The fabrication of periodic nanostructures has garnered significant attention. Despite the investigation into the mechanical properties and deformation behaviors of graphene coated on metal surfaces during single indentation, there remains a dearth of research on the mechanical response and deformation behaviors of graphene/Cu systems, as well as the effects of different crystal orientations during continuous nanoindentation. The present study employed molecular dynamics simulations to investigate the effects of crystal orientation and coated graphene on surface morphology, elastic recovery, and dislocation evolution in Cu and graphene/Cu systems under continuous indentation-induced deformation. The results revealed that the force required for continuous indentation was approximately 1.36 times higher than that for initial indentation at the same depth on Gr/Cu, indicating a significant work hardening effect induced by the first indentation. Moreover, the continuous indentation enhances the surface pile-up effect and promotes the formation of more atoms in the overlap region between adjacent indentations. The presence of graphene coatings significantly influences the contact area, suppressing dislocation nucleation while increasing dislocation density. Furthermore, during continuous indentation, the depth at which dislocation nucleation occurs is shallower compared to that observed during initial indentation. The subsurface damage caused by the initial indentation was comparatively more severe than that induced during continuous indentation. Notably, the extent of dislocation propagation resulting from continuous indentation on graphene/Cu surpassed that observed on Cu alone. These findings significantly contribute to our comprehension of the metal-graphene interaction mechanism during continuous indentation and offer valuable insights for optimizing indentation quality.
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