ABSTRACT Scanning jet electrodeposition (SJE) is a promising method for electrodeposition. Integrated with automation and machine learning, intelligent electrodeposition can be achieved. In this study, a machine learning method was used to develop the relationship between the process parameters and properties of Ni-Co alloys produced by SJE. To evaluate the various models, the coefficient of determination (R 2), mean absolute percentage error (MAPE), and root mean square error (RMSE) were calculated as performance metrics. The multivariate nonlinear regression (MNR) model shows a higher R 2, lower MAPE and RMSE values, and better performance in both the training and testing sets, indicating superior approximation and prediction accuracies for microhardness. A back-propagation artificial neural network (BP-ANN) shows stable R 2 value of closest to 1, and the lowest MAPE and RMSE for corrosion current density and presents an exceptional generalisation ability. Finally, under the present experimental conditions, the highest microhardness and corresponding process parameters were determined using the MNR model, and the lowest corrosion current density was optimised using the BP-ANN model.
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