Optomechanical Applications Research Articles

Analysis and Simulation of the Optical Properties of a Quantum Dot on a Graphene Nanoribbon System

In this work, we theoretically study the optical properties of a graphene nanoribbon with a quantum dot (QD) on it. The system consists of a graphene nanoribbon with dimensions of 400 × 3100 (nm2) and a quantum dot with a nanoscale radius. The quantum dot is symmetrically located at the center of the graphene nanoribbon to simplify the mathematical model. To calculate the optical properties (susceptibility) of the system, a broadband electromagnetic wave (0.5–2.5 μm) is applied to the structure to model dipole-dipole interaction. Considering the input field and calculating the total induced polarization, the optical susceptibility of the system is calculated. The applied electromagnetic field excites the surface plasmon on the graphene nanoribbon and the excitons of QDs. The induced dipoles in the graphene nanoribbon and the QD will interact with each other. We show that the parameters of both materials strongly influence dipole-dipole interaction. In particular, the effect of QDs (location on graphene and radius) on the optical properties of the considered system was studied. The obtained results can be used to introduce periodic optical structures in nanoscale by inserting QDs in a periodic array on graphene nanoribbon. Additionally, applications such as reflectors, couplers, and wavelength filters can be designed. Considering the presented theoretical framework, we can describe all the optoelectronic and optomechanical applications of complex nanoscale graphene and QD systems.

Polarization-independent optical spatial differentiation with a doubly-resonant one-dimensional guided-mode grating.

We report on the design and experimental characterization of a suspended silicon nitride subwavelength grating possessing a polarization-independent guided-mode resonance at oblique incidence. At this resonant wavelength we observe that the transverse intensity profile of the transmitted beam is consistent with a first-order spatial differentiation of the incident beam profile in the direction of the grating periodicity, regardless of the incident light polarization. These observations are corroborated by full numerical simulations. The simple one-dimensional and symmetric design, combined with the thinness and excellent mechanical properties of these essentially loss-free dieletric films, is attractive for applications in optical processing, sensing and optomechanics.

Single-mode, single-polarization and dispersion-flattened waveguides based on silicon carbide and diamond

Fundamental properties of an optical waveguide are mainly related to its guided modes and associated loss, dispersion, polarization and nonlinearity. Single-mode and single-polarization waveguiding has long been of interest, i.e., so-called truly single mode. We propose SiC- and diamond-based waveguides, which are truly single-mode and simultaneously dispersion-flattened. This is preferred for broadband nonlinear applications, such as octave-spanning supercontinuum and frequency comb generation. An ultra-low and flat dispersion profile with four zero-dispersion wavelengths (ZDWs) can be obtained over an octave-spanning bandwidth from 1.8 to 3.6 μm. Meanwhile, only TE00 mode is supported in the proposed waveguide over the low-dispersion bandwidth. Scattering loss of the waveguide is greatly reduced by 8.6 times, compared to a standard strip waveguide. Fabrication of the proposed waveguide is easier than previous dispersion-tailored waveguides, without dry etching SiC and diamond. It is expected that the proposed waveguides can find applications in nonlinear photonics, optomechanics and quantum optics.

Electromechanical feedback control of nanoscale superflow

Superfluid 4He is a promising material for optomechanical and electromechanical applications due to its low acoustic loss. Some of the more intriguing aspects of superfluidity—the macroscopic coherence, topological nature of vorticity, and capability of supporting non-classical flows—remain, however, poorly explored resources in opto- and electro-mechanical systems. Here, we present an electromechanical coupling to pure superflow inside a nanofluidic Helmholtz resonator with viscously clamped normal fluid. The system is capable of simultaneous measurement of displacement and velocity of the Helmholtz mechanical mode weakly driven by incoherent environmental noise. Additionally, we implement feedback capable of inducing self-oscillation of the non-classical acoustic mode, damping the motion below the ambient level, and tuning of the mode frequency.

Collimation and finite-size effects in suspended resonant guided-mode gratings.

The optical transmission of resonant guided-mode gratings patterned on suspended silicon nitride thin films and illuminated at normal incidence with a Gaussian beam is investigated both experimentally and theoretically. Effects due to the beam focusing and its finite size are accounted for by a phenomenological coupled-mode model whose predictions are found to be in very good agreement with the experimentally measured spectra for various grating structures and beam sizes, and which allow for a detailed analysis of the respective magnitude of these effects. These results are highly relevant for the design and optimization of such suspended structured films that are widely used for photonics, sensing, and optomechanics applications.

Tunable Optical Diffusers Based on the UV/Ozone-Assisted Self-Wrinkling of Thermal-Cured Polymer Films.

Tunable optical diffusers have attracted attention because of the rapid development of next generation stretchable optoelectronics and optomechanics applications. Flexible wrinkle structures have the potential to change the light path and tune the diffusion capability, which is beneficial to fabricate optical diffusers. The generation of wrinkles usually depends on an external stimulus, thus resulting in complicated fabricating equipment and processes. In this study, a facile and low-cost method is proposed to fabricate wrinkle structures by the self-wrinkling of thermal-cured polymer for tunable optical diffusers. The uncured polydimethylsiloxane (PDMS) precursors were exposed to UV/ozone to obtain hard silica layers and then crosslinked via heating to induce the wrinkle patterns. The wrinkle structures were demonstrated as strain-dependent tunable optical diffusers and the optical diffusion of transmitted light via the deformable wrinkle structures was studied and adjusted. The incident light isotropically diffused through the sample at the initial state. When the wrinkle structures deformed, it showed a more pronounced isotropic optical diffusion with uniaxial tensile strain. The optical diffusion is anisotropical with a further increase in uniaxial tensile strain. The proposed method of fabricating wrinkles by UV/ozone-assisted self-wrinkling of thermal-cured polymer films is simple and cost-effective, and the obtained structures have potential applications in tunable optical diffusers.

Fabrication of Photonic Resonators in Bulk 4H‐SiC

AbstractThe design and engineering of photonic architectures, suitable to enhance, collect and guide light on chip is needed for applications in quantum photonics and quantum optomechanics. In this work, a Faraday cage‐based oblique angle etch method is applied to fabricate various functional photonic devices from 4H Silicon Carbide (SiC)—a material that has attracted attention in recent years, due to its potential in optomechanics, nonlinear optics, and quantum information. The processing conditions are detailed and the geometrical and optical characteristics of the fabricated devices are thoroughly addressed. Employing photoluminescence measurements high‐quality factors are demonstrated for suspended microring resonators of up to 3500 in the visible range. Such devices will be applicable in the future to augment the properties of SiC in integrated on chip quantum photonics.

Experimental localisation of quantum entanglement through monitored classical mediator

Quantum entanglement is a form of correlation between quantum particles that cannot be increased via local operations and classical communication. It has therefore been proposed that an increment of quantum entanglement between probes that are interacting solely via a mediator implies non-classicality of the mediator. Indeed, under certain assumptions regarding the initial state, entanglement gain between the probes indicates quantum coherence in the mediator. Going beyond such assumptions, there exist other initial states which produce entanglement between the probes via only local interactions with a classical mediator. In this process the initial entanglement between any probe and the rest of the system "flows through" the classical mediator and gets localised between the probes. Here we theoretically characterise maximal entanglement gain via classical mediator and experimentally demonstrate, using liquid-state NMR spectroscopy, the optimal growth of quantum correlations between two nuclear spin qubits interacting through a mediator qubit in a classical state. We additionally monitor, i.e., dephase, the mediator in order to emphasise its classical character. Our results indicate the necessity of verifying features of the initial state if entanglement gain between the probes is used as a figure of merit for witnessing non-classical mediator. Such methods were proposed to have exemplary applications in quantum optomechanics, quantum biology and quantum gravity.

Nonsuspended optomechanical crystal cavities using As2S3 chalcogenide glass

An optomechanical crystal cavity with nonsuspended structure using As 2 S 3 material is proposed. The principle of mode confinement in the nonsuspended cavity is analyzed, and two different types of optical and acoustic defect modes are calculated through appropriate design of the cavity structure. An optomechanical coupling rate of 82.3 kHz is obtained in the proposed cavity, and the designed acoustic frequency is 3.44 GHz. The acoustic mode coupling between two nonsuspended optomechanical crystal cavities is also demonstrated, showing that the proposed cavity structure has great potential for realizing further optomechanical applications in multicavity systems.

Low-loss and high-resolution mechanical mode tuning in microspheres.

Lack of tunability impedes the wide application of optomechanical systems; however, little research exists on mechanical frequency tuning. Herein, ultra-fine low-loss dynamical mechanical frequency tuning is achieved by compressing a microsphere along the axial direction. The tuning resolution reaches approximately 4% of the mechanical linewidth, and the variation range of the mechanical quality factor (Qm) is within 2.9% of the untouched Qm. The roles of geometric deformation, spring effect, and stiffness were also evaluated through simulation and experimental analysis. Furthermore, sine function modulation was displayed, with a Pearson coefficient exceeding 99.3%, to achieve arbitrary-function mechanical resonance tuning. This method paves the way for scalable optomechanical applications, such as mechanical vibration synchronization or optomechanics-based optical wavelength conversion.

Mode Localization and Eigenfrequency Curve Veerings of Two Overhanged Beams.

Overhang provides a simple but effective way of coupling (sub)structures, which has been widely adopted in the applications of optomechanics, electromechanics, mass sensing resonators, etc. Despite its simplicity, an overhanging structure demonstrates rich and complex dynamics such as mode splitting, localization and eigenfrequency veering. When an eigenfrequency veering occurs, two eigenfrequencies are very close to each other, and the error associated with the numerical discretization procedure can lead to wrong and unphysical computational results. A method of computing the eigenfrequency of two overhanging beams, which involves no numerical discretization procedure, is analytically derived. Based on the method, the mode localization and eigenfrequency veering of the overhanging beams are systematically studied and their variation patterns are summarized. The effects of the overhang geometry and beam mechanical properties on the eigenfrequency veering are also identified.

Modified Stoney’s equation with anisotropic substrates undergoing large deformations

Thin film deposition is a key fabrication step in several opto-mechanical and electronics applications. For instance, thin film coatings can act as reflective interfaces, protective coatings or they can be used to modify the thermal behavior of the film-substrate system. For effective design, it is important to understand the deformation of the system in response to residual stresses during thin film deposition. The widely used Stoney’s equation to measure this deformation assumes isotropic elasticity of the substrate together with infinitesimal strains and rotations. In this work we relax both constraints, where we study the deformation of commonly used substrates made of single crystal Si(001) and Si(111) wafers that undergo large rotations. We derive relations between normalized substrate curvature and thin film mismatch strain and validate our analysis with numerical results. The methodology presented can be used for more accurate understanding of a broad range of film-substrate systems in semiconductors.

Colossal switchable photocurrents in topological Janus transition metal dichalcogenides

Nonlinear optical properties, such as bulk photovoltaic effects, possess great potential in energy harvesting, photodetection, rectification, etc. To enable efficient light–current conversion, materials with strong photo-responsivity are highly desirable. In this work, we predict that monolayer Janus transition metal dichalcogenides (JTMDs) in the 1T′ phase possess colossal nonlinear photoconductivity owing to their topological band mixing, strong inversion symmetry breaking, and small electronic bandgap. 1T′ JTMDs have inverted bandgaps on the order of 10 meV and are exceptionally responsive to light in the terahertz (THz) range. By first-principles calculations, we reveal that 1T′ JTMDs possess shift current (SC) conductivity as large as 2300 nm μA V−2, equivalent to a photo-responsivity of 2800 mA/W. The circular current (CC) conductivity of 1T′ JTMDs is as large as ∼104 nm μA V−2. These remarkable photo-responsivities indicate that the 1T′ JTMDs can serve as efficient photodetectors in the THz range. We also find that external stimuli such as the in-plane strain and out-of-plane electric field can induce topological phase transitions in 1T′ JTMDs and that the SC can abruptly flip their directions. The abrupt change of the nonlinear photocurrent can be used to characterize the topological transition and has potential applications in 2D optomechanics and nonlinear optoelectronics.

Single-Phonon Addition and Subtraction to a Mechanical Thermal State.

Adding or subtracting a single quantum of excitation to a thermal state of a bosonic system has the counter-intuitive effect of approximately doubling its mean occupation. We perform the first experimental demonstration of this effect outside optics by implementing single-phonon addition and subtraction to a thermal state of a mechanical oscillator via Brillouin optomechanics in an optical whispering-gallery microresonator. Using a detection scheme that combines single-photon counting and optical heterodyne detection, we observe this doubling of the mechanical thermal fluctuations to a high precision. The capabilities of this joint click-dyne detection scheme adds a significant new dimension for optomechanical quantum science and applications.

Recent Advances in Single Crystal Diamond Device Fabrication for Photonics, Sensing and Nanomechanics.

In the last two decades, the use of diamond as a material for applications in nanophotonics, optomechanics, quantum information, and sensors tremendously increased due to its outstanding mechanical properties, wide optical transparency, and biocompatibility. This has been possible owing to advances in methods for growth of high-quality single crystal diamond (SCD), nanofabrication methods and controlled incorporation of optically active point defects (e.g., nitrogen vacancy centers) in SCD. This paper reviews the recent advances in SCD nano-structuring methods for realization of micro- and nano-structures. Novel fabrication methods are discussed and the different nano-structures realized for a wide range of applications are summarized. Moreover, the methods for color center incorporation in SCD and surface treatment methods to enhance their properties are described. Challenges in the upscaling of SCD nano-structure fabrication, their commercial applications and future prospects are discussed.

Optimisation and scaling effect of dual-waveguide optical trapping in the SOI platform.

Optical trapping has potential applications in biological manipulation, particle trapping, Raman spectroscopy, and quantum optomechanics. Among the various optical trapping schemes, on-chip dual-waveguide traps combine benefits of stable trapping and mass production. However, no systematic research has been conducted to optimise on-chip dual-waveguide traps so that the trapping capability is maximised. Here, a numerical simulation of an on-chip silicon on insulator (SOI) dual-waveguide optical trap based on Lumerical FDTD Solutions is carried out to optimise the on-chip dual-waveguide trap. It was found that the waveguide thickness is a crucial parameter when designing a dual-waveguide trap, and its optical trapping capability largely depends on the distance between the two waveguides. We show that the optimal waveguide thickness to achieve the maximum trapping capability generally increases with the gap distance, accompanied by a periodic feature due to the interference and the resonant effects within the gap. This optimal waveguide thickness and gap distance are analysed to have clear scaling effects over the input optical wavelength, which paves the way for the design and optimisation of dual-waveguide traps for various applications.

Optical Rotation and Thermometry of Laser Tweezed Silicon Nanorods.

Optical rotation of laser tweezed nanoparticles offers a convenient means for optical to mechanical force transduction and sensing at the nanoscale. Plasmonic nanoparticles are the benchmark system for such studies, but their rapid rotation comes at the price of high photoinduced heating due to Ohmic losses. We show that Mie resonant silicon nanorods with characteristic dimensions of ∼220 × 120 nm2 can be optically trapped and rotated at frequencies up to 2 kHz in water using circularly polarized laser light. The temperature excess due to heating from the trapping laser was estimated by phonon Raman scattering and particle rotation analysis. We find that the silicon nanorods exhibit slightly improved thermal characteristics compared to Au nanorods with similar rotation performance and optical resonance anisotropy. Altogether, the results indicate that silicon nanoparticles have the potential to become the system of choice for a wide range of optomechanical applications at the nanoscale.

Mechanical reinforcement of polymer colloidal crystals by supercritical fluids

Colloidal crystals realized by self-assembled polymer nanoparticles have prominent attraction as a platform for various applications from assembling photonic and phononic crystals, acoustic metamaterials to coating applications. However, the fragility of these systems limits their application horizon. In this work the uniform mechanical reinforcement and tunability of 3D polystyrene colloidal crystals by means of cold soldering are reported. This structural strengthening is achieved by high pressure gas (N2 or Ar) plasticization at temperatures well below the glass transition. Brillouin light scattering is employed to monitor in-situ the mechanical vibrations of the crystal and thereby determine preferential pressure, temperature and time ranges for soldering, i.e. formation of physical bonding among the nanoparticles while maintaining the shape and translational order. This low-cost method is potentially useful for fabrication and tuning of durable devices including applications in photonics, phononics, acoustic metamaterials, optomechanics, surface coatings and nanolithography.

Large visible-light-driven photostriction in Bi(Ni2/3Nb1/3)O3–PbTiO3 ferroelectrics

Photostrictive effect that has been discovered for over half a century is getting renewed interest in recent years in view of the great potentials for optomechanical applications. Ferroelectric materials represented by lead lanthanum zirconated titanate have been widely studied in this field because of their relatively large photostriction and fast photoresponse, but their wide bandgaps with limit response to visible light hinder further practical application. Here, visible-light-driven photostrictions of the order of 10−3 are discovered in Bi(Ni2/3Nb1/3)O3–PbTiO3 (BNNPT) ferroelectric solid solutions. Three BNNPT compositions with different phase structures, exhibiting notably different piezoelectric and photovoltaic properties, are selected to conduct the photostriction investigation, and their analogous photostrictive behaviors contradict with previous acknowledgment that the photostriction of ferroelectrics originates from the photovoltage-induced inverse piezoresponse. The nonuniform shifts of the XRD diffraction peaks under external laser illumination and the redshifts of the laser power dependent Raman modes disclose that the photostriction is mainly attributed to the light-induced distortion of BO6 octahedra. This study sheds insight into the mechanism of the photostriction of ferroelectrics.

S-band delay lines in suspended lithium niobate

Thin-film lithium niobate is an attractive platform for GHz-frequency applications in low-power RF analog signal processing, optomechanics, and quantum devices due to its high coupling, low loss, excellent optical properties, and compatibility with superconducting quantum circuits. We demonstrate aluminum interdigitated transducers (IDTs) in this platform for horizontal shear (SH) waves between 1.2 and 3.3 GHz and longitudinal waves between 2.1 and 5.4 GHz. For the SH waves, we measure a piezoelectric coupling coefficient of 13% and 6.0 dB/mm propagation losses in delay lines up to 1.2 mm with a 300 ns delay in air at room temperature. In these high keff2 transducers, electrical loading gives rise to large reflections and resonances. Finite element method models and an experimental finger-pair sweep are used to characterize the role of resonance in these transducers, illuminating the physics behind the large motional admittances of these small-footprint IDTs.