Ocean Cloud Research Articles

Southern Ocean Cloud Properties Derived From CAPRICORN and MARCUS Data

AbstractThe properties of Southern Ocean (SO) liquid phase non precipitating clouds (hereafter clouds) are examined using shipborne data collected during the Measurements of Aerosols, Radiation and Clouds over the Southern Ocean and the Clouds Aerosols Precipitation Radiation and atmospheric Composition Over the SoutheRN ocean I and II campaigns that took place south of Australia during Autumn 2016 and Summer 2017–2018. Cloud properties are derived using data from W‐band radars, lidars, and microwave radiometers using an optimal estimation algorithm. The SO clouds tended to have larger liquid water paths (LWP, 115 ± 117 g m−2), smaller effective radii (re, 8.7 ± 3 μm), and higher number concentrations (Nd, 90 ± 107 cm−3) than typical values of eastern ocean basin stratocumulus. The clouds demonstrated a tendency for the LWP to increase with Nd presumably due to precipitation suppression up to Nd of approximately 100 cm−3 when mean LWP decreased with increasing Nd. Due to higher optical depth, cloud albedos were less susceptible to changes in Nd compared to subtropical stratocumulus. The highest latitude clouds of the datasets, observed along and near the Antarctic coast, presented a distinctly bimodal character. One mode had the properties of marine clouds further north. The other mode occurred in an aerosol environment characterized by high cloud condensation nuclei concentrations and elevated sulfate aerosol without obvious continental aerosol markers. These regions of higher cloud condensation nuclei tended to have higher Nd, smaller re and higher LWP suggesting sensitivity of cloud properties to seasonal biogenic aerosol production in the high latitude SO.

Turbulent and boundary layer characteristics during VOCALS-REx

Abstract. Boundary layer and turbulent characteristics (surface fluxes, turbulent kinetic energy – TKE, turbulent kinetic energy dissipation rate – ϵ), along with synoptic-scale changes in these properties over time, are examined using data collected from 18 research flights made with the CIRPAS Twin Otter Aircraft. Data were collected during the Variability of the American Monsoon Systems (VAMOS) Ocean–Cloud–Atmosphere–Land Study Regional Experiment (VOCALS-REx) at Point Alpha (20∘ S, 72∘ W) in October and November 2008 off the coast of South America. The average boundary layer depth is found to be 1148 m, with 28 % of the boundary layer profiles analyzed displaying decoupling. Analysis of correlation coefficients indicates that as atmospheric pressure decreases, the boundary layer height (zi) increases. As has been shown previously, the increase in zi is accompanied by a decrease in turbulence within the boundary layer. As zi increases, cooling near cloud top cannot sustain mixing over the entire depth of the boundary layer, resulting in less turbulence and boundary layer decoupling. As the latent heat flux (LHF) and sensible heat flux (SHF) increase, zi increases, along with the cloud thickness decreasing with increasing LHF. This suggests that an enhanced LHF results in enhanced entrainment, which acts to thin the cloud layer while deepening the boundary layer. A maximum in TKE on 1 November (both overall average and largest single value measured) is due to sub-cloud precipitation acting to destabilize the sub-cloud layer while acting to stabilize the cloud layer (through evaporation occurring away from the surface, primarily confined between a normalized boundary layer height, z/zi, of 0.40 to 0.60). Enhanced moisture above cloud top from a passing synoptic system also acts to reduce cloud-top cooling, reducing the potential for mixing of the cloud layer. This is observed in both the vertical profiles of the TKE and ϵ, in which it is found that the distributions of turbulence for the sub-cloud and in-cloud layer are completely offset from one another (i.e., the range of turbulent values measured have slight or no overlap for the in-cloud and sub-cloud regions), with the TKE in the sub-cloud layer maximizing for the analysis period, while the TKE in the in-cloud layer is below the average in-cloud value for the analysis period. Measures of vertical velocity variance, TKE, and the buoyancy flux averaged over all 18 flights display a maximum near cloud middle (between normalized in-cloud height, Z*, values of 0.25 and 0.75). A total of 10 of the 18 flights display two peaks in TKE within the cloud layer, one near cloud base and another near cloud top, signifying evaporative and radiational cooling near cloud top and latent heating near cloud base. Decoupled boundary layers tend to have a maximum in turbulence in the sub-cloud layer, with only a single peak in turbulence within the cloud layer.

Opinion: Cloud-phase climate feedback and the importance of ice-nucleating particles

Abstract. Shallow clouds covering vast areas of the world's middle- and high-latitude oceans play a key role in dampening the global temperature rise associated with CO2. These clouds, which contain both ice and supercooled water, respond to a warming world by transitioning to a state with more liquid water and a greater albedo, resulting in a negative “cloud-phase” climate feedback component. Here we argue that the magnitude of the negative cloud-phase feedback component depends on the amount and nature of the small fraction of aerosol particles that can nucleate ice crystals. We propose that a concerted research effort is required to reduce substantial uncertainties related to the poorly understood sources, concentration, seasonal cycles and nature of these ice-nucleating particles (INPs) and their rudimentary treatment in climate models. The topic is important because many climate models may have overestimated the magnitude of the cloud-phase feedback, and those with better representation of shallow oceanic clouds predict a substantially larger climate warming. We make the case that understanding the present-day INP population in shallow clouds in the cold sector of cyclone systems is particularly critical for defining present-day cloud phase and therefore how the clouds respond to warming. We also need to develop a predictive capability for future INP emissions and sinks in a warmer world with less ice and snow and potentially stronger INP sources.

The Use of SSL and TLS Protocols in Providing a Secure Environment for e-commerce Sites

The problem is that e-commerce is not reliable and people are afraid to buy things and make transactions with commercial websites. Only some well-known companies have a known digital document from where it was issued. To solve this problem and to document any individual commercial website, We suggested to design a personal commercial website, it is a website to buy books and enable access to a domain by purchasing it from the digital ocean cloud, then a server is installed in this domain and then we connect it to the digital certification from the website (lets encrypt), where certain software are added to client (certbot, root) server assistant program, and we have linked the server and the certification together via Linux instructions and codes. The commercial website. (PHP3.PHP) has been tested in SSL laboratories and the results are the division of service sites into three categories: current, best current, and worst currently with details of categories, and what are the weaknesses.

Phase Characterization of Cold Sector Southern Ocean Cloud Tops: Results From SOCRATES

AbstractFor a given cloud, whether the cloud top is predominately made up of ice crystals or supercooled liquid droplets plays a large role in the clouds overall radiative effects. This study uses collocated airborne radar, lidar, and thermodynamic data from 12 high‐altitude flight legs during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) to characterize Southern Ocean (SO) cold sector cloud top phase (i.e., within 96 m of top) as a function of cloud top temperature (CTT). A training data set was developed to create probabilistic phase classifications based on High Spectral Resolution Lidar data and Cloud Radar data. These classifications were then used to identify dominant cloud top phase. Case studies are presented illustrating examples of supercooled liquid water at cloud top at different CTT ranges over the SO (−3°C < CTTs < −28°C). During SOCRATES, 67.4% of sampled cloud top had CTTs less than 0°C. Of the subfreezing cloud tops sampled, 91.7% had supercooled liquid water present in the top 96 m and 74.9% were classified entirely as liquid‐bearing. Liquid‐bearing cloud tops were found at CTTs as cold as −30°C. Horizontal cloud extent was also determined as a function of median cloud top height.

How Well Do Large‐Eddy Simulations and Global Climate Models Represent Observed Boundary Layer Structures and Low Clouds Over the Summertime Southern Ocean?

AbstractClimate models struggle to accurately represent the highly reflective boundary layer clouds overlying the remote and stormy Southern Ocean. We use in situ aircraft observations from the Southern Ocean Clouds, Radiation and Aerosol Transport Experimental Study (SOCRATES) to evaluate Southern Ocean clouds in a cloud‐resolving large‐eddy simulation (LES) and two coarse resolution global atmospheric models, the CESM Community Atmosphere Model (CAM6) and the GFDL Atmosphere Model (AM4), run in a nudged hindcast framework. We develop six case studies from SOCRATES data which span the range of observed cloud and boundary layer properties. For each case, the LES is run once forced purely using reanalysis data (fifth generation European Centre for Medium‐Range Weather Forecasts atmospheric reanalysis, “ERA5 based”) and once strongly nudged to an aircraft profile(“Obs based”). The ERA5‐based LES can be compared with the global models, which are also nudged to reanalysis data and are better for simulating cumulus. The Obs‐based LES closely matches an observed cloud profile and is useful for microphysical comparisons and sensitivity tests and simulating multilayer stratiform clouds. We use two‐moment Morrison microphysics in the LES and find that it simulates too few frozen particles in clouds occurring within the Hallett‐Mossop temperature range. We tweak the Hallett‐Mossop parameterization so that it activates within boundary layer clouds, and we achieve better agreement between observed and simulated microphysics. The nudged global climate models (GCMs) simulate liquid‐dominated mixed‐phase clouds in the stratiform cases but excessively glaciate cumulus clouds. Both GCMs struggle to represent two‐layer clouds, and CAM6 has low droplet concentrations in all cases and underpredicts stratiform cloud‐driven turbulence.

Simulating Observations of Southern Ocean Clouds and Implications for Climate

AbstractSouthern Ocean (S. Ocean) clouds are important for climate prediction. Yet previous global climate models failed to accurately represent cloud phase distributions in this observation‐sparse region. In this study, data from the Southern Ocean Clouds, Radiation, Aerosol, Transport Experimental Study (SOCRATES) experiment is compared to constrained simulations from a global climate model (the Community Atmosphere Model, CAM). Nudged versions of CAM are found to reproduce many of the features of detailed in situ observations, such as cloud location, cloud phase, and boundary layer structure. The simulation in CAM6 has improved its representation of S. Ocean clouds with adjustments to the ice nucleation and cloud microphysics schemes that permit more supercooled liquid. Comparisons between modeled and observed hydrometeor size distributions suggest that the modeled hydrometeor size distributions represent the dual peaked shape and form of observed distributions, which is remarkable given the scale difference between model and observations. Comparison to satellite observations of cloud physics is difficult due to model assumptions that do not match retrieval assumptions. Some biases in the model's representation of S. Ocean clouds and aerosols remain, but the detailed cloud physical parameterization provides a basis for process level improvement and direct comparisons to observations. This is crucial because cloud feedbacks and climate sensitivity are sensitive to the representation of S. Ocean clouds.

Structure of an Atmospheric River Over Australia and the Southern Ocean: II. Microphysical Evolution

AbstractAn atmospheric river affecting Australia and the Southern Ocean on 28–29 January 2018 during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) is analyzed using nadir‐pointing W‐band cloud radar measurements and in situ microphysical measurements from a Gulfstream‐V aircraft. The AR had a two‐band structure, with the westernmost band associated with a cold frontal boundary. The bands were primarily stratiform with distinct radar bright banding. The microphysical evolution of precipitation is described in the context of the tropical‐ and midlatitude‐sourced moisture zones above and below the 0°C isotherm, respectively, identified in Part I. In the tropical‐sourced moisture zone, ice particles at temperatures less than −8°C had concentrations on the order of 10 L−1, with habits characteristic of lower temperatures, while between −8°C and −4°C, an order of magnitude increase in ice particle concentrations was observed, with columnar habits consistent with Hallett‐Mossop secondary ice formation. Ice particles falling though the 0°C level into the midlatitude‐sourced moisture region and melting provided “seed” droplets from which subsequent growth by collision‐coalescence occurred. In this region, raindrops grew to sizes of 3 mm and precipitation rates averaged 16 mm hr−1.

Structure of an Atmospheric River Over Australia and the Southern Ocean. Part I: Tropical and Midlatitude Water Vapor Fluxes

AbstractAn atmospheric river (AR) impacting Tasmania, Australia, and the Southern Ocean during the austral summer on 28–29 January 2018 during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study campaign is analyzed using a modeling and observational approach. Gulfstream‐V dropsonde measurements and Global Precipitation Measurement radar analyses were used in conjunction with Weather Research and Forecasting model simulations with water vapor tracers to investigate the relative contributions of tropical and midlatitude moisture sources to the AR. Moisture associated with a monsoonal tropical depression became entrained into a midlatitude frontal system that extended to 60°S, reaching the associated low‐pressure system 850 km off the coast of Antarctica—effectively connecting the tropics and the polar region. Tropical moisture contributed to about 50% of the precipitable water within the AR as the flow moved over the Southern Ocean near Tasmania. The tropical contribution to precipitation decreased with latitude, from >70% over Australia, to ~50% off the Australian coast, to less than 5% poleward of 55°S. The integrated vapor transport (IVT) through the core of the AR reached above 500 kg m−1 s−1 during 1200 UTC 28 January to 0600 UTC 29 January, 1.29 times the average amount of water carried by the world's largest terrestrial river, the Amazon. The high IVT strength might be attributed to the higher water vapor content associated with the warmer temperatures across Australia and the Southern Ocean in austral summer.

Spatiotemporal variability of total cloud cover measured by visual observation stations and their comparison with ERA5 reanalysis over South Korea

AbstractThis analysis investigates the spatiotemporal variation of total cloud cover (TCC) across South Korea from 96 visual observation stations (VOS) during the years 2010–2019. The thin‐plate spline interpolation technique is used to interpolate the spatial variation of TCC within the country. The annual average of TCC distribution is closely related to topographical features and does not show excessive variation, with 50–56% over land. The seasonal TCC distribution has the lowest (highest) pattern in spring (summer), with a minimum (maximum) pattern of approximately 45% (95%). The lowest pattern in spring and highest pattern in summer may be due to the combined effect of lower cloud cover with TCC during March, and higher cloud cover with TCC from June to July. Interpolated VOS data are compared with the TCC obtained from ERA5 reanalysis products. The correlation coefficient between VOS and ERA5 is higher than 0.80 on the eastern coast, and approximately 0.20–0.40 on the western coast, indicating a strong and poor sampling effect. The largest variability between VOS and ERA5 is observed during the winter season, with a percentage deviation of −70–20%, possibly due to inaccurate cloud detection under cold low‐level atmospheric temperatures or snow cover. In summer, variability is −35–40%, which is slightly less than that in winter, possibly because of the incorrect detection of frequently occurring cumulus clouds. Principal component analysis of the TCC variability used to examine the relationship with other climate parameters. The first principal component, containing the major portion, correlated with precipitation, diurnal temperature, humidity, atmospheric pressure, and wind speed, with correlation coefficients of 0.293, 0.246, −0.360, −0.258, and 0.470, respectively, indicating positive or negative relationship. We believe the outcomes from this study will contribute a better understanding of climate over South Korea and establish links between East Asia and the Pacific Ocean cloud formation.

Improving the Southern Ocean cloud albedo biases in a general circulation model

Abstract. The present generation of global climate models is characterised by insufficient reflection of short-wave radiation over the Southern Ocean due to a misrepresentation of clouds. This is a significant concern as it leads to excessive heating of the ocean surface, sea surface temperature biases and subsequent problems with atmospheric dynamics. In this study, we modify cloud microphysics in a recent version of the Met Office's Unified Model and show that choosing a more realistic value for the shape parameter of atmospheric ice crystals, in better agreement with theory and observations, benefits the simulation of short-wave radiation. In the model, for calculating the growth rate of ice crystals through deposition, the default assumption is that all ice particles are spherical in shape. We modify this assumption to effectively allow for oblique shapes or aggregates of ice crystals. Along with modified ice nucleation temperatures, we achieve a reduction in the annual-mean short-wave cloud radiative effect over the Southern Ocean by up to ∼4 W m−2 and seasonally much larger reductions compared to the control model. By slowing the growth of the ice phase, the model simulates substantially more supercooled liquid cloud.

Microphysical Properties of Generating Cells Over the Southern Ocean: Results From SOCRATES

AbstractThe bulk microphysical properties and number distribution functions (N(D)) of supercooled liquid water (SLW) and ice inside and between ubiquitous generating cells (GCs) observed over the Southern Ocean (SO) during the Southern Ocean Clouds Radiation Aerosol Transport Experimental Study (SOCRATES) measured by in situ cloud probes onboard the NCAR/NSF G‐V aircraft are compared. SLW was detected inside all GCs with an average liquid water content of 0.31 ± 0.19 g m−3, 11% larger than values between GCs. The N(D) of droplets (maximum dimension D < 50 μm) inside and between GCs had only slight differences. For ice particles, on the other hand, the mean concentration (median mass diameter) with D > 200 μm inside GCs was 2.0 ± 3.3 L−1 (323 ± 263 μm), 65% (37%) larger than values outside GCs. As D increases, the percentage differences became larger (up to ~500%). The more and larger ice particles inside GCs suggest the GC updrafts provide a favorable environment for particle growth by deposition and riming and that mixing processes are less efficient at redistributing larger particles. The horizontal scale of observed GCs ranged from 200 to 600 m with a mean of 395 ± 162 m, smaller than GC widths observed in previous studies. This study expands knowledge of the microphysical properties and processes acting in GCs over a wider range of conditions than previously available.

Evaluation of Southern Ocean cloud in the HadGEM3 general circulation model and MERRA-2 reanalysis using ship-based observations

Abstract. Southern Ocean (SO) shortwave (SW) radiation biases are a common problem in contemporary general circulation models (GCMs), with most models exhibiting a tendency to absorb too much incoming SW radiation. These biases have been attributed to deficiencies in the representation of clouds during the austral summer months, either due to cloud cover or cloud albedo being too low. The problem has been the focus of many studies, most of which utilised satellite datasets for model evaluation. We use multi-year ship-based observations and the CERES spaceborne radiation budget measurements to contrast cloud representation and SW radiation in the atmospheric component Global Atmosphere (GA) version 7.1 of the HadGEM3 GCM and the MERRA-2 reanalysis. We find that the prevailing bias is negative in GA7.1 and positive in MERRA-2. GA7.1 performs better than MERRA-2 in terms of absolute SW bias. Significant errors of up to 21 W m−2 (GA7.1) and 39 W m−2 (MERRA-2) are present in both models in the austral summer. Using ship-based ceilometer observations, we find low cloud below 2 km to be predominant in the Ross Sea and the Indian Ocean sectors of the SO. Utilising a novel surface lidar simulator developed for this study, derived from an existing Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) – active remote sensing simulator (ACTSIM) spaceborne lidar simulator, we find that GA7.1 and MERRA-2 both underestimate low cloud and fog occurrence relative to the ship observations on average by 4 %–9 % (GA7.1) and 18 % (MERRA-2). Based on radiosonde observations, we also find the low cloud to be strongly linked to boundary layer atmospheric stability and the sea surface temperature. GA7.1 and MERRA-2 do not represent the observed relationship between boundary layer stability and clouds well. We find that MERRA-2 has a much greater proportion of cloud liquid water in the SO in austral summer than GA7.1, a likely key contributor to the difference in the SW radiation bias. Our results suggest that subgrid-scale processes (cloud and boundary layer parameterisations) are responsible for the bias and that in GA7.1 a major part of the SW radiation bias can be explained by cloud cover underestimation, relative to underestimation of cloud albedo.

Evaluation of Southern Ocean cloud in the HadGEM3 general circulation model and MERRA-2 reanalysis using ship-based observations

Evaluation of Southern Ocean cloud in the HadGEM3 general circulation model and MERRA-2 reanalysis using ship-based observations

Evaluation of Cloud Microphysical Properties Derived From MODIS and Himawari‐8 Using In Situ Aircraft Measurements Over the Southern Ocean

AbstractCloud microphysical properties from aircraft measurements during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study are used to evaluate the cloud products from the geostationary satellite Himawari‐8 (H‐8) and the polar‐orbiting satellite the Moderate Resolution Imaging Spectroradiometer (MODIS). Compared to the in situ aircraft observations when aircraft flew horizontally near cloud tops, the cloud droplet effective radius (re) and number concentration (Nd) from H‐8 (MODIS) are 33% (26%–31%) and 2% (9–13%) larger. Both the H‐8 and MODIS retrievals behave similarly for liquid‐only and mixed‐phase low‐level clouds, indicating the weak sensitivity of the satellite cloud retrieval performance to cloud phase. The re and Nd of the cloud profiles from aircraft measurements were also used to compare with the satellite product. It shows that H‐8 re and Nd agree better with aircraft measurements when considering only the in situ data acquired in the upper portions (highest 20%) of the clouds. Roughly, the re overestimation by H‐8 decreases from 18% to 3% when considering the upper portions of clouds compared to all cloud layer averages, except for one case with drizzles appeared. In addition, the performance of MODIS re and Nd is highly dependent on the wavelengths the retrieval method uses. The droplet re retrievals using wavelength of 1.6 μm have much larger biases than that using the other two channels. The potential effects of the cloud vertical variation and the photon penetration depth, the cloud heterogeneity, the cloud droplet size spectra, and the drizzle on satellite retrievals have also been discussed.

Sea-spray regulates sulfate cloud droplet activation over oceans

Sulfate aerosols are typically the dominant source of cloud condensation nuclei (CCN) over remote oceans and their abundance is thought to be the dominating factor in determining oceanic cloud brightness. Their activation into cloud droplets depends on dynamics (i.e. vertical updrafts) and competition with other potential CCN sources for the condensing water. We present new experimental results from the remote Southern Ocean illustrating that, for a given updraft, the peak supersaturation reached in cloud, and consequently the number of droplets activated on sulfate nuclei, is strongly but inversely proportional to the concentration of sea-salt activated despite a 10-fold lower abundance. Greater sea-spray nuclei availability mostly suppresses sulfate aerosol activation leading to an overall decrease in cloud droplet concentrations; however, for high vertical updrafts and low sulfate aerosol availability, increased sea-spray can augment cloud droplet concentrations. This newly identified effect where sea-salt nuclei indirectly controls sulfate nuclei activation into cloud droplets could potentially lead to changes in the albedo of marine boundary layer clouds by as much as 30%.

Evaluation of an E–ε and Three Other Boundary Layer Parameterization Schemes in the WRF Model over the Southeast Pacific and the Southern Great Plains

Abstract To accurately simulate the atmospheric state within the planetary boundary layer (PBL) by PBL parameterization scheme in different regions with their dominant weather/climate regimes is important for global/regional atmospheric models. In this study, we introduce the turbulence kinetic energy (TKE) and TKE dissipation rate (ε) based 1.5-order closure PBL parameterization (E–ε, EEPS) in the Weather Research and Forecasting (WRF) Model. The performances of the newly implemented EEPS scheme and the existing Yonsei University (YSU) scheme, the University of Washington (UW) scheme, and Mellor–Yamada–Nakanishi–Niino (MYNN) scheme are evaluated over the stratocumulus dominated southeast Pacific (SEP) and over the Southern Great Plains (SGP) where strong PBL diurnal variation is common. The simulations by these PBL parameterizations are compared with various observations from two field campaigns: the Variability of American Monsoon Systems Project (VAMOS) Ocean–Cloud–Atmosphere–Land Study (VOCALS) in 2008 over the SEP and the Land–Atmosphere Feedback Experiment (LAFE) in 2017 over the SGP. Results show that the EEPS and YSU schemes perform comparably over both regions, while the MYNN scheme performs differently in many aspects, especially over the SEP. The EEPS (MYNN) scheme slightly (significantly) underestimates liquid water path over the SEP. Compared with observations, the UW scheme produces the best PBL height over the SEP. The MYNN produces too high PBL height over the western part of the SEP while both the YSU and EEPS schemes produce too low PBL and cloud-top heights. The differences among the PBL schemes in simulating the PBL features over the SGP are relatively small.

Constraining the Surface Flux of Sea Spray Particles From the Southern Ocean

AbstractModeling the shortwave radiation balance over the Southern Ocean region remains a challenge for Earth system models. To investigate whether this is related to the representation of aerosol‐cloud interactions, we compared measurements of the total number concentration of sea spray‐generated particles within the Southern Ocean region to model predictions thereof. Measurements were conducted from a container laboratory aboard the R/V Tangaroa throughout an austral summer voyage to the Ross Sea. We used source‐receptor modeling to calculate the sensitivity of our measurements to upwind surface fluxes. From this approach, we could constrain empirical parameterizations of sea spray surface flux based on surface wind speed and sea surface temperature. A newly tuned parameterization for the flux of sea spray particles based on the near‐surface wind speed is presented. Comparisons to existing model parameterizations revealed that present model parameterizations led to overestimations of sea spray concentrations. In contrast to previous studies, we found that including sea surface temperature as an explanatory variable did not substantially improve model‐measurement agreement. To test whether or not the parameterization may be applicable globally, we conducted a regression analysis using a database of in situ whitecap measurements. We found that the key fitting parameter within this regression agreed well with the parameterization of sea spray flux. Finally, we compared calculations from the best model of surface flux to boundary layer measurements collected onboard an aircraft throughout the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES), finding good agreement overall.

Reassessing the Effect of Cloud Type on Earth’s Energy Balance in the Age of Active Spaceborne Observations. Part I: Top of Atmosphere and Surface

AbstractThis study revisits the classical problem of quantifying the radiative effects of unique cloud types in the era of spaceborne active observations. The radiative effects of nine cloud types, distinguished based on their vertical structure defined by CloudSat and CALIPSO observations, are assessed at both the top of the atmosphere and the surface. The contributions from single- and multilayered clouds are explicitly diagnosed. The global, annual mean net cloud radiative effect at the top of the atmosphere is found to be −17.1 ± 4.2 W m−2 owing to −44.2 ± 2 W m−2 of shortwave cooling and 27.1 ± 3.7 W m−2 of longwave heating. Leveraging explicit cloud base and vertical structure information, we further estimate the annual mean net cloud radiative effect at the surface to be −24.8 ± 8.7 W m−2 (−51.1 ± 7.8 W m−2 in the shortwave and 26.3 ± 3.8 W m−2 in the longwave). Multilayered clouds are found to exert the strongest influence on the top-of-atmosphere energy balance. However, a strong asymmetry in net cloud radiative cooling between the hemispheres (8.6 W m−2) is dominated by enhanced cooling from stratocumulus over the southern oceans. It is found that there is no corresponding asymmetry at the surface owing to enhanced longwave emission by southern ocean clouds in winter, which offsets a substantial fraction of their impact on solar absorption in summer. Thus the asymmetry in cloud radiative effects is entirely realized as an atmosphere heating imbalance between the hemispheres.

Response of Arctic mixed-phase clouds to aerosol perturbations under different surface forcings

Abstract. The formation and persistence of low-lying mixed-phase clouds (MPCs) in the Arctic depends on a multitude of processes, such as surface conditions, the environmental state, air mass advection, and the ambient aerosol concentration. In this study, we focus on the relative importance of different instantaneous aerosol perturbations (cloud condensation nuclei and ice-nucleating particles; CCN and INPs, respectively) on MPC properties in the European Arctic. To address this topic, we performed high-resolution large-eddy simulation (LES) experiments using the Consortium for Small-scale Modeling (COSMO) model and designed a case study for the Aerosol-Cloud Coupling and Climate Interactions in the Arctic (ACCACIA) campaign in March 2013. Motivated by ongoing sea ice retreat, we performed all sensitivity studies over open ocean and sea ice to investigate the effect of changing surface conditions. We find that surface conditions highly impact cloud dynamics, consistent with the ACCACIA observations: over sea ice, a rather homogeneous, optically thin, mixed-phase stratus cloud forms. In contrast, the MPC over the open ocean has a stratocumulus-like cloud structure. With cumuli feeding moisture into the stratus layer, the cloud over the open ocean features a higher liquid (LWP) and ice water path (IWP) and has a lifted cloud base and cloud top compared to the cloud over sea ice. Furthermore, we analyzed the aerosol impact on the sea ice and open ocean cloud regime. Perturbation aerosol concentrations relevant for CCN activation were increased to a range between 100 and 1000 cm−3 and ice-nucleating particle perturbations were increased by 100 % and 300 % compared to the background concentration (at every grid point and at all levels). The perturbations are prognostic to allow for fully interactive aerosol–cloud interactions. Perturbations in the INP concentration increase IWP and decrease LWP consistently in both regimes. The cloud microphysical response to potential CCN perturbations occurs faster in the stratocumulus regime over the ocean, where the increased moisture flux favors rapid cloud droplet formation and growth, leading to an increase in LWP following the aerosol injection. In addition, IWP increases through new ice crystal formation by increased immersion freezing, cloud top rise, and subsequent growth by deposition. Over sea ice, the maximum response in LWP and IWP is delayed and weakened compared to the response over the open ocean surface. Additionally, we find the long-term response to aerosol perturbations to be highly dependent on the cloud regime. Over the open ocean, LWP perturbations are efficiently buffered after 18 h simulation time. Increased ice and precipitation formation relax the LWP back to its unperturbed range. On the contrary, over sea ice the cloud evolution remains substantially perturbed with CCN perturbations ranging from 200 to 1000 CCN cm−3.