This article proposes a nonlinear feedback control methodology for spatially inhomogeneous aerosol processes for which the manipulated inputs, the control objectives and the measurements are distributed in space. Initially, a general nonlinear partial integro-differential equation model which describes the spatio-temporal evolution of the aerosol size distribution, as well as the evolution of the concentrations of species and temperature of the continuous phase is presented. The model accounts for simultaneous chemical reaction, nucleation, condensation, coagulation and convective transport. Then, under the assumption of lognormal aerosol size distribution, the method of moments is employed to reduce the original model into a set of first-order hyperbolic partial differential equations (PDEs) which accurately describes the spatio-temporal evolution of the three leading moments needed to precisely characterize the aerosol size distribution. This hyperbolic PDE system is then used as the basis for the synthesis of nonlinear distributed output feedback controllers that enforce closed-loop stability and achieve an aerosol size distribution with desired characteristics. The proposed nonlinear control method is successfully applied through simulations to a typical aerosol process and is shown to outperform a conventional proportional integral control scheme and deal effectively with disturbances in the feed to the process.
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