Parametric Down-conversion Source Research Articles

Experimental Bounds on Classical Random Field Theories

Alternative theories to quantum mechanics motivate important fundamental tests of our understanding and descriptions of the smallest physical systems. Here, using spontaneous parametric downconversion as a heralded single-photon source, we place experimental limits on a class of alternative theories, consisting of classical field theories which result in power-dependent normalized correlation functions. In addition, we compare our results with standard quantum mechanical interpretations of our spontaneous parametric downconversion source over an order of magnitude in intensity. Our data match the quantum mechanical expectations, and do not show a statistically significant dependence on power, limiting quantum mechanics alternatives which require power-dependent autocorrelation functions.

Nonlinear interaction between single photons.

Harnessing nonlinearities strong enough to allow single photons to interact with one another is not only a fascinating challenge but also central to numerous advanced applications in quantum information science. Here we report the nonlinear interaction between two single photons. Each photon is generated in independent parametric down-conversion sources. They are subsequently combined in a nonlinear waveguide where they are converted into a single photon of higher energy by the process of sum-frequency generation. Our approach results in the direct generation of photon triplets. More generally, it highlights the potential for quantum nonlinear optics with integrated devices and, as the photons are at telecom wavelengths, it opens the way towards novel applications in quantum communication such as device-independent quantum key distribution.

Exploring entanglement with the help of quantum state measurement

We have performed a series of experiments using a spontaneous parametric down-conversion source to produce pairs of photons in either entangled or non-entangled polarization states. We determine the full quantum mechanical polarization state of one photon, conditioned on the results of measurements performed on the other photon. For non-entangled states, we find that the measured state of one photon is independent of measurements performed on the other. However, for entangled states, the measured state does depend on the results of measurements performed on the other photon. This is possible because of the nonlocal nature of entangled states. These experiments are suitable for an undergraduate teaching laboratory.

Observation of Quantum Interference in the Plasmonic Hong-Ou-Mandel Effect

We report direct evidence of the bosonic nature of surface plasmon polaritons (SPPs) in a scattering-based beamsplitter. A parametric down-conversion source is used to produce two indistinguishable photons, each of which is converted into a SPP on a metal-stripe waveguide and then made to interact through a semi-transparent Bragg mirror. In this plasmonic analog of the Hong-Ou-Mandel experiment, we measure a coincidence dip with a visibility of 72%, a key signature that SPPs are bosons and that quantum interference is clearly involved.

Characterization of a Spontaneous Parametric Downconversion Source for Use in Single Photon Tests of Quantum Mechanics

Characterization of a Spontaneous Parametric Downconversion Source for Use in Single Photon Tests of Quantum Mechanics

High-visibility nonclassical interference of photon pairs generated in a multimode nonlinear waveguide

We report measurements of two-photon interference using a cw-pumped type-II spontaneous parametric down-conversion source based on a multimode perodically poled potassium titanyl phosphate (PPKTP) waveguide. We have used the recently demonstrated technique of controlling the spatial characteristics of the down-conversion process via intermodal dispersion to generate photon pairs in fundamental transverse modes, thus ensuring their spatial indistinguishability. Good overlap of photon modes within the pairs has been verified using the Hong-Ou-Mandel interferometer and the preparation of polarization entanglement in the Shih-Alley configuration, yielding visibilities consistently above 90%.

On-demand generation of indistinguishable polarization-entangled photon pairs

An on-demand source of indistinguishable and entangled photon pairs is a fundamental component for different quantum information applications such as optical quantum computing, quantum repeaters, quantum teleportation and quantum communication. Parametric down-conversion and four-wave mixing sources of entangled photons have shown high degrees of entanglement and indistinguishability but the probabilistic nature of their generation process also creates zero or multiple photon pairs following a Poissonian distribution. This limits their use in complex algorithms where many qubits and gate operations are required. Here we show simultaneously ultra-high purity (g^(2)(0) < 0.004), high entanglement fidelity (0.81 +/- 0.02), high two-photon interference non-post selective visibilities (0.86 +/- 0.03 and 0.71 +/- 0.04) and on-demand generation of polarization-entangled photon pairs from a single semiconductor quantum dot. Through a two-photon resonant excitation scheme, the biexciton population is deterministically prepared by a Pi-pulse. Applied on a quantum dot showing no exciton fine structure splitting, this results in the deterministic generation of indistinguishable entangled photon pairs.

Bright integrated photon-pair source for practical passive decoy-state quantum key distribution

We report on a bright, nondegenerate type-I parametric down-conversion source, which is well suited for passive decoy-state quantum key distribution. We show the photon-number-resolved analysis over a broad range of pump powers and we prove heralded higher-order $n$-photon states up to $n=4$. The inferred photon click statistics exhibit excellent agreements to the theoretical predictions. From our measurement results we conclude that our source meets the requirements to avert photon-number-splitting attacks.

A monolithic polarization-independent frequency-filter system for filtering of photon pairs

We set up a long-term stable filtering system that consists of cascaded monolithic Fabry-Pérot filters to enhance the suppression and free spectral range. An effective free spectral range of hundreds of GHz allows the system to be used as a high resolution monochromator, with a linewidth of 192 MHz. As an important application a single mode is filtered from photon pairs generated by a parametric down-conversion source, and their indistinguishability is proven by measuring the Hong-Ou-Mandel effect with a visibility of 96%. We report that undesired birefringence, which is often encountered with monolithic cavities, can be avoided by stress-free mounting.

Multiplexing photons with a binary division strategy

We present a scheme to produce clock-synchronized photons from a single parametric downconversion source with a binary division strategy. The time difference between a clock and detections of the herald photons determines the amount of delay that must be imposed to a photon by actively switching different temporal segments, so that all photons emerge from the output with their wavepackets temporally synchronized with the temporal reference. The operation is performed using a binary division configuration which minimizes the passages through switches. Finally, we extend this scheme to the production of many synchronized photons and find expressions for the optimal amount of correction stages as a function of the pair generation rate and the target coherence time. Our results show that, for the generation of this heralded single-photon per output state at an optimized input photon flux, the output rate of our scheme scales essentially with the reciprocal of the target output photon number. With current technology, rates of up to 104 synchronized pairs per second could be observed with only 7 correction stages.

Direct observation of the degree of correlations using photon-number-resolving detectors

Optical parametric down-conversion is a common source for the generation of nonclassical correlated photonic states. Using a parametric down-conversion source and photon-number-resolving detectors, we measure the two-mode photon-number distribution of up to 10 photons for different degrees of correlation. The degree of correlation is controlled by collecting different spatial and spectral single modes for each polarization and varying the amount of spectral and spatial overlap between them. Clear evidence for photon-number correlations is presented despite detector imperfections such as low detection efficiency and other distorting effects. Two criteria, derived directly from the raw data, are shown to be good measures for the degree of correlation. Additionally, using a fitting technique, we find a connection between the measured photon-number distribution and the degree of correlation of the reconstructed original two-mode state. These observations are only possible as a result of the detection of high photon number events.

Capacitive readout and gating of superconducting single photon detectors

We propose and develop a readout scheme for superconducting single-photon detectors based on an integrated circuit, relaxing the need for large bandwidth amplification and resulting in voltage steps proportional to the number of detected photons. We also demonstrate time gating, to filter scattered light in time and reduce dark counts. This could lead to a higher signal-to-noise ratio. The gate pulse is generated on the detection of a photon created by a spontaneous parametric down-conversion source, heralding the presence of a second photon. These two schemes could find applications within advanced multi-array imaging detection systems.

An efficient integrated two-color source for heralded single photons

We present a pulsed and integrated, highly non-degenerate parametric down-conversion (PDC) source of heralded single photons at telecom wavelengths, paired with heralding photons around 800 nm. The active PDC section is combined with a passive, integrated wavelength division demultiplexer on-chip, which allows for the spatial separation of signal and idler photons with efficiencies of more than 96.5%, as well as with multi-band reflection and anti-reflection coatings which facilitate low incoupling losses and a pump suppression at the output of the device of more than 99%. Our device is capable of preparing single photons with efficiencies of 60% with a coincidences-to-accidentals ratio exceeding 7400. Likewise, it shows practically no significant background noise compared to continuous wave realizations. For low pump powers, we measure a conditioned second-order correlation function of g(2) = 3.8 × 10−3, which proves almost pure single-photon generation. In addition, our source can feature a high brightness of 〈npulse〉 = 0.24 generated photon pairs per pump pulse at pump power levels below 100 μW. The high quality of the pulsed PDC process in conjunction with the integration of highly efficient passive elements makes our device a promising candidate for future quantum networking applications, where an efficient miniaturization plays a crucial role.

Photon entanglement detection by a single atom

We use a single trapped 40Ca+ ion as a resonant, polarization-sensitive absorber to detect and characterize the entanglement of tunable narrowband photon pairs from a spontaneous parametric down-conversion source. Single-photon absorption is marked by a quantum jump in the ion and heralded by coincident detection of the partner photon. For three polarization basis settings of the absorption and detection of the herald, we find maximum coincidences always for orthogonal polarizations. The polarization entanglement is further evidenced by tomographic reconstruction of the biphoton quantum state with an overlap fidelity of 93% with the Bell singlet state. This is an essential step toward a single-ion based quantum memory for photonic entanglement.

Optimal photon-pair single-mode coupling in narrow-band spontaneous parametric downconversion with arbitrary pump profile

A theoretical investigation of the performance of single-mode coupled spontaneous parametric downconversion sources is proposed, which only requires very few assumptions of practical interest: quasi-degenerate collinear generation and narrow bandwidth obtained through spectral filtering. Other assumptions, such as pump-beam spatial and temporal envelopes, target single-mode profile and size, and nonlinear susceptibility distribution, are only taken into account in the final step of the computation, thus making the theory general and flexible. Figures of merit for performance include absolute coupled brightness and conditional coupling efficiency. Their optimization is investigated using functions that only depend on dimensionless parameters, so that the results provide the best experimental configuration for a whole range of design choices (e.g., crystal length, pump power, etc.). A particular application of the theory is validated by an experimental optimization obtained under compatible assumptions. A comparison with other works and proposals for numerically implementing the theory under less stringent assumptions is also provided.

Event-by-event simulation of nonclassical effects in two-photon interference experiments

A corpuscular simulation model for second-order intensity interference phenomena is discussed. It is shown that both the visibility predicted for two-photon interference experiments with two independent sources and the visibility predicted for two-photon interference experiments with a parametric down-conversion source can be explained in terms of a locally causal, modular, adaptive, corpuscular, classical (non-Hamiltonian) dynamical system. Hence, there is no need to invoke quantum theory to explain the so-called nonclassical effects in the interference of signal and idler photons in parametric down conversion. A revision of the commonly accepted criterion of the nonclassical nature of light is needed.

Proposal for a new scheme for producing a two-photon, high dimensional hyperentangled state

We propose an experimentally feasible scheme for generating a two 2 × 4 × 4 dimensional photon hyperentangled state, entangled in polarization, frequency and spatial mode. This scheme is mainly based on a parametric down-conversion source and cross-Kerr nonlinearities, which avoids the complicated uncertain post-selection. Our method can be easily expanded to the production of hyperentangled states with more photons in multidimensions. Hence the expectation for vast quantities of information in quantum information processing will possibly come true. Finally, we put forward a realizable quantum key distribution (QKD) protocol based on the high dimensional hyperentangled state.

Quantum Storage of Heralded Polarization Qubits in Birefringent and Anisotropically Absorbing Materials

Storage of quantum information encoded into heralded single photons is an essential constituent of long-distance quantum communication based on quantum repeaters and of optical quantum information processing. The storage of photonic polarization qubits is, however, difficult because many materials are birefringent and have polarization-dependent absorption. Here we present a simple scheme that eliminates these polarization effects, and we demonstrate it by storing heralded polarization qubits into a solid-state quantum memory. The quantum memory is implemented with a biaxial yttrium orthosilicate (Y2SiO5) crystal doped with rare-earth ions. Heralded single photons generated from a filtered spontaneous parametric down-conversion source are stored, and quantum state tomography of the retrieved polarization state reveals an average fidelity of 97.5±0.4%, which is significantly higher than what is achievable with a measure-and-prepare strategy.

Limits on the deterministic creation of pure single-photon states using parametric down-conversion

Parametric down-conversion (PDC) is one of the most widely used methods to create pure single-photon states for quantum information applications. However little attention has been paid to higher-order photon components in the PDC process, yet these ultimately limit the prospects of generating single-photons of high quality. In this paper we investigate the impacts of higher-order photon components and multiple frequency modes on the heralding rates and single-photon fidelities. This enables us to determine the limits of PDC sources for single-photon generation. Our results show that a perfectly single-mode PDC source in conjunction with a photon-number resolving detector is ultimately capable of creating single-photon Fock states with unit fidelity and a maximal state creation probability of 25%. Hence an array of 17 switched sources is required to build a deterministic (>99% emission probability) pure single-photon source.

Measurements of the dependence of the photon-number distribution on the number of modes in parametric down-conversion

Optical parametric down-conversion (PDC) is a central tool in quantum optics experiments. The number of collected down-converted modes greatly affects the quality of the produced photon state. We use Silicon Photomultiplier (SiPM) number-resolving detectors in order to observe the photon-number distribution of a PDC source, and show its dependence on the number of collected modes. Additionally, we show how the stimulated emission of photons and the partition of photons into several modes determine the overall photon number. We present a novel analytical model for the optical crosstalk effect in SiPM detectors, and use it to analyze the results.