Nonlocal Transport Research Articles

Contact-induced charge contributions to non-local spin transport measurements in Co/MgO/graphene devices

Recently, it has been shown that oxide barriers in graphene-based non-local spin-valve structures can be the bottleneck for spin transport. The barriers may cause spin dephasing during or right after electrical spin injection which limits spin transport parameters such as the spin lifetime of the whole device. An important task is to characterize the quality of the oxide barriers of both spin injection and detection contacts in a fabricated device. To address this issue, we discuss the influence of spatially inhomogeneous oxide barriers and especially conducting pinholes within the barriers on the background signal in non-local measurements of graphene/MgO/Co spin-valve devices. By both simulations and reference measurements on devices with non-ferromagnetic electrodes, we demonstrate that the background signal can be caused by an inhomogeneous current flow through the oxide barriers. As a main result, we demonstrate the existence of charge accumulation besides the actual spin accumulation signal in non-local voltage measurements, which can be explained by a redistribution of charge carriers by a perpendicular magnetic field similar to the classical Hall effect. Furthermore, we present systematic studies of the phase of the low frequency non-local ac voltage signal which is measured in non-local spin measurements when applying ac lock-in techniques. This phase has so far widely been neglected in the analysis of non-local spin transport. We demonstrate that this phase is another hallmark of the homogeneity of the MgO spin injection and detection barriers. We link backgate dependent changes of the phase to the interplay between the capacitance of the oxide barrier and the quantum capacitance of graphene.

Microscopic studies of nonlocal spin dynamics and spin transport (invited)

Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.

Equivalence of gradient flows and entropy solutions for singular nonlocal interaction equations in 1D

We prove the equivalence between the notion of Wasserstein gradient flow for a one- dimensional nonlocal transport PDE with attractive/repulsive Newtonian potential on one side, and the notion of entropy solution of a Burgers-type scalar conservation law on the other. The solution of the former is obtained by spatially differentiating the solution of the latter. The proof uses an intermediate step, namely the L 2 gradient flow of the pseudo-inverse distribution function of the gradient flow solution. We use this equivalence to provide a rigorous particle-system approximation to the Wasserstein gradient flow, avoiding the regularization effect due to the singularity in the repulsive kernel. The abstract particle method relies on the so-called wave-front-tracking algorithm for scalar conservation laws. Finally, we provide a characterization of the subdifferential of the functional involved in the Wasserstein gradient flow.

Optothermal Modeling of Plasmonic Nanofocusing Structures With Nonlocal Optical Response and Ballistic Heat Transport

Nanoscale optical energy focusing using plasmonic structures is crucial for many applications, such as imaging and lithography. Thermal management for these nanostructures is of great importance to maintain their reliabilities but has not been investigated extensively yet, especially when the strong nonlocalities present in the nanostructures. Here, we report a multiphysics model to study the coupled optical and thermal responses of plasmonic nanofocusing structures. We applied the hydrodynamic Drude model to describe the nonlocality in the optical response and derived ballistic–diffusive equations for both electrons and phonons to model the nonlocal thermal transport. Strong nonlocal optothermal responses were observed.

Influence of spatial geometrical curvature on nonlocal electron heat transport in expanding plasmas

The electron thermal transport in fluid theory would be inaccurate when the collisionality is not enough, and the Fokker-Planck (FP) simulations are usually employed to resolve the inadequacies. In this paper, the one-dimensional Fokker-Planck code is extended to handle the cylindrical and spherical geometries in which the electron distribution functions are solved in the reference frame of the ion fluid. The FP code is validated in the fluid limit by comparing with fluid (MULTI) simulations. Then, the expansions of plasmas in different spatial geometries are simulated with the FP and fluid codes. As the main characters of nonlocal transport, the electron thermal transport inhibition and preheating are investigated in expanding plasmas. The spherical nonlocal theory can give the thermal transport inhibition and preheating phenomenon, which is exploited to fit the heat flux with variation of fitting parameter . The spherical nonlocal theory will reproduce Spizer-Hrm expression as = 0. Then we analyze the heat flux after the plasma expanding 200 ps with a uniform initial temperature T = 100 eV and density ne= 1 1021 /cm3. By comparing the heat flux computed by spherical nonlocal thermal transport theory and FP simulation, it is found that (n-1)/r term in Eq. (3a) cannot be neglected when the radius is small and the geometrical curvature effect will decrease the nonlocality of transport in outer expanding plasmas. The geometrical curvature effect leads to a smaller thermal transport inhibition and preheating in the expanding plasmas as comparing the spherical case with the planar one. The expansions of plasmas in different spatial geometries are also simulated with the FP and fluid codes under the initial conditions which are similar to the inertial confinement fusion. The same influence of geometrical curvature on nonlocal electron thermal transport are also obtained.

Representation of the Subgrid-Scale Turbulent Transport in Convective Boundary Layers at Gray-Zone Resolutions

Abstract Parameterization of the unresolved vertical transport in the planetary boundary layer (PBL) is one of the key physics algorithms in atmospheric models. This study attempts to represent the subgrid-scale (SGS) turbulent transport in convective boundary layers (CBLs) at gray-zone resolutions by investigating the effects of grid-size dependency in the vertical heat transport parameterization for CBL simulations. The SGS transport profile is parameterized based on the 2013 conceptual derivation by Shin and Hong. First, nonlocal transport via strong updrafts and local transport via the remaining small-scale eddies are separately calculated. Second, the SGS nonlocal transport is formulated by multiplying a grid-size dependency function with the total nonlocal transport profile fit to the large-eddy simulation (LES) output. Finally, the SGS local transport is formulated by multiplying a grid-size dependency function with the total local transport profile, which is calculated using an eddy-diffusivity formula. The new algorithm is evaluated against the LES output and compared with a conventional nonlocal PBL parameterization. For ideal CBL cases, by considering the scale dependency in the parameterized vertical heat transport, improvements over the conventional nonlocal K-profile model appear in mean profiles, resolved and SGS vertical transport profiles with their grid-size dependency, and the energy spectrum. Real-case simulations for convective rolls show that the simulated roll structures are more robust with stronger intensity when the new algorithm is used.

Towards an emerging understanding of non-locality phenomena and non-local transport

In this paper, recent progress on experimental analysis and theoretical models for non-local transport (non-Fickian fluxes in real space) is reviewed. The non-locality in the heat and momentum transport observed in the plasma, the departures from linear flux-gradient proportionality, and externally triggered non-local transport phenomena are described in both L-mode and improved-mode plasmas. Ongoing evaluation of ‘fast front’ and ‘intrinsically non-local’ models, and their success in comparisons with experimental data, are discussed

Spin transport in graphene nanostructures

Graphene is an interesting material for spintronics, showing long spin relaxation lengths even at room temperature. For future spintronic devices it is important to understand the behavior of the spins and the limitations for spin transport in structures where the dimensions are smaller than the spin relaxation length. However, the study of spin injection and transport in graphene nanostructures is highly unexplored. Here we study the spin injection and relaxation in nanostructured graphene with dimensions smaller than the spin relaxation length. For graphene nanoislands, where the edge length to area ratio is much higher than for standard devices, we show that enhanced spin-flip processes at the edges do not seem to play a major role in the spin relaxation. On the other hand, contact induced spin relaxation has a much more dramatic effect for these low dimensional structures. By studying the nonlocal spin transport through a graphene quantum dot we observe that the obtained values for spin relaxation are dominated by the connecting graphene islands and not by the quantum dot itself. Using a simple model we argue that future nonlocal Hanle precession measurements can obtain a more significant value for the spin relaxation time for the quantum dot by using high spin polarization contacts in combination with low tunneling rates.

Local electrical tuning of the nonlocal signals in a Cooper pair splitter

A Cooper pair splitter consists of a central superconducting contact, S, from which electrons are injected into two parallel, spatially separated quantum dots (QDs). This geometry as well as electron interactions can lead to correlated electrical currents due to the spatial separation of spin-singlet Cooper pairs from S. We present experiments on such a device with a series of bottom gates, which allows for spatially resolved tuning of the tunnel couplings between the QDs and the electrical contacts and between the two QDs. Our main findings are gate-induced transitions between positive conductance correlation in the QDs due to Cooper pair splitting and negative correlations due to QD dynamics. Using a semiclassical rate equation model we show that the experimental findings are consistent with in situ electrical tuning of the local and nonlocal quantum transport processes. In particular, we illustrate how the competition between Cooper pair splitting and local processes can be optimized in such hybrid nanostructures.

APTWG: The 4th Asia-Pacific Transport Working Group Meeting

This conference report summarizes the contributions to, and discussions at, the 4th Asia-Pacific Transport Working Group Meeting held at Kyushu University, Japan, during 10–13 June 2014. The topics of the meeting were organized under five main headings: turbulence suppression and transport barrier formation, effect of magnetic topology on MHD activity and transport, non-diffusive contribution of momentum and particle transport, non-local transport and turbulence spreading and coupling, energetic particles and instability. The Young Researchers' Forum which was held in this meeting is also described in this report.

Nonlocal transport mediated by spin supercurrents

In thin film ferromagnets with perfect easy-plane anisotropy, the component of total spin perpendicular to the easy plane is a good quantum number and the corresponding spin supercurrent can flow without dissipation. In this Letter we explain how spin supercurrents couple spatially remote spin-mixing vertical transport channels, even when easy-plane anisotropy is imperfect, and discuss the possibility that this effect can be used to fabricate new types of electronic devices.

Noncollinear Andreev reflections in semiconductor nanowires

We show that noncollinear Andreev reflections can be induced at interfaces of semiconductor nanowires with spin-orbit coupling, Zeeman splitting, and proximity-induced superconductivity. In a noncollinear local Andreev reflection, the spin polarizations of the injected and the retro-reflected carriers are typically at an angle that is tunable via system parameters. While in a nonlocal transport, this noncollinearity enables us to identify and block, at different voltage configurations, the noncollinear cross Andreev reflection and the direct charge transfer processes. We demonstrate that the intriguing noncollinearity originates from the spin-dependent coupling between carriers in the lead and the lowest discrete states in the wire, which, for a topological superconducting nanowire, are related to the overlap-induced hybridization of Majorana edge states in a finite system. These interesting phenomena can be observed in semiconductor nanowires of experimentally relevant lengths, and are potentially useful for spintronics.

Spintronics with graphene-hexagonal boron nitride van der Waals heterostructures

Hexagonal boron nitride (h-BN) is a large bandgap insulating isomorph of graphene, ideal for atomically thin tunnel barrier applications. In this letter, we demonstrate large area chemical vapor deposited (CVD) h-BN as a promising spin tunnel barrier in graphene spin transport devices. In such structures, the ferromagnetic tunnel contacts with h-BN barrier are found to show robust tunneling characteristics over a large scale with resistances in the favorable range for efficient spin injection into graphene. The non-local spin transport and precession experiments reveal spin lifetime ≈500 ps and spin diffusion length ≈1.6 μm in graphene with tunnel spin polarization ≈11% at 100 K. The electrical and spin transport measurements at different injection bias current and gate voltages confirm tunnel spin injection through h-BN barrier. These results open up possibilities for implementation of large area CVD h-BN in spintronic technologies.

Nonlocal thermal transport across embedded few-layer graphene sheets

Thermal transport across the interfaces between few-layer graphene sheets and soft materials exhibits intriguing anomalies when interpreted using the classical Kapitza model, e.g. the conductance of the same interface differs greatly for different modes of interfacial thermal transport. Using atomistic simulations, we show that such thermal transport follows a nonlocal flux-temperature drop constitutive law and is characterized jointly by a quasi-local conductance and a nonlocal conductance instead of the classical Kapitza conductance. The nonlocal model enables rationalization of many anomalies of the thermal transport across embedded few-layer graphene sheets and should be used in studies of interfacial thermal transport involving few-layer graphene sheets or other ultra-thin layered materials.

Nonlocal nonlinear coupling of kinetic sound waves

Abstract. We study three-wave resonant interactions among kinetic-scale oblique sound waves in the low-frequency range below the ion cyclotron frequency. The nonlinear eigenmode equation is derived in the framework of a two-fluid plasma model. Because of dispersive modifications at small wavelengths perpendicular to the background magnetic field, these waves become a decay-type mode. We found two decay channels, one into co-propagating product waves (forward decay), and another into counter-propagating product waves (reverse decay). All wavenumbers in the forward decay are similar and hence this decay is local in wavenumber space. On the contrary, the reverse decay generates waves with wavenumbers that are much larger than in the original pump waves and is therefore intrinsically nonlocal. In general, the reverse decay is significantly faster than the forward one, suggesting a nonlocal spectral transport induced by oblique sound waves. Even with low-amplitude sound waves the nonlinear interaction rate is larger than the collisionless dissipation rate. Possible applications regarding acoustic waves observed in the solar corona, solar wind, and topside ionosphere are briefly discussed.

Non-local parallel transport in BOUT++

Non-local closures allow kinetic effects on parallel transport to be included in fluid simulations. This is especially important in the scrape-off layer, but to be useful there the non-local model requires consistent kinetic boundary conditions at the sheath. A non-local closure scheme based on solution of a kinetic equation using a diagonalized moment expansion has been previously reported. We derive a method for imposing kinetic boundary conditions in this scheme and discuss their implementation in BOUT++. To make it feasible to implement the boundary conditions in the code, we are lead to transform the non-local model to a different moment basis, better adapted to describe parallel dynamics. The new basis has the additional benefit of enabling substantial optimization of the closure calculation, resulting in an O(10) speedup of the non-local code.

Exotic circuit elements from zero-modes in hybrid superconductor–quantum-Hall systems

Heterostructures formed by quantum Hall systems and superconductors have recently been shown to support widely coveted Majorana fermion zero-modes and still more exotic `parafermionic' generalizations. Here we establish that probing such zero-modes using quantum Hall edge states yields non-local transport signatures that pave the way towards a variety of novel circuit elements. In particular, we demonstrate quite generally that at low energies the zero-modes convert chirally moving quasiparticles into oppositely charged quasiholes propagating in the same direction---that is, they swap the sign of the chiral edge currents. One may then construct new and potentially useful circuit elements using this `perfect Andreev conversion' process, including superconducting current and voltage mirrors as well as transistors for fractional charge currents. Characterization of these circuit elements should provide striking evidence of the zero-mode physics.

Transport equation describing fractional Lévy motion of suprathermal ions in TORPEX

Suprathermal ions, created by fusion reactions or by additional heating, will play an important role in burning plasmas such as the ones in ITER or DEMO. Basic plasma experiments, with easy access for diagnostics and well-controlled plasma scenarios, are particularly suitable to investigate the transport of suprathermal ions in plasma waves and turbulence. Experimental measurements and numerical simulations have revealed that the transport of fast ions in the presence of electrostatic turbulence in the basic plasma toroidal experiment TORPEX is generally non-classical. Namely, the mean-squared radial displacement of the ions does not scale linearly with time, but 〈r2(t)〉 ∼ tγ, with γ ≠ 1 generally, γ > 1 corresponding to superdiffusion and γ < 1 to subdiffusion. A generalization of the classical model of diffusion, the so-called fractional Lévy motion, which encompasses power-law (Lévy) statistics for the displacements and correlated temporal increments, leads to non-classical dynamics such as that observed in the experiments. On a macroscopic scale, this results in fractional differential operators, which are used to model non-Gaussian, non-local anomalous transport in a growing number of applied fields, including plasma physics. In this paper, we show that asymmetric fractional Lévy motion can be described by a diffusion equation using space-fractional differential operator with skewness. Numerical simulations of tracers in TORPEX turbulence are performed. The time evolution of the radial particle position distribution is shown to be described by solutions of the fractional diffusion equation corresponding to asymmetric fractional Lévy motion in sub- and superdiffusive cases.

Scale-invariant quantum anomalous Hall effect in magnetic topological insulators beyond the two-dimensional limit.

We investigate the quantum anomalous Hall effect (QAHE) and related chiral transport in the millimeter-size (Cr(0.12)Bi(0.26)Sb(0.62))₂Te₃ films. With high sample quality and robust magnetism at low temperatures, the quantized Hall conductance of e²/h is found to persist even when the film thickness is beyond the two-dimensional (2D) hybridization limit. Meanwhile, the Chern insulator-featured chiral edge conduction is manifested by the nonlocal transport measurements. In contrast to the 2D hybridized thin film, an additional weakly field-dependent longitudinal resistance is observed in the ten-quintuple-layer film, suggesting the influence of the film thickness on the dissipative edge channel in the QAHE regime. The extension of the QAHE into the three-dimensional thickness region addresses the universality of this quantum transport phenomenon and motivates the exploration of new QAHE phases with tunable Chern numbers. In addition, the observation of scale-invariant dissipationless chiral propagation on a macroscopic scale makes a major stride towards ideal low-power interconnect applications.

Manifestation of two-channel nonlocal spin transport in the shapes of Hanle curves

Dynamics of charge-density fluctuations in a system of two tunnel-coupled wires contains two diffusion modes with dispersion iw=Dq^2 and iw =Dq^2+2/tau_t, where D is the diffusion coefficient and tau_t is the tunneling time between the wires. The dispersion of corresponding spin-density modes depends on magnetic field as a result of spin precession with Larmour frequency, w_L. The presence of two modes affects the shape of the Hanle curve describing the spin-dependent resistance, R, between ferromagnetic strips covering the non-magnetic wires. We demonstrate that the relative shapes of the R(w_L)-curves, one measured within the same wire and the other measured between the wires, depends on the ratio tau_t/tau_s, where tau_s is the spin-diffusion time. If the coupling between the wires is local, i.e. only at the point x=0, then the difference of the shapes of intra-wire and inter-wire Hanle curves reflects the difference in statistics of diffusive trajectories which "switch" or do not switch near x=0. When one of the coupled wires is bent into a loop with a radius, a, the shape of the Hanle curve reflects the statistics of random walks on the loop. This statistics is governed by the dimensionless parameter, a/(D tau_s)^(1/2).