Parametric Down-conversion Research Articles

Amplification of cascaded down-conversion by reusing photons with a switchable cavity

The ability to efficiently produce and manipulate nonclassical states of light is a critical requirement for the development of quantum optical technologies. In recent years, experiments have demonstrated that cascaded spontaneous parametric down-conversion is a promising approach to implement photon precertification, providing a way to overcome photon transmission losses for quantum communication, as well as to directly produce entangled three-photon states and heralded Bell pairs. However, the low efficiency of this process has so far limited its applicability beyond basic experiments. Here, we propose a scheme to amplify triplet production rates by using a fast switch and a delay loop to reuse photons that fail to convert on the first pass through the cascade's second nonlinear crystal. We construct a theoretical model to predict amplification rates and verify them in an experimental implementation. Our proof-of-concept device increases the rate of detected photon triplets as predicted, demonstrating that the method has the potential to dramatically improve the usefulness of cascaded down-conversion for device-independent quantum communication and entangled state generation.

Measurement-Device-Independent Quantum Key Distribution Based on Decoherence-Free Subspaces with Logical Bell State Analyzer.

Measurement-device-independent quantum key distribution (MDI-QKD) enables two legitimate users to generate shared information-theoretic secure keys with immunity to all detector side attacks. However, the original proposal using polarization encoding is sensitive to polarization rotations stemming from birefringence in fibers or misalignment. To overcome this problem, here we propose a robust QKD protocol without detector vulnerabilities based on decoherence-free subspaces using polarization-entangled photon pairs. A logical Bell state analyzer is designed specifically for such encoding. The protocol exploits common parametric down-conversion sources, for which we develop a MDI-decoy-state method, and requires neither complex measurements nor a shared reference frame. We have analyzed the practical security in detail and presented a numerical simulation under various parameter regimes, showing the feasibility of the logical Bell state analyzer along with the potential that double communication distance can be achieved without a shared reference frame.

Degenerate polarization entangled photon source based on a single Ti-diffusion lithium niobate waveguide in a polarization Sagnac interferometer

Combining a Ti-diffusion periodically poled lithium niobate (PPLN) waveguide with a Sagnac interferometer, two opposite directions type-II spontaneous parametric down conversions (SPDC) occur coherently and yield a high brightness, high stability polarization entanglement source. The source produces degenerate photon pairs at 1540.4 nm with a brightness of B = (1.36 ± 0.03) × 106 pairs/(s⋅nm⋅mW). We perform quantum state tomography to reconstruct the density matrix of the output state and obtain a fidelity of F = 0.983 ± 0.001. The high brightness and phase stability of our waveguide source enable a wide range of quantum information experiments operating at a low pump power as well as hold the advantage in mass production which can promote the practical applications of quantum technologies.

Polarization Entanglement from Parametric Down-conversion with an LED Pump

Spontaneous parametric down-conversion (SPDC) is a reliable platform for entanglement generation. Routinely, a coherent laser beam is an essential prerequisite for pumping the nonlinear crystal. Here we break this barrier to generate polarization-entangled photon pairs by using a commercial light-emitting diode (LED) source to serve as the pump beam. This effect is counterintuitive, as the LED source is of extremely low spatial coherence, which is transferred during the down-conversion process to the biphoton wave function. However, the type-II phase matching condition naturally filters the specific frequency and wavelength of LED light exclusively to participate in SPDC such that localized polarization Bell states can be generated, regardless of the global incoherence over the full transverse plane. In our experiment, we characterize the degree of LED light-induced polarization entanglement in the standard framework of the violation of Bell's inequality. We achieve the Bell value $S=2.33\ifmmode\pm\else\textpm\fi{}0.097$, obviously surpassing the classical bound $S=2$ and thus witnessing the quantum entanglement. Our work can be extended to prepare polarization entanglement by using other natural light sources, such as sunlight and biolight, which holds promise for electricity-free quantum communications in outer space.

High-flux, high-visibility entangled photon source obtained with a non-collinear type-II PPKTP crystal pumped by a broadband continuous-wave diode laser

We demonstrated a high-brightness, polarization-entangled bi-photon source generated in a type-II phase-matched non-collinear PPKTP crystal pumped by a 405 nm continuous-wave (cw) broadband diode laser. Basing on the single-pass configuration, we investigated the distribution characteristics of the bi-photon cone and the wavelength tunability with crystal temperatures. Overcoming the degradation of the bi-photon generation rate and the spectral correlation induced by the broadband pump laser, we obtained a bi-photon generation rate of 7.48×103/s/mW/nm and an interference visibility over 95% via a Hong–Ou–Mandel (HOM) configuration. We established a theoretical model to address the bi-photon time-delayed HOM dip pumped by the broadband cw diode laser in spontaneous parametric down-conversion and obtained the complete analytic solution of the bi-photon coincidence counting rates.

Generation of hyperentangled photon pairs based on lithium niobate waveguide

Generation of hyperentangled photon pairs is investigated based on the lithium niobate straight waveguide. We propose to use the nonlinear optical process of spontaneous parametric down-conversion (SPDC) and a well-designed lithium niobate waveguide structure to generate a hyperentangled (in the polarization dimension and the energy-time dimension) two-photon state. By performing numerical simulations of the waveguide structure and calculating the possible polarization states, joint spectral amplitudes (JSA), and joint temporal amplitudes (JTA) of the generated photon pair, we show that the generated photon pair is indeed hyperentangled in both the polarization dimension and the energy-time dimension.

Realization of a source-device-independent quantum random number generator secured by nonlocal dispersion cancellation

Quantum random number generators (QRNGs) can provide genuine randomness by exploiting the intrinsic probabilistic nature of quantum mechanics, which play important roles in many applications. However, the true randomness acquisition could be subjected to attacks from untrusted devices involved or their deviations from the theoretical modeling in real-life implementation. We propose and experimentally demonstrate a source-device-independent QRNG, which enables one to access true random bits with an untrusted source device. The random bits are generated by measuring the arrival time of either photon of the time–energy entangled photon pairs produced from spontaneous parametric downconversion, where the entanglement is testified through the observation of nonlocal dispersion cancellation. In experiment, we extract a generation rate of 4 Mbps by a modified entropic uncertainty relation, which can be improved to gigabits per second by using advanced single-photon detectors. Our approach provides a promising candidate for QRNGs with no characterization or error-prone source devices in practice.

Simultaneous transmission of hyper-entanglement in three degrees of freedom through a multicore fiber

Entanglement distribution is at the heart of most quantum communication protocols. Inevitable loss of photons along quantum channels is a major obstacle for distributing entangled photons over long distances, as the no-cloning theorem forbids the information to simply be amplified along the way as is done in classical communication. It is therefore desirable for every successfully transmitted photon pair to carry as much entanglement as possible. Spontaneous parametric down-conversion (SPDC) creates photons entangled in multiple high-dimensional degrees of freedom simultaneously, often referred to as hyper-entanglement. In this work, we use a multicore fiber (MCF) to show that energy-time and polarization degrees of freedom can simultaneously be transmitted in multiple fiber cores, even maintaining path entanglement across the cores. We verify a fidelity to the ideal Bell state of at least 95% in all degrees of freedom. Furthermore, because the entangled photons are created with a center wavelength of 1560 nm, our approach can readily be integrated into modern telecommunication infrastructure, thus paving the way for high-rate quantum key distribution and many other entanglement-based quantum communication protocols.

Measuring the Schmidt number of parametric down conversion by exploiting photon distribution

The Schmidt number quantifies the number of modes and is mainly used as a measure for the quality of entanglement. We theoretically compute the photon distribution of type-I spontaneous parametric down conversion (SPDC) with an arbitrary Schmidt number. The photon distribution is used for a novel method to measure the Schmidt number. This method requires only two on–off single-photon detectors with no photon number or temporal resolution. The method works in the strong pumping regime where high photon numbers are non-negligible. We experimentally demonstrate the method for type-II SPDC. The easy and fast measurement of the Schmidt number has a broad range of applications from the calibration of strong pump SPDC and entanglement sources to multi-photon quantum interference and Gaussian boson sampling.

High-sensitivity quantum sensing with pump-enhanced spontaneous parametric down-conversion

Recent years have seen the development of quantum sensing concepts utilizing nonlinear interferometers based on correlated photon pairs generated by spontaneous parametric down-conversion (SPDC). Using SPDC far from frequency degeneracy allows a “division of labor” between the mid-infrared photon for the strongest sample interaction and the correlated near-infrared photon for low-noise detection. The small number of photons provided by SPDC and the resulting inferior signal-to-noise ratio are, however, a limiting factor preventing the wide applicability of the novel sensing concept. Here, we demonstrate a nonlinear interferometer based on pump-enhanced SPDC with strongly improved emission rates while maintaining broadband spontaneous emission. For validation of the concept, we demonstrate high-resolution mid-infrared spectroscopy with near-infrared detection, showcasing improved accuracy. Although the number of mid-infrared photons is about five orders of magnitude smaller than in classical spectrometers, the sensitivity of the quantum spectrometer becomes comparable, marking an essential step toward real-world applications.

Spatial-spectral mapping to prepare frequency entangled qudits.

Entangled qudits, the high-dimensional entangled states, play an important role in the study of quantum information. How to prepare entangled qudits in an efficient and easy-to-operate manner is still a challenge in quantum technology. Here, we demonstrate a method to engineer frequency entangled qudits in a spontaneous parametric downconversion process. The proposal employs an angle-dependent phase-matching condition in a nonlinear crystal, which forms a classical-quantum mapping between the spatial (pump) and spectral (biphotons) degrees of freedom. In particular, the pump profile is separated into several bins in the spatial domain, and thus shapes the down-converted biphotons into discrete frequency modes in the joint spectral space. Our approach provides a feasible and efficient method to prepare a high-dimensional frequency entangled state. As an experimental demonstration, we generate a three-dimensional entangled state by using a homemade variable slit mask.

Optical spin–orbit interaction in spontaneous parametric downconversion

Optical spin–orbit interaction (SOI), which can be used to simultaneously control the spin and orbital angular momentum of light, is important for both classical and quantum information applications. In linear and nonlinear optics, the SOI of light has been extensively explored in both artificial structures and conventional optical crystals. However, optical SOI in quantum nonlinear optical processes, such as spontaneous parametric downconversion (SPDC), has not been studied before. Here, we experimentally demonstrate that optical SOI in the SPDC process can be realized through a nonlinear crystal with threefold rotational symmetry. Two-photon quantum states with controlled angular momentum can be generated through the symmetry selection rules in nonlinear optics and the SOI of the pump wave. The proposed methodology may facilitate the generation and control of spin and orbital angular momentum of entangled photons.

Reinterpretation of the Grangier experiment using a multiple-triggering single-photon model

The classic Grangier et al. (1996) experiment is revisited to suggest an alternative model of a single photon. Photon-counting experiments using spontaneous parametric down conversion (SPDC) show that not every single-photon incident on a detector triggers it, and that coincident triggering of detectors can occur during a single gate. The latter is usually interpreted as being caused by spurious photons entering the gate from different SPDC events. However, a pseudo-classical-type model is suggested which dispenses with these intruder photons. Here, a single-photon manifests as a transversely-iterated front of non-rotating screw threads. Each advancing thread has the potential to trigger a detector, and each allows the transfer of spin angular momentum (SAM). On exiting a beam splitter, a single-photon front can produce multiple triggering of detectors on different parts of the front with a probability of at most [Formula: see text] for the experiments presented.

Background-Free Near-Infrared Biphoton Emission from Single GaAs Nanowires.

The generation of photon pairs from nanoscale structures with high rates is still a challenge for the integration of quantum devices, as it suffers from parasitic signals from the substrate. In this work, we report type-0 spontaneous parametric down-conversion at 1550 nm from individual bottom-up grown zinc-blende GaAs nanowires with lengths of up to 5 μm and diameters of up to 450 nm. The nanowires were deposited on a transparent ITO substrate, and we measured a background-free coincidence rate of 0.05 Hz in a Hanbury-Brown-Twiss setup. Taking into account transmission losses, the pump fluence, and the nanowire volume, we achieved a biphoton generation of 60 GHz/Wm, which is at least 3 times higher than that of previously reported single nonlinear micro- and nanostructures. We also studied the correlations between the second-harmonic generation and the spontaneous parametric down-conversion intensities with respect to the pump polarization and in different individual nanowires.

Quantum ghost imaging based on a "looking back" 2D SPAD array.

Quantum ghost imaging (QGI) is an intriguing imaging protocol that exploits photon-pair correlations stemming from spontaneous parametric down-conversion (SPDC). QGI retrieves images from two-path joint measurements, where single-path detection does not allow us to reconstruct the target image. Here we report on a QGI implementation exploiting a two-dimensional (2D) single-photon avalanche diode (SPAD) array detector for the spatially resolving path. Moreover, the employment of non-degenerate SPDC allows us to investigate samples at infrared wavelengths without the need for short-wave infrared (SWIR) cameras, while the spatial detection can be still performed in the visible region, where the more advanced silicon-based technology can be exploited. Our findings advance QGI schemes towards practical applications.

Generation of a time–bin Greenberger–Horne–Zeilinger state with an optical switch

Multipartite entanglement is a critical resource in quantum information processing that exhibits much richer phenomenon and stronger correlations than in bipartite systems. This advantage is also reflected in its multi-user applications. Although many demonstrations have used photonic polarization qubits, polarization-mode dispersion confines the transmission of photonic polarization qubits through an optical fiber. Consequently, time–bin qubits have a particularly important role to play in quantum communication systems. Here, we generate a three-photon time–bin Greenberger–Horne–Zeilinger (GHZ) state using a 2 × 2 optical switch as a time-dependent beam splitter to entangle time–bin Bell states from a spontaneous parametric down-conversion source and a weak coherent pulse. To characterize the three-photon time–bin GHZ state, we performed measurement estimation, showed a violation of the Mermin inequality, and used quantum state tomography to fully reconstruct a density matrix, which shows a state fidelity exceeding 70%. We expect that our three-photon time–bin GHZ state can be used for long-distance multi-user quantum communication.

Telecom quantum photonic interface for a 40Ca+ single-ion quantum memory

Entanglement-based quantum networks require quantum photonic interfaces between stationary quantum memories and photons, enabling entanglement distribution. Here we present such a photonic interface, designed for connecting a 40Ca+ single-ion quantum memory to the telecom C-band. The interface combines a memory-resonant, cavity-enhanced spontaneous parametric down-conversion photon pair source with bi-directional polarization-conserving quantum frequency conversion. We demonstrate preservation of high-fidelity entanglement during conversion, fiber transmission over up to 40 km and back-conversion to the memory wavelength. Even for the longest distance and bi-directional conversion the entanglement fidelity remains larger than 95% (98%) without (with) background correction.

Experimental generation of polarization entanglement from spontaneous parametric down-conversion pumped by spatiotemporally highly incoherent light

The authors experimentally demonstrate the generation of polarization entanglement through spontaneous parametric down-conversion pumped by a spatiotemporally highly incoherent light beam. However, polarization entanglement from the spatiotemporally incoherent pump is susceptible to degradation. Theoretical analysis shows that the degradation stems from the coupling between the spatiotemporal and polarization degrees of freedom, which is introduced by the birefringence and dispersion of the nonlinear crystal.

General simulation method for spontaneous parametric down- and parametric up-conversion experiments

Spontaneous parametric down-conversion (SPDC) sources are an important technology for quantum sensing and imaging. We demonstrate a general simulation method, based on modeling from first principles, reproducing the spectrally and spatially resolved absolute counts of a SPDC experiment. By additionally simulating parametric up- and down-conversion processes with thermal photons as well as effects of the optical system we accomplish good agreement with the experimental results. This method is broadly applicable and allows for the separation of contributing processes, virtual characterization of SPDC sources, and enables the simulation of many quantum based applications.

Continuous variable spin-orbit total angular momentum entanglement on the higher-order Poincaré sphere.

Optical spin-orbit coupling is an important phenomenon and has fruitful applications. Here, we investigate the spin-orbit total angular momentum entanglement in the optical parametric downconversion process. Four pairs of entangled vector vortex modes are experimentally generated directly using a dispersion- and astigmatism-compensated single optical parametric oscillator, and for the first time, to the best of our knowledge, the spin-orbit quantum states are characterized on the quantum higher-order Poincaré sphere, and the relationship of spin-orbit total angular momentum Stokes entanglement is demonstrated. These states have potential applications in high-dimensional quantum communication and multiparameter measurement.