Particle Collection Efficiency Research Articles

Controlling the Magnetic Responsiveness of Cellulose Nanofiber Particles Embedded with Iron Oxide Nanoparticles.

2,2,6,6-tetramethylpiperidine-1-oxyl (TEMPO)-oxidized cellulose nanofiber (TOCN) particles, an innovative biobased material derived from wood biomass, have garnered significant interest, particularly in the biomedical field, for their distinctive properties as biocompatible particle adsorbents. However, their microscopic size complicates their separation in liquid media, thereby impeding their application in various domains. In this study, superparamagnetic magnetite nanoparticles (NPs), specifically iron oxide Fe3O4 NPs with an average size of 15 nm, were used to enhance the collection efficiency of TOCN-Fe3O4 composite particles synthesized through spray drying. These composite particles exhibited a remarkable ζ-potential (approximately -50 mV), indicating their high stability in water, as well as impressive magnetization properties (up to 47 emu/g), and rapid magnetic responsiveness within 60 s in water (3 wt % Fe3O4 to TOCN, 1 T magnet). Furthermore, the influence of Fe3O4 NP concentrations on the measurement of the speed of magnetic separation was quantitatively discussed. Additionally, the binding affinity of the synthesized particles for proteins was assessed on a streptavidin-biotin binding system, offering crucial insights into their binding capabilities with specific proteins and underscoring their significant potential as functionalized biomedical materials.

Review on Sampling Methods and Health Impacts of Fine (PM2.5, ≤2.5 µm) and Ultrafine (UFP, PM0.1, ≤0.1 µm) Particles

Airborne particulate matter (PM) is of great concern in the modern-day atmosphere owing to its association with a variety of health impacts, such as respiratory and cardiovascular diseases. Of the various size fractions of PM, it is the finer fractions that are most harmful to health, in particular ultrafine particles (PM0.1; UFPs), with an aerodynamic diameter ≤ 100 nm. The smaller size fractions, of ≤2.5 µm (PM2.5; fine particles) and ≤0.1 µm (PM0.1; ultrafine particles), have been shown to have numerous linkages to negative health effects; however, their collection/sampling remains challenging. This review paper employed a comprehensive literature review methodology; 200 studies were evaluated based on the rigor of their methodologies, including the validity of experimental designs, data collection methods, and statistical analyses. Studies with robust methodologies were prioritised for inclusion. This review paper critically assesses the health risks associated with fine and ultrafine particles, highlighting vehicular emissions as the most significant source of particulate-related health effects. While coal combustion, diesel exhaust, household wood combustors’ emissions, and Earth’s crust dust also pose health risks, evidence suggests that exposure to particulates from vehicular emissions has the greatest impact on human health due to their widespread distribution and contribution to air pollution-related diseases. This article comprehensively examines current sampling technologies, specifically focusing on the collection and sampling of ultrafine particles (UFP) from ambient air to facilitate toxicological and physiochemical characterisation efforts. This article discusses diverse approaches to collect fine and ultrafine particulates, along with experimental endeavours to assess ultrafine particle concentrations across various microenvironments. Following meticulous evaluation of sampling techniques, high-volume air samplers such as the Chem Vol Model 2400 High Volume Cascade Impactor and low-volume samplers like the Personal Cascade Impactor Sampler (PCIS) emerge as effective methods. These techniques offer advantages in particle size fractionation, collection efficiency, and adaptability to different sampling environments, positioning them as valuable tools for precise characterisation of particulate matter in air quality research and environmental monitoring.

Numerical study on staggered needle-plate electrode configuration for improved particulate matter collection in electrostatic precipitator

The electrostatic precipitator (ESP) utilizes corona discharge to effectively separate particles from polluted air. The arrangement of electrode is a crucial role in achieving higher efficiency. Needle discharge electrodes can generate concentrated corona discharge at lower applied voltages. In this study, a staggered needle-plate electrode configuration was presented to expand the domain for particle charging, and thereby improve collection efficiency. A three-dimensional model was established to describe the multi-physics phenomenon in the ESP. The ion charge distribution, electric field, and particle collection efficiency were investigated under various conditions. The staggered model showed an average ion charge density that was 20% higher than that of the aligned arrangement. Particles introduced via staggered model acquired higher charge and showed improved collection efficiency across inflow velocities of 0.5 to 1.5 m/s and particle diameters of 0.1 to 50 μm. In the staggered model, particles predominantly escaped near the sidewall of the ESP.

Performance and techno-economic evaluation of a high-efficiency electrospray cyclone

"Nowadays, because of the global air pollution issue caused by fine dust, fine dust collection and removal technologies are crucial for enhancing living environments and human health. This research proposes a new pilot-scale electrospray cyclone (ESC) designed for the collection of submicron dust particles. The experimental apparatuses comprised a cyclone dust collector and an insulating tank. Initially, laboratory-scale single-nozzle visualization tests were conducted to investigate the droplets’ number and size under various operating conditions. Subsequently, based on the visualization research outcomes, electrospray module was inserted to the industrial cyclone, which was designated by ESC. Performance assessments of the pilot-scale ESC were conducted under diverse water flowrates, applied voltages and nozzle sizes. The capture efficiencies for PM10, PM2.5, and PM1.0 were measured up to 98.2%, 95.4%, and 90.3%, respectively. Both the environmental and economic viabilities of the newly-proposed ESC in this study were evaluated based on three aspects: 1) capacitive particle collection efficiency; 2) capacitive installation cost; and 3) rated power and operational cost. This evaluation method has been defined as the Levelized Cost of Precipitator (LCOP), and it is intended to assess the environmental and economic performance of 5-convenstional dust collectors. In these results, the ESC shows relatively high performance in terms of the environmental and economic aspects. Based on these indices, we assess that the ESC has one of the promising alternatives of commercial precipitators."

Measurement report: Evaluation of the TOF-ACSM-CV for PM1.0 and PM2.5 measurements during the RITA-2021 field campaign

Abstract. The recently developed time-of-flight aerosol chemical speciation monitor with a capture vaporizer and a PM2.5 aerodynamic lens (TOF-ACSM-CV-PM2.5) aims to improve the collection efficiency and chemical characterization of aerosol particles with a diameter smaller than 2.5 µm. In this study, comprehensive cross-comparisons were performed between real-time online measurements and offline filter analysis with 24 h collection time. The goal was to evaluate the capabilities of the TOF-ACSM-CV-PM2.5 lens, as well as the accuracy of the TOF-ACSM-CV-PM2.5. The experiments were conducted at Cabauw Experimental Site for Atmospheric Research (CESAR) during the RITA-2021 campaign. The non-refractory fine particulate matter (PM1.0 and PM2.5) was measured by two collocated TOF-ACSM-CV-PM2.5 instruments by placing them behind a PM2.5 and PM1.0 inlet, respectively. A comparison between the ACSMs and PM2.5 and PM1.0 filter samples showed a much better accuracy than ±30 % less given in the previous reports, with average differences less than ±10 % for all inorganic chemical species. In addition, the ACSMs were compared to the Monitoring Instrument for Aerosol and Gas (MARGA) (slope between 0.78 and 0.97 for inorganic compounds, R2≥ 0.93) and a mobility particle size spectrometer (MPSS), measuring the particle size distribution from around 10 to 800 nm (slope was around 1.00, R2= 0.91). The intercomparison of the online measurements and the comparison between the online and offline measurements indicated a low bias (< 10 % for inorganic compounds) and demonstrated the high accuracy and stability of the TOF-ACSM-CV-PM2.5 lens for the atmospheric observations of particle matter. The two ACSMs exhibited an excellent agreement, with differences less than 7 %, which allowed a quantitative estimate of PM1.0 vs. PM2.5 chemical composition. The result showed that the PM1.0 accounted for about 70 %–80 % of the PM2.5 on average. The NO3 mass fraction increased, but the organic carbon (OC) mass fraction decreased from PM1.0 to PM2.5, indicating the size dependence on chemical composition.

Enhancing the sub-micrometer performance of a uniflow cyclone separator using a built-in stainless steel mesh filter

Although the uniflow cyclone separator has low pressure drop and high collection efficiency compared to other existing cyclone separators, it still has room to improve its collection efficiency of submicron particles. For this reason, we present a new uniflow cyclone separator with an installed mesh filter called the MFUC. The MFUC cyclone body is not made of a solid wall but a stainless steel mesh with porosity. Our research newly revealed that the pressure gradient in the radial direction at the front region of the mesh filter is reversed in the rear region, which can help to remove sub-micrometer particles which are difficult to collect using a basic cyclone separator. The measured MFUC performance showed the synergetic effect of filtration and inertial separation for the removal of fine particles. As the inlet flow rate increases, the inertial separation becomes more effective than filtration. In addition, the cut-off diameter of the MFUC was 0.83 μm at 500 lpm, which is 56.6 % smaller than that of the basic cyclone separator.

Simulation study on rotor speed of combined rotary separator in coal pneumatic conveying

The separator is a key component of coal pneumatic conveying systems, which plays an important role in improving particle collection efficiency and reducing dust pollution. In this paper, a combined rotary separator was designed. Based on the traditional cyclone separator, the rotor blades were installed and matched with the guide vanes to increase the material separation and collection performance. The influence of rotor speed on the characteristics of the separator was studied by computational fluid dynamics simulation, and the flow field velocity and pressure distribution and the particle trajectory and separation degree were obtained. The results showed that the flow field tangential velocity plays a dominant role in the separation process and is approximately symmetrically distributed with the rotor axis as the center. The velocity of the flow field in the inner rotor is approximately positively correlated with the rotor speed, and the tangential velocity gradually decreases with the increase in the flow field height. The static pressure of the flow field is approximately axisymmetric along the rotor axis, and there is a pressure gradient from the outer separation cone to the rotor axis. The particles in the separator show a separation phenomenon based on the different sizes, and the change trend of the separation degree under different rotor speeds is similar. When the rotor speed is 160 rpm, the particles maintain the highest integrity. The rotor speed of 320 rpm has a protective effect on coarse particles above 1000 µm.

Numerical Study of the Influence of Using Semicircular Corrugated Collecting Plate and Inverted Semicircular Corrugated on the Electrostatic Precipitator

Electrostatic precipitators (ESPs) play a crucial role in removing harmful particles in various industries. Ongoing studies continuously strive to improve their performance and efficiency, leveraging the inherent advantages of ESPs. Researchers are exploring various types of collecting and discharge electrodes to achieve this. This study specifically focuses on comparing two types of collecting electrodes, Semicircular Corrugated Plates (SCPs) and inverted Semicircular Corrugated Plates (InvSCPs), against Flat Plates (FPs) as a reference case. Three distinct forms of ESPs were simulated, and the SCP and InvSCP designs were evaluated against the FPs, specifically assessing the impact of modifying the collecting electrode design on key electrostatic precipitator characteristics, such as electrical field distribution, space charge density distribution, particle trajectories, and particle collection efficiency. Notably, the study found that using SCP resulted in the highest particle collection efficiency compared to InvSCP and FP for the same range of particles.

Particle removal performance of a novel ESP type air cleaning system for indoor air quality in a subway station

A novel electrostatic precipitation type air cleaning technology with near zero ozone emission for indoor air quality of a subway station was developed. To minimize ozone emission and achieve high particle removal performance against ultrafine particulate matters (PMs), a multi-channel charging method using soft ionization by micrometre carbon fibers and a narrow gap collection method using high electric field by thin conductive plastic sheets as a high voltage electrode were used. In this study, the novel electrostatic charging and collection technologies were applied to a real scale air cleaning system in an Air Handling Unit (AHU) with air flow rate of 950 m3/min in Yuseong Oncheon subway station with an area of 3000 m2 in Daejeon, South Korea. The particle removal performance of the demonstration system was evaluated with real suspended particles in the subway station during test period with high PM concentrations in Korea over 40 μg/m3. Particle collection efficiency, pressure drop and ozone emission were evaluated, and compared to those of the a minimum efficiency reporting value (MERV) 10 and 14 filters used in the typical subway stations in Korea. In the field researches, the developed ESP achieved over 80% of the PM collection efficiency higher than those of the filters with MERV-10 and -14, and even 10% higher efficiency against PM1.0, while generating only 10% of pressure drop and also emitting nearly zero ozone. It is concluded that a novel ESP type air cleaning system with near zero ozone emission could be a promising air cleaning method for a large indoor environment such as a subway station where polluted air with ultrafine particles flowed in with a very high flow rate.

Computational Fluid Dynamics Analysis of Wet Dust Removal in High-Gravity Countercurrent Rotating Packed Bed

High-gravity wet dust removal technology has attracted much attention because of its potential to cut liquid into smaller liquid droplets and lower energy consumption. However, the complex structure and the high-speed rotation of the rotating packed bed do not allow us to analyze the flow field using conventional methods, and thus the capture mechanism of fine particles in a high-gravity environment is poorly understood. In this study, a two-dimensional computational fluid dynamics model was established to investigate the distribution of the gas–liquid two-phase flow field inside of a rotating packed bed. The characteristics of the flow field, such as the liquid form, gas–liquid contact time, and gas flow path, were investigated, and the droplet size distribution and gas–liquid slip velocity were quantitatively analyzed. The inertial capture efficiency was calculated using the Stokes number, and the dust removal efficiency distribution in the rotating packed bed was compared. The reason for the high collection efficiency of fine particles by the high-gravity wet dust removal technology was explained by numerical simulations. Two new structures were designed to improve the total dust removal efficiency.

Influence of Acoustic Streams on the Efficiency of Ultrasonic Particle Agglomeration

The article is devoted to the study of ultrasonic agglomeration of PM 2.5 in homogeneous and inhomogeneous ultrasonic fields. The possibility of increasing the efficiency of ultrasonic agglomeration by initiating acoustic streams in a resonant inhomogeneous ultrasonic field is shown. A inhomogeneous ultrasonic field with zones of high and low sound pressure levels formed using a bending-oscillating disk transmitter made it possible to initiate acoustic vortex-type streaming that promotes the movement of particles into the nodal areas of a standing wave and between them. Due to the formation of a inhomogeneous ultrasonic field, the efficiency of particle collection is increased: for PM 2.5, the efficiency reaches 95%; PM 1.5—92%; PM 0.5—85%. The results were obtained under the following conditions: concentration 2 × 10−2 g/m3, sound pressure level 165 dB, flow rate 6.2 m3/h. For comparison, when a homogeneous ultrasonic field is formed in the agglomeration chamber (under similar conditions), the efficiency of particle capture by inertial gas cleaning equipment does not exceed the following: for PM 2.5—89%; PM 1.5—85%; and PM 0.5—76%. The obtained research results made it possible to propose a design for an agglomeration chamber that can greatly increase the productivity of ultrasonic flow processing.

Performance of the porous media model for simulating flow through an electrostatic precipitator

An electrostatic precipitator (ESP), which filters the fine particles present in the exhaust gas generated from a power plant, has a better particle-collection efficiency when there exists a uniform flow in the dust collection chamber. However, most former investigations examined the flow distribution via numerical approaches that modeled the perforated plates within the inlet diffuser as porous media, which have not been adequately validated. Therefore, the aim of this study was to examine the performance of the porous media model for simulating the flow through perforated plates of an ESP diffuser by numerical simulation and experiment. Simulation results using the porous media model were compared with those obtained with a fully resolved mesh precisely describing the complete geometry of the entire perforated plate. The results obtained with both these methods were consistent with experimental results obtained upstream of the inlet diffuser, but the porous media model could not accurately simulate the flow distribution across the perforated plates. Overall, this model failed to predict the deflection of incoming flow on the solid bars and the wakes behind the bars, and could not reflect the vena contracta phenomenon occurring within the holes of the plate. As a result, the simulated flow distribution at the entrance of the main dust-collection chamber differed from that observed in the experiment, which resulted in poor prediction of the flow field inside the chamber. Therefore, this porous media model requires further improvement for wide-scale adoption in industrial practical applications, e.g., ESP for flue gas treatment in power plants.

Effect of operation conditions on particulate matter removal by a packed-bed wet scrubber for a small-scale biofuel boiler

In 2013 the EU’s Clean Air Policy Package was established, aiming to reduce air pollution to half by 2030 compared to the level in 2005. Small-scale (<500 kW)biofuel boilers play a key role in particulate matter emission, and exposure to particulate matter even in the short term can cause different diseases. With the aim of reducing particulate matter emission in Europe, this study presents an approach to improve the removal of particulate matter emitted by small-scale boilers. A biofuel combustion boiler was equipped with a packed-bed wet scrubber, and the flue gas emitted through combustion was cleaned through the wet scrubber using a saltwater mixture. The performance of a packed-bed wet scrubber was investigated under different operating conditions. The effect of the salt concentration of the absorption solution, the temperature of the absorption solution fed to the absorber, and the height of the packed-bed material on the particle collection efficiency were measured. The operating conditions were selected based on the results obtained in a previous computational fluid dynamic simulation study. The results obtained in the present study show that an absorption solution temperature of 30 °C and an absorption solution concentration of 75 % with a full height of the packed-bed material lead to the best performance in the system. Totally keeping the absorption solution temperature as low as possible, increasing the absorption solution concentration, and raising the packed-bed material height could improve the particle collection efficiency by enhancing the effect of the diffusiophoresis and thermophoresis forces and the contact time between the flue gas and solution.

Microscale modelling of electret filters using disordered 2-D domains

This paper reports on a computational study about the impact of fiber dipole orientation on particle collection efficiency of a bipolarly charged filter. The simulations were carried out using ANSYS software in a series of 2-D geometries comprised of randomly distributed fibers. The simulations were enhanced with in-house subroutines to incorporate Coulomb and dielectrophoretic forces in calculating particle trajectories and thereby simulating filter efficiency. The highest and lowest efficiencies were observed for dipole orientations that were perpendicular and parallel to the airflow direction, respectively. The simulation results were also compared with the predictions of the popular semi-empirical correlations from the literature and good general agreement was observed, without the need for any empirical correction factors. In addition, it was observed that the predictions of the semi-empirical correlations better agreed with the simulation results obtained for media comprised of fibers with random dipole orientations when challenged with neutralized particles.

Study on Gas-solid Two-phase Flow Field of Ramon Mill Classifier

To reveal the working principle and internal flow field law of the grading machine, the numerical simulation of the gas-solid two-phase flow field was carried out. In this paper, the numerical simulation method based on Fluent is used to obtain the internal velocity distribution and pressure distribution of the grading machine. The flow field of gas-solid two-phase was studied based on the CFD-DEM coupling, and the particle motion trajectory in the grading machine and the particle motion law in the flow field at different times were obtained; The influence of the operating parameters of the internal flow field on the force of particles in the grading machine was analyzed, and combined with the change of particle number, the particle collection efficiency of the grading machine under different operating parameters was further given. It is of guiding significance to adjust the parameters of the grading machine, improve the output and the product quality of the longitudinal mill, and reduce the energy consumption of the longitudinal mill.

A dynamic collection efficiency formulation implemented in the icing code DICEPS

The Technical University of Braunschweig developed the 2D icing code DICEPS, used for the simulation of ice accretion on aircraft components exposed to icing conditions. In its formulations, DICEPS presents an improvement in the traditional formulation which icing codes use for the calculation of the collection efficiency, which works together with a multi-sub-step algorithm used for the surface deformation during an icing-step. This new formulation continuously updates the impingement mass flow based on the change of the wall-normal as the surface deforms during the multi-sub-step routine in an icing-step, resulting in a dynamic collection efficiency. In the current work, DICEPS and its dynamic collection efficiency formulation (DCEF) are presented and validated through several test cases under three categories: prediction of collection efficiency, rime ice shapes and glaze ice shapes. DICEPS managed to successfully replicate distributions of collection efficiency along with an implemented splashing model. A substantial improvement in the prediction of rime ice shapes via single-step simulations was achieved using the DCEF, while the traditional formulation requires several icing-steps to obtain a converged ice shape. This is also seen when rime ice results are compared to those of FENSAP-ICE, which require as well several icing-steps. In the case of glaze ice, the DCEF presents a time limit since prominent ice features will heavily influence the real collection efficiency, making the DCEF inaccurate after this limit. Nevertheless, the effects that geometrical changes have over parameters such as the heat transfer imply that a multi-step approach is eventually required. By analyzing the results, the DCEF shows that it effectively resembles the physical behavior that geometrical changes impose on the collection efficiency for particles with large inertia, while smaller particles present some inaccuracies, suggesting a proper extension of DCEF for these cases.

The effect of the corona wire distribution with W-type of collecting plates on the characteristics of electrostatic precipitators

Electrostatic precipitators (ESPs) are commonly applied to eliminate particles in various industrial sectors. A numerical study is conducted to evaluate the use of different arrangements of W-type collecting plates compared to flat plates (FPs) for a single stage of ESP. The modeling was done for six different ESP cases, and the W-type results obtained are compared to FPs to determine the consequence of corona wires spacing at different ratios of Lww/Lwp (Lww is a wire–wire space and Lwp is a wire–plate space) on the distribution especially of the electrical field, space charge density, and particle collection. The electric field close to the grounded collecting plates continued to rise when Lww/Lwp is reduced for both shapes. Furthermore, when compared to FPs, the use of W-types improves particle collection efficiency.

PM0.1 non-bouncing impactor (NBI) for ultrafine particle mass and number measurements

This study designed and tested a 30 L/min PM0.1 non-bouncing impactor (PM0.1 NBI) for ultrafine particle (UFP) mass concentration measurement. The PM0.1 NBI uses a wetted glass fiber filter with continuous water injection to maintain a clean surface, preventing particle loading and bounce effects. Lab tests showed the 30 L/min PM0.1 NBI outperformed the PM0.1 stage of NCTU micro-orifice cascade impactor (NMCI, non-rotating) with a silicon oil-coated aluminum foil substrate in collecting solid particles, as the particle collection efficiency of the latter decreased obviously with increasing particle aerodynamic diameter for particles larger than ca. 300 nm, an apparent particle bounce phenomenon. The ambient field tests showed very close UFP mass concentrations between the PM0.1 NBI sampler (the PM0.1 NBI preceded by 3 stages with 18, 10, and 2.5 μm cutoff sizes) and the reference rotating 10-stages NMCI with the difference of ±0.5 μg/m3 only. In addition, the 3 L/min PM0.1 NBI was combined with a condensation particle counter to measure the UFP number concentrations which were shown to be very close to those of the reference with the difference of ±5% only in the laboratory tests for loaded particle mass up to 300 μg. Good agreement was also found in the field tests. Therefore, the current 3 L/min PM0.1 NBI and the future PM NBI with smaller flow rates (0.2–2.1 L/min) and larger cut-sizes (such as 0.4–0.9 μm) can be used as viable UFP classifiers for improving UFP measurement accuracy both in mass concentrations and number concentrations and reducing the maintenance needs for the UFP classifiers which are important to long-term sampling and monitoring.

Effects of the nozzle-to-nozzle distance on the performance of the water condensation growth-based virus aerosol concentrator

Efficient collection of airborne viruses is crucial for monitoring and preventing the spread of respiratory diseases. The laminar flow water condensation-based growth tube collector (GTC) is a microbial sampler extensively used to collect virus aerosol particles owing to its high recovery of viable viruses. The GTC involves multiple nozzles and eight tubes for sampling flow rates of 6–8 L per minute (LPM). To allow the GTC to operate at a higher flow rate, optimizing GTC performance through investigation of the effects of nozzle-to-nozzle distance is essential. Herein, we examined these effects on the collection efficiency and viability of airborne MS2 viruses collected by the growth-based virus aerosol concentrator (GVC), which is a lab-made single-tubed GTC, at flow rates of up to 6 LPM per tube. The flow interactions between adjacent jets were analyzed by observing the particle deposition patterns. The collection efficiencies of MS2 virus aerosol particles and the enrichment ratio of the GVC increased with increasing nozzle-to-nozzle distance. The infectious virus concentration relative to that in the virus suspension (RIVC) ranged from 0.0093 to 0.095 for 5 min of sampling. At flow rates of 1 and 6 LPM, the RIVC decreased as the nozzle-to-nozzle distance decreased, which may be ascribed to the higher shear stress at shorter nozzle-to-nozzle distances applied to the viruses collected through the cross-flows driven by adjacent jets. These measured RIVC values are much larger than those collected by the BioSampler. These findings can provide important insights into optimizing multiple nozzles in high-flow-rate GTCs.

Improvement and validation of containment spray removal aerosol models based on single droplet collection particle mechanism

Nuclear safety is the lifeline for the development and application of nuclear energy. In severe nuclear power plant accidents, aerosols are the major carriers of fission products, which may leak into the environment and cause potential radioactive contamination. Containment spray is an important mitigation measure for severe accidents in nuclear power plants. It can effectively reduce containment atmospheric pressure and radioactive aerosol concentration. This paper improves the containment spray removal models so as to address the low accuracy of the original models of the ISAA code. Based on single droplet collection particle mechanism, new inertial impaction and interception models were used to accurately calculate the collection efficiency of large particles. Additionally, a new correlation was used to explain the Brownian diffusion collection mechanism of small particles. Moreover, thermophoresis and diffusiophoresis models were introduced to consider the contribution of steam condensation in the containment to the collection efficiency. A rear capture model was introduced to incorporate the influence of recirculation within the wake of large droplets on the collection efficiency. Furthermore, THAI, TOSQAN and CSE experiments were selected to validate and evaluate the improved ISAA code. According to the calculation results, the improved models can simulate the attenuation trend of suspended aerosols with higher accuracies and significantly improves the calculation accuracy of the spray removal constants. This work contributes to understand of the scavenging mechanism of aerosol particle by containment spray droplets, and provides an analysis method with higher simulation accuracy. At the same time, it points out shortcomings in the simulation of aerosol behavior in the current ISAA code and discusses future improvements to the code.