We review the operating principles of noncollinear acousto-optic tunable filters (AOTF's), emphasizing the use of two orthogonally polarized beams for narrow-band imaging. Spectral characterization and spectral broadening measurements of commercially available AOTF's agree with theoretical predictions and reveal difficulties associated with imaging noncollimated light. An AOTF imaging spectropolarimeter for ground-based astronomy that uses CCD's has been constructed at NASA Goddard Space Flight Center. It uses a TeO(2) noncollinear AOTF and a simple optical relay assembly to produce side-by-side orthogonally polarized spectral images. We summarize the instrument design and initial performance tests. We include sample spectral images acquired at the Goddard Geophysical and Astronomical Observatory.