Nuclear Physics Research Articles

Introduction to Special Issue on the Early History of Nuclear Fusion

This introductory paper to the special issue of Fusion Science and Technology commemorates early research on fusion conducted at Los Alamos (the singular entity denoted Los Alamos Laboratory/Los Alamos Scientific Laboratory/Los Alamos National Laboratory at different times is designated “Los Alamos” in this paper) in support of the eventual H-bomb program. We survey the historical origins of the thermonuclear program, what was known of fusion reactions at the outbreak of the war, and the remarkable breakthroughs involving particularly the prospect of deuterium-tritium (DT) reactions conducted during the war, and we summarize the papers in this volume. Much of the nuclear fusion technical history presented herein has not been previously reported. Papers describe aspects of fusion science during these days, on shock hydrodynamics and on electron-radiation coupling, and on nuclear physics including the discoveries of resonances in both the DT cross section and in the lithium tritium-breeding cross section. Three papers follow our colleague Mark Paris’s finding Arthur Ruhlig’s 1938 paper on the first observation of DT fusion: one on how it influenced subsequent Manhattan Project research, another on a modern calculation of that historic experiment, and a third that has repeated the experiment using modern experimental capabilities. Other papers discuss how the first H-bomb test, Ivy Mike, led to the discovery of the new elements einsteinium and fermium and how the DT fusion processes played a key role in our universe’s development after the Big Bang. We also present a paper that analyzes the pioneering Cambridge University 1934 experiment by Marcus Oliphant, Paul Harteck, and Ernest Rutherford where deuterium-deuterium fusion was first observed and that describes how Ernest Lawrence missed identifying fusion in 1933. Finally, we present a summary of early concepts for controlled fusion energy that grew out of wartime discussions at Los Alamos. The papers show how J. Robert Oppenheimer played a leading technical role in the early developments of the H-bomb, before his later opposition—our first paper in this issue addresses the U.S. Department of Energy’s 2022 vacating of the earlier 1954 decision to revoke his security clearance.

First Structured Uranium‐Based Monoliths Produced via Vat Photopolymerization for Nuclear Applications

AbstractUranium plays an unquestionable role in the framework of nuclear physics, biology, and radiopharmacy. Moreover, uranyl ion UO22+ offers an immense variety of applications due to the unique photosensitivity of its complexes. The excited state of uranyl cation is indeed accessible under ultraviolet‐visible (UV–vis) light, readily producing radical species UO22+* upon light irradiation. Herein, an innovative synthesis protocol is presented to explore the use of uranyl cations as photocatalyst systems for photocurable sol–gel‐based formulations, coupling the photochemical reactions of uranyl cations with photopolymerization‐based additive manufacturing processes. Additive manufacturing has nowadays revolutionized the production of complex structures with arbitrary geometries and has opened up enticing opportunities for innovative technological breakthroughs and highly tailorable systems. The fabrication of micro‐architected components is shown via vat photopolymerization, namely, the Digital Light Processing technique, and ‐3D) printed parts are converted into uranium dicarbide (UC2)/carbon nanocomposite upon carbothermal reduction. This uranyl‐mediated additive manufacturing process constitutes the first application of the synergistic role of uranyl motifs in a photopolymer platform, demonstrating for the first time the possibility to directly pattern uranium‐based materials in complex structures.

Symmetry energy in holographic QCD

We study the symmetry energy (SE), an important quantity in nuclear physics, in the Witten-Sakai-Sugimoto model and in a much simpler hard-wall model of holographic QCD. The SE is the energy contribution to the nucleus due to having an unequal number of neutrons and protons. Using a homogeneous Ansatz representing smeared instantons and quantizing their isospin, we extract the SE and the proton fraction assuming charge neutrality and beta-equilibrium, using quantization of the isospin zeromode. We also show the equivalence between our method adapted from solitons and the usual way of the isospin controlled by a chemical potential at the holographic boundary. We find that the SE can be well described in the WSS model if we allow for a larger ’t Hooft coupling and lower Kaluza-Klein scale than is normally used in phenomenological fits.

Extraction method for superimposed coherent transition radiation using Fresnel reflection in a ring-type resonator

To generate terahertz pulses with a high peak power, a pulse train of coherent transition radiation (CTR) is superimposed by circulating it in a ring-type resonator at an L-band electron linear accelerator facility at the Kyoto University Institute for Integrated Radiation and Nuclear Science. By extracting the superimposed CTR pulses from the ring-type resonator via Fresnel reflection on a low-loss parallel substrate, we show that the cavity loss can be suppressed without being affected by the wavenumber of the CTR pulses. The power of the superimposed CTR pulse is increased to approximately four times that of a CTR generated by plane mirrors in the resonator at a wavenumber of 8.5cm−1, where the diffraction loss of the resonator is lower. Using shorter electron bunches to generate CTR pulses with higher wavenumbers increases the amplification factor caused by superposition and allows CTR pulses with a higher peak power to be generated.

Relativistic Time‐dependent Density Functional Theory Approach to Nuclear Physics Fission

A thorough knowledge of the stationary characteristics of the nuclei of atoms, their stimulation wavelengths, how they react to outside factors, and how they disintegrate is the aim of nuclear structural science. Although achieving these objectives within just one structure is difficult and prevents the existence of a nuclear "standard model," it is evident that radioactive Density Functional Theory (DFT) offers perhaps the broadest variety of applications to date. We attempt to place DFT in a larger perspective in this study by making frequent allusions to electrical DFT. We also provide a brief overview of the numerous uses and an explanation of the connections between beginning techniques and Useful Field Concepts (EFTs) in particular. The article tries to promote collaborations with different scientific fields while being published from a subjective and perhaps biased point of view.

Modeling in Nuclear Physics of Visual Approach to the Semi-empirical Mass Formula SEMF

An empirical framework that accurately describes radioactive binding energies is the Somewhat Empirical Mass Equation (SEMF). They showcase many implementations and uses of the idea that rely on graphics and printed objects. A key new addition is a contrast with real experiments, as well as a visualization of the energy environment as supplied by the SEMF. The shortcomings of the empirical theory are shown by our visualization of this differential energy scenery, which also highlights the significance of what is known as magic numbers—an explanation provided by the outermost approach, which was developed much more recently than the water drop theory. This provides a great chance to talk about the advantages and limitations of simulations everywhere within the framework of science teaching.

Lunar Lithium-7 Sensing (δ7Li): Spectral Patterns and Artificial Intelligence Techniques.

Lithium, a critical natural resource integral to modern technology, has influenced diverse industries since its discovery in the 1950s. Of particular interest is lithium-7, the most prevalent lithium isotope on Earth, playing a vital role in applications such as batteries, metal alloys, medicine, and nuclear research. However, its extraction presents significant environmental and logistical challenges. This article explores the potential for lithium exploration on the Moon, driven by its value as a resource and the prospect of cost reduction due to the Moon's lower gravity, which holds promise for future space exploration endeavors. Additionally, the presence of lithium in the solar wind and its implications for material transport across celestial bodies are subjects of intrigue. Drawing from a limited dataset collected during the Apollo missions (Apollo 12, 15, 16, and 17) and leveraging artificial intelligence techniques and sample expansion through bootstrapping, this study develops predictive models for lithium-7 concentration based on spectral patterns. The study areas encompass the Aitken crater, Hadley Rima, and the Taurus-Littrow Valley, where higher lithium concentrations are observed in basaltic lunar regions. This research bridges lunar geology and the formation of the solar system, providing valuable insights into celestial resources and enhancing our understanding of space. The data used in this study were obtained from the imaging sensors (infrared, visible, and ultraviolet) of the Clementine satellite, which significantly contributed to the success of our research. Furthermore, the study addresses various aspects related to statistical analysis, sample quality validation, resampling, and bootstrapping. Supervised machine learning model training and validation, as well as data import and export, were explored. The analysis of data generated by the Clementine probe in the near-infrared (NIR) and ultraviolet-visible (UVVIS) spectra revealed evidence of the presence of lithium-7 (Li-7) on the lunar surface. The distribution of Li-7 on the lunar surface is non-uniform, with varying concentrations in different regions of the Moon identified, supporting the initial hypothesis associating surface Li-7 concentration with exposure to solar wind. While a direct numerical relationship between lunar topography and Li-7 concentration has not been established due to morphological diversity and methodological limitations, preliminary results suggest significant economic and technological potential in lunar lithium exploration and extraction.

Burnup and neutronic parameter analysis of GAMA molten salt reactor (GAMA-MSR)

The GAMA molten salt reactor (GAMA-MSR) is a small modular MSR design developed by the Nuclear Reactor Research Team of the Department of Nuclear Engineering and Engineering Physics, Universitas Gadjah Mada. In the GAMA-MSR design, the reactor core is placed above the primary heat exchanger. The primary heat exchanger is partially filled with fuel in normal operation, allowing room to be filled with the fuel drained from the reactor. Thus, in addition to control rods, the design of GAMA-MSR provides unique reactivity control through the balance of fuel salt fuel from the reactor core to the primary heat exchanger vice versa by adjusting fuel pump capacity. This design allows to shutdown the reactor by switching off the fuel pump. The reactor is initially fueled with 7LiF-ThF4-UF4 with 75: 20.1: 4.9 mol composition. The uranium has 19.75 % U-235 mol fraction. The reactor criticality and nuclide composition in the reactor fuel are calculated using OpenMC code during the reactor operation lifetime, with periodic adjustments to the fuel composition to simulate the effects of the fissile and fertile additions to the fuel and the extraction of actinides and fission products from the fuel. The calculated reactor thermal power is 60 MWth in this paper. The reactor is operated until it achieves a burnup value of 34,000 MWd/tHM. At this burnup value, the U-235 inventory is consumed and the amount is reduced from 794 kg to 250 kg. The U-233, Pu-239 and Pu-241 are produced with the amount are 246 kg, 24 kg and 8 kg respectively at the end of reactor operation. The effects of temperature, fuel density change, and fission product neutron poisons are also calculated. The average temperature reactivity coefficient value is approximately -4.4395×10-5Δk/k per °C. The effect of thermal expansion has been included in the calculation of this temperature reactivity coefficient value. The average value of the void reactivity coefficient is +1.2606×10-3Δk/k per % of void fraction for the void fraction value range up to 50 %. However, molten salt fuel suffers only small changes in density during operation. The negative value of the temperature reactivity coefficient will be dominant; thus, the GAMA-MSR becomes inherently safe. The GAMA-MSR is designed for a 30-year operation time. The effect of the fission product to the reactor reactivity is -1.4597×10-2Δk/k. Full draining of the fuel to primary heat exchanger brings the reactor to shutdown condition with the reactivity of −0.20525. Results showed that this reactor has an inherently safe characteristic and has an effective shutdown system, especially due to the fuel draining system.

Acceleration of uranium beam to record power of 10.4 kW and observation of new isotopes at Facility for Rare Isotope Beams

The Facility for Rare Isotope Beams (FRIB) is a major nuclear physics facility for research with fast, stopped, and reaccelerated beams that was successfully commissioned in May 2022. A key capability of FRIB is the production of an acceleration of the uranium beam, but this capability requires the facility to work at the design limits of the lowest charge-to-mass ratio and the highest power density on the beam intercepting devices. This paper presents techniques for overcoming the significant challenges in accelerating the uranium beam, culminating in the demonstration of 10.4 kW on target, and the discovery of three new isotopes. The high-power uranium beam enabled us to produce and identify G88a, A93s, and S96e, within the first 24 h of operation. The successful uranium operation at FRIB sets a new record for accelerated uranium beam power above 10 kW and opens a new avenue of research with rare isotopes. Published by the American Physical Society 2024

High-Performance Wave Union Time-to-Digital Converter Implementation Based on Routing Path Delays of FPGA

Time-to-digital converters (TDCs) with superior performance are in high demand in application domains like light detection and ranging (LIDAR), nuclear physics, and time interval counters. One of the interesting architectures for field-programmable gate array (FPGA)-based TDCs is the tapped delay line (TDL) approach with carry chains as delay elements. However, the resolution of TDL-TDCs is limited, and linearity is weakened by the ultra-wide bins that correspond to the FPGA’s long routing wires crossing into another clock area. This paper presents wave union TDC using FPGA internal routing wires as delay elements to subdivide ultra-wide bins. The Zynq Evaluation and Development (ZED) board is used to implement and test the wave union types: A (WU-A) and B (WU-B) TDCs. According to experimental data, the WU-A TDC based on an 8 × 128 matrix of counters has a resolution of 5.7 ps, an integral nonlinearity (INL) of 1.1170 LSB (RMS), and a differential nonlinearity of 0.329 LSB (RMS). WU-A TDC improves DNL and INL by 19% and 57%, respectively, over ordinary TDC. The WU-B TDC uses an average of sixteen different time measurements, resulting in an effective resolution of up to 0.356 ps, a DNL of 0.60 LSB (RMS), and an INL of 1.04 LSB (RMS). These characteristics make the TDC suitable for time-of-flight applications such as LIDAR and for other general-purpose scientific instruments.

Development of a human reliability analysis framework for nominal human error probability estimate of the TRIGA research reactor in Thailand

Human reliability analysis (HRA) of nuclear research reactors often encounters a lack of human performance data, a challenge that is also faced by the TRIGA reactor of Thailand having no specific full method or human error database for HRA. To overcome this challenge, in 2023, HRA teams from the Korea Atomic Energy Research Institute (KAERI) and the Thailand Institute of Nuclear Technology (TINT) jointly developed an HRA framework for the TRIGA reactor. In the HRA framework development, the HRA practitioners applied KAERI's three main HRA tools, namely 1) the EMpirical data-Based crew Reliability Assessment and Cognitive Error analysis (EMBRACE) method, 2) the Human Reliability data EXtraction (HuREX) database, and 3) the TAsk COMplexity (TACOM) method. The HRA framework covers the overall process including the classification of documents and human error types as well as nominal human error extraction for estimating nominal human error probabilities. According to the results of the first use of the HRA framework on the TRIGA reactor in Thailand, the HRA framework provided an effective way to improve the procedures and systematically identify nominal human errors of actions in the emergency procedures.

Strengthening nuclear symmetry energy constraints using multiple resonant shattering flares of neutron stars with realistic mass uncertainties

ABSTRACT With current and planned gravitational-wave (GW) observing runs, coincident multimessenger timing of resonant shattering flares (RSFs) and GWs may soon allow for neutron star (NS) asteroseismology to be used to constrain the nuclear symmetry energy, an important property of fundamental nuclear physics that influences the composition and equation of state of NSs. In this work, we examine the effects of combining multiple RSF detections on these symmetry energy constraints, and consider how realistic uncertainties in the masses of the progenitor NSs may weaken them. We show that the detection of subsequent multimessenger events has the potential to substantially improve constraints beyond those obtained from the first, and that this improvement is insensitive to the mass of the NSs that produce the RSFs and its uncertainty. This sets these asteroseismic constraints apart from bulk NS properties such as radius, for which the NS mass is highly important, meaning that any multimessenger RSF and GW events can equally improve our knowledge of fundamental physics.

Enhancing radiation resistance of silicone rubber through the addition of polydopamine-modified cerium dioxide

With the widespread use of nuclear science and technology, slowing down the aging of polymers in a radiation environment has become a matter of great concern. In this work, cerium dioxide (CeO2) and CeO2 encapsulated with dopamine (PDA@CeO2) were selected as special fillers to prepare the silicone rubber (SR) composites, and their radiation resistance were investigated by comparing the mechanical properties and thermal performance before and after irradiation. The interfacial bridge formed by PDA results in a greater elongation at break for PDA@CeO2/SR5.0 (770.0 ± 33.6 %) than for CeO2/SR (686.0 ± 15.0 %). After irradiation with γ-rays, the retention of elongation at break of both CeO2/SR0.1 and PDA@CeO2/SR0.1 were larger than SR. Furthermore, PDA@CeO2/SR0.1 showed an impressive retention of 90.5 ± 2.7 % of the tensile strength retention after exposure to an absorbed dose of 200 kGy. The disparity in crosslink density prior to and following irradiation indicated that both CeO2 and PDA@CeO2 were efficacious in reducing radiation crosslinking within the SR. An electron paramagnetic resonance spectrometer and an ultraviolet lamp (UV-EPR) were used to observe in real time the free radical scavenging ability of CeO2 and PDA@CeO2 inside the SR. These results indicated that CeO2 and PDA@CeO2 was expected to prevent further chain reactions in silicone rubber by scavenging free radicals generated in SR, thus improving the radiation resistance of SR.

Simulating the impact of electron beam energy deposition on lead target temperature

This study delves into the thermal dynamics induced by an electron beam sourced from the CIRCE III accelerator, focusing on a lead target previously employed at the National Centre for Nuclear Science and Technology (CNSTN) in Tunisia for neutron and photon production. Leveraging FLUKA software, we simulate the intricate interplay between electrons and the target surface, analyzing variations in deposited energy across different target thicknesses. Beyond elucidating the electron-target interaction, our investigation extends to predicting crucial parameters such as the maximum operational threshold and surface temperature distribution of the target. To achieve this, a computational model harnessing the finite volume method is employed, offering insights into the thermal response dynamics and paving the way for optimized operational protocols and target design refinements. Through this comprehensive analysis, we aim to advance the understanding of thermal phenomena in electron-target interactions, thereby bolstering the efficiency and safety of particle accelerator operations in diverse scientific applications.

Nuclear-matter saturation and symmetry energy within Δ -full chiral effective field theory

Nuclear saturation and the symmetry energy are key properties of low-energy nuclear physics that depend on fine details of the nuclear interaction. The equation of state around saturation is also an important anchor for extrapolations to higher densities and studies of neutron stars. Here we develop a unified statistical framework that uses realistic nuclear forces to link the theoretical modeling of finite nuclei and infinite nuclear matter. We construct fast and accurate emulators for nuclear-matter observables and employ an iterative history-matching approach to explore and reduce the enormous parameter domain of Δ-full chiral interactions. We perform rigorous uncertainty quantification and find that model calibration including O16 observables gives saturation predictions that are more precise than those that only use few-body data. Published by the American Physical Society 2024

BRAVER challenges students in radiation protection training in an international training

The nuclear industry is currently facing a significant demand for well-trained personnel. Due to the high market demand, it is essential to raise awareness among new target groups, including high school pupils and (pre-service) STEM teachers, about the potential and opportunities of pursuing a nuclear career. With this in mind, a new strategic partnership has been established under the Erasmus+ project ‘BRAVER’ (Blended and Remote teaching Activities supported by Virtual rEality for Radiation sciences). Within this 2-year project, international staff, and students from 7 partners of the CHERNE (Cooperation of Higher Education on Radiological and Nuclear Engineering) network collaborate with industry, regulatory and research institutes in developing educational virtual tools (VR and virtual online escape rooms) for nuclear sciences and engineering. The project aims to develop blended international training programs that incorporate technical, generic, and networking skills for both students and professors. This initiative can serve as a model for other scientific fields, extending its benefits to students and educators across different disciplines.

A Vision for the Science of Rare Isotopes

The field of nuclear science has considerably advanced since its beginning just over a century ago. Today, the science of rare isotopes is on the cusp of a new era with theoretical and computing advances complementing experimental capabilities at new facilities internationally. In this article we present a vision for the science of rare isotope beams (RIBs). We do not attempt to cover the full breadth of the field; rather, we provide a perspective and address a selection of topics that reflect our own interests and expertise. We focus in particular on systems near the drip lines, where one often finds nuclei that are referred to as exotic and where the role of the nuclear continuum is only just starting to be explored. An important aspect of this article is its attempt to highlight the crucial connections between nuclear structure and the nuclear reactions required to fully interpret and leverage the rich data to be collected in the next years at RIB facilities. Further, we connect the efforts in structure and reactions to key questions of nuclear astrophysics.

Dense Polarized Positrons from Beam-Solid Interaction.

Relativistic positron sources with high spin polarization have important applications in nuclear and particle physics and many frontier fields. However, it is challenging to produce dense polarized positrons. Here we present a simple and effective method to achieve such a positron source by directly impinging a relativistic high-density electron beam on the surface of a solid target. During the interaction, a strong return current of plasma electrons is induced and subsequently asymmetric quasistatic magnetic fields as high as megatesla are generated along the target surface. This gives rise to strong radiative spin flips and multiphoton processes, thus leading to efficient generation of copious polarized positrons. With three-dimensional particle-in-cell simulations, we demonstrate the production of a dense highly polarized multi-GeV positron beam with an average spin polarization above 40% and nC-scale charge per shot. This offers a novel route for the studies of laserless strong-field quantum electrodynamics physics and for the development of high-energy polarized positron sources.

Effects of Micro- and Nanosilica on the Mechanical and Microstructural Characteristics of Some Special Mortars Made with Recycled Concrete Aggregates.

In this paper, we study the influence of densified microsilica and colloidal nanosilica admixtures on the mechanical strength and the microstructural characteristics of special mortars used for immobilizing radioactive concrete waste. The experimental program focused on the replacement of cement with micro- and/or nanosilica, in different proportions, in the basic composition of a mortar made with recycled aggregates. The technical criteria imposed for such cementitious systems, used for the encapsulation of low-level radioactive waste, imply high fluidity, increased mechanical strength and lack of segregation and of bleeding. We aimed to increase the structural compactness of the mortars by adding micro- and nanosilica, all the while maintaining the technical criteria imposed, to obtain a cement matrix with high durability and increased capacity for immobilizing radionuclides. The samples from all the compositions obtained were analyzed from the point of view of mechanical strength. Also, micro- and nanosilica as well as samples of the optimal mortar compositions were analyzed physically and microstructurally. Experimental data showed that the mortar samples present maximum compressive strength for a content between 6 and 7.5% wt. of microsilica, respectively, for a content of 2.25% wt. nanosilica. The obtained results suggest a synergistic effect of micro- and nanosilica when they are used simultaneously in cementitious compositions. Thus, among the analyzed compositional variants, the mortar composition with 3% wt. microsilica and 2.25% wt. nanosilica showed the best performance, with an increase in compressive strength of 23.5% compared to the control sample (without micro- and nanosilica). Brunauer-Emmett-Teller (BET) analysis and scanning electron microscopy (SEM) images highlighted the decrease in pore diameter and the increase in structural compactness, especially for mortar samples with nanosilica content or a mixture of micro- and nanosilica. This study is useful in the field of recycling radioactive concrete resulting from the decommissioning of nuclear research or nuclear power reactors.

Analysis on the relationship between the Higgs boson and the standard model

In 1964, Peter Higgs proposed the Higgs mechanism, a theory explaining the generation mechanism of the property mass for gauge bosons. After that, physicists proposed many theories and experiments to prove the existence of the Higgs boson. Then in 2013, the European Organization for Nuclear Research (CERN) discovered the Higgs boson, and in the next ten years, physicists did a large amount of research about the boson, the other possible kinds of Higgs boson, and the pairs of Higgs boson. However, it is hard to prove those theories through experiments mainly due to the large mass of the Higgs boson. In this paper, the author discusses the process of particles getting mass and the significance of the Higgs boson. The history of the Higgs boson and its impact on the world is summarized, and some probable predictions of the future research orientation are proposed by summarizing the past research papers and concluding from those articles. Overall, physicists can do more research on the interactions between the Higgs bosons, whose sensitivity can be used to discover those possible particles in the future.