Particle Number Concentration Levels Research Articles

Contrasting intra-urban variability of ultrafine particle number and fine particle mass concentrations in Dhaka, Bangladesh, and Pittsburgh, USA

In this study, we investigated the intra-urban variability of fine particle mass (PM2.5) and ultrafine particle number concentration (PNC) in Dhaka (Bangladesh), and Pittsburgh (USA), two cities with vastly different pollution sources and levels. We collected measurements of PNC and PM2.5 at a wide range of sites spanning a variety of urban land use attributes (35 sites in Dhaka and 30 sites in Pittsburgh). We found that PNC levels exhibited a 3-4-fold variability between sites in each city, ranging from 20,000–100,000 # cm−3 in Dhaka and 7,000–28,000 # cm−3 in Pittsburgh. PM2.5 levels varied within 50% of the urban background level, ranging from 80 to 110 μg m−3 in Dhaka and 6–12 μg m−3 in Pittsburgh. We observed a moderate level of spatial correlation between PNC and PM2.5 measurements in both cities (R2 0.3 in Dhaka, and 0.4 in Pittsburgh), and consistent within-city spatial patterns in different meteorological seasons. Compared to the Pittsburgh levels, both PNC and PM2.5 levels in Dhaka were significantly higher, however, PM2.5 was disproportionately higher (10–12 times higher) than PNC (3–4 times higher). The slope of PNC versus PM2.5 varied significantly between the two cities, suggesting that the sources and size distribution of particles that make up the majority of the PM2.5 were different in the two cities. The results found in Dhaka indicate that aerosol particles are influenced by solid fuel combustion, including solid biomass burning, waste burning, and road dust, which have a greater impact on particle mass concentration due to their larger size. Contrary, in Pittsburgh, traffic (gasoline and diesel combustion) particles, relatively smaller in size compared to solid fuel combustion particles, play a dominant role in determining the within-city variability of PNC and PM2.5. Our findings suggest that while controlling traffic emissions can contribute to reducing PNC, substantial efforts will be required to mitigate accumulation mode particles from various region-specific sources in order to decrease PM2.5 mass concentrations in Dhaka.

In-vehicle ultrafine and fine particulate matter exposures during commuting in a South Asian megacity: Dhaka, Bangladesh

We measured ultrafine particle number concentration (PNC) and fine particulate matter mass concentration (PM2.5) levels in public buses and private cars under three conditions: windows open, windows closed with air recirculation off, and windows closed with air recirculation on in Dhaka, Bangladesh—an extremely polluted megacity in South Asia. We collected measurements on ∼10 repeated round trips on unique days for each selected transportation mode, covering various routes that spanned multiple arterial roads over several months (January to March 2020 and November to December 2020) and different times of the day to account for the variability in traffic and meteorological conditions. We used a condensation particle counter (CPC) to measure PNC and a PurpleAir sensor to measure PM2.5 mass concentrations. We applied corrections to the raw data and analyzed quality-assured data to investigate exposure differences across modes, pollutants, locations, and times. Public buses and private cars with open windows had mean PNC levels of 112,000 # cm−3 and 117,000 # cm−3, approximately 5–6 times higher than the mean urban background level of around 20,000 # cm−3. PM2.5 levels in these vehicles were approximately ∼100 μg m−3, about 20% higher than the urban background PM2.5 level of 85 μg m−3. With closed windows and air recirculation off, concentrations were 15% lower for PNC and 10% lower for PM2.5. Under closing windows and keeping air recirculation on, mean PNC and PM2.5 levels were 60,000 # cm−3 and 70 μg m−3, respectively, representing a 50% reduction for PNC and a 30% reduction for PM2.5 compared to open windows. Our findings suggest that commuters in public buses and private cars with open windows have higher and similar exposure levels, whereas those commute in private cars with closed windows and air recirculation on have lower exposure levels.

Occupational Exposure during the Production and the Spray Deposition of Graphene Nanoplatelets-Based Polymeric Coatings.

Graphene-based polymer composites are innovative materials which have recently found wide application in many industrial sectors thanks to the combination of their enhanced properties. The production of such materials at the nanoscale and their handling in combination with other materials introduce growing concerns regarding workers' exposure to nano-sized materials. The present study aims to evaluate the nanomaterials emissions during the work phases required to produce an innovative graphene-based polymer coating made of a water-based polyurethane paint filled with graphene nanoplatelets (GNPs) and deposited via the spray casting technique. For this purpose, a multi-metric exposure measurement strategy was adopted in accordance with the harmonized tiered approach published by the Organization for Economic Co-operation and Development (OECD). As a result, potential GNPs release has been indicated near the operator in a restricted area not involving other workers. The ventilated hood inside the production laboratory guarantees a rapid reduction of particle number concentration levels, limiting the exposure time. Such findings allowed us to identify the work phases of the production process with a high risk of exposure by inhalation to GNPs and to define proper risk mitigation strategies.

Revisiting Total Particle Number Measurements for Vehicle Exhaust Regulations

Road transport significantly contributes to air pollution in cities. Emission regulations have led to significantly reduced emissions in modern vehicles. Particle emissions are controlled by a particulate matter (PM) mass and a solid particle number (SPN) limit. There are concerns that the SPN limit does not effectively control all relevant particulate species and there are instances of semi-volatile particle emissions that are order of magnitudes higher than the SPN emission levels. This overview discusses whether a new metric (total particles, i.e., solids and volatiles) should be introduced for the effective regulation of vehicle emissions. Initially, it summarizes recent findings on the contribution of road transport to particle number concentration levels in cities. Then, both solid and total particle emission levels from modern vehicles are presented and the adverse health effects of solid and volatile particles are briefly discussed. Finally, the open issues regarding an appropriate methodology (sampling and instrumentation) in order to achieve representative and reproducible results are summarized. The main finding of this overview is that, even though total particle sampling and quantification is feasible, details for its realization in a regulatory context are lacking. It is important to define the methodology details (sampling and dilution, measurement instrumentation, relevant sizes, etc.) and conduct inter-laboratory exercises to determine the reproducibility of a proposed method. It is also necessary to monitor the vehicle emissions according to the new method to understand current and possible future levels. With better understanding of the instances of formation of nucleation mode particles it will be possible to identify its culprits (e.g., fuel, lubricant, combustion, or aftertreatment operation). Then the appropriate solutions can be enforced and the right decisions can be taken on the need for new regulatory initiatives, for example the addition of total particles in the tailpipe, decrease of specific organic precursors, better control of inorganic precursors (e.g., NH3, SOx), or revision of fuel and lubricant specifications.

Ultrafine particle exposure for bicycle commutes in rush and non-rush hour traffic: A repeated measures study in Copenhagen, Denmark

Ultrafine particles (UFP), harmful to human health, are emitted at high levels from motorized traffic. Bicycle commuting is increasingly encouraged to reduce traffic emissions and increase physical activity, but higher breathing rates increase inhaled UFP concentrations while in traffic. We assessed exposure to UFP while cycling along a fixed 8.5 km inner-city route in Copenhagen, on weekdays over six weeks (from September to October 2020), during morning and afternoon rush-hour, as well as morning non-rush-hour, traffic time periods starting from 07:45, 15:45, and 09:45 h, respectively. Continuous measurements were made (each second) of particle number concentration (PNC) and location. PNC levels were summarized and compared across time periods. We used generalized additive models to adjust for meteorological factors, weekdays and trends. A total of 61 laps were completed, during 28 days (∼20 per time period). Overall mean PNC was 18,149 pt/cm3 (range 256–999,560 pt/cm3) with no significant difference between morning rush-hour (18003 pt/cm3), afternoon rush-hour (17560 pt/cm3) and late morning commute (17560 pt/cm3) [p = 0.85]. There was substantial spatial variation of UFP exposure along the route with highest PNC levels measured at traffic intersections (∼38,000-42000 pt/cm3), multiple lane roads (∼38,000-40000 pt/cm3) and construction sites (∼44,000-51000 pt/cm3), while lowest levels were measured at smaller streets, areas with open built environment (∼12,000 pt/cm3), as well as at a bus-only zone (∼15,000 pt/cm3). UFP exposure in inner-city Copenhagen did not differ substantially when bicycling in either rush-hour or non-rush-hour, or morning or afternoon, traffic time periods. UFP exposure varied substantially spatially, with highest concentrations around intersections, multiple lane roads, and construction sites. This suggests that exposure to UFP is not necessarily reduced by avoiding rush-hours, but by avoiding sources of pollution along the bicycling route.

Occupational exposure to graphene and silica nanoparticles. Part I: workplace measurements and samplings

Few-Layers Graphene (FLG) are able to improve the performance of materials, due to their chemical-physical properties. Engineered amorphous silica nanoparticles (SiO2NPs) are among the most widespread nanomaterials (NMs) in the world. Such nanomaterials are two case studies of the research project ‘NanoKey’ that integrated the exposure assessment through personal measurements and sampling in the workplace, as described in the present work (part I), with the biomonitoring of exposed workers (reported in part II). Measurement campaigns were conducted according to OECD and WHO harmonized approach in two production sites. The set of instruments included real-time devices for high-resolution measurements at the nanoscale and time-integrated samplers for the off-line gravimetric analysis and chemical and morphological (SEM-EDS) characterization of exposure in order to identify the contribution of production compared to the background. Values of particle number concentration (PNC) and lung deposited surface area (LDSA) within the FLG production resulted higher than the background far field (FF), even if they are always similar to the near field (NF) ones: the average diameter (Davg) during the production was higher than the NF background but always lower than the FF values. SEM-EDS analysis highlighted the presence of structures comparable to those produced. During the SiO2NPs production, the PBZ values showed PNC and LDSA levels higher than the background, with a decrease in the Davg probably due to NPs emission. SEM-EDS confirms the presence of rare silica nanoparticles. Since the exposure to airborne NMs cannot be excluded in both production sites, a prevention-through-design approach to mitigate the potential risk for workers has been recommended.

Studies of Atmospheric PM2.5 and its Inorganic Water Soluble Ions and Trace Elements around Southeast Asia: a Review

Air pollution is a worldwide issue that is mainly caused from excessive inhalation of hazardous PM2.5 pollutant that is emitted into the air. The objective of this study is to assess the fundamental knowledge revolving PM2.5 (particles aerodynamic diameter of lower than or equal to 2.5 μm) and its inorganic composition in ambient air of urban areas, mainly in Malaysia in comparison to other Southeast Asia countries. This research also investigates the theory of particle number concentration (PNC) with PM2.5, also the health effects and origins of the emissions. The factors affecting the PM2.5 mass include the local emission, El Nino phenomenon, land, meteorological effects, monsoons, rainfall events, sea breeze, transboundary pollution and seasonal changes. 24 h mean PM2.5 mass concentration for metropolitan regions in the SEA is in the range of 11 μgm−3 and 72.3 μgm−3, while between 5.30 μgm−3 and 55.89 μgm−3 for semi-urban zones. For rural area, the 24 h mean PM2.5 value is about 30 μgm−3. The findings indicate that metals in PM2.5 emission are frequently Pb, Se, Zn, Cd, As, Bi, Ba, Cu, Rb, V, Ni, Fe, Ca, Mn, Cr, Al, Si and K, where Zn has the uppermost range of 133.50 to 419.30 ngm−3 while the major water-soluble ions exist are NH4+, K+, Ca2+, Na+, in which Na+, NH4+ and Cl- are present in aged sea salt and mixed industrial, Ca2+ and Mg2+ present in mineral dust, NH4+, K+ and SO42− present in mixture of SIA and biomass burning. There is a high correlation between the particle mass concentration and PNC level, especially the ones in accumulation mode (PNC0.1–1.0) which are mostly originated from the emission of heavy traffic streets.

Ultrafine particles and PM2.5 in the air of cities around the world: Are they representative of each other?

Can mitigating only particle mass, as the existing air quality measures do, ultimately lead to reduction in ultrafine particles (UFP)? The aim of this study was to provide a broader urban perspective on the relationship between UFP, measured in terms of particle number concentration (PNC) and PM2.5 (mass concentration of particles with aerodynamic diameter < 2.5 μm) and factors that influence their concentrations. Hourly average PNC and PM2.5 were acquired from 10 cities located in North America, Europe, Asia, and Australia over a 12-month period. A pairwise comparison of the mean difference and the Kolmogorov-Smirnov test with the application of bootstrapping were performed for each city. Diurnal and seasonal trends were obtained using a generalized additive model (GAM). The particle number to mass concentration ratios and the Pearson's correlation coefficient were calculated to elucidate the nature of the relationship between these two metrics.Results show that the annual mean concentrations ranged from 8.0 × 103 to 19.5 × 103 particles·cm−3 and from 7.0 to 65.8 μg·m−3 for PNC and PM2.5, respectively, with the data distributions generally skewed to the right, and with a wider spread for PNC. PNC showed a more distinct diurnal trend compared with PM2.5, attributed to the high contributions of UFP from vehicular emissions to PNC. The variation in both PNC and PM2.5 due to seasonality is linked to the cities' geographical location and features. Clustering the cities based on annual median concentrations of both PNC and PM2.5 demonstrated that a high PNC level does not lead to a high PM2.5, and vice versa. The particle number-to-mass ratio (in units of 109 particles·μg−1) ranged from 0.14 to 2.2, >1 for roadside sites and <1 for urban background sites with lower values for more polluted cities. The Pearson's r ranged from 0.09 to 0.64 for the log-transformed data, indicating generally poor linear correlation between PNC and PM2.5. Therefore, PNC and PM2.5 measurements are not representative of each other; and regulating PM2.5 does little to reduce PNC. This highlights the need to establish regulatory approaches and control measures to address the impacts of elevated UFP concentrations, especially in urban areas, considering their potential health risks.

Application of a sensor network of low cost optical particle counters for assessing the impact of quarry emissions on its vicinity

The adverse health effects of inhaled particulate matter (PM) are global concern. Yet, in general, estimating the exposure to PM is challenging due to the sparsity of standard air quality monitoring stations and the low accuracy of dispersion models when high spatial resolution is required. The city of Elad, Israel, is situated less than 1 km from the Migdal Tzedek stone quarry, and public concerns were raised regarding the impact of the quarry's PM emissions on the city air quality.This work describes a year-long campaign of continuous measurements of particle number concentration (PNC) in few locations in the city and its vicinity, using a network of low cost optical particle counters (OPCs). To assess the possible impact of the quarry on the city we examined the OPCs' accuracy, coherency, and their capability to detect the quarry's impact on the PNC levels in the city. Using PNC time series in two size channels from a network of five nodes, PM10 and PM2.5 records from a nearby reference air quality monitoring station, and meteorological data, we could conclude that the quarry's impact on the city was small relative to the background PNC levels. Yet, more importantly, this work demonstrates the use of a network of low cost OPCs for responding to an environmental query for which the sparse standard air quality monitoring observations were not sufficient. The trade-offs between deployment of a network of cheap low-quality instruments and the use of a single high-end device are discussed.

Characterization of aerosol particles over the southern and South-Eastern Baltic Sea

Abstract Studies of aerosol particle number concentration (PNC) level over open sea in the southern and south-eastern Baltic Sea regions were performed during five cruises (2005–2006, 2008–2010) by RV Oceania and at the coastal Preila station (Lithuania). A comparative analysis was performed of aerosol PNC variation at open sea versus measurements taken at the coastal site under various conditions (breaking waves, fog events, NPF), considering transport of forest fire products and advection of different air mass types to the investigation sites. It was found that the average PNC over the open sea (3000–4000 cm− 3) was generally higher than at the coastal site (2000–3000 cm− 3). Breaking waves caused by the latitudinal or longitudinal long-lasting (3–4 days) constant-direction wind under stormy conditions had the strongest effect on the aerosol PNC over the Baltic Sea. The aerosol PNC in the marine boundary layer (MBL) of the south-eastern Baltic Sea during fog did not depend on the air mass type over open sea, in contrast to the coastal site, that is, the average PNC level (3000–4000 cm− 3) in the MBL, which could be constantly affected by specific environmental factors as a source of condensation nuclei for the fog formation. Short-term increases of aerosol PNC in the MBL (5000–10,000 cm− 3) were higher than in the same periods of the time scale at the coastal site (3000–6000 cm− 3) during NPF events, and therefore the open sea environment may facilitate a more favourable condition for the NPF, that is, exhaust and biogenic emissions from ships and the marine environment.

Observation of new particle formation on Curonian Spit located between continental Europe and Scandinavia

This study presents results of the research on atmospheric aerosol particles in the coastal environment, focusing on the investigation of new particle formation (NPF) events. Continuous measurements of the particle number size distribution (8.7–840nm) were performed at the Preila station throughout the year 2013. An estimation of the aerosol particle number concentration (PNC) of nucleation (8.7–20nm), Aitken (20–100nm) and accumulation modes (100–840nm) and their input to the total PNC were performed. The annual average value of the total PNC was 3.9·103cm−3. The seasonal variations of the total PNC essentially comprised the maximum monthly average in March (6.3·103cm−3) and the minimum in November (1.9·103cm−3). The highest input (44–64%) into the total PNC was influenced by Aitken mode particles. The particles of the accumulation mode made up 23% of the total PNC during spring, summer and autumn months, and comprised about 48% during winter months. The monthly average input of the nucleation mode particles to the total PNC varied from 11% to 20%. However, the diurnal average input of each nucleation mode particles to the total PNC had higher variations and showed the limits of the nucleation mode input to the total PNC depending on the inputs of Aitken and accumulation modes. It should be noted that the described limits of the nucleation mode input to the total PNC were constant for NPF event days and non-event day׳s datasets. During whole 2013 year were observed 111 NPF events, which were classified as Class I (18 days) and Class II (93 days). The average particle formation and growth rates were 0.45cm−3s−1 and 3.7nmh−1, respectively. The average condensation sink was 1.53·10−3s−1. The highest number of NPF days was observed when the air masses advected from northern directions (Scandinavia, the North Sea, and the Arctic) and contrary the NPF events were observed very rarely during advection of polluted continental air masses. Thus, the parameters estimated for the NPF events observed at the Preila station are partially similar to the Northern Europe stations. However, the PNC level, low seasonal PNC cycle and heterogeneous air masses showed similarity with Central Europe aerosol.

Personal exposure to ultrafine particles: Two-level statistical modeling of background exposure and time-activity patterns during three seasons.

Personal exposure to air pollution is associated with time- and location-specific factors including indoor and outdoor air pollution, meteorology and time activities. Our investigation aims at the description and identification of factors determining personal exposure to particle number concentration (PNC) in everyday situations. Ten volunteers recorded their personal exposure to PNC and kept an activity diary in three different seasons besides stationary measurements of ambient air pollution and meteorology. Background exposure to PNC was modelled using the most predictive variables. In a second step, the effects of the activities were calculated adjusted for the background exposure. The average personal PNC level was highest in winter and was three times higher than the mean stationary PNC level while staying indoors and two times higher while staying outdoors. Personal indoor PNC levels were significantly increased during the use of candles, cooking and the occurrence of smell of food. High stationary outdoor PNC levels and low dew point temperatures were associated with increased personal outdoor PNC levels. Times spent in public transport were associated with lower personal PNC levels than other times spent in transportation. Personal PNC levels in everyday situations exhibited a large variability because of seasonal, microenvironment-specific and activity-specific influences.

Influence of medium range transport of particles from nucleation burst on particle number concentration within the urban airshed

Abstract. An elevated particle number concentration (PNC) observed during nucleation events could play a significant contribution to the total particle load and therefore to the air pollution in the urban environments. Therefore, a field measurement study of PNC was commenced to investigate the temporal and spatial variations of PNC within the urban airshed of Brisbane, Australia. PNC was monitored at urban (QUT), roadside (WOO) and semi-urban (ROC) areas around the Brisbane region during 2009. During the morning traffic peak period, the highest relative fraction of PNC reached about 5% at QUT and WOO on weekdays. PNC peaks were observed around noon, which correlated with the highest solar radiation levels at all three stations, thus suggesting that high PNC levels were likely to be associated with new particle formation caused by photochemical reactions. Wind rose plots showed relatively higher PNC for the NE direction, which was associated with industrial pollution, accounting for 12%, 9% and 14% of overall PNC at QUT, WOO and ROC, respectively. Although there was no significant correlation between PNC at each station, the variation of PNC was well correlated among three stations during regional nucleation events. In addition, PNC at ROC was significantly influenced by upwind urban pollution during the nucleation burst events, with the average enrichment factor of 15.4. This study provides an insight into the influence of regional nucleation events on PNC in the Brisbane region and it the first study to quantify the effect of urban pollution on semi-urban PNC through the nucleation events.

SPATIO-TEMPORAL VARIATION OF PARTICLE NUMBER CONCENTRATIONS IN A SWISS URBAN CITY

Background and Aims: This study is part of the Swiss Cohort Study on Air Pollution and Lung and Heart Diseases in Adults (SAPALDIA), a nearly 20-year old cohort study spread in 8 geographically diverse areas in Switzerland. Innovative exposure modeling has been conducted in SAPALDIA earlier for PM10 and NO2, however, exposure to specific traffic related pollutants such as ultrafine particles and PM constituents has not been assessed. The overarching aim is to provide the estimates of individual long-term outdoor traffic-related air pollution exposures of the cohort participants. This paper focuses on the spatial and temporal variation of home outdoor particle number concentration (PN) in one of the SAPALDIA area, Basel. Methods: The PN measurements will be conducted at 20 residences each in four of the eight areas in three seasons over a period of 2 years, 2011-2012. Indoors and outdoors monitoring will be conducted biweekly for PM2.5, PM10, NO2 and weekly for PN. Particle counts are measured using a particle counting device, miniDiSC (miniature diffusion size classifier). It is a portable device and measures nanometer sized (10-300nm) particles with a resolution of one second. Results: Mean weekly averaged PN levels are observed 14529±3296, 13659±1878 and 11545 particles/cm3 at street, urban and regional background locations respectively. Median correlation coefficient for all sites is 0.70 (range 0.36-0.91) and 0.83 (range 0.39-0.99) for hourly and daily PN respectively. Median coefficient of divergence, a measure of spatial heterogeneity, for all site pairs is 0.15 (range 0.05-0.27), showing a low to mid spatial heterogeneity in daily PN in Basel. These winter season observations will be compared across seasons and further with concurrent PM2.5, PM10 and NO2 measurements. Conclusions: Our first results show significant differences in PN levels in home outdoor locations and document the differential impact of traffic on PN levels in the city.

커먼레일 디젤엔진의 운전조건이 나노크기 입자상 물질 배출특성에 미치는 영향에 관한 실험적 연구

본 논문은 커먼레일 디젤엔진의 정속운전시 배출되는 나노크기의 입자상 물질을 분석하는데 초점을 두었다. 디젤산화촉매 후단에서 나노입자상 물질의 개수농도 저감수준은 크지 않았으나 매연여과장치 후단에서 분석한 결과 1,000배 정도 저감되는 결과를 확인하였다. 고속ㆍ고부하 조건에서는 매연여과 장치의 자연재생 효과로 인해 입자상 물질은 증가하였다. 연료분사시기를 BTDC 6℃A 에서 ATDC 4℃A까지 지각시킨 결과 입자상 물질의 개수농도는 감소하였지만 최지각 조건인 ATDC 9℃A에서는 증가하는 결과를 확인하였다. EGR 적용시 핵화모드 입자상 물질은 저감되는 경향을 보였으며 축적모든 입자는 증가하였다.

Corona Ions from Overhead Transmission Voltage Powerlines: Effect on Direct Current Electric Field and Ambient Particle Concentration Levels

Along with their essential role in electricity transmission and distribution, some powerlines also generate large concentrations of corona ions. This study aimed at the comprehensive investigation of corona ions, vertical direct current electric field (dc e-field), ambient aerosol particle charge, and particle number concentration levels in the proximity of some high/subtransmission voltage powerlines. The influence of meteorology on the instantaneous value of these parameters and the possible existence of links or associations between the parameters measured were also statistically investigated. The presence of positive and negative polarities of corona ions was associated with variation in the mean vertical dc e-field, ambient ion, and particle charge concentration level. Though these variations increased with wind speed, their values also decreased with distance from the powerlines. Predominately positive polarities of ions were recorded up to a distance of 150 m (with the maximum values recorded 50 m downwind of the powerlines). At 200 m from the source, negative ions predominated. Particle number concentration levels, however, remained relatively constant (10(3) particle cm(-3)), irrespective of the sampling site and distance from the powerlines. Meteorological factors of temperature, humidity, and wind direction showed no influence on the electrical parameters measured. The study also discovered that e-field measurements were not necessarily a true representation of the ground-level ambient ion/particle charge concentrations.

Experimental investigation of nanoparticle formation characteristics from advanced gasoline and diesel fueled light duty vehicles under different certification driving modes

This paper mainly focused on the comparison of nanoparticle size distribution and number concentration level characteristics with gasoline and diesel fueled light duty vehicles. In the engine research, particle size distribution and number concentrations were analyzed by a DMS500 with engine parameters. Time-resolved particle number concentration levels from test vehicles were measured by a golden particle measurement system (GPMS) as recommended by a Particle Measurement Programme (PMP) on certification modes such as New European Driving Cycle (NEDC), Federal Test Procedure (FTP)-75, and Highway Fuel Economy Test (HWFET). In addition, particle emission characteristics from vehicles were analyzed by DMS500 during transient and high-speed driving conditions. From the results, we found that the formation of particles was highly dependent on vehicle speed and load conditions for each mode. The diesel vehicle equipped with a particulate filter showed substantial reduction of the total particle number whose number concentration was equivalent to that of the gasoline vehicle. The nucleation mode particles from gasoline fuel were mainly emitted; however, the accumulation mode particles from the diesel fuel were generally analyzed.

Inter-laboratory correlation exercise on a light-duty diesel passenger vehicle to verify nano-particle emission characteristics by Korea particle measurement program

The Light Duty Inter-Laboratory Correlation Exercise (ILCE) final report, performed with the ‘PMP Golden Vehicle’ at nine laboratories in the EU, Korea and Japan to demonstrate repeatability and reproducibility of the particle number concentration emissions measurement techniques proposed by the Particle Measurement Program (PMP), was released in 2007. The ILCE was conducted by the Korea Particle Measurement Program (KPMP) with a domestic diesel passenger vehicle equipped with a diesel particulate filter (DPF) between three certification laboratories and the research center of an automotive manufacturer to meet future regulations (EURO 5 and EURO 6) of particle number concentration for light-duty vehicles in early 2008. This research focused on measuring the particulate matter emission (particle number and mass) levels of a representative light-duty diesel passenger vehicle during new European driving cycle (NEDC) mode to analyze the repeatability and reproducibility between laboratories in Korea. From the ILCE test results in Korea, the mean total particle number concentration levels ranged from 5.43E+10 #/km to 1.58E+11 #/km and 0.0003 g/km to 0.0036 g/km for particle mass. Repeatability between participating laboratories ranged from 32% to 66% for particle number, 11% to 70% for particle mass; the reproducibility level was 46% for particle number, and 66% for particle mass emission.

Spatial and temporal variation of particle number concentration in Augsburg, Germany

Epidemiological studies on health effects of outdoor air pollution are largely based on a single monitoring site to estimate the exposure of people living in urban areas. For such an approach two aspects are important: the temporal correlation and the spatial variation of the absolute levels of concentrations measured at different sites in an urban area. Whereas many studies have shown small spatial variability of fine particles in urban areas, little is known on how well a single monitoring station could represent the temporal and spatial variation of ultrafine particles across urban areas. In our study we investigated the temporal and spatial variation of particle number concentration (PNC) at four background sites in Augsburg, Germany. Two of them were influenced by traffic, one was placed in the outskirts of the city. The average PNC levels at two urban background sites with traffic impact were 16,943 cm − 3 and 20,702 cm − 3 , respectively, compared to 11,656 cm − 3 at the urban background site without traffic impact (ratio 1.5 to 1.8). The Spearman correlation coefficients between the monitoring sites were high ( r > 0.80). The pronounced differences in absolute PNC levels suggest that the use of a single monitoring station in long-term epidemiological studies must be insufficient to attribute accurate exposure levels of PNC to all study subjects. On the other hand, the high temporal correlations of PNC across the city area of Augsburg implicate that in epidemiological time-series studies the use of one single ambient monitoring site is an adequate approach for characterizing exposure to ultrafine particles.

Particle Emission Characteristics of Office Printers

In modern society, printers are widely used in the office environment. This study investigated particle number and PM2.5 emissions from printers using the TSI SMPS, TSI CPC 3022, and 3025A TSI P-Trak and DustTrak. The monitoring of particle characteristics in a large open-plan office showed that particles generated by printers can significantly (p = 0.01) affect the submicrometer particle number concentration levels in the office. An investigation of the submicrometer particle emissions produced by each of the 62 printers used in the office building was also conducted and based on the particle concentrations in the immediate vicinity of the printers, after a short printing job, the printers were divided into four classes: non-emitters, and low, medium, and high emitters. It was found that approximately 60% of the investigated printers did not emit submicrometer particles and of the 40% that did emit particles, 27% were high particle emitters. Particle emission characteristics from three different laser printers were also studied in an experimental chamber, which showed that particle emission rates are printer-type specific and are affected by toner coverage and cartridge age. While a more comprehensive study is still required, to provide a better database of printer emission rates, as well as their chemical characteristics, the results from this study imply that submicrometer particle concentration levels in an office can be reduced by a proper choice of the printers.