The unstable Adams-Novikov spectral sequence for a space X is a sequence of groups {Er(X)}9 r = 2, 3,..., which converge to the homotopy groups of X, and whose £2term depends on the complex cobordism groups of X. We investigate this spectral sequence when X is the infinite special unitary group SU, or one of the finite groups SU(n), or when X is an odd sphere S2+1. The reader is referred to [2] for the construction and properties of the unstable Adams-Novikov spectral sequence. For some purposes, it is convenient to localize at a prime p, in which case the complex cobordism homology theory, based on the spectrum MU, is replaced by Brown-Peterson homology, based on the spectrum BP. We then have a useful spectral sequence with many of the properties of the stable Adams-Novikov spectral sequence. Namely, the nitrations are less than or equal to the filtrations in the unstable Adams spectral sequence based on mod-p homology. When X is a space for which H*(X; BP) is free over the coefficient ring n*(BP) and cofree as a coalgebra, then the E2-term is isomorphic to an Ext group in an abelian category (see §2; also [2, § 7]). Furthermore, this Ext group may be computed as the homology of an unstable cobar complex which we describe explicitly in Section 2. In particular, these considerations apply to the cases X = SU, X = SU(ri), or X = S2n+1. We first consider the situation where X is a p-local H-space with torsion-free homotopy and torsion-free homology. The results of Wilson [10] and the