Nonlocal Correlations Research Articles

Underwater single photon 3D imaging with millimeter depth accuracy and reduced blind range.

Mono-static system benefits from its more flexible field of view and simplified structure, however, the backreflection photons from mono-static system lead to count loss for target detection. Counting loss engender range-blind, impeding the accurate acquisition of target depth. In this paper, count loss is reduced by introducing a polarization-based underwater mono-static single-photon imaging method, and hence reduced blind range. The proposed method exploits the polarization characteristic of light to effectively reduce the count loss of the target, thus improving the target detection efficiency. Experiments demonstrate that the target profile can be visually identified under our method, while the unpolarization system can not. Moreover, the ranging precision of system reaches millimeter-level. Finally, the target profile is reconstructed using non-local pixel correlations algorithm.

Bell Inequalities with Overlapping Measurements.

Which nonlocal correlations can be obtained, when a party has access to more than one subsystem? While traditionally nonlocality deals with spacelike separated parties, this question becomes important with quantum technologies that connect devices by means of small shared systems. Here, we study Bell inequalities where measurements of different parties can have overlap. This allows us to accommodate problems in quantum information such as the existence of quantum error correction codes in the framework of nonlocality. The scenarios considered show an interesting behavior with respect to Hilbert space dimension, overlap, and symmetry.

Quantifying hole-motion-induced frustration in doped antiferromagnets by Hamiltonian reconstruction

Unveiling the microscopic origins of quantum phases dominated by the interplay of spin and motional degrees of freedom constitutes one of the central challenges in strongly correlated many-body physics. When holes move through an antiferromagnetic spin background, they displace the positions of spins, which induces effective frustration in the magnetic environment. However, a concrete characterization of this effect in a quantum many-body system is still an unsolved problem. Here we present a Hamiltonian reconstruction scheme that allows for a precise quantification of hole-motion-induced frustration. We access non-local correlation functions through projective measurements of the many-body state, from which effective spin-Hamiltonians can be recovered after detaching the magnetic background from dominant charge fluctuations. The scheme is applied to systems of mixed dimensionality, where holes are restricted to move in one dimension, but SU(2) superexchange is two-dimensional. We demonstrate that hole motion drives the spin background into a highly frustrated regime, which can quantitatively be described by an effective J1–J2-type spin model. We exemplify the applicability of the reconstruction scheme to ultracold atom experiments by recovering effective spin-Hamiltonians of experimentally obtained 1D Fermi-Hubbard snapshots. Our method can be generalized to fully 2D systems, enabling promising microscopic perspectives on the doped Hubbard model.

Bipartite and tripartite steering by a nonlinear medium in a cavity

Nonlocal quantum correlations are important for potential applications in quantum optics and quantum information. Multipartite quantum correlations are relevant to access to high-dimensional systems such as qudits. There are also different proposals for the generation of quantum steering based on nonlinear systems and cavities. Here, we consider the Hamiltonian of a triple photon parametric down-conversion process to investigate the regions where bipartite and tripartite steering are generated. In this model, three beams interact with a nonlinear medium inside a cavity through the process of parametric down-conversion, creating three output fields. The positive P representation is used to analyze this system and steady-state solutions are obtained. We calculated the intracavity fluctuation spectra to analyze steering in the frequency domain and used different criteria to certify this quantum correlation. We certified bipartite steering for the three output fields from the cavity. In the case of full tripartite two-way steering inseparability, it is also present for all the bipartitions under consideration. Our results show regimes where bipartite and tripartite steering is certified for this model.

Bell nonlocality in maximal-length quantum mechanics

In this paper, we investigate the consequences of maximal length as well as minimal momentum scales on nonlocal correlations shared by two parties of a bipartite quantum system. To this aim, we rely on a general phenomenological scheme which is usually associated with the non-negligible spacetime curvature at cosmological scales, namely the extended uncertainty principle. In so doing, we find that quantum correlations are degraded if the deformed quantum mechanical model mimics a positive cosmological constant. This opens up the possibility to recover classicality at sufficiently large distances.

Coherently driven quantum features using a linear optics-based polarization-basis control

Quantum entanglement generation is generally known to be impossible by any classical means. According to Poisson statistics, coherent photons are not considered quantum particles due to the bunching phenomenon. Recently, a coherence approach has been applied for quantum correlations such as the Hong–Ou–Mandel (HOM) effect, Franson-type nonlocal correlation, and delayed-choice quantum eraser to understand the mysterious quantum features. In the coherence approach, the quantum correlation has been now understood as a direct result of selective measurements between product bases of phase-coherent photons. Especially in the HOM interpretation, it has been understood that a fixed sum-phase relation between paired photons is the bedrock of quantum entanglement. Here, a coherently excited HOM model is proposed, analyzed, and discussed for the fundamental physics of two-photon correlation using linear optics-based polarization-basis control. For this, polarization-frequency correlation in a Mach–Zehnder interferometer is coherently excited using synchronized acousto-optic modulators, where polarization-basis control is conducted via a selective measurement process of the heterodyne signals. Like quantum operator-based destructive interference in the HOM theory, a perfectly coherent analysis shows the same HOM effects of the paired coherent photons on a beam splitter, whereas individual output intensities are uniform.

Regionwise Generative Adversarial Image Inpainting for Large Missing Areas.

Recently, deep neural networks have achieved promising performance for in-filling large missing regions in image inpainting tasks. They have usually adopted the standard convolutional architecture over the corrupted image, leading to meaningless contents, such as color discrepancy, blur, and other artifacts. Moreover, most inpainting approaches cannot handle well the case of a large contiguous missing area. To address these problems, we propose a generic inpainting framework capable of handling incomplete images with both contiguous and discontiguous large missing areas. We pose this in an adversarial manner, deploying regionwise operations in both the generator and discriminator to separately handle the different types of regions, namely, existing regions and missing ones. Moreover, a correlation loss is introduced to capture the nonlocal correlations between different patches, and thus, guide the generator to obtain more information during inference. With the help of regionwise generative adversarial mechanism, our framework can restore semantically reasonable and visually realistic images for both discontiguous and contiguous large missing areas. Extensive experiments on three widely used datasets for image inpainting task have been conducted, and both qualitative and quantitative experimental results demonstrate that the proposed model significantly outperforms the state-of-the-art approaches, on the large contiguous and discontiguous missing areas.

Anatomy of localisation protected quantum order on Hilbert space

Many-body localised (MBL) phases of disordered, interacting quantum systems allow for exotic localisation protected quantum order in eigenstates at arbitrarily high energy densities. In this work, we analyse the manifestation of such order on the Hilbert-space anatomy of eigenstates. Quantified in terms of non-local Hilbert-spatial correlations of eigenstate amplitudes, we find that the spread of the eigenstates on the Hilbert-space graph is directly related to the order parameters which characterise the localisation protected order, and hence these correlations, in turn, characterise the order or lack thereof. Higher-point eigenstate correlations also characterise the different entanglement structures in the many-body localised phases, with and without order, as well as in the ergodic phase. The results pave the way for characterising the transitions between MBL phases and the ergodic phase in terms of scaling of emergent correlation lengthscales on the Hilbert-space graph.

Quantum correlations on the no-signaling boundary: self-testing and more

In device-independent quantum information, correlations between local measurement outcomes observed by spatially separated parties in a Bell test play a fundamental role. Even though it is long-known that the set of correlations allowed in quantum theory lies strictly between the Bell-local set and the no-signaling set, many questions concerning the geometry of the quantum set remain unanswered. Here, we revisit the problem of when the boundary of the quantum set coincides with the no-signaling set in the simplest Bell scenario. In particular, for each Class of these common boundaries containing k zero probabilities, we provide a (5−k)-parameter family of quantum strategies realizing these (extremal) correlations. We further prove that self-testing is possible in all nontrivial Classes beyond the known examples of Hardy-type correlations, and provide numerical evidence supporting the robustness of these self-testing results. Candidates of one-parameter families of self-testing correlations from some of these Classes are identified. As a byproduct of our investigation, if the qubit strategies leading to an extremal nonlocal correlation are local-unitarily equivalent, a self-testing statement provably follows. Interestingly, all these self-testing correlations found on the no-signaling boundary are provably non-exposed. An analogous characterization for the set M of quantum correlations arising from finite-dimensional maximally entangled states is also provided. En route to establishing this last result, we show that all correlations of M in the simplest Bell scenario are attainable as convex combinations of those achievable using a Bell pair and projective measurements. In turn, we obtain the maximal Clauser-Horne-Shimony-Holt Bell inequality violation by any maximally entangled two-qudit state and a no-go theorem regarding the self-testing of such states.

Computational Studies of Energetic Property Peculiarities in Trinitrophenyl-Substituted Nitramines

This research was performed using Becke’s three-parameter hybrid functional approach with non-local correlation provided by Lee, Yang, and Parr and the cc-pVTZ basis set. The geometry, total energy, and heat of formation of the most stable conformers of the nitramines under study were obtained to obtain the density, resistance to shock stimuli, detonation pressure, and velocity of the materials under study. The results obtained allow us to predict new multipurpose energetic materials with a good balance between energy and stability. Our findings show that N-(2-nitroethyl)-N-(2,4,6-trinitrophenyl)nitramine, N-(2,4,6-trinitrophenyl)-N-[(3,4,5-trinitro-1H-pyrazol-1-yl)methyl]nitramine, N-(2,2-dinitroethyl)-N-(2,4,6-trinitrophenyl)nitramine, N-(2,2,2-trinitroethyl)-N-(2,4,6-trinitrophenyl)nitramine, and N-(trinitromethyl)-N-(2,4,6-trinitrophenyl)nitramine possess better explosive properties and a greater stability compared to tetryl, although they remain sensitive to shock stimuli. Referring to the results obtained, we recommend new tetryl analogs containing dinitroethyl, trinitroethyl, and trinitromethyl substituents for practical usage.

PHAM-YOLO: A Parallel Hybrid Attention Mechanism Network for Defect Detection of Meter in Substation

Accurate detection and timely treatment of component defects in substations is an important measure to ensure the safe operation of power systems. In this study, taking substation meters as an example, a dataset of common meter defects, such as a fuzzy or damaged dial on the meter and broken meter housing, is constructed from the images of manual inspection in power systems. There are several challenges involved in accurately detecting defects in substation meter images, such as the complex background, different meter sizes and large differences in the shapes of meter defects. Therefore, this paper proposes the PHAM-YOLO (Parallel Hybrid Attention Mechanism You Only Look Once) network for automatic detection of substation meter defects. In order to make the network pay attention to the key areas against the complex background of the meter defect images and the differences between different defect features, a Parallel Hybrid Attention Mechanism (PHAM) module is designed and added to the backbone of YOLOv5. PHAM integration of local and non-local correlation information can highlight these differences while remaining focused on the meter defect features. To improve the expressive ability of the feature map, a Spatial Pyramid Pooling Fast (SPPF) module is introduced, which pools the input feature map using a continuous fixed convolution kernel, fusing the feature maps of different receptive fields. Bounding box regression (BBR) is the key way to determine object positioning performance in defect detection. EIOU (Efficient Intersection over Union) is, therefore, introduced as a boundary loss function to solve the ambiguity of the CIOU (Complete Intersection Over Union) loss function, making the BBR regression more accurate. The experimental results show that the Average Precision Mean (mAP), Precision (P) and Recall (R) of the proposed PHAM-YOLO network in the dataset are 78.3%, 78.3%, and 79.9%, respectively, with mAP being improved by 2.7% compared to the original model and higher than SSD, Fast R-CNN, etc.

Strong-correlation density functionals made simple

Recent work on incorporating strong-correlation (sc) corrections into the scLH22t local hybrid functional [A. Wodyński and M. Kaupp, J. Chem. Theory Comput. 18, 6111–6123 (2022)] used a hybrid procedure, applying a strong-correlation factor derived from the reverse Becke–Roussel machinery of the KP16/B13 and B13 functionals to the nonlocal correlation term of a local hybrid functional. Here, we show that adiabatic-connection factors for strong-correlation-corrected local hybrids (scLHs) can be constructed in a simplified way based on a comparison of semi-local and exact exchange-energy densities only, without recourse to exchange-hole normalization. The simplified procedure is based on a comparative analysis of Becke’s B05 real-space treatment of nondynamical correlation and that in LHs, and it allows us to use, in principle, any semi-local exchange-energy density in the variable used to construct local adiabatic connections. The derivation of competitive scLHs is demonstrated based on either a modified Becke–Roussel or a simpler Perdew–Burke–Ernzerhof (PBE) energy density, leading to the scLH23t-mBR and scLH23t-tPBE functionals, which both exhibit low fractional spin errors while retaining good performance for weakly correlated situations. We also report preliminary attempts toward more detailed modeling of the local adiabatic connection, allowing a reduction of unphysical local maxima in spin-restricted bond-dissociation energy curves (scLH23t-mBR-P form). The simplified derivations of sc-factors reported here provide a basis for future constructions and straightforward implementation of exchange-correlation functionals that escape the zero-sum game between low self-interaction and static-correlation errors.

Creating nonlocality using geometric phases between partially distinguishable photons

The geometric (Berry-Pancharatnam) phase originates from the intrinsic geometry of the space of quantum states and can be observed in different situations, such as a cyclic evolution of a quantum system. Here, we utilize the geometric phase to obtain a surprising insight: It is possible to create nonlocal correlations in a fixed interferometer with independent photon inputs by varying the photons' internal states. In particular, we consider a cyclic interferometer that is fixed, i.e., that has no variable internal phase shifts or subsequent measurement settings. Instead, the measurement choices of the different parties correspond to the internal states of the input photons which influence the observed correlations via a collective $N$-photon geometric phase, constituting a different approach for the generation of nonlocality with respect to the usual paradigm. We observe a trade-off between the geometric phases and the visibility of the many-photon interference, impeding the generation of nonlocality. However, by making use of the dynamical quantum Zeno effect, we show that nonlocality can be created in the fixed cyclic interferometer using 12 (or more) independent photons.

Exchange interactions in iron and nickel: DFT+DMFT study in paramagnetic phase

We analyze possible ways to calculate magnetic exchange interactions within the density functional theory plus dynamical mean-field theory (DFT+DMFT) approach in the paramagnetic phase. Using the susceptibilities obtained within the ladder DMFT approach together with the random phase approximation result for the Heisenberg model, we obtain bilinear exchange interactions. We show that the earlier obtained result of Stepanov et al. [Phys. Rev. Lett. 121, 037204 (2018); Phys. Rev. B 105, 155151 (2022)] corresponds to considering individual magnetic moments in each orbital in the leading-order approximation in the non-local correlations. We consider a more general approach and apply it to evaluate the effective magnetic parameters of iron and nickel. We show that the analysis, based on the inverse orbital-summed susceptibilities, yields reasonable results for both, weak and strong magnets. For iron we find, in the low-temperature limit, the exchange interaction $J_0\simeq 0.20$ eV, while for nickel we obtain $J_0\simeq 1.2$ eV. The considered method also allows one to describe the spin-wave dispersion at temperatures $T\sim T_C$, which is in agreement with the experimental data.

Introducing a novel C50N10 azafullerene with chained nitrogen atoms on a buckyball pole: structure, stability, vibration, and electronic properties.

Fullerenes are of high significance due to their unique chemical properties and various applications in technology, particularly materials science, drug delivery, electronics, and nanoelectronics. In the recent years, many attempts have been focused to introduce new heteroatom-doped fullerenes having advanced chemical properties and tunable electronic traits, which make them a potential candidate for application in many branches of sciences. In this study, a novel C50N10 azafullerene with a fascinating structure of chained nitrogen atoms on a buckyball pole, with different electronic and optical properties compared to its other analogs, is introduced and trace of N-N substructures on the surface of C60 fullerene cage is investigated. For this molecule, four structural isomers including 3 structures with chain N atoms on a fullerene buckyball pole (NP isomers) and one isomer with separated N atoms (SN isomer) have been studied. All isomers have been studied with and without symmetry constraints, and the symmetry influence on the structure and stability of each isomer has been investigated. Although the studied NP structures have lower stability than the SN isomer, some reasons (such as their more all-carbon hexagonal rings, breaking some of their N-N bonds for partial opening of the cage and creating bigger rings in order to get rid of the unfavorable strain, as well as decreasing the N-N lone pair repulsions) lead to the acceptable stability of these structures with the bonded N atoms. The results of atomization energy and vibrational frequency calculations indicate that isomers with the bonded N atoms have acceptable stabilities and do not decompose into their constituent components. Investigation on the structural parameters demonstrates important roles of the number of all-carbon hexagonal rings, the number of N-N junction, and the molecule symmetry in the stability of the structures with the bonded N atoms. Study on the electronic and optical properties indicates that the target structures exhibit high electronic polarizability, relatively small HOMO/LUMO gap, high first- and second-order hyperpolarizability, and also large third-order nonlinear optical properties. All calculations have been performed using Gaussian G09 software using density functional theory (DFT) approach. Three-parameter Beck hybrid exchange functional (B3) hybridized with nonlocal correlation functional of Lee, Yang, and Parr (LYP) has been employed as the level of DFT calculations. All optimizations have been performed at double-zeta polarized (DZP) split valence 6-31G(d,p) and also at split valence TZP 6-311G(d,p) basis sets. The global minimum structures have been confirmed by frequency calculations at the same level of optimizations. The natural bond orbital (NBO) analyses, frontier orbital surfaces imaging, atomic charges, and charge transfer analyses have been achieved by GenNBO program package.

Distilling Nonlocality in Quantum Correlations.

Nonlocality, as established by the seminal Bell's theorem, is considered to be the most striking feature of correlations present in spacelike separated events. Its practical application in device independent protocols, such as secure key distribution, randomness certification, etc., demands identification and amplification of such correlations observed in the quantum world. In this Letter we study the prospect of nonlocality distillation, wherein, by applying a natural set of free operations (called wirings) on many copies of weakly nonlocal systems, one aims to generate correlations of higher nonlocal strength. In the simplest Bell scenario, we identify a protocol, namely, logical OR-AND wiring, that can distill nonlocality to a significantly high degree starting from arbitrarily weak quantum nonlocal correlations. As it turns out, our protocol has several interesting facets: (i)it demonstrates that a set of distillable quantum correlations has nonzero measure in the full eight-dimensional correlation space, (ii)it can distill quantum Hardy correlations by preserving its structure, (iii)it shows that (nonlocal) quantum correlations sufficiently close to the local deterministic points can be distilled by a significant amount. Finally, we also demonstrate efficacy of the considered distillation protocol in detecting postquantum correlations.

Scalable Bell inequalities for graph states of arbitrary prime local dimension and self-testing

Bell nonlocality—the existence of quantum correlations that cannot be explained by classical means—is certainly one of the most striking features of quantum mechanics. Its range of applications in device-independent protocols is constantly growing. Many relevant quantum features can be inferred from violations of Bell inequalities, including entanglement detection and quantification, and state certification applicable to systems of arbitrary number of particles. A complete characterisation of nonlocal correlations for many-body systems is, however, a computationally intractable problem. Even if one restricts the analysis to specific classes of states, no general method to tailor Bell inequalities to be violated by a given state is known. In this work we provide a general construction of Bell expressions tailored to the graph states of any prime local dimension. These form a broad class of multipartite quantum states that have many applications in quantum information, including quantum error correction. We analytically determine their maximal quantum values, a number of high relevance for device-independent applications of Bell inequalities. Importantly, the number of expectation values to determine in order to test the violation of our inequalities scales only linearly with the system size, which we expect to be the optimal scaling one can hope for in this case. Finally, we show that these inequalities can be used for self-testing of multi-qutrit graph states such as the well-known four-qutrit absolutely maximally entangled state AME(4,3).

CASPI: collaborative photon processing for active single-photon imaging

Image sensors capable of capturing individual photons have made tremendous progress in recent years. However, this technology faces a major limitation. Because they capture scene information at the individual photon level, the raw data is sparse and noisy. Here we propose CASPI: Collaborative Photon Processing for Active Single-Photon Imaging, a technology-agnostic, application-agnostic, and training-free photon processing pipeline for emerging high-resolution single-photon cameras. By collaboratively exploiting both local and non-local correlations in the spatio-temporal photon data cubes, CASPI estimates scene properties reliably even under very challenging lighting conditions. We demonstrate the versatility of CASPI with two applications: LiDAR imaging over a wide range of photon flux levels, from a sub-photon to high ambient regimes, and live-cell autofluorescence FLIM in low photon count regimes. We envision CASPI as a basic building block of general-purpose photon processing units that will be implemented on-chip in future single-photon cameras.

DFT screening exchange sX-LDA approach to study the origin of the indirect band gap of hexagonal boron nitride in its most stable phase

The present study is a theoretical work of the effect of the nonlocal screened exchange within the local density approximation (sX-LDA) functional on the structural and electronic properties of hexagonal Boron Nitride (h-BN). We obtained a visible renormalization of the band structure due to the inclusion of nonlocal correlation effects. Furthermore, we demonstrated that h-BN with AA’ stacking have an indirect band gap and the origin of the h-BN band gap width and its nature are strongly affected by Nitrogen electronic band structure. Here, we discuss also the exact nature of h-BN band gap and its value to give a sense to the wide variety of results obtained in the literature.

Thermal Fisher and Wigner–Yanase information correlations in two-qubit Heisenberg XYZ chain

Using Wigner–Yanase and Fisher information [including local quantum uncertainty (LQU) and local quantum Fisher information (LQFI)] as well as log-negativity, we investigate the thermal non-local correlations of two-qubit Heisenberg XYZ non-X states produced in the presence of the Dzyaloshinskii–Moriya (DM) interaction. The two-spin XYZ-Heisenberg non-local correlation decay can be weakened by increasing the DM interaction as well as the spin–spin XYZ-Heisenberg interactions. The LQFI correlation has greater resistance to thermal degradation. The spin–spin y-component antiferromagnetic coupling has a higher ability to protect the generated spin–spin nonlocal correlations against high temperatures. The emergence of the phenomena of the sudden death of log-negativity and the sudden change of the LQFI and LQU depend on the spin–spin XYZ-Heisenberg and DM interactions as well as on the bath temperature. The generated asymmetric correlations resulting due to the x,y-component spin interactions confirm that the antiferromagnetic coupling has a high ability to generate a maximally correlated two-qubit state. While the generated correlations, due to two-spin z-component interaction, present symmetric dynamics, and its amount depends on the x-component spin interaction.