration, low- and high-temperature ignition, and turbulent flame dynamics, while in-vessel pressure is used in concert with the optical diagnostics to assess the ignition delay time of the high-temperature ignition events. The PLIF and line-of-sight measurements, documenting the position and timing for formation and consumption of CH2O and the inception and distribution of PAH downstream with changes in ambient oxygen concentration and injection pressure, provide a unique database for detailed evaluation of single-event (e.g. LES) or ensemble-average CFD.

Effect of H2 addition on the local extinction, flame structure, and flow field hydrodynamics in non-premixed bluff body stabilized flames

We examined the effect of hydrogen (H2) enrichment on the primary fuel methane (CH4) in a canonical non-premixed bluff-body stabilized burner operating under typical central jet-dominated flame mode. In the chosen mode of operation, globally, the flow field and flame feature three important successive spatial zones: the recirculation zone, the neck zone, and the jet-like flame zone. The flame is exposed to a higher stretch rate in the neck zone in such a configuration and eventually undergoes local extinction. Such local extinction and subsequent re-ignition/reconnection of broken flame branches have substantial implications for the hydrodynamic instability of the coaxial annular air shear layer. It is well known that H2 addition increases the flame extinction strain rate (κext) and thus alters the local extinction phenomenon. To understand this, we performed experiments at 0%, 10%, 20%, 30%, 50%, 80%, and 100% hydrogen proportion in the H2-CH4 blend. High repetition rate (5 kHz) Particle Image Velocimetry and OH Planar Laser Induced Fluorescence (PLIF) measurements are simultaneously implemented to gain quantitative insight into the flow field and flame structure. A detailed analysis performed over the instantaneous OH–PLIF datasets reveals the absence of local extinctions in flames with H2 enrichment &amp;gt;30% due to an increased extinction strain rate (κext). Furthermore, it is found that H2 enrichment plays a significant role in the reconnection/re-ignition of the broken flame branches formed during the local extinction. For instance, a high reconnection probability is observed in flames with an H2 addition of ≥20%. Consequently, variations in the mean reaction zone height are witnessed for different H2 enrichment levels. Further analysis of the influence of variation in reaction zone height on flow field hydrodynamics is explored using Proper Orthogonal Decomposition (POD) and Continuous Wavelet Transform (CWT). The results obtained from POD and CWT indicated the suppression of vortex shedding at the annular air shear layer for H2 addition greater than 20% and irregular wrinkling of flame fronts. Thus, they quantified the beneficial effect of H2 addition in turbulent flame stabilization.

A generative adversarial network (GAN) approach to creating synthetic flame images from experimental data

Modern diagnostic tools in turbulent combustion allow for highly-resolved measurements of reacting flows; however, they tend to generate massive data-sets, rendering conventional analysis intractable and inefficient. To alleviate this problem, machine learning tools may be used to, for example, discover features from the data for downstream modeling and prediction tasks. To this end, this work applies generative adversarial networks (GANs) to generate realistic flame images based on a time-resolved data set of hydroxide concentration snapshots obtained from planar laser induced fluorescence measurements of a model combustor. The generative model is able to generate flames in attached, lifted, and intermediate configurations dictated by the user. Using k-means clustering and proper orthogonal decomposition, the synthetic image set produced by the GAN is shown to be visually similar to the real image set, with recirculation zones and burned/unburned regions clearly present, indicating good GAN performance in capturing the experimental data statistical structure. Combined with techniques for controlling the configuration of generated flames, this work opens new avenues towards tractable statistical analysis and modeling of flame behavior, as well as rapid and inexpensive flame data generation.

Investigation of 10 kHz Filtered Rayleigh Scattering and CH2O Planar Laser-Induced Fluorescence Measurement in Two-Stage Swirl Combustor

Investigation of 10 kHz Filtered Rayleigh Scattering and CH₂O Planar Laser-Induced Fluorescence Measurement in Two-Stage Swirl Combustor

On polyhedral structures of lean methane/hydrogen Bunsen flames: Combined experimental and numerical analysis

In premixed flame propagation of lean hydrogen or hydrogen-enriched blends, both hydrodynamic and thermo-diffusive instabilities are governing the flame front shape and affect its propagation velocity. As a result, different types of cellular patterns can occur along the flame front in a laminar scenario. In this context, an interesting phenomenon is the formation of polyhedral flames which can be observed in a Bunsen burner. It is the objective of this work to systematically characterize the polyhedral structures of premixed methane/hydrogen Bunsen flames in a combined experimental and numerical study. A series of lean flames with hydrogen content varying between 20 and 85% at two equivalence ratios is investigated. The experiments encompass chemiluminescence imaging together with Planar Laser-induced Fluorescence (PLIF) measurements of the OH radical. Characteristic cell sizes are quantified from the experiments and related to the characteristic length scales obtained from a linear stability analysis. In the experiments, it is observed that the cell sizes at the base of the polyhedral Bunsen flames decrease almost linearly with hydrogen addition and only a weak dependence on the equivalence ratio is noted. These trends are well reflected in the numerical results and the length scale comparison further shows that the wavelength with the maximum growth rate predicted by the linear stability analysis is comparable to the cell size obtained from the experiment. The correlation between the experimental findings and the linear stability analysis is discussed from multiple perspectives considering the governing time and length scales, furthermore drawing relations to previous studies on cellular flames.

Effect of flame retardants on side-wall quenching of partially premixed laminar flames

A combined experimental and numerical investigation of partially premixed laminar methane-air flames undergoing side-wall quenching (SWQ) is performed. A well-established SWQ burner is adapted to allow the seeding of the main flow with additional gaseous products issued from a (secondary) wall inlet close to the flame’s quenching point. First, the characteristics of the partially premixed flame that quenches at the wall are assessed using planar laser-induced fluorescence measurements of the OH radical, and a corresponding numerical simulation with fully-resolved transport and chemistry is conducted. A boundary layer of enriched mixture is formed at the wall, leading to a reaction zone parallel to the wall for high injection rates from the wall inlet. Subsequently, in a numerical study, the wall inflow is mixed with dimethylmethylphosphonat (DMMP), a phosphor-based flame retardant. The DMMP addition allows the assessment of the combined effects of heat loss and flame retardants on the flame structure during flame-wall interaction. With an increasing amount of DMMP in the injected mixture, the flame stabilizes further away from the wall and shows a decrease in the local heat-release rate. Thereby, the maximum wall heat flux is significantly reduced. That results in a lower thermal load on the quenching wall. The flame structure analysis shows an accumulation of the intermediate species HOPO at the wall similar to the CO accumulation during the quenching of premixed flames without flame retardant addition. The study shows how the structure of a partially premixed flame is influenced by a wall that releases either additional fuel or a mixture of fuel and flame retardant. The insights gained from the canonical configuration can lead to a better understanding of the combined effects of flame retardants and heat losses in near-wall flames.

Influence of flow structures and combustion on cross-scale turbulent kinetic energy transfer in premixed swirl flames.

This paper experimentally analyzes the simultaneous influence of combustion and large-scale vortex structures on the transfer of kinetic energy across scales around the laminar flame thickness δL0 in a turbulent premixed swirl flame and a non-reacting swirl flow. High-resolution tomographic particle image velocimetry and formaldehyde planar laser induced fluorescence measurements are used to obtain 3D velocity fields and estimates of the progress variable and density fields. The kinetic energy transfer across a filter scale of Δ=1.5δL0 was then quantified using physical space analysis. Coherent flow structures were identified using the swirling strength and proper orthogonal decomposition was used to identify the dominant periodic flow structure. While non-reacting regions of the flow show mean down-scale energy transfer (forward-scatter), mean back-scatter is observed internal to the flame. Importantly, the back-scatter magnitude in the flame increases in regions undergoing flame/vortex interaction. That is, the mean back-scatter magnitude at locations simultaneously inside the flame and a large-scale coherent vortex is higher than regions in the flame and not in a vortex, with the mean back-scatter magnitude increasing with the swirling strength. This increased back-scatter may be due to locally higher heat release rates in locations of flame/vortex interaction. Overall, the results demonstrate the importance of kinetic energy back-scatter at scales around the flame thickness and the complicated relationship between back-scatter and local flame/flow structure; these results should be considered when modeling turbulence in flames.

Stabilization and Emission Characteristics of Gliding Arc-Assisted NH3/CH4/Air Premixed Flames in a Swirl Combustor

This paper investigates the effects of gliding arc (GA) discharge on the stabilization and emission characteristics of premixed NH3/CH4/air swirl flames under various ammonia contents, flow rates, and global equivalence ratios. First, the lean blowout (LBO) limits are measured. We find that although blending CH4 extends the LBO limit of the ammonia flame to 0.6–0.8, the GA discharge further remarkably extends it to 0.3–0.4. Then, the flow and flame structures are visualized by simultaneous OH planar laser-induced fluorescence and particle imaging velocimetry measurements. The results reveal that the discharge increases the OH radical concentration and expands the inner recirculation zone, leading to improved flame stability. Second, the NOx emissions are investigated over a wide range of global equivalence ratios and ammonia contents. It is seen that the GA discharge slightly increases the NOx emission by less than 7% at low NH3 contents (<0.6), which can be attributed to the thermal and OH-involved reaction pathway of NOx formation. However, as the NH3 content further increases (which is accompanied by the rapid growth of the NOx emission), the GA discharge effectively reduces the NOx emission by up to 30%. This effect might be due to the more intensive NOx-consuming reactions by plasma-induced NH2 radicals at a higher ammonia content, which is confirmed by the strengthened NH2* chemiluminescence under GA discharge conditions. Finally, a chemical reactor network analysis gives reasonable NOx predictions without GA discharge and highlights the NOx-reduction effects of NH2 radicals under high ammonia contents.

Pilot impact on turbulent premixed methane/air and hydrogen-enriched methane/air flames in a laboratory-scale gas turbine model combustor

The impact of pilot flame operation on the combustion of pure methane and hydrogen-enriched methane (H2/CH4: 50/50 in vol%) fuels was investigated in a gas turbine model combustor under atmospheric conditions. The burner assembly was designed to mimic the geometry of an industrial burner, the Siemens DLE Burner, in which a concentric annular ring equipped with pilot flame burners is implemented in the dome of the combustor. Two pilot burner configurations have been investigated: a non-premixed and a partially premixed pilot arrangement. The performance of the pilot burners was evaluated for varying Reynolds number (Re) and H2 enrichment. High-speed OH∗ chemiluminescence imaging, as well as simultaneous planar laser-induced fluorescence measurements of the OH radicals and formaldehyde (CH2O) were used for evaluating the dynamics and structures of the flames for different conditions. Furthermore, emission measurements were carried out to determine the influence of hydrogen dilution on the NOx and CO emission levels. The main findings are (a) the effect of the pilot flame is sensitive to the Reynolds number of the main flame and the type of the pilot flame, (b) the stability range becomes narrower with increasing hydrogen ratio, due to the tendency to flashback, (c) non-premixed pilot flames lower the NOx and increase the CO emissions, albeit rather small differences in the emissions have been detected, and (d) the NOx and CO emissions become significantly lower with increasing hydrogen ratio.

Flame features and oscillation characteristics in near-blowout swirl-stabilized flames using high-speed OH-PLIF and mode decomposition methods

Flame features and dynamics are important to the explanation and prediction of a lean blowout (LBO) phenomenon. In this paper, recognition of near-LBO flame features and oscillation characterization methods were proposed based on flame spectroscopic images. High-speed planar laser-induced fluorescence measurements of OH were used to capture unique dynamic features such as the local extinction and reignition feature and entrained reactant pockets. The Zernike moment demonstrated a good performance in recognition of stability and near-LBO conditions, though the geometric moment had more advantages to characterize frequency characteristics. Low-frequency oscillations, especially at the obvious self-excited oscillation frequency around 200 Hz, were found when approaching an LBO condition, which can be expected to be used as a novel prediction characteristic parameter of the flameout limit. Proper orthogonal decomposition (POD) and dynamic mode decomposition (DMD) were used to conduct dynamic analysis of near-LBO flames. POD modes spectra showed the unique frequency characteristics of stable and near-LBO flames, which were basically in line with those at the heat-release frequency. The primary POD modes demonstrated that the radial vibration mode dominated in a stable flame, while the rotation mode was found to exist in a near-LBO flame. Analysis of modal decomposition showed that flame shedding and agminated entrained reactant pockets were responsible for generating self-excited flame oscillations.

Experimental analysis of a non-isothermal confined impinging single plume using time-resolved particle image velocimetry and planar laser induced fluorescence measurements

In this study, the experimental results of the flow behavior of a non-isothermal confined impinging single plume were analyzed. Experimental measurements were performed in the upper plenum of a high-temperature gas-cooled reactor (HTGR) that was scaled, designed, and assembled at Texas A&M University. The goal was to investigate flow mixing, thermal stratification, and plume impingement in the upper plenum of the HTGR under a loss-of-forced-coolant accident and provide a high-fidelity experimental database for validating computational fluid dynamics (CFD) and system codes. Time-resolved particle image velocimetry (TR-PIV) and planar laser-induced fluorescence (P-LIF) measurements were performed in the central plane of the plume flow in the upper plenum. A total power of 0.4 kW of heat was applied to the system. Convergence was achieved for the statistical results from the TR-PIV and P-LIF snapshots. The TR-PIV velocity vectors presented statistical characteristics of the plume flow, such as the mean velocity, root-mean-square fluctuating velocity, and Reynolds stress. The results revealed that the flow reached the maximum velocity far from the jet inlet at y/Dj=2. Furthermore, two-point velocity cross-correlation was performed on the TR-PIV velocity vector fields. Finally, the statistical results were calculated from the P-LIF temperature snapshots and the mean temperature. Furthermore, the temperature profiles were plotted. It was observed that the flow reached the maximum temperature near the plume inlet and decreased downstream.