Particle Trapping Research Articles

Compensating loss via non-Hermiticity in optically trapped and bounded particles

The non-Hermiticity in the optical trapping and binding originates from their open nature. Once the non-Hermiticity is sufficiently large such that it pushes the system across the exceptional point, the non-Hermitian force will provide an effective gain to the systems. In this scenario, the trapped particles acquire additional energies as a consequence of the non-Hermitian force field, which effectively serve as a gain. Conversely, these trapped or bound particles can also dissipate energy as a result of the damping effect experienced during oscillation within optical trapping or binding. People usually employ vacuum extraction to extend the lifetime of particles’ vibrational modes. However, low-pressure environments can induce instability in the systems. Here, we propose using the “non-Hermitian gain” to compensate for damping loss and enhance the quality factor (lifetime, Q-factor) of vibrational modes. Our study also takes into account the Brownian motion in optical trapping. Nevertheless, even after taking the Brownian motion into account, the Q-factors remained high. We further unveil the physical mechanism that can enhance or diminish non-Hermitian forces, such as increasing particle radius and refractive index and utilizing propagating or standing waves

Influence of astigmatic aberration on partially coherent Gaussian-Schell vortex beam focused by lensacon

Based on the mathematical framework of the partially coherent Gaussian Schell model vortex (PCGSMV) beam and the Huygens-Fresnel integral, we conducted a study to analyze the intensity distribution and depth of focus (DOF) of the PCGSMV beam as it propagates through a classical axicon. Our numerical results indicate the influence of factors such as the beam width, spatial degree of coherence, topological charge, and axicon base angle on the intensity distribution and DOF. In addition, we investigated the relationship between the beam spot size and propagation distance, as well as the effects of the spatial degree of coherence and propagation distance on the intensity profile. Our findings highlight the importance of the intensity values along the DOF for various applications, including the optical trapping and manipulation of micro particles.

Controlling the initial separation distance between two electron plasma vortices in a Malmberg–Penning trap

This paper presents a novel method to continuously control the initial separation distance d between two plasma vortices of electrons. In this method, the two electron columns are initially confined individually in two coaxial Malmberg–Penning traps with different axial lengths. They rotate around the trap axis at different rotation frequencies due to the \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\varvec{E}\ imes \\varvec{B}$$\\end{document} drift. Their different rotation rates cause periodic changes in their relative azimuthal positions. The initial conditions are established when the two columns are stretched along magnetic field lines of a unified Malmberg–Penning trap. This method precisely provides a simple and continuous adjustment of the initial d and facilitates efficient investigation of the interaction of the two plasma electron vortices.

Interaction of driven ``cold'' electron plasma wave with thermal bulk via ion spatial inhomogeneity

Abstract Using high resolution Vlasov - Poisson simulations, evolution of driven ``cold" electron plasma wave (EPW) in the presence of stationary inhomogeneous background of ions is studied. Mode coupling dynamics between ``cold'' EPW with phase velocity $v_{\phi}$ greater than thermal velocity i.e $v_{\phi} \gg v_{thermal}$ and its inhomogeneity induced sidebands is illustrated as an initial value problem. In driven cases, formation of BGK like phase space structures corresponding to sideband modes due to energy exchange from primary mode to bulk particles via wave-wave and wave-particle interactions leading to particle trapping is demonstrated for inhomogeneous plasma. Qualitative comparison studies between initial value perturbation and driven problem is presented, which examines the relative difference in energy transfer time between the interacting modes. Effect of variation in background ion inhomogeneity amplitude as well as ion inhomogeneity scale length on the driven EPWs is reported.

Impact of ageostrophic dynamics on the predictability of Lagrangian trajectories in surface-ocean turbulence

Turbulent flows at the surface of the ocean deviate from geostrophic equilibrium on scales smaller than about 10 km. These scales are associated with important vertical transport of active and passive tracers, and should play a prominent role in the heat transport at climate scales and for plankton dynamics. Measuring velocity fields on such small scales is notoriously difficult but new, high-resolution satellite altimetry is starting to reveal them. However, the satellite-derived velocities essentially represent the geostrophic flow component, and the impact of unresolved ageostrophic motions on particle dispersion needs to be understood to properly characterize transport properties. Here, we investigate ocean fine-scale turbulence using a model that represents some of the processes due to ageostrophic dynamics. We take a Lagrangian approach and focus on the predictability of the particle dynamics, comparing trajectories advected by either the full flow or by its geostrophic component only. Our results indicate that, over long times, relative dispersion is marginally affected after filtering out the ageostrophic component. Nevertheless, advection by the geostrophic-only flow leads to an overestimation of the typical pair-separation rate, and to a bias on trajectories (in terms of displacement from the actual ones), whose importance grows with the Rossby number. We further explore the intensity of the transient particle clustering induced by ageostrophic motions and find that it can be significant, even for small flow compressibility. Indeed, we show that clustering is here due to the interplay between compressibility and persistent flow structures that trap particles, enhancing their aggregation. Published by the American Physical Society 2024

On-The-Flight trapping, LIBS analysis and discrimination of single meteorite particles generated by laser ablation

BackgroundThousands of micrometeorites fall to the Earth on a daily basis. Most of these meteorites have a rocky composition, but others are mainly composed of iron and nickel. Due to their small size, often ca. 100 μm in diameter, the process of searching for, collecting, and identifying these samples is remarkably tedious. In this work, we introduce a minimally invasive methodology for evaluating the full elemental composition of micrometeorites using optical emission spectroscopy of single particles produced by laser ablation of bulk targets. ResultsBulk meteorite samples were directly ablated within an ablation cell. From few micrograms of ablated matrix, we originated dry aerosols consisting of multielemental particles which were representative of the sample chemistry. SEM images confirmed that the generated particles exhibited spherical geometry. Particles were first optically trapped in air and, then, analyzed by laser-induced breakdown spectroscopy (LIBS). LIBS spectra evidenced compositional differences among samples. For example, Campo de Cielo meteorite featured a high iron content due to its metallic nature whereas LIBS results for Jbilet Winselwan and NWA 869 suggested that pyroxene components dominated the composition of the samples. In contrast, NWA 13739 and Vaca Muerta contained high aluminum intensity, thus indicating that the feldspathic component was dominant, as then verified by XRD. The intra-sample compositional variability were quite satisfactory, as revealed by the RSD data, below 45 %. For quantitative analysis, the percentages of FeO, SiO2, Al2O3, Na2O, MgO, TiO2, CaO, K2O, MnO, SrO, Cr2O3, and Li2O were calculated using CF-LIBS. SignificanceThis work demonstrates the applicability of laser excitation of individual particles in an optical trap for the multielemental analysis of meteorites. The methodology provides a complete overview of the samples, is capable of classificating them according to their main phases and yield preliminary quantitative information about those phases. Therefore, we present a minimally destructive pathway to be used as the first step in the inspection of these delicate samples. If the particles represent nanostructures inherent to the meteorites, it would constitute a major step in the analysis of extraterrestrial material that may provide fundamental insights into the structure and composition of the original materials at the microscale, a topic that remains an active area of research worldwide.

Acoustic metagrating focusing and Bessel vortexes

Acoustic focusing and Bessel vortexes have great potential in medical ultrasound, particle trapping, and information processing. Based on the generalized Snell's law (GSL), metasurface focusing and Bessel vortexes were achieved by using in-plane phase profiles to shape wavefronts. Recent developments in acoustic metagratings (AMs) have demonstrated an extension of the GSL capable of switching transmitted and reflected vortexes that are determined by the parity of the number of wave propagation trips. However, these metagratings were designed with a certain one-dimensional phase gradient along the azimuthal direction, and the propagation of vortexes were generally fixed into cylindrical waveguides owing to energy divergence. The propagation and manipulation of acoustic vortexes in three-dimensional (3D) free space, caused by AMs with two-dimensional (2D) aperiodic phase gradients, still pose a great challenge. Here, we experimentally demonstrate two types of switchable acoustic lenses with focusing and Bessel vortexes. Based on the GSL extension, by separating and attaching 2D dual-layer aperiodic AMs in both lenses, the switch between the reflected focusing vortex and transmitted focusing/Bessel vortex with the same focus length and topological charge in 3D free space can be observed. The designed dual-layer AMs can realize the short-range and long-range focusing vortexes in 3D free space and also have the advantage of convenient function switching, which may pave the way for designing switchable focusing vortex lenses with practical applications.

Plasma edge and scrape-off layer turbulence in gyrokinetic simulations of negative triangularity plasmas

Abstract Gyrokinetic simulations in the long-wavelength or drift-kinetic limit are carried out of DIII-D inner-wall-limited (IWL) plasmas to investigate the effect of triangularity on edge and scrape-off layer (SOL) turbulence. The effect of neutral interactions and triangularity on plasma blobs is explored due to the impact blobs can have in setting the SOL width or introducing impurities through interactions with plasma-facing components. Seeded blob simulations with neutrals in shaped SOL scenarios demonstrate that increasing elongation, triangularity, or Shafranov shift decreases radial blob velocities, but neutral interactions have a minor effect. Fully turbulent simulations of DIII-D IWL plasmas include both open- and closed-field-line regions. The negative triangularity (NT) simulation has lower average core Te , lower normalized Te fluctuations, and lower fluxes, but a greater number of coherent structures (blobs) identified with increased size and velocity, on average. Density and electron temperature profiles are within a factor of 2 of experimental values. The increased trapped electron particle fraction in NT simulations is consistent with previous studies.

The optimisation of the STEP electron cyclotron current drive concept

Abstract A fusion reactor based on the spherical tokamak is very likely to be completely non-inductive for the majority of the plasma ramp-up and steady-state phases, due to the limitations imposed on the central coil assemblies by the compact design. Efficiency gains from solenoid-driven current cannot be relied upon. It is also critical that an electricity-producing plant maximises the wall-plug efficiency of its heating and current drive (HCD) system, this being one of the largest consumers of recirculating power. It is therefore essential that the HCD system is well-optimised for current drive efficiency in order to meet the goal of net electricity production. The UK’s Spherical Tokamak for Energy Production (STEP) reactor design program has recently taken the decision to use exclusively microwave-based heating and current drive actuators for its reactor concepts. We present the optimisation of an electron cyclotron current drive scheme for a spherical tokamak reactor, based around the STEP concept, arriving at a solution which overcomes the limitations imposed by the spherical tokamak geometry in terms of microwave access and high trapped particle fraction. The solution uses high-field side absorption and a mix of fundamental and 2nd harmonic O mode, with overall power requirements reducing with increasing number of frequencies used. An additional fundamental frequency is also added to further boost the efficiency during non-inductive plasma ramp.

Spectral line broadening of the Raman scattered waves in laser plasmas

Parametric instabilities are of a great concern especially in the context of laser fusion. Electromagnetic waves scattered by these instabilities can reach high amplitudes, thereby diverting a significant portion of the energy from the incident laser beam, which is essential for compressing and heating the fuel capsule. In addition, the emerging electrostatic wave can trap and accelerate electrons, which, upon impact, can preheat the target and thus prevent its effective compression. Here, we focus on the stimulated Raman scattering and the associated processes. Spectral broadening of the backward Raman scattering daughter wave is theoretically described process, which is caused by so-called trapped particle instability. The existence of trapped and freely moving electrons in plasma influenced by high amplitude electron plasma wave leads also to the anomalous dispersion of this wave. It is reflected in the shifts in the electrostatic spectrum which, on the other hand, must be visible also in the electromagnetic spectrum via the feed-back loop of the instability. In the present paper, we discuss scattered wave modes spectral broadening using results of numerical simulations.

Tunable Acoustic Tweezer System for Precise Three-Dimensional Particle Manipulation

This study introduces a tunable acoustic tweezer system designed for precise three-dimensional particle trapping and manipulation. The system utilizes a dual-liquid-layer acoustic lens, which enables the dynamic control of the focal length through the adjustable curvature of a latex membrane. This tunability is essential for generating the acoustic forces necessary for effective manipulation of particles, particularly along the direction of acoustic wave propagation (z-axis). Experiments conducted with spherical particles as small as 1.5 mm in diameter demonstrated the system’s capability for stable trapping and manipulation. Performance was rigorously evaluated through both z-axis and 3D manipulation tests. In the z-axis experiments, the system achieved a manipulation range of 33.4–53.4 mm, with a root-mean-square error and standard deviation of 0.044 ± 0.045 mm, which highlights its precision. Further, the 3D manipulation experiments showed that particles could be accurately guided along complex paths, including multilayer rectangular and helical trajectories, with minimal deviation. A visual feedback-based particle navigation system significantly enhanced positional accuracy, reducing errors relative to open-loop control. These results confirm that the tunable acoustic tweezer system is a robust tool for applications requiring precise control of particles with diameter of 1.5 mm in three-dimensional environments. Considering its ability to dynamically adjust the focal point and maintain stable trapping, this system is well suited for tasks demanding high precision, such as targeted particle delivery and other applications involving advanced material manipulation.

Photovoltaic Charge Lithography on Passive Dielectric Substrates Using Fe:LiNbO3 Stamps

AbstractPhotovoltaic Fe:LiNbO3 is an outstanding material platform able to photo‐generate versatile charge patterns, useful for a broad variety of applications. However, in some cases, its photorefractive effect, light absorption, and active ferroelectric properties may interfere with the optimum operation of certain devices based on Fe:LiNbO3. Here, a novel optoelectronic method is proposed and demonstrated to transfer photovoltaic charge patterns from Fe:LiNbO3 to non‐photovoltaic passive substrates, thus removing these possible limitations. The method, denominated as photovoltaic charge lithography (PVCL), resembles the operation of a stamp and does not require external high‐voltage supplies or electron/ion beams. Upon contact between the active Fe:LiNbO3 stamp and a passive dielectric substrate, the light‐induced charge pattern can be faithfully mirrored on the passive substrate. The imprinted pattern is probed and characterized by dielectrophoretic and electrophoretic particle trapping. The results reveal that the charge builds up on the passive substrate during contact, allowing charge tunability. Moreover, arbitrary charge distributions can be flexibly tailored, using scanning laser beams or spatially structured light. Overall, PVCL opens the possibility of printing complex 1D/2D charge patterns of controlled polarity on different passive dielectric materials, enhancing the technological potential of Fe:LiNbO3 photovoltaic platforms.

Single particle tracking reveals through-membrane diffusion of bacteriophage during process disruption of virus filtration

In the biopharmaceutical industry, virus filters are crucial for ensuring the removal of endogenous and adventitious viruses as part of the viral clearance strategy. Although traditionally described as a size-exclusion mechanism, virus retention has a process-dependent nature where challenging conditions, such as process disruptions, may compromise membrane retention and significantly increase virus filtrate concentrations. The detailed mechanisms underlying this loss of retention are challenging to determine using traditional breakthrough experiments. In this work, single particle tracking and kinetic simulations were employed to connect individual particle behavior to the observed macroscopic losses in virus retention. Our experiments, using fluorescently labeled ΦX174 bacteriophage as a model parvovirus, replicated conditions representative of process disruptions within the Pegasus SV4, a homogeneous polymeric virus filtration membrane. During flow, phage particles retained were trapped within relatively large cavity spaces that had downstream constrictions aligned with the flow direction; the trapped particles were dynamic and exhibited significant intra-cavity motion. Upon flow stoppage, particles escaped from these retention locations rapidly, with approximately 90 % of previously trapped particles being remobilized for process disruption times ranging from 2 to 10 min, suggesting that local cavity escape had reached saturation at these timescales. Diffusion experiments within the membrane revealed isotropic and Fickian motion, hindered by more than an order of magnitude compared to diffusion in unconfined liquid. Despite the reduced mobility within the membrane, the substantial diffusion coefficient of 4.19 ± 0.06 μm2/s indicated that virus particles could travel tortuous but non-retentive pathways through the membrane on length scales equal to or greater than the membrane thickness during a disruption event. A 1D kinetic Monte-Carlo simulation successfully connected single-particle behavior to macroscopically observed virus release, indicating that significant diffusive release into the filtrate can occur even without the resumption of flow. This work provides crucial insights into the retention behavior of homogeneous membranes during periods of disruption, enabling the design of more robust mitigation strategies and filter designs.

Spiral microchannels with concave cross-section for enhanced cancer cell inertial separation.

Inertial microfluidic technologies have proven effective for particle focusing and separation in many microchannels, typically the channels with the rectangular and trapezoidal shapes. To advance particle focusing in complex channels, we propose a spiral channel combining rectangular and concave cross-sections for high-resolution particle and cell focusing and separation. Numerical simulations were conducted to illustrate the effects of channel geometry on secondary flow distribution and particle focusing positions. The simulation shows the concave cross-section generates two asymmetrical Dean vortices skewing towards the inner and outer channel walls, resulting to stronger flow velocity magnitudes near the walls than the channel center. Consequently, larger particles focus near the inner wall, while smaller particles are trapped closer to the outer wall under the influence of the stronger velocity magnitude near the walls. A microfluidic chip with the proposed channelgeometry, along with a traditional rectangular channel, was fabricated by 3D printing and PDMS casting. Fluorescent microbeads were used to investigate inertial focusing and separation behaviors in the microfluidicchips. Experimental results show that the concave channel facilitates particle focusing or trapping much closer to the walls than the traditional rectangular channel, achieving better separation resolution. Finally, the proposed channel was applied to separate lung cancer A549 cells from human blood, achieving a cancer cell recovery rate of ~ 84.78% (enrichment ratio over 820-fold) and a blood cell rejection rate of ~ 99.88%. This innovative channel design in inertial microfluidics offers new insights for enhanced particle focusing and holds significant promise for cell manipulation with improved separation resolution.

Investigating sediment dynamics on a continental shelf mud patch under the influence of a macrotidal estuary: A numerical modeling analysis

Shelf mud patches represent major sinks for fine-grained particles on continental shelves, as well as for carbon and contaminants of continental origin. The West Gironde Mud Patch (WGMP) is an interesting example of such offshore marine systems as it is an active mud deposition area located offshore the Gironde estuarine mouth (France) at depths between 30 and 70 m. It is known to be the trap of fine particles coming from the estuary, but the contribution of this material to the total mass of the depocenter is poorly quantified. In addition, despite the economic and ecological issues at stake, the response of such subtidal sedimentary structure to the combination of tidal currents, waves, and river supply remain poorly understood. Thus, using a realistic 3-D hydrodynamic and mixed (mud/sand) sediment transport model, this study aims at investigating the sediment dynamics of the WGMP under different hydrometeorological conditions. The analysis of the residual fluxes at the estuarine mouth exhibited large discrepancies between the different sediment classes as well as for contrasted hydro-and meteorological conditions induced by different dominant transport mechanisms. During winter, the reinforced density gradients drive strong up-estuary baroclinic circulation at the bottom that dominates the sediment dynamics over the barotropic export of mud particles. The model also reproduced the signature of a subtidal mud accumulation area over the continental shelf around 30–40 m water depth, on the proximal side of the observed WGMP. On average over two years, 26% of the mud mass accumulating on the simulated subtidal mudflat comes from the estuary. The trapping efficiency of this mud patch is negatively correlated with the significant wave height. Moreover, due to the estuarine turbid plume being more concentrated and developed at the surface during high river discharge, the trapping efficiency of the mud body is enhanced compared to lower discharge. This study highlights the sensitivity of mud and sand fluxes to vertical and horizontal residual circulation, and points out the uncertainties associated with the simulation of short-term (i.e., years) fine particle deposits compared to long-term (i.e., centuries) sediment accumulation trends. In addition, these results show the primordial effects of both wave action and riverine sediment supply on the dynamics of such subtidal muddy structures, which raises concern about their fate facing climate change and human activities in the future.

Tunable Elliptical Cylinders for Rotational Mechanical Studies of Single DNA Molecules.

The angular optical trap (AOT) is a powerful technique for measuring the DNA topology and rotational mechanics of fundamental biological processes. Realizing the full potential of the AOT requires rapid torsional control of these processes. However, existing AOT quartz cylinders are limited in their ability to meet the high rotation rate requirement while minimizing laser-induced photodamage. In this work, we present a novel trapping particle design to meet this challenge by creating small metamaterial elliptical cylinders with tunable trapping force and torque properties. The optical torque of these cylinders arises from their shape anisotropy, with their optical properties tuned via multilayered SiO 2 and Si 3 N 4 deposition. We demonstrate that these cylinders can be rotated at about 3 times the rate of quartz cylinders without slippage while enhancing the torque measurement resolution during DNA torsional elasticity studies. This approach opens new opportunities for previously inaccessible rotational studies of DNA processing.

Coupled modes analysis of stimulated Brillouin scattering in the regimes of nonlinear ion acoustic waves

The nonlinear saturation of stimulated Brillouin scattering (SBS) in long scale length plasmas is studied in detail through coupled mode equations. Our model incorporates harmonic and subharmonic generation of ion acoustic waves (IAWs), as well as nonlinear Landau damping and the nonlinear frequency shift of IAWs induced by particle trapping. Numerical simulations are carried out across various IAW wavenumbers (k a λ De ) and electron-ion temperature ratios (Z i T e /T i ) within different SBS instability regimes. The results demonstrate that our model can distinguish the importance of each effect contributing to the nonlinear behavior in SBS under different plasma conditions. Furthermore, we examine the scaling of SBS reflectivity with laser intensity under conditions relevant to inertial confinement fusion.

Precise mass measurements of A = 133 isobars with the Canadian Penning Trap: Resolving the [formula omitted] anomaly at 133Te

We report precision mass measurements of 133Sb, 133g,mTe, and 133g,mI, produced at CARIBU at Argonne National Laboratory's ATLAS facility and measured using the Canadian Penning Trap mass spectrometer. These masses clarify an anomaly in the 133Te β-decay. The masses reported in the 2020 Atomic Mass Evaluation (M. Wang et al., 2021) produce Qβ−(133Te)=2920(6) keV; however, the highest-lying 133I level populated in this decay is observed at Ei=2935.83(15) keV, resulting in an anomalous Qβ−i=−16(6) keV. Our new measurements give Qβ−(Te133)=2934.8(11) keV, a factor of five more precise, yielding Qβi=−1.0(12) keV, a 3σ shift from the previous results. This resolves this anomaly, but indicates further anomalies in our understanding of the structure of this isotope.

Intrinsic angular momentum, spin and helicity of higher-order Poincaré modes

Abstract The availability of coherent sources of higher order Poincaré optical beams have opened up new opportunities for applications such as in the optical trapping of atoms and small particles, the manipulation of chirally-sensitive systems and in improved encoding schemes for broad-bandwidth communications. Here we determine the intrinsic properties of integer order m ⩾ 0 Poincaré Laguerre–Gaussian (LG) modes which have so far neither been evaluated, nor their significance highlighted. The theoretical framework we adopt here is both novel and essential because it emphasises the crucial role played by the normally ignored axial components of the twisted light fields of these modes. We show that the inclusion of the axial field components enables the intrinsic properties of the Poincaré modes, notably their angular momentum, both spin and orbital as well as their helicity and chirality, to be determined. We predict significant enhancements of the intrinsic properties of these modes when compared with those due to the zero order LG modes. In particular, we show that higher order LG Poincaré modes exhibit super-chirality and, significantly so, even in the case of the first order m = 1.

Mineralogical characterization of magnesium-based nanoparticles recovered from a swirl-stabilized magnesium flame by analytical and scanning/transmission electron microscopy

Abstract. The current climate emergency and the related energy transition require the development of technology producing zero-carbon energy. One viable option entails the utilization of recyclable metal fuels. The primary energy stored by the reduction in metal oxides can be transported and later released by metal combustion. Mg is among the most promising metal as a regenerable energetic vector, having an energy density of 25 MJ kg−1. The exploitation of the Mg oxidation and reduction loop has recently been demonstrated, and the loop combustion products are made of metal oxides. The mineralogical characterization of the MgO crystals generated by the Mg combustion is of utter importance for the optimization of the particle trapping capacity in the combustion system during the closed oxidation and reduction loop. In this paper we characterize MgO particles generated in a swirl-stabilized Mg flame by using powder X-ray diffraction, transmission electron microscopy and selected area electron diffraction, and atomic-resolution microscopy combined with energy-dispersive X-ray spectroscopy and dual-electron energy-loss spectroscopy. The MgO combustion products were chemically homogeneous at this level of investigation. Three representative morphologies (cubic, truncated octahedron, and spherical) and two isostructural phases were identified in the MgO combustion product. These findings may contribute to the optimization of system development, particularly in terms of the collection efficiency of the combustion end product.