Because of the improved physical, mechanical and crack–resistant properties, smart cementitious materials have garnered significant attention in civil engineering. However, the method of predicting performance of smart cementitious materials remains a formidable task. To address this issue, this study develops a neural network optimized by particle swarm algorithm, specifically designed for predicting the strength of smart cementitious materials. Particle swarm optimization is used to determine the initial weights and biases of the neural network in this algorithm. Two types of smart cementitious materials, namely 3D printed fiber reinforced concrete and graphene nanoparticles–reinforced cementitious composites, are studied as examples. Utilizing the PSO–BPNN method and data gathered from the existing articles, the predictive models for the mechanical properties of these materials are developed. Five commonly used statistical metrics are applied to evaluate the predictive performance. The results indicate suggest the PSO–BPNN outperforms the traditional back propagation neural network. Thus, a reliable and robust performance predictive model can be built for smart cementitious materials using the proposed approach.
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