Parametric Down-conversion Research Articles

Wavelength variable generation and detection of photon pairs in visible and mid-infrared regions via spontaneous parametric downconversion

We report an experimental demonstration of wavelength variable generation and detection of photon pairs in the visible and mid-infrared (MIR) regions over a wide spectral range of 2–5 µm via spontaneous parametric downconversion. Despite the recent increase in interest in such a photon-pair source, there have been few detailed evaluations of emitted photons generated via the downconversion process in the low gain regime, due to the lack of suitable single-photon detectors. By changing the angle of the nonlinear crystal, we continuously tune the phase-matching condition and generate photon pairs as signal photons in the wavelength range of 600–965 nm and idler photons in the wavelength range of 1186–4694 nm. We evaluate the generated photon pairs using single and coincidence counts by superconducting nanowire single-photon detectors up to a wavelength of 2 µm and detect the intensity using an InSb detector with a lock-in detection system up to 5 µm. From this analysis, a pair generation rate of 10 5 s − 1 per mW of pump power is experimentally obtained for this wavelength range. This work provides a basis for the realization of applications such as heralded MIR single-photon sources, infrared imaging, and infrared spectroscopy based on quantum technologies in the MIR region.

Experimental realization of Schumacher's information geometric Bell inequality

Quantum mechanics can produce correlations that are stronger than classically allowed. This stronger–than–classical correlation is the “fuel” for quantum computing. In 1991 Schumacher forwarded a beautiful geometric approach, analogous to the well-known result of Bell, to capture non-classicality of this correlation for a singlet state. He used a well-established information distance defined on an ensemble of identically–prepared states. He calculated that for certain detector settings used to measure the entangled state, the resulting geometry violated a triangle inequality — a violation that is not possible classically. This provided a novel information–based geometric Bell inequality in terms of a “covariance distance.” Here we experimentally reproduce his construction and demonstrate a definitive violation for a Bell state of two photons based on the usual spontaneous parametric down-conversion in a paired BBO crystal. The state we produced had a visibility of Vad=0.970. We discuss generalizations to higher dimensional multipartite quantum states.

Azimuthal eigenmodes at strongly non-degenerate parametric down-conversion

Quantum-optical technologies based on parametric light down-conversion are not yet applied in the terahertz frequency range. This is owing to the complexity of detecting single photons in the terahertz frequency range and the strong entanglement of modes of optical-terahertz biphotons. This study investigates the angular structure of scattered radiation generated by strongly non-degenerate parametric down-conversion when the frequency of the idler radiation does not exceed several terahertz. We demonstrate that under certain approximations, it is possible to obtain azimuthal eigenmodes for the nonlinear-interaction operator. The solution of the evolution equations for the field operators in these eigenmodes has the form of the Bogolyubov transformation, which allows a scattering matrix to be obtained for arbitrary values of the parametric gain. This scattering matrix describes both the production of biphoton pairs and the generation of intense fluxes of correlated optical-terahertz fields that form a macroscopic quantum state of radiation in two spectral ranges.

Photon Pairs from Resonant Metasurfaces.

All-dielectric optical metasurfaces are a workhorse in nano-optics, because of both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to 2 orders of magnitude, compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons—a new promising platform for quantum optics experiments.

Full-mode characterization of correlated photon pairs generated in spontaneous downconversion.

Spontaneous parametric downconversion is the primary source to generate entangled photon pairs in quantum photonics laboratories. Depending on the experimental design, the generated photon pairs can be correlated in the frequency spectrum, polarization, position-momentum, and spatial modes. Exploring the spatial modes' correlation has hitherto been limited to the polar coordinates' azimuthal angle, and a few attempts to study Walsh mode's radial states. Here, we study the full-mode correlation, on a Laguerre-Gauss basis, between photon pairs generated in a type-I crystal. Furthermore, we explore the effect of a structured pump beam possessing different spatial modes onto bi-photon spatial correlation. Finally, we use the capability to project over arbitrary spatial mode superpositions to perform the bi-photon state's full quantum tomography in a 16-dimensional subspace.

Generation of hyper-entangled states in strongly coupled topological defects.

We investigate spontaneous parametric downconversion (SPDC) in a waveguide array supporting two strongly coupled topological guided modes. We show that it is possible to generate photon pairs that are hyper-entangled in energy and path. We study the state robustness against positional disorder of the waveguides, in terms of Schmidt number (SN), fidelity, and density matrix. We show that quantum correlations are in general robust due to the peculiar interplay between structure topology and second-order nonlinear interaction.

Engineering multipartite coupling in doubly pumped parametric down-conversion processes

We investigate the quantum state generated by optical parametric down-conversion in a $\chi^{(2) } $ medium driven by two noncollinear light modes. The analysis shows the emergence of multipartite, namely 3- or 4-partite, entangled states in a subset of the spatio-temporal modes generated by the process. These appear as bright spots against the background fluorescence, providing an interesting analogy with the phenomenology recently observed in two-dimensional nonlinear photonic crystals. We study two realistic setups: i) Non-critical phase-matching in a periodically poled Lithium Tantalate slab, characterized by a 3-mode entangled state among hot spots. ii) A type I setup in a Beta-Barium Borate crystal, where the spatial walk-off between the two pumps can be exploited to make a transition to a quadripartite entangled state. In both cases we show that the properties of the state can be controlled by modulating the relative intensity of two pump waves, making the device a versatile tool for quantum state engineering.

Improving the purity of heralded single-photon sources through spontaneous parametric down-conversion process* *Project supported by the National Key Research and Development Program of China (Grant Nos. 2018YFA0306400 and 2017YFA0304100), the National Natural Science Foundation of China (Grant Nos. 12074194, 11774180, and U19A2075), and the Leading-edge Technology Program of Jiangsu Natural Science Foundation, China (Grant No. BK20192001).

The high-purity single-photon source plays an important role in the field of quantum information. Usually, it is generated through spontaneous parametric down-conversion process. In this paper, we investigate and summarize a few approaches on obtaining single-photon sources with a high purity using either PPKTP or PPLN nonlinear crystals. Moreover, we present improved schemes to increase the purity based on existing work, corresponding applicable conditions and procedures are discussed and analyzed. Besides, we carry out numerical simulations and show that nearly perfect purity can be reached even without using any filters. Therefore, this work might provide valuable references for the generation and application of high purity single-photon sources.

Spectral characterization of SPDC-based single-photon sources for quantum key distribution

In our laboratory, we employ two biphoton sources for quantum key distribution. The first is based on cw parametric down-conversion of photons at 404 nm in PPKTP waveguide chips, while the second is based on the pulsed parametric down-conversion of 775 nm photons in PPLN waveguides. The spectral characterization is important for the determination of certain side-channel attacks. A Hong-Ou-Mandel experiment employing the first photon source revealed a complex structure of the common Hong-Ou-Mandel dip. By measuring the spectra of the single photons at 808 nm, we were able to associate these structures to the superposition of different transverse modes of the pump photons in our waveguide chips. The pulsed source was characterized by means of single-photon spectra measured by a sensitive spectrum analyzer as well as dispersion-based measurements. Finally, we also describe Hong-Ou-Mandel experiments using the photons from the second source.

Enhancement of microwave squeezing via parametric down-conversion in a superconducting quantum circuit.

We propose an experimentally accessible superconducting quantum circuit, consisting of two coplanar waveguide resonators (CWRs), to enhance the microwave squeezing via parametric down-conversion (PDC). In our scheme, the two CWRs are nonlinearly coupled through a superconducting quantum interference device embedded in one of the CWRs. This is equivalent to replacing the transmission line in a flux-driven Josephson parametric amplifier (JPA) by a CWR, which makes it possible to drive the JPA by a quantized microwave field. Owing to this design, the PDC coefficient can be considerably increased to be about tens of megahertz, satisfying the strong-coupling condition. Using the Heisenberg-Langevin approach, we numerically show the enhancement of the microwave squeezing in our scheme. In contrast to the JPA, our proposed system becomes stable around the critical point and can generate stronger transient squeezing. In addition, the strong-coupling PDC can be used to engineer the photon blockade.

Positive operator-valued measure for two-photon detection via sum-frequency generation

Spontaneous parametric down conversion (PDC), in the perturbative limit, can be considered as a probabilistic splitting of one input photon into two output photons. Conversely, sum-frequency generation (SFG) implements the reverse process of combining two input photons into one. Here we show that a single-photon projective measurement in the temporal-mode basis of the output photon of a two-photon SFG process effects a generalized measurement on the input two-photon state. We describe the positive-operator-valued measure (POVM) associated with such a measurement, and show that its elements are proportional to the two-photon states produced by the time-reversed PDC process. Such a detection acts as a joint measurement on two photons, and is thus an important component of many quantum information processing protocols relying on photonic entanglement. Using the retrodictive approach, we analyze the properties of the two-photon POVM that are relevant for quantum protocols exploiting two-photon states and measurements.

Effect of source statistics on utilizing photon entanglement in quantum key distribution

A workflow for evaluation of entanglement source quality is proposed. Based on quantum state density matrices obtained from theoretical models and experimental data, we make an estimate of a potential performance of a quantum entanglement source in quantum key distribution protocols. This workflow is showcased for continuously pumped spontaneous parametric down-conversion (SPDC) source, where it highlights the trade-off between entangled pair generation rate and entanglement quality caused by multiphoton nature of the generated quantum states. We employ this characterization technique to show that secure key rate of down-converted photon pairs is limited to 0.029 bits per detection window due to intrinsic multiphoton contributions. We also report that there exists one optimum gain for continuous-wave down-conversion sources. We find a bound for secure key rate extracted from SPDC sources and make a comparison with perfectly single-pair quantum states, such as those produced by quantum dots.

Study of Type II SPDC in Lithium Niobate for High Spectral Purity Photon Pair Generation

Recent advances of high-quality lithium niobate (LN) on insulator technology have revitalized the progress of novel chip-integrated LN-based photonic devices and accelerated application research. One of the promising technologies of interest is the generation of entangled photon pairs based on spontaneous parametric down-conversion (SPDC) in LNs. In this paper, we investigated, theoretically and numerically, Type II SPDC in two kinds of LNs—undoped and 5-mol% MgO doped LNs. In each case, both non-poled and periodically poled crystals were considered. The technique is based on the SPDC under Type II extended phase matching, where the phase matching and the group velocity matching are simultaneously achieved between interacting photons. The proposed approach has not yet been reported for LNs. We discussed all factors required to generate photon pairs in LNs, in terms of the beam propagation direction, the spectral position of photons, and the corresponding effective nonlinearities and walk-offs. We showed that the spectral positions of the generated photon pairs fall into the mid-infrared region with high potential for free-space quantum communication, spectroscopy, and high-sensitivity metrology. The joint spectral analyses showed that photon pairs can be generated with high purities of 0.995–0.999 with proper pump filtering.

Directional emission of down-converted photons from a dielectric nanoresonator

Creation of correlated photon pairs is one of the key topics in contemporary quantum optics. Here, we theoretically describe the generation of photon pairs in the process of spontaneous parametric down-conversion in a resonant spherical nanoparticle made of a dielectric material with bulk $\chi^{(2)}$ nonlinearity. We pick the nanoparticle size that satisfies the condition of resonant eigenmodes described by Mie theory. We reveal that highly directional photon-pair generation can be observed utilising the nonlinear Kerker-type effect, and that this regime provides useful polarisation correlations.

Heralded Nondestructive Quantum Entangling Gate with Single-Photon Sources

Heralded entangling quantum gates are an essential element for the implementation of large-scale optical quantum computation. Yet, the experimental demonstration of genuine heralded entangling gates with free-flying output photons in linear optical system, was hindered by the intrinsically probabilistic source and double-pair emission in parametric down-conversion. Here, by using an on-demand single-photon source based on a semiconductor quantum dot embedded in a micropillar cavity, we demonstrate a heralded controlled-NOT (CNOT) operation between two single photons for the first time. To characterize the performance of the CNOT gate, we estimate its average quantum gate fidelity of (87.8±1.2)%. As an application, we generated event-ready Bell states with a fidelity of (83.4±2.4)%. Our results are an important step towards the development of photon-photon quantum logic gates.

Continuous variable multimode quantum states via symmetric group velocity matching

Configurable and scalable continuous variable (CV) quantum networks for measurement-based quantum information protocols or multipartite quantum communication schemes can be obtained via parametric down conversion (PDC) in non-linear waveguides. In this work, we exploit symmetric group velocity matching (SGVM) to engineer the properties of the squeezed modes of the PDC. We identify type II PDC in a single waveguide as the best suited process, since multiple modes with non-negligible amount of squeezing can be obtained. We explore, for the first time, the waveguide dimensions, usually only set to ensure single-mode guiding, as an additional design parameter ensuring indistinguishability of the signal and idler fields. We investigate here potassium titanyl phosphate (KTP), which offers SGVM at telecommunications wavelengths, but our approach can be applied to any non-linear material and pump wavelength. This work paves the way toward the engineering of future large-scale quantum networks in the CV regime.

Entangled photon-pair sources based on three-wave mixing in bulk crystals.

Entangled photon pairs are a critical resource in quantum communication protocols ranging from quantum key distribution to teleportation. The current workhorse technique for producing photon pairs is via spontaneous parametric down conversion (SPDC) in bulk nonlinear crystals. The increased prominence of quantum networks has led to a growing interest in deployable high performance entangled photon-pair sources. This manuscript provides a review of the state-of-the-art bulk-optics-based SPDC sources with continuous wave pump and discusses some of the main considerations when building for deployment.

Practical amplification for a single photon qudit encoded in three degrees of freedom

A single-photon qudit encoded in more than one degree of freedom (DOF) can effectively enlarge a single photon’s capacity and has great potential for applications in future high-capacity quantum communication fields. During the photon transmission in practical noisy channels, photon qudits may suffer from photon transmission loss, which largely limits their application. In this paper, we propose a practical noiseless linear amplification (NLA) protocol for protecting the single-photon qudit encoded in polarization and double-longitudinal momentum DOFs. This NLA adopts the imperfect entangled state generated from a practical spontaneous parametric down-conversion (SPDC) source as the auxiliary state and can be realized under current experimental conditions. After performing the NLA protocol, the fidelity of the target single-photon qudit can be increased and the encoded information in all DOFs can be well preserved. We show the adoption of the imperfect entangled state generated from SPDC source is superior to that of the imperfect single-photon state from practical heralded single-photon source. Our NLA protocol has application potential in current and future quantum communications.

Impact of higher-order optical fiber modes for photon-triplet generation

This paper presents a study of the phasematching properties of the third-order parametric down-conversion process in multimode optical fibers with a step-index profile. Through this process, entangled photon triplets can be generated in the spontaneous regime. We show that phasematching is achieved in a wide range of fiber geometries, provided that the pump field propagates in a higher-order mode. Furthermore, we show the nonlinear coefficient and the absolute emitted flux for each source configuration, evaluated from expressions derived by us in previous theoretical studies concerning the spontaneous and stimulated emission regimes.

Study on a polarization-entangled photon-pair source based on niobium-doped potassium titanyl phosphate

We investigate the high-purity polarization-entangled photon-pair generation in niobium-doped potassium titanyl phosphate (Nb:KTP). The technique is based on Type II spontaneous parametric down-conversion (SPDC). Two kinds of Nb:KTPs with Nb-doping concentrations of 3.4 mol% and 7.5 mol% will be considered in each periodically poled and non-poled case. The properties of Type II SPDC, including the range of the beam propagation direction (or the spectral range of photons) and the corresponding effective nonlinearities and beam walk-offs, will be discussed in detail both theoretically and numerically. This is followed by a joint spectral analysis is followed to quantify the heralded-state spectral purities of the photon pairs generated by Type II SPDC. The results show that photon-pairs can be generated with high purities of 0.995–0.997 with proper pump filtering. We will also show that the spectral positions of photon pairs can be chosen from a wide range, including 1520.0 nm, 1582.4 nm, 1811.6–1837.4 nm, and 1998.6–2026.8 nm.