Optical Manipulation Research Articles

Optically controllable deformation and phase change in VO2/Si3N4/Au hybrid nanostructures with polarization selectivity

Optically spatial displacement and material modification hold great potential for the appealing applications in nanofabrication and reconfiguration of functional optical devices. Here, we propose and demonstrate a scheme to achieve simultaneous deformation and phase change in vanadium dioxide (VO2)/Si3N4/Au hybrid nanostructures by laser stimuli. Low triggering threshold and significant deformation characteristics of VO2, based on controllable phase transition, are demonstrated in microscale cantilevers. The plasmonic properties of the nanostructure array are further utilized to achieve a polarization-selective dynamic response. The persistence of deformation and dynamical optical modulation are further demonstrated. Such high-precision fabrication methods and non-contact reconfiguration methods are useful for future applications in dynamic optical manipulation.

Dynamical characteristics of tightly focused flat-topped double vortex beam for enhanced optical manipulation

The Flat-topped Vortex (FTV) beam has shown remarkable utility in a diverse range of industrial procedures, primarily attributed to its central intensity plateau. Nevertheless, the substantial potential of the FTV beam in particle trapping and manipulation has been largely underappreciated. In this work, we conducted the first study on the focusing properties and dynamic characteristics of the Flat-topped double vortex (FTDV) beam under different polarization for the absorption of Rayleigh particles. Through superimposing linearly two FTV beams with equal but opposite topological charges, the FTDV beam emerged naturally. Moreover, a comprehensive numerical analysis was subsequently performed to decode the interactions between the focusing field of the FTDV beam and Rayleigh particles. The analysis demonstrated that the focusing field of FTDV beam can perform multi-particle capture and effectively manipulate particles by modulating the topological charge |m|, the flatness order n, and the polarization state of the FTDV. Furthermore, a comparison between the focusing field of FTDV beam with that of vector vortex (VV) beam revealed that the FTDV beam was capable to generate spin angular momentum (SAM) density and spin torque at least an order of magnitude higher. These findings highlight the superior capabilities of FTDV beam in optical manipulation, and provide essential theoretical support for its utilization in particle capture and management.

Optical manipulation based on fusion spliced all-fiber optical tweezers

Optical manipulation based on fusion spliced all-fiber optical tweezers

Coupling of photonic topological states and their dynamical control based on liquid crystal

Optical field manipulation inspired by topology theory has recently drawn great research attention in nanophotonic. For flexible and programmable light management, the capacity to dynamically regulate the photonic topological states in fixed optical artificial microstructures is essential. Here, we propose a dynamic light manipulation of a two-dimensional (2D) photonic lattice aided by liquid crystals, which is composed of all-dielectric photonic crystals with distinct topological phases. In brief, by submerging the well-designed photonic lattice into a liquid crystal (LC), the topological edge and corner states can be actively modulated by applying external bias voltage, which offers an electrically switchable tuning capability, enabling the coupling between higher-order topological states in a structurally deterministic photonic structure. As a proof-of-principle, we use the 1D topological edge states and 0D topological corner states in one sample, respectively, to mimic line-waveguides and corner-cavities, and demonstrate their selective couplings with Fano-like profile driven by electric bias. Our work offers an effective and flexible way for light control in the potential active topological photonic devices.

Mode-Symmetry-Assisted Optical Pulling by Bound States in the Continuum.

Aside from optical pushing and trapping that have been implemented successfully, the transportation of objects backward to the source by the optical pulling forces (OPFs) has attracted tremendous attention, which was usually achieved by increasing the forward momentum of light. However, the limited momentum transfer between light and object greatly constrains the amplitudes of OPFs. Here, we present a mechanism to generate strong interactions between object and background through the bound states in the continuums, which can generate large OPFs without increasing the forward momentum of light. The underlying physics is the extraction of momentum from the designed background lattice units assisted by mode symmetry. This work paves the way for extraordinary optical manipulations and shows great potential for exploring the momenta of light in media.

Controllable multi-autofocusing of chirped multi-Pearcey beams and their trapping performance on Rayleigh particles

The exploration of structured light created through autofocusing beams has attracted widespread attention in optical manipulation. Here, we investigate the propagation dynamics of chirped multi-Pearcey beams (CMPBs) in theory and experiment, especially exploring the impact of chirped factors on the autofocusing characteristics of CMPBs. It is found that the autofocusing characteristics of the beams can be significantly modulated by introducing first-order and second-order chirped factors. Specifically, the first-order chirped factor greatly improves the autofocusing coefficient of CMPBs, while the second-order chirped factor introduces multiple autofocusing propagations. By analyzing the transverse power flow of CMPBs both without and with chirped factors, we explain why the chirped factors can remarkably strengthen the autofocusing performance of CMPBs. Finally, our theoretical analysis on trapping force on Rayleigh particles indicates that the introduction of chirped factors optimizes the intensity gradient and trapping capability of CMPBs, potentially enabling multiple longitudinal trapping positions. These findings offer a comprehensive insight into the propagation dynamics of CMPBs, opening avenues for flexible optical manipulation of multiple particles.

Dynamic control of optical skyrmions in cylindrical waveguide

In recent times, the optical skyrmions have received an increasing amount of interest owing to its applications in optical manipulation, super-resolution imaging and microscopy, quantum technologies. However, few studies are focused on the dynamic control of optical skyrmions. It is found that Neel-type photonic skyrmions were discovered in evanescent electromagnetic waves. Here, we find the Bloch-type skyrmions in a three-dimensional cylindrical waveguide. By modulating the amplitude ratio of two incident vortex beams, the new types of skyrmions such as Twisted-type skyrmions and Planar-type skyrmions can be found. Further more, we have also achieved arbitrary modulation ratios of internal spin components. It is believed that our findings greatly enrich the types of photonic skyrmions and provide a method to freely control the photonic skyrmions.

Diarylethene derivative photoionization control via two-color two-laser optical manipulation in the presence of cyclodextrins

In this study, the photodynamics of 1,2-bis(2,4-dimethyl-5-phenyl-3-thienyl)-3,3,4,4,5,5-hexafluoro-1-cyclopentene (DE) was investigated in the presence of α-, β- and γ-cyclodextrin (CD) inclusion complexes and under the influence of one- and two-laser excitations. Thus, this study aimed to elucidate the ionization quantum yield of DE and how it is affected by the type of CD and laser configuration. Specifically, DE/CD was flash photolyzed using a single laser (355 nm) or a double laser (355 nm and 532 nm) and observed at a wavelength of 720 nm to examine the transient absorption of hydrated electrons. The ionization efficiency with the two lasers was found to exceed that with the single laser. This suggests the existence of a two-step process involving S0→S1 and S1→Sn singlet transitions in the two-photon ionization (TPI) of DE. Furthermore, when the ring-closing isomer of DE was initiated via laser irradiation at 532 nm, the photoionization efficiency increased, especially in the presence of γ-CD. This implies that the 532-nm irradiation, which is not directly involved in TPI, contributed to promoting the TPI of DE, thus increasing its photo-steady state (saturation). Thus, the possibility of using CD-containing lasers to control photochemical reactions with photo-steady state processes was demonstrated. This investigation contributes to a broader understanding of the potential applications and underlying mechanisms of photochromic materials influenced by multi-laser interactions.

Controllable optical tweezer and spanner in evanescent fields via a single plasmonic metasurface

A dual-functional plasmonic metasurface is proposed to realize trapping and rotation of microparticles in evanescent fields by simply changing the polarization of incident light. The metasurface is constituted with subwavelength rectangular nanoslit that is perforated in an Au film on the glass substrate. Simulated near-field intensity distributions show that surface plasmon vortex with designed topological charge and focused point with enhanced intensity can be controllably generated in the center region of the designed metasurface by different circularly polarized lights. Calculated optical force and optical potential on a polystyrene sphere further demonstrate the good performances of rotating and trapping a microparticle with the generated vortex and focused surface plasmon polaritons. Moreover, two examples designed with different topological charges demonstrate the flexibility of these metasurfaces in tuning the rotation radius of microparticles. The advantages of the proposed metasurface in design flexibility, multifunctionality, and small size may provide new possibilities for applications of integrated optical manipulation devices and systems.

Amorphous to Crystalline Phase Transformation Enables Tunable Persistent Luminescence for Multi‐Mode Optical Information Storage

AbstractMulti‐mode luminescence tuning through in situ crystallization of topological glass holds significance for photonics applications. Here, NaAlSiO4:Eu2+‐based glass ceramics are presented as stable persistent luminescence (PersL) materials by controlling the phase transformation in Eu2+ doped Na2O‐Al2O3‐SiO2 from amorphous glass to crystalline nepheline phase. X‐ray and UV excited PersL colors from blue to yellow are realized by adjusting the crystallization duration time, and trap statuses reveal the dynamic PersL process with a trap redeployment from 0.83 to 1.09 eV during the transformation. Optical information storage model is constructed with a structure of stacked emitting layers to enhance storage capacity. X‐ray excited luminescence time‐lapse imaging is further demonstrated with optical memory longer than 5 days. These findings advance the development of superior stable PersL glass ceramics and offer optical manipulation tactics for multi‐mode optical information storage applications.

Switchable dual-functional optical vortex manipulation via cylindrical phase-change metagratings

Subwavelength artificial engineering microstructures, such as metasurfaces and metagratings, can realize superior optical properties that many natural materials cannot finish. However, most functionalities achieved are mostly single and fixed. The appearance of phase-change materials makes it possible to extend the functions of metagratings. Here, we propose and demonstrate a structural design of cylindrical phase-change metagratings based on VO2, which can achieve switchable dual-functional optical vortex manipulation in the terahertz range. Specifically, by excitation of the temperature-sensitive metallic and insulating states of VO2, the simple two-dimensional cylindrical gear-like structure can achieve dual-functionality for vortex waves with orbital angular momentum, namely efficient retroreflection and near-perfect absorption. In addition, we also discussed the influence of the gear-like structure dimensions on the transmissivity and absorptivity of dual-function vortex wave manipulation. This work provides a simple and effective approach for the tunable and multifunctional control of vortex waves in subwavelength artificial devices, with potential applications in automated device design and terahertz (THz) communications.

Ultracold LiCr : A New Pathway to Quantum Gases of Paramagnetic Polar Molecules

Quantum gases of doubly polar molecules represent appealing frameworks for a variety of cross-disciplinary applications, encompassing quantum simulation and computation, controlled quantum chemistry, and precision measurements. Through a joint experimental and theoretical study, here we explore a novel class of ultracold paramagnetic polar molecules combining lithium alkali and chromium transition metal elements. Focusing on the specific bosonic isotopologue 6Li53Cr, leveraging on the Fermi statistics of the parent atomic mixture and on suitable Feshbach resonances recently discovered, we produce up to 50×103 ultracold LiCr molecules at peak phase-space densities exceeding 0.1, prepared within the least bound rotationless level of the LiCr electronic ground state X6Σ+. By also developing new probing methods, we thoroughly characterize the molecular gas, demonstrating the paramagnetic nature of LiCr dimers and the precise control of their quantum state. We investigate their stability against inelastic processes and identify a parameter region where pure LiCr samples exhibit lifetimes exceeding 0.2 s. Parallel to this, we employ state-of-the-art quantum chemical calculations to accurately predict the properties of LiCr ground and excited electronic states. This model, able to reproduce the experimental Li-Cr high-spin, scattering length, allows us to identify both efficient paths to coherently transfer weakly bound LiCr dimers to their absolute ground state, and suitable transitions for their subsequent optical manipulation. Our studies establish Li-Cr as a prime candidate to realize ultracold gases of doubly polar molecules with significant electric (3.3 D) and magnetic (5μB) dipole moments. Published by the American Physical Society 2024

Optical manipulation of the charge-density-wave state in RbV3Sb5.

Broken time-reversal symmetry in the absence of spin order indicates the presence of unusual phases such as orbital magnetism and loop currents1-4. The recently discovered kagome superconductors AV3Sb5 (where A is K, Rb or Cs)5,6 display an exotic charge-density-wave (CDW) state andhave emerged as astrong candidate for materialshosting a loop currentphase. The idea that the CDW breaks time-reversal symmetry7-14 is, however, being intensely debated due to conflicting experimental data15-17. Here we use laser-coupled scanning tunnelling microscopy to study RbV3Sb5. By applying linearly polarized light along high-symmetry directions, we show that the relative intensities of the CDW peaks can be reversibly switched, implying a substantial electro-striction response, indicative of strong nonlinear electron-phonon coupling. A similar CDW intensity switching is observed with perpendicular magnetic fields, which implies an unusual piezo-magnetic response that, in turn, requires time-reversal symmetry breaking. We show that the simplest CDW that satisfies these constraints is an out-of-phase combination of bond charge order and loop currents that we dub a congruent CDW flux phase. Our laser scanning tunnelling microscopy data open the door to the possibility of dynamic optical control of complex quantum phenomenon in correlated materials.

Dynamically crosslinked chiral optics sensing for ultra-sensitive VOCs detection

Chiroptical sensing with real-time colorimetrical detection has been emerged as quantifiable properties, enantioselective responsiveness, and optical manipulation in environmental monitoring, food safety and other trace identification fields. However, the sensitivity of chiroptical sensing materials remains an immense challenge. Here, we report a dynamically crosslinking strategy to facilitate highly sensitive chiroptical sensing material. Chiral nematic cellulose nanocrystals (CNC) were co-assembled with amino acid by a two-step esterification, of which a precisely tunable helical pitch, a unique spiral conformation with hierarchical and numerous active sites in sensing performance could be trigged by dynamic covalent bond on amines. Such a CNC/amino acid chiral optics features an ultra-trace amount of 0.08 mg/m3 and a high sensitivity of 60 nm/(mg/m3) for formaldehyde gas at a molecule level detection, which is due to the three synergistic adsorption enhancement of dynamic covalent bonded interaction, hydrogen bonded interaction and van der Waals interaction. Meanwhile, an enhancement hierarchical adsorption of CNC/amino acid chiral materials can be readily representative to the precise helical pitch and colorimetrical switch for sensitive visualization reorganization.

A Cocaine-Activated Ensemble Exerts Increased Control Over Behavior While Decreasing in Size

BackgroundSubstance use disorder is characterized by long-lasting changes in reward-related brain regions, such as the nucleus accumbens. Previous work has shown that cocaine exposure induces plasticity in broad, genetically defined cell types in the nucleus accumbens; however, in response to a stimulus, only a small percentage of neurons are transcriptionally active—termed an ensemble. Here, we identify an Arc-expressing neuronal ensemble that has a unique trajectory of recruitment and causally controls drug self-administration after repeated, but not acute, cocaine exposure. MethodsUsing Arc-CreERT2 transgenic mice, we expressed transgenes in Arc+ ensembles activated by cocaine exposure (either acute [1 × 10 mg/kg intraperitoneally] or repeated [10 × 10 mg/kg intraperitoneally]). Using genetic, optical, and physiological recording and manipulation strategies, we assessed the contribution of these ensembles to behaviors associated with substance use disorder. ResultsRepeated cocaine exposure reduced the size of the ensemble while simultaneously increasing its control over behavior. Neurons within the repeated cocaine ensemble were hyperexcitable, and their optogenetic excitation was sufficient for reinforcement. Finally, lesioning the repeated cocaine, but not the acute cocaine, ensemble blunted cocaine self-administration. Thus, repeated cocaine exposure reduced the size of the ensemble while simultaneously increasing its contributions to drug reinforcement. ConclusionsWe showed that repeated, but not acute, cocaine exposure induced a physiologically distinct ensemble characterized by the expression of the immediate early gene Arc, which was uniquely capable of modulating reinforcement behavior.

Optical manipulation of ratio-designable Janus microspheres

Angular optical trapping based on Janus microspheres has been proven to be a novel method to achieve controllable rotation. In contrast to natural birefringent crystals, Janus microspheres are chemically synthesized of two compositions with different refractive indices. Thus, their structures can be artificially regulated, which brings excellent potential for fine and multi-degree-of-freedom manipulation in the optical field. However, it is a considerable challenge to model the interaction of heterogeneous particles with the optical field, and there has also been no experimental study on the optical manipulation of microspheres with such designable refractive index distributions. How the specific structure affects the kinematic properties of Janus microspheres remains unknown. Here, we report systematic research on the optical trapping and rotating of various ratio-designable Janus microspheres. We employ an efficient T-matrix method to rapidly calculate the optical force and torque on Janus microspheres to obtain their trapped postures and rotational characteristics in the optical field. We have developed a robust microfluidic-based scheme to prepare Janus microspheres. Our experimental results demonstrate that within a specific ratio range, the rotation radii of microspheres vary linearly and the orientations of microsphere are always aligned with the light polarization direction. This is of great importance in guiding the design of Janus microspheres. And their orientations flip at a particular ratio, all consistent with the simulations. Our work provides a reliable theoretical analysis and experimental strategy for studying the interaction of heterogeneous particles with the optical field and further expands the diverse manipulation capabilities of optical tweezers.

Multifunctional Meta-Devices for Full-Polarization Rotation and Focusing in the Near-Infrared.

The creation of multi-channel focused beams with arbitrary polarization states and their corresponding optical torques finds effective applications in the field of optical manipulation at the micro-nanoscale. The existing metasurface-based technologies for polarization rotation have made some progress, but they have been limited to single functions and have not yet achieved the generation of full polarization. In this work, we propose a multi-channel and spatial-multiplexing interference strategy for the generation of multi-channel focusing beams with arbitrary polarization rotation based on all-dielectric birefringent metasurfaces via simultaneously regulating the propagation phase and the geometric phase and independently controlling the wavefronts at different circular polarizations. For the proof of concept, we demonstrate highly efficient multi-channel polarization rotation meta-devices. The meta-devices demonstrate ultra-high polarization extinction ratios and high focusing efficiencies at each polarization channel. Our work provides a compact and versatile wavefront-shaping methodology for full-polarization control, paving a new path for planar multifunctional meta-optical devices in optical manipulation at micro-nano dimensions.

Construction of vector vortex beams on hybrid-order Poincaré sphere through highly scattering media

Vector vortex beams (VVBs) have attracted extensive attention due to their unique properties and their wide applications in fields such as optical manipulation and optical imaging. However, the wavefronts of the vector vortex beams are highly scrambled when they encounter highly scattering media (HSM), such as thick biological tissues, which greatly prevents the applications of VVBs behind HSM. To address this issue, we propose a scheme to construct VVBs of freewill position on the surface of hybrid-order Poincaré sphere (HyOPS) through HSM. With the measurement of two orthogonal scalar transmission matrices, the conjugated wavefronts for constructing orbital angular momentum beams with arbitrary topological charge in right and left circularly polarized states through HSM can be calculated, respectively. When an input wavefront superimposed by the two conjugated wavefronts with an appropriate ratio and phase delay, impinges on the HSM, the desired VVB can be created through HSM. To demonstrate the viability of our scheme, a series of VVBs on different locations of various HyOPSs have been reconstructed through a ZnO scattering layer experimentally. Furthermore, to characterize the polarization distribution of the generated beams, the polarization maps of these beams are derived by measuring the four Stokes parameters, which agree well with the theoretical distributions. This work will promote the applications of VVBs in highly scattering environments.

Propagation behaviors of two-dimensional chirped finite-energy Pearcey beams in free space

We introduce two-dimensional chirped finite energy Pearcey beams (FEPBs) for the first time and investigate the propagation dynamics. First, we applied the Huygens–Fresnel integral to derive an explicit analytical expression which is suitable for describing FEPB propagation in free space. It is interesting to find that FEPBs will experience three typical propagation patterns, i.e. the single-autofocusing case, dual-autofocusing case and non-autofocusing diffraction case, only depending on the value of the input asymmetric chirp. We further arrive at the critical condition of these three patterns analytically. However, by changing the sign, another input symmetric chirp acts to strengthen or weaken the autofocusing intensity but does not affect the focal distance. Our findings suggest that two-dimensional chirped FEPBs have more potential in controlling linear self-focusing and optical particle manipulation, when compared with the corresponding Airy field or conventional Gaussian field.

Wideband and low-spurious optical waveform generator for optically addressable quantum systems manipulation and control

Optical manipulation of quantum systems requires stable laser sources able to produce complex waveforms over a large frequency range. In the visible region, such waveforms can be generated using an acousto-optic modulator driven by an arbitrary waveform generator, but these suffer from a limited tuning range typically of a few tens of MHz. Visible-range electro-optic modulators are an alternative option offering a larger modulation bandwidth, however they have limited output power which drastically restricts the scalability of quantum applications. There is currently no architecture able to perform phase-stabilized waveforms over several GHz in the visible or near infrared region while providing sufficient optical power for quantum applications. Here we propose and develop a modulation and frequency conversion set-up able to deliver optical waveforms over a large frequency range, with a high spurious extinction ratio, scalable to the entire visible/near infrared region with high optical power. The optical waveforms are first generated at telecom wavelength and then converted to the emitter wavelength through a sum frequency generation process. By adapting the pump laser frequency, the optical waveforms can be tuned to interact with a broad range of optical quantum emitters or qubits such as alkali atoms, trapped ions, rare earth ions, or fluorescent defects in solid-state matrices. Using this architecture, we were able to detect and study a single erbium ion in a nanoparticle. We also generated high bandwidth signals at 606 nm, which would enable frequency multiplexing of on-demand read-out Pr3+:Y2SiO5 quantum memories.