Picosecond Optical Parametric Oscillator Research Articles

Near to Mid-Infrared (1.3–5 μm) Widely Tunable, High Power Picosecond Pulsed Laser

We present a high-power, widely tunable, synchronously pumped picosecond pulsed optical parametric oscillator (OPO) generating emissions in the near to mid-infrared wavelength ranges. The OPO is pumped using a Nd:YVO4 picosecond pulsed laser and utilizes a fan-shaped, multi-grating MgO doped PPLN crystal (MgO:PPLN). The system generates near to mid-infrared output across the wavelength range 1.3–5 µm, with a high overall conversion efficiency of 75.15%.

15-µJ picosecond hollow-core-fiber-feedback optical parametric oscillator.

We report a high-energy, picosecond, mid-infrared (MIR) optical parametric oscillator (OPO), in which a length of hollow-core-fiber (HCF) is employed to enable operation at 1-MHz repetition rate in a compact cavity format. The OPO is synchronously pumped by an ytterbium-doped-fiber (YDF) master-oscillator-power-amplifier (MOPA) system, seeded by a 1040-nm gain-switched laser diode (GSLD). Using periodically poled lithium niobate (PPLN) as the nonlinear crystal, the OPO generates signal and idler beams with tunable wavelengths in the range of 1329-1641 nm and 2841-4790 nm, respectively. The OPO provides 137-ps pulses with a maximum signal energy of 10.05 µJ at 1600 nm and a maximum idler energy of 5.13 µJ at 2967 nm. This, to the best of our knowledge, represents the highest energy MIR pulses, as well as the highest total converted pulse energy (15.18 µJ), ever achieved from a fiber laser pumped picosecond OPO.

Yb-fiber-pumped high-average-power picosecond optical parametric oscillator tunable across 1.3−1.5 μm

We report the generation of high-repetition-rate picosecond pulses in the 1.3-1.5µm spectral range by internal second harmonic generation (SHG) of an idler-resonant optical parametric oscillator (OPO) based on MgO-doped periodically-poled LiNbO3 (MgO:PPLN), synchronously pumped by ∼20 ps pulses at 80 MHz using an Yb-fiber laser at 1.064 µm. By taking advantage of the high spatial quality of the resonant idler beam in the 2503-3030 nm wavelength range and using a second MgO:PPLN crystal with fanout grating structure for intracavity SHG, we have achieved spectral coverage across 1272-1515 nm with up to 1.23 W average power. The second harmonic output exhibits a power stability of 3% rms over 1 hour in pulses of 8.3 ps with Gaussian beam profile. The described approach overcomes the spectral limitation of 1.064 µm-pumped OPOs based on MgO:PPLN and other oxide-based nonlinear crystals, where signal generation below ∼1.45 µm is precluded by multi-phonon absorption of idler radiation above ∼4µm.

Synchronously Intracavity-Pumped Picosecond Optical Parametric Oscillators for Sensors.

The research and development of laser systems for intracavity phase interferometry is described. These systems are based on an intracavity synchronously pumped optical parametric oscillator (OPO), enabling the generation of two trains of picosecond pulses inside a single cavity. In such a configuration, it is possible to measure the beat note frequency between two pulses and to very precisely determine the phase difference between them. The pump source is a diode-pumped passively mode-locked Nd:YVO laser. A periodically poled magnesium-doped lithium niobate crystal is used as the optical parametric oscillator crystal coupling the pump and the signal cavities. We designed a synchronously pumped OPO in a linear and ring cavity configuration allowing generation in a dual-pulse regime. By a mutual detuning of both cavity lengths, the quasi-synchronous regime of pumping was achieved and high harmonics of repetition rate frequencies were generated. Such a system can be useful for applications such as pump-probe spectroscopy or for testing telecommunication systems. We also realized the subharmonic OPO cavity as a source of two independent trains of picosecond pulses suitable for intracavity phase interferometry; we also measured the beat note signal.

A 45-μJ, 10-kHz, burst-mode picosecond optical parametric oscillator synchronously pumped at a second harmonic cavity

A novel high-energy picosecond optical parametric oscillator (OPO) was realized by placing an OPO in a second-harmonic (SH) cavity. In a proof-of-principle experiment, we demonstrated excellent burst energy of 45 μJ for the OPO signal at 900 nm that operates at a pulse repetition rate of 10 kHz and a pulse width of 46.8 ps. The beam quality was measured as and in the orthogonal directions, corresponding to an average beam factor M 2 = 1.42. So far, this study is the first to investigate high-energy ps OPO synchronously pumped in a second-harmonic cavity.

Tunable, high-power, high-order optical vortex beam generation in the mid-infrared.

We report the generation of tunable high-order optical vortices in the mid-infrared (mid-IR) using a picosecond optical parametric oscillator (OPO). The OPO is based on MgO:PPLN as the nonlinear gain medium and synchronously pumped by a mode-locked Yb-fiber laser at 1064 nm. Using a singly-resonant oscillator configuration for the OPO, we have achieved direct transfer of pump optical vortices to the non-resonant idler beam, with the resonant signal in the Gaussian cavity mode. We demonstrate the successful transfer of pump optical vortices of order, lp = 1 to 5, to the idler beam of the same order across the mid-IR, with an output power of 630 mW to 130 mW across 2538 nm to 4035 nm for the highest idler vortex order, li = 5. To the best of our knowledge, this is the first report of an OPO pumped by a vortex beam of order as high as lp = 5 and generating idler vortices of high order in the mid-IR.

High resolution ZrF4-fiber-delivered multi-species infrared spectroscopy

Using coherent broadband mid-infrared light from a picosecond optical parametric oscillator we introduce a flexible, easy to use, high-resolution technique which can be utilized to conduct remote stand-off, or fiber delivered, multi-species spectroscopy in a spectroscopically cluttered environment. In particular, both narrow line-like and broad continuum-like species can be handled simultaneously. If only species with narrow line-like absorptions are present, this can be done without the need for an explicit reference spectrum. We demonstrate the approach by performing absorption spectroscopy of H2O, CH4, CH3OH and C2H7NO (MEA) at high optical resolution (≈0.033 cm−1) and via fiber delivery, opening the possibility of conducting multi-species spectroscopy in remote and hazardous environments. Spectral co-fitting of all absorption features and of the spectrum of the light-source provides a robust means of determining species concentrations, with detection limits of 290 ppb and 890 ppb obtained for CH4 and MEA respectively using a 10.5-m Herriott cell and 32 seconds measurement time.

Compact picosecond mid-IR PPLN OPO with controllable peak powers

We report a high-repetition-rate, compact, mid-infrared picosecond (ps) optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN). The OPO is synchronously pumped by an ytterbium-doped-fibre (YDF) master-oscillator-power-amplifier (MOPA) system, seeded by a 1040-nm gain-switched laser diode (GSLD). Under continuous-wave (cw) pulsed operation, at a 1.5-GHz repetition rate and 14-W pump power, an idler average power of 2.4 W (∼30 W peak power) was achieved, with an idler wavelength tunability of 2260–3573 nm. Through the addition of an electro-optic modulator (EOM) to the MOPA system, acting as a time gate to suppress a variable number of pulses per 1 µs, a quasi-cw pumping regime was realized, allowing burst-mode operation of the OPO at a 1-MHz inter-burst repetition rate. By varying the burst window time with the EOM, controllable idler peak powers of up to 1.2 kW were then realized.

Phase-locked picosecond optical parametric oscillator.

We report a degenerate self-phase-locked picosecond optical parametric oscillator (OPO) synchronously pumped by a mode-locked Yb-fiber laser at 1064 nm, delivering broadband output near 2 µm with 2.8 W of average power at ∼80MHz repetition rate. By exploiting a 50-mm-long MgO:PPLN crystal providing high gain and low group velocity dispersion under type-0 (e→ee) phase matching, the OPO generates a phase-locked degenerate output spectrum with a bandwidth of ∼202nm centered at 2128 nm in pulses of ∼21ps duration with excellent passive long-term power and spectral stability in high spatial beam quality. Phase-locked operation results in spectral and power stabilization at exact degeneracy and is further validated by f-2f interferometry and radio frequency measurements of OPO output. To the best of our knowledge, this is the first degenerate self-phase-locked OPO in picosecond time scale, and the highest average power reported for a phase-locked ultrafast OPO to date.

High-average-power picosecond mid-infrared OP-GaAs OPO.

We report a high-average-power mid-infrared picosecond (ps) optical parametric oscillator (OPO) based on orientation-patterned gallium arsenide (OP-GaAs), with wide wavelength tunability. The OP-GaAs OPO is synchronously pumped by a thulium-doped-fiber (TDF) master oscillator power amplifier (MOPA), seeded by a gain-switched laser diode. At a pump power of 35.3 W and a repetition rate of 100 MHz, a maximum OPO total average output power of 9.7 W (signal 5.7 W (0.60 kW peak power), idler 4.0 W (0.42 kW peak power)) is obtained at signal and idler wavelengths of 3093 nm and 5598 nm, and a thermally induced power roll-off is observed. To mitigate the thermal effects, an optical chopper is placed before the OPO to provide burst mode operation and a reduced thermal load. We achieved a linear growth in OPO output power over the full range of available pump powers in this instance confirming thermal effects as the origin of the roll-off observed under continuous pumping. We estimate the maximum peak powers of the signal and idler are estimated to be over 0.79 kW and 0.58 kW, respectively in this instance. A wide mid-infrared wavelength tuning range of 2895-3342 nm (signal) and 4935-6389 nm (idler) is demonstrated.

Yb-fiber-pumped, high-beam-quality, idler-resonant mid-infrared picosecond optical parametric oscillator.

We report an Yb-fiber-pumped picosecond optical parametric oscillator (OPO) delivering high average power in excellent beam quality throughout the mid-infrared (mid-IR). Using MgO:PPLN as the nonlinear crystal and configured as a singly-resonant oscillator in the mid-IR idler wave, the OPO provides up to 3.5 W average power in high spatial quality with M2<1.8 across a continuous tuning range of 4028-2198 nm, with M2<1.5 at 4000 nm. It can also deliver as much as 4.3 W of signal power in an output beam with M2<1.4 across 1446-2062 nm. The extracted idler exhibits a passive power stability better than 0.46% rms over 1 hour across the entire mid-IR tuning range. We have also investigated OPO cavity length detuning behavior about the zero-group-velocity-mismatch crossing point and its effects on output power.

High-beam-quality, watt-level, widely tunable, mid-infrared OP-GaAs optical parametric oscillator

We demonstrate near-diffraction-limited performance from a mid-infrared, idler-resonant, fiber-laser-pumped, widely tunable, picosecond optical parametric oscillator (OPO) based on orientation-patterned gallium arsenide (OP-GaAs). The OP-GaAs OPO is synchronously pumped by a picosecond Tm:fiber master–oscillator-power-amplifier system. An OPO tuning range of 4394–6102 nm (idler) and 2997–3661 nm (signal) is achieved, with maximum average powers of 1.18 (idler, 5580 nm) and 0.51 W (signal, 3136 nm). The idler beam has M2 values of 1.06 (x-direction) by 1.03 (y-direction).

A high energy, wavelength and repetition rate tunable eye-safe picosecond optical parametric oscillator

A wavelength and pulse repetition rate (PRR) tunable eye-safe picosecond (ps) optical parametric oscillator (OPO) with high energy is developed using a novel method that operates the OPO in a ps regenerative amplifier (RA). With this method, the PRR can be conveniently tuned and a compact kHz ps OPO can be achieved with a pulse energy of 1–3 orders of magnitude higher than previous works. Based on an angle phase matching type II (θ = 41.4°, φ = 0°) KTA crystal, signal wavelength tunability from 1501 nm to 1565 nm is realized at the PRRs of 5 kHz and 10 kHz, respectively. The highest pulse energy of 21.6 µJ with a pulse width of about 6 ps is obtained at the PRR of 5 kHz and a wavelength of 1532 nm.

Pulse length variation causing spectral distortions in OPO-based hyperspectral coherent Raman scattering microscopy

Picosecond optical parametric oscillators (OPOs) with broad wavelength tunability are frequently used as light sources in hyperspectral coherent Raman scattering (CRS) microscopy. We investigate how changes in the pulse length during OPO wavelength tuning of the pump beam affect hyperspectral CRS imaging. We find that significant distortions of the resulting CRS spectra occur if the OPO is operated without monitoring pulse length variations. By utilizing a custom-written MATLAB based control program to counteract changes in pulse length, normalized and reproducible data sets can be acquired. We demonstrate this by comparing hyperspectral data obtained from pure substances, as well as relevant biological specimens.

Long-wave infrared generation from femtosecond and picosecond optical parametric oscillators based on orientation-patterned gallium phosphide

Optical parametric oscillators synchronously pumped with 1-µm femtosecond and picosecond lasers are used to generate long-wave mid-infrared radiation using the nonlinear material orientation-patterned gallium phosphide. The output spectra from the femtosecond OPO are measured, demonstrating tuning based on grating period and temperature from 5.5 to 13.0 µm. The picosecond OPO produces 137 mW at 7.87 µm, representing the first picosecond-pumped OPO using orientation gallium phosphide.

Yb-fiber-pumped mid-infrared picosecond optical parametric oscillator tunable across 6.2–6.7 µm

We report a high-average-power picosecond optical parametric oscillator (OPO) tunable in the mid-infrared (mid-IR) based on CdSiP2 synchronously pumped by an Yb-fiber laser at ~ 80 MHz repetition rate. Successful operation of this high-repetition-rate singly-resonant picosecond OPO has been enabled by the improved CSP crystal quality over a long interaction length. The OPO can be tuned across 1264–1284 nm in the near-IR signal and 6205–6724 nm in the mid-IR idler by temperature tuning the CSP crystal over 39–134 °C. By deploying a 5% output coupler for the resonant signal, we have extracted up to 44 mW of average power in the near-IR and up to 95 mW of non-resonant idler power at 6205 nm at 6.3% total conversion efficiency, with > 50 mW over > 55% of the mid-IR tuning range. We have investigated temperature-tuning characteristics of the OPO and compared the data with the theoretical calculations using the recent Sellmeier and thermo-optic coefficients for CdSiP2. The signal pulses from the OPO exhibit a Gaussian pulse duration of 19 ps centered at 1284 nm. We have also studied the output power stability of the OPO, resulting in a passive stability better than 1.9% rms for the near-IR signal and 2.4% rms for the mid-IR idler, measured over > 17 h, with both beams in high spatial quality.

30.5-μJ, 10-kHz, picosecond optical parametric oscillator pumped synchronously and intracavity by a regenerative amplifier.

We have proposed a novel approach to realize a high-energy ultrafast optical parametric oscillator (OPO) by intracavity pumping in a regenerative amplifier. In this way, we have experimentally demonstrated an unprecedented pulse energy of 30.5μJ from a 1.5-μm singly resonant synchronously pumped OPO at a pulse repetition rate of 10kHz with a pulse width of 7.0ps. To the best of our knowledge, this is the highest pulse energy from an ultrafast laser OPO.

High-repetition-rate, deep-infrared, picosecond optical parametric oscillator based on CdSiP2.

We report a high-repetition-rate picosecond optical parametric oscillator (OPO) based on CdSiP2 (CSP) that is synchronously pumped by an Yb-fiber laser at 1064nm and provides high average power in the deep-infrared (deep-IR) at 79.5MHz. The OPO is tunable across 6205-6710nm in the idler, providing as much as 105mW of average power at 6205nm and >55 mW over nearly the entire tuning range. The deep-IR idler output exhibits passive power stability better than 2.3% rms over 12h in good beam quality. The near-IR signal pulses from the OPO have a Gaussian pulse duration of ∼19 ps, measured at 1284nm. We have investigated the temperature tuning characteristics of the OPO and compared the data with the theoretical calculations using the most recent Sellmeier equations and thermo-optic coefficients for the crystal. To the best of our knowledge, this is the first picosecond OPO based on CSP operating at MHz repetition rates.

Picosecond difference-frequency-generation in orientation-patterned gallium phosphide.

We report the generation of tunable high-repetition-rate picosecond radiation in the mid-infrared using the new quasi-phase-matched nonlinear material of orientation-patterned gallium phosphide (OP-GaP). The source is realized by single-pass difference-frequency-generation (DFG) between the output signal of a picosecond optical parametric oscillator (OPO) tunable across 1609-1637 nm with input pump pulses at 1064 nm in OP-GaP, resulting in tunable radiation across 3040-3132 nm. Using a 40-mm-long crystal, we have generated up to 57 mW of DFG average power at ~80 MHz repetition rate for a pump power of 5 W and signal power of 0.9 W, with >30 mW over >50% of the tuning range. The DFG source exhibits a passive power stability better than 3.2% rms over 1 hour in good spatial beam quality. To the best of our knowledge, this is the first picosecond frequency conversion source based on OP-GaP.

Wide and fast dispersion tuning of a picosecond OPO based on aperiodic quasi-phase matching using an axially chirped volume Bragg grating.

We report on a widely tunable synchronously pumped picosecond optical parametric oscillator (OPO) combining an aperiodically poled MgO-doped LiNbO3 crystal as a broadband gain medium and an axially chirped volume Bragg grating as a spectral filtering dispersive element. Translation of the Bragg grating along the beam axis enables wavelength tuning over 215nm around 3.82μm and provides spectral narrowing. Rapid continuous tuning over 150nm in 100ms is demonstrated.