Odd-frequency Superconductivity Research Articles

Odd-frequency pairing in a superconductor coupled to two parallel nanowires

We study the behavior of Cooper pair amplitudes that emerge when a two-dimensional superconductor is coupled to two parallel nanowires, focusing on the conditions for realizing odd-frequency pair amplitudes in the absence of spin-orbit coupling or magnetism. In general, any finite tunneling between the superconductor and the two nanowires induces odd-frequency spin-singlet pair amplitudes in the substrate as well as a substantial odd-frequency interwire pairing, both of which vanish locally. Interestingly, in the regime of strong superconductor-nanowire tunneling, we find that the presence of two nanowires allows for the conversion of non-local odd-frequency pairing to local even-frequency pairing. By studying this higher-order symmetry conversion process, we are able to identify a notable effect of the odd-frequency pairing in the superconductor on local quantities accessible by experiments. Specifically, we find that the odd-frequency pairing plays a direct role in the emergence of certain subgap features in the local density of states, and, importantly, it is responsible for a reduction of the maximum Josephson current between the two nanowires, measurable using Josephson scanning tunneling microscopy. We discuss ways to control the sizes of these effects induced by odd-frequency superconductivity by tuning the parameters describing the nanowires.

Even- and Odd-Frequency Superconductivity in Q1D Organic Superconductors Under Magnetic Field

One of the quasi-one-dimensional organic superconductors $$(\hbox {TMTSF})_2X$$ , called Bechgaard salts, has attracted a lot of interest since its discovery in 1980. These compounds have high critical magnetic field $$H_{\mathrm {c}2}$$ in the direction parallel to the layers, and their pairing symmetries seem to be different between low-field phase and high-field phase. In addition, recently, the possibility of the realization of odd-frequency superconductivity was pointed out. Therefore, we study pairing symmetries of Bechgaard salts under magnetic field with frequency-dependent pairing interaction due to spin and charge fluctuation. The model is given by the extended Hubbard model on a quasi-one-dimensional square lattice, and the spin susceptibility and charge susceptibility for the effective pairing interactions are derived by random-phase approximation under magnetic field. The odd-frequency s-wave and even-frequency f-wave regions expand as the magnetic field is increased.

Gapless odd-frequency superconductivity induced by the Sachdev-Ye-Kitaev model

We show that a single-fermion quantum dot acquires odd-frequency Gor'kov anomalous averages in proximity to strongly correlated Majorana zero modes, described by the Sachdev-Ye-Kitaev (SYK) model. Despite the presence of finite anomalous pairing, the superconducting gap vanishes for the intermediate coupling strength between the quantum dot and Majoranas. The increase of the coupling leads to smooth suppression of the original quasiparticles. This effect might be used as a characterization tool for recently proposed tabletop realizations of the SYK model.

Odd-frequency superconductivity revealed by thermopower

Superconductivity is characterized by a nonvanishing superconducting pair amplitude. It has a definite symmetry in spin, momentum and frequency (time). While the spin and momentum symmetry have been probed experimentally for different classes of superconductivity, the odd-frequency nature of certain superconducting correlations has not been demonstrated yet in a direct way. Here we propose the thermopower as an unambiguous way to assess odd-frequency superconductivity. This is possible since the thermoelectric coefficient given by Andreev-like processes is only finite in the presence of odd-frequency superconductivity. We illustrate our general findings with a simple example of a superconductor-quantum dot-ferromagnet hybrid.

Odd-frequency pairing in the edge states of superconducting pnictides in the coexistence phase with antiferromagnetism

In several members of the pnictide materials, spin density wave order coexists with superconductivity over a range of dopings and temperature. In this paper we show that odd-frequency superconductivity emerges on the edges of pnictides in such a coexistence phase. In particular, the breaking of spin-rotation symmetry by SDW and translation symmetry by the edge can lead to the development of odd-frequency spin-triplet Cooper pairing on edges of superconducting pnictide samples. In this case, the odd-frequency pairing has even parity components, which are immune to disorder. Our results show that pnictides are a natural platform to realize odd frequency superconductivity, which is a new quantum phase and has been mainly searched for in heterostructures of magnetic and superconducting materials. The emergence of odd-frequency pairing on the edges and in the defects can be potentially detected in magnetic response measurements.

Local impedance on a rough surface of a chiral p -wave superconductor

We develop a self-consistent approach for calculating the local impedance at a rough surface of a chiral $p$-wave superconductor. Using the quasiclassical Eilenberger-Larkin-Ovchinnikov formalism, we numerically find the pair potential, pairing functions, and the surface density of states taking into account diffusive electronic scattering at the surface. The obtained solutions are then employed for studying the local complex conductivity and surface impedance in the broad range of microwave frequencies (ranging from subgap to above-gap values). We identify anomalous features of the surface impedance caused by generation of odd-frequency superconductivity at the surface. The results are compared with experimental data for Sr$_2$RuO$_4$ and provide a microscopic explanation of the phenomenological two-fluid model suggested earlier to explain anomalous features of the microwave response in this material.

Conductance signatures of odd-frequency superconductivity in quantum spin Hall systems using a quantum point contact

Topological superconductors give rise to unconventional superconductivity, which is mainly characterized by the symmetry of the superconducting pairing amplitude. However, since the symmetry of the superconducting pairing amplitude is not directly observable, its experimental identification is rather difficult. In our work, we propose a system, composed of a quantum point contact and proximity induced s-wave superconductivity at the helical edge of a two dimensional topological insulator, for which we demonstrate the presence of odd-frequency pairing and its intimate connection to unambiguous transport signatures. Notably, our proposal requires no time-reversal symmetry breaking terms. We discover the domination of crossed Andreev reflection over electron cotunneling in a wide range of parameter space, which is a quite unusual transport regime.

Mixing Effect of Even-Frequency on Odd-Frequency Pairings in Strongly Correlated Electron Systems under Magnetic Field

Even- and odd-frequency superconductivity coexist due to broken time-reversal symmetry under magnetic field. In order to describe this mixing, we extend the linearized Eliashberg equation for the spin and charge fluctuation mechanism in strongly correlated electron systems. We apply this extended Eliashberg equation to the odd-frequency superconductivity on a quasi-one-dimensional isosceles triangular lattice under in-plane magnetic field and examine the effect of the even-frequency component.

Symmetry analysis of odd- and even-frequency superconducting gap symmetries for time-reversal symmetric interactions

Odd-frequency superconductivity describes a class of superconducting states where the superconducting gap is an odd function in relative time and Matsubara frequency. We present a group theoretical analysis based on the linearized gap equation in terms of Shubnikov groups of the second kind. By discussing systems with spin-orbit coupling and an interaction kernel which is symmetric under the reversal of relative time, we show that both even- and odd-frequency gaps are allowed to occur. Specific examples are discussed for the square lattice, the octahedral lattice, and the tetragonal lattice. For irreducible representations that are even under reversal of relative time the common combinations of $s$- and d-wave spin singlet and p-wave spin triplet gaps are revealed, irreducible representations that are odd under reversal of relative time give rise to $s$- and d-wave spin triplet and p-wave spin singlet gaps. Furthermore, we discuss the construction of a generalized Ginzburg-Landau theory in terms of the associated irreducible representations. The result complements the established classification of superconducting states of matter.

Odd-Frequency Superconductivity in Sr_{2}RuO_{4} Measured by Kerr Rotation.

We establish the existence of bulk odd-frequency superconductivity in Sr_{2}RuO_{4} and show that an intrinsic Kerr effect is direct evidence of this state. We use both general two- and three-orbital models, as well as a realistic tight-binding description of Sr_{2}RuO_{4} to demonstrate that odd-frequency pairing arises due to finite hybridization between different orbitals in the normal state, and is further enhanced by finite interorbital pairing.

Odd-frequency superconductivity induced in topological insulators with and without hexagonal warping

We study the effect of the Fermi surface anisotropy on the odd-frequency spin-triplet pairing component of the induced pair potential. We consider a superconductor/ ferromagnetic insulator (S/FI) hybrid structure formed on the 3D topological insulator (TI) surface. In this case three ingredients ensure the possibility of the odd-frequency pairing: (1) the topological surface states, (2) the induced pair potential, and (3) the magnetic moment of a nearby ferromagnetic insulator. We take into account the strong anisotropy of the Dirac point in topological insulators when the chemical potential lies well above the Dirac cone and its constant energy contour has a snowflake shape. Within this model, we propose that the S/FI boundary should be properly aligned with respect to the snowflake constant energy contour to have an odd-frequency symmetry of the corresponding pairing component and to insure the Majorana bound state at the S/FI boundary. For arbitrary orientation of the boundary, the Majorana bound state is absent. This provides a selection rule to the realization of Majorana modes in S/FI hybrid structures, formed on the topological insulator surface.

Majorana STM as a perfect detector of odd-frequency superconductivity

We propose a novel scanning tunneling microscope (STM) device in which the tunneling tip is formed by a Majorana bound state (MBS). This peculiar bound state exists at the boundary of a one-dimensional topological superconductor. Since the MBS has to be effectively spinless and local, we argue that it is the smallest unit that shows itself odd-frequency superconducting pairing. Odd-frequency superconductivity is characterized by an anomalous Green function which is an odd function of the time arguments of the two electrons forming the Cooper pair. Interestingly, our Majorana STM can be used as the perfect detector of odd-frequency superconductivity. The reason is that a supercurrent between the Majorana STM and any other superconductor can only flow if the latter system exhibits itself odd-frequency pairing. To illustrate our general idea, we consider the tunneling problem of the Majorana STM coupled to a quantum dot in vicinity to a conventional superconductor. In such a (superconducting) quantum dot, the effective pairing can be tuned from even- to odd-frequency behavior if an external magnetic field is applied to it.

Odd-frequency superconductivity in a nanowire coupled to Majorana zero modes

Odd-frequency superconductivity, originally proposed by Berezinskii in 1974, is an exotic phase of matter in which Cooper pairing between electrons is entirely dynamical in nature. The pair potential is an odd function of frequency, leading to a vanishing static superconducting order parameter and exotic types of pairing seemingly inconsistent with Fermi statistics. Motivated by recent experimental progress in the realization of Majorana zero modes in semiconducting nanowires, we show that odd-frequency superconductivity generically appears in a spin-polarized nanowire coupled to Majorana zero modes. We explicitly calculate the superfluid response and show that it is characterized by a paramagnetic Meissner effect.

Spontaneous Orbital-Selective Mott Transitions and the Jahn-Teller Metal of A_{3}C_{60}.

The alkali-doped fullerides A_{3}C_{60} are half-filled three-orbital Hubbard systems which exhibit an unconventional superconducting phase next to a Mott insulator. While the pairing is understood to arise from an effectively negative Hund coupling, the highly unusual Jahn-Teller metal near the Mott transition, featuring both localized and itinerant electrons, has not been understood. This property is consistently explained by a previously unrecognized phenomenon: the spontaneous transition of multiorbital systems with negative Hund coupling into an orbital-selective Mott state. This symmetry-broken state, which has no ordinary orbital moment, is characterized by an orbital-dependent two-body operator (the double occupancy) or an orbital-dependent kinetic energy and may be regarded as a diagonal-order version of odd-frequency superconductivity. We propose that the recently discovered Jahn-Teller metal phase of Rb_{x}Cs_{3-x}C_{60} is an experimental realization of this novel state of matter.

奇周波数超伝導 : 同時刻で消える奇妙なペア(最近の研究から)

奇周波数超伝導 : 同時刻で消える奇妙なペア(最近の研究から)

Pure odd-frequency superconductivity at the cores of proximity vortices

After more than a decade, direct observation of the odd frequency triplet pairing state in super- conducting hybrid structures remains elusive. We propose an experimentally feasible setup that can unambiguously reveal the zero energy peak due to proximity-induced equal spin superconducting triplet correlations. We theoretically investigate a two dimensional Josephson junction in the diffu- sive regime. The nanostructure consists of a normal metal sandwiched between two ferromagnetic layers with spiral magnetization patterns. By applying an external magnetic field perpendicular to the junction plane, vortices nucleate in the normal metal. The calculated energy and spatially resolved density of states, along with the pair potential, reveal that remarkably, only triplet Cooper pairs survive in the vortex cores. These isolated odd frequency triplet correlations result in well defined zero energy peaks in the local density of states that can be identified through tunneling spectroscopy experiments. Moreover, the diffusive regime considered here rules out the possibility of Andreev bound states in the vortex core as contributors to the zero energy peaks.

Odd-frequency superconductivity in driven systems

We show that Berezinskii's classification of the symmetries of Cooper pair amplitudes holds for driven systems even in the absence of translation invariance. We then consider a model Hamiltonian for a superconductor coupled to an external driving potential and, treating the driving potential as a perturbation, we investigate the corrections to the anomalous Green's function, density of states, and spectral function. We find that in the presence of an external drive the anomalous Green's function develops terms that are odd in frequency and that the same mechanism responsible for these odd-frequency terms generates additional features in the density of states and spectral function.

General Conditions for Proximity-Induced Odd-Frequency Superconductivity in Two-Dimensional Electronic Systems.

We obtain the general conditions for the emergence of odd-frequency superconducting pairing in a two-dimensional (2D) electronic system proximity coupled to a superconductor, making minimal assumptions about both the 2D system and the superconductor. Using our general results we show that a simple heterostructure formed by a monolayer of a group VI transition metal dichalcogenide, such as molybdenum disulfide, and an s-wave superconductor with Rashba spin-orbit coupling exhibits odd-frequency superconducting pairing. Our results allow the identification of a new class of systems among van der Waals heterostructures in which odd-frequency superconductivity should be present.

Tunneling and Josephson effects in odd-frequency superconductor junctions: A study on multichannel Kondo chain

Junction systems of odd-frequency (OF) superconductors are investigated based on a mean-field Hamiltonian formalism. One-dimensional two-channel Kondo lattice (TCKL) is taken as a concrete example of OF superconductors. Properties of normal and Andreev reflections are examined in a normal metal/superconductor junction. Unlike conventional superconductors, normal reflection is always present due to the normal self energy that necessarily appears in the present OF pairing state. The conductance reflects the difference between repulsive and attractive potentials located at the interface, which is in contrast with the preexisting superconducting junctions. Josephson junction is also constructed by connecting TCKL with the other types of superconductors. The results can be understood from symmetry of the induced Cooper pairs at the edge in the presence of spin/orbital symmetry breaking. It has also been demonstrated that the symmetry argument for Cooper pairs is useful in explaining Meissner response in bulk.

21aPS-102 磁場下でのナノ構造超伝導における奇周波数超伝導と渦糸構造の関係

21aPS-102 磁場下でのナノ構造超伝導における奇周波数超伝導と渦糸構造の関係