non-Fermi Liquid Behavior Research Articles

Charge Kondo circuit as a detector for electron-electron interactions in a Luttinger liquid

We investigate the effects of the electron-electron interactions on the quantum transport through a charge Kondo circuit. The setup consists of a quantum dot sandwiched between two leads by two nearly transparent single mode quantum point contacts. The size of the interacting area $L$ in the Luttinger liquid formed in the vicinities of the narrow constrictions is assumed to be much smaller compared to the size of the quantum dot $a$. We predict that the interplay between the electron-electron interactions in the Luttinger liquid and the fingerprints of the non-Fermi liquid behavior in the vicinity of the two channel Kondo intermediate coupling fixed point allows to determine the interaction strength through the power-law temperature scaling of the electric conductance.

Non-Hertz-Millis scaling of the antiferromagnetic quantum critical metal via scalable Hybrid Monte Carlo

A key component of the phase diagram of many iron-based superconductors and electron-doped cuprates is believed to be a quantum critical point (QCP), delineating the onset of antiferromagnetic spin-density wave order in a quasi-two-dimensional metal. The universality class of this QCP is believed to play a fundamental role in the description of the proximate non-Fermi liquid behavior and superconducting phase. A minimal model for this transition is the O(3) spin-fermion model. Despite many efforts, a definitive characterization of its universal properties is still lacking. Here, we numerically study the O(3) spin-fermion model and extract the scaling exponents and functional form of the static and zero-momentum dynamical spin susceptibility. We do this using a Hybrid Monte Carlo (HMC) algorithm with a novel auto-tuning procedure, which allows us to study unprecedentedly large systems of 80 × 80 sites. We find a strong violation of the Hertz-Millis form, contrary to all previous numerical results. Furthermore, the form that we do observe provides good evidence that the universal scaling is actually governed by the analytically tractable fixed point discovered near perfect “hot-spot’" nesting, even for a larger nesting window. Our predictions can be directly tested with neutron scattering. Additionally, the HMC method we introduce is generic and can be used to study other fermionic models of quantum criticality, where there is a strong need to simulate large systems.

Probing a Bose metal via electrons: inescapable non-Fermi liquid scattering and pseudogap physics

Non-Fermi liquid behavior and pseudogap formation are among the most well-known examples of exotic spectral features observed in several strongly correlated materials such as the hole-doped cuprates, nickelates, iridates, ruthenates, ferropnictides, doped Mott organics, transition metal dichalcogenides, heavy fermions, d- and f-electron metals, etc. We demonstrate that these features are inevitable consequences when fermions couple to an unconventional Bose metal (Hegg et al 2021 Proc. Natl. Acad. Sci. 118) mean field consisting of lower-dimensional coherence. Not only do we find both exotic phenomena, but also a host of other features that have been observed e.g. in the cuprates including nodal anti-nodal dichotomy and pseudogap asymmetry (symmetry) in momentum (real) space. Obtaining these exotic and heretofore mysterious phenomena via a mean field offers a simple, universal, and therefore widely applicable explanation for their ubiquitous empirical appearance.

Non-Fermi liquid behavior at flat hot spots from quantum critical fluctuations at the onset of charge- or spin-density wave order

We analyze quantum fluctuation effects at the onset of charge- or spin-density wave order with a $2{k}_{F}$ wave vector $\mathbf{Q}$ in two-dimensional metals, for the special case where $\mathbf{Q}$ connects a pair of hot spots situated at high symmetry points of the Fermi surface with a vanishing Fermi surface curvature. We compute the order parameter susceptibility and the fermion self-energy in one-loop approximation. The susceptibility has a pronounced peak at $\mathbf{Q}$, and the self-energy displays non-Fermi liquid behavior at the hot spots, with a linear frequency dependence of its imaginary part. The real part of the one-loop self-energy exhibits logarithmic divergencies with universal prefactors as a function of both frequency and momentum, which may be interpreted as perturbative signatures of power laws with universal anomalous dimensions. As a result, one obtains a non-Fermi liquid metal with a vanishing quasiparticle weight at the hot spots, and a renormalized dispersion relation with anomalous algebraic momentum dependencies near the hot spots.

Pressure induced insulator to metal transition in quantum spin liquid candidate NaYbS2

Pressure induced insulator to metal transition followed by the appearance of superconductivity has been observed recently in inorganic quantum spin liquid candidate NaYbSe2. In this paper, we study the properties of isostructural compound NaYbS2 under pressure. It is found that the resistance of NaYbS2 single crystal exhibits an insulating state below 82.9 GPa, but with a drop of more than six orders of magnitude at room temperature. Then a minimum of resistance is observed at about 100.1 GPa and it moves to lower temperature with further compression. Finally, a metallic state in the whole temperature range is observed at about 130.3 GPa accompanied by a non-Fermi liquid behavior below 100 K. The insulator to metal transition, non-monotonic resistance feature and non-Fermi liquid behavior of NaYbS2 under pressure are similar to those of NaYbSe2, suggesting that these phenomena might be the universal properties in NaLnCh 2 (Ln = rare earth, Ch = O, S, Se) system.

Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La2O3Fe2Se2

The insulator-metal transition in Mott insulators, known as the Mott transition, is usually accompanied with various novel quantum phenomena, such as unconventional superconductivity, non-Fermi liquid behavior and colossal magnetoresistance. Here, based on high-pressure electrical transport and XRD measurements, and first-principles calculations, we find that a unique pressure-induced Mott transition from an antiferromagnetic Mott insulator to a ferromagnetic Weyl metal in the iron oxychalcogenide La2O3Fe2Se2 occurs around 37 GPa without structural phase transition. Our theoretical calculations reveal that such an insulator-metal transition is mainly due to the enlarged bandwidth and diminishing of electron correlation at high pressure, fitting well with the experimental data. Moreover, the high-pressure ferromagnetic Weyl metallic phase possesses attractive electronic band structures with six pairs of Weyl points close to the Fermi level, and its topological property can be easily manipulated by the magnetic field. The emergence of Weyl fermions in La2O3Fe2Se2 at high pressure may bridge the gap between nontrivial band topology and Mott insulating states. Our findings not only realize ferromagnetic Weyl fermions associated with the Mott transition, but also suggest pressure as an effective controlling parameter to tune the emergent phenomena in correlated electron systems.

Interplay of superconductivity and localization near a two-dimensional ferromagnetic quantum critical point

We study the superconducting instability of a two-dimensional disordered Fermi liquid weakly coupled to the soft fluctuations associated with proximity to an Ising-ferromagnetic quantum critical point. We derive interaction-induced corrections to the Usadel equation governing the superconducting gap function, and show that diffusion and localization effects drastically modify the interplay between fermionic incoherence and strong pairing interactions. In particular, we obtain the phase diagram, and demonstrate that (i) there is an intermediate range of disorder strength where superconductivity is enhanced, eventually followed by a tendency towards the superconductor-insulator transition at stronger disorder; and (ii) diffusive particle-particle modes (so-called ``Cooperons'') acquire anomalous dynamical scaling $z=4$, indicating strong non-Fermi liquid behavior.

Free energy and specific heat near a quantum critical point of a metal

We analyze free energy and specific heat for fermions interacting with gapless bosons at a quantum-critical point (QCP) in a metal. We use the Luttinger-Ward-Eliashberg formula for the free energy in the normal state, which includes contributions from bosons, fermions, and their interaction, all expressed via fully dressed fermionic and bosonic propagators. The sum of the last two contributions is the free energy $F_\gamma$ of an effective low-energy model of fermions with boson-mediated dynamical 4-fermion interaction $V (\Omega_m) \propto 1/|\Omega_m|^\gamma$ (the $\gamma-$model). This purely electronic model has been used to analyze the interplay between non-Fermi liquid (non-FL) behavior and pairing near a QCP, which are both independent of the upper energy cutoff $\Lambda$. However, the specific heat $C_\gamma (T)$, obtained from $F_\gamma$, does depend on $\Lambda$. We argue that this dependence is spurious and cancels out, once we include the contribution from bosons. We compare our $C(T)$ with the one obtained within the $\gamma-$model using recently proposed regularization of $F_\gamma$. We argue that for $\gamma <1$, the full $C(T)$ and the regularized $C_\gamma (T)$ differ by a $\gamma-$dependent prefactor, while for $\gamma >1$, the full $C(T)$ is the sum of $ C_\gamma (T)$ and the specific heat of free bosons with fully dressed mass. For these $\gamma$, $C_\gamma (T)$ is negative. The authors of Ref. [1] argued that a negative $ C_\gamma (T)$ implies that the normal state becomes unstable at some distance to a QCP. In our calculation, both terms in $C(T)$ come from the same source, and $ C_\gamma (T)$ is smaller as long as vertex corrections can be safely neglected. We then argue that the normal state remains stable even at a QCP.

Nematicity-enhanced superconductivity in systems with a non-Fermi liquid behavior

We explore the interplay between nematicity (spontaneous breaking of the sixfold rotational symmetry), superconductivity, and non-Fermi liquid behavior in partially flat-band (PFB) models on the triangular lattice. A key result is that the nematicity (Pomeranchuk instability), which is driven by many-body effect and stronger in flat-band systems, enhances superconducting transition temperature in a systematic manner on the T c dome. There, a plausible -wave symmetry, in place of the conventional -wave, governs the nematicity-enhanced pairing with a sharp rise in the T c dome on the filling axis. When the sixfold symmetry is spontaneously broken, the pairing interaction is shown to become stronger with more compact pairs in real space than when the symmetry is enforced. These are accompanied by a non-Fermi character of electrons in the PFBs with many-body interactions.

Monte Carlo simulation of the topological quantities in fractional quantum Hall systems

Generally speaking, for a fractional quantum Hall (FQH) state, the electronic occupation number for each Landau orbit could be obtained from numerical methods such as exact diagonalization, density matrix renormalization group or algebraic recursive schemes (Jack polynomial). In this work, we apply a Metroplis Monte Carlo method to calculate the occupation numbers of several FQH states in cylinder geometry. The convergent occupation numbers for more than 40 particles are used to verify the chiral bosonic edge theory and determine the topological quantities via momentum polarization or dipole moment. The guiding center spin, central charge and topological spin of different topological sectors are consistent with theoretical values and other numerical studies. Especially, we obtain the topological spin of $e/4$ quasihole in Moore-Read and 331 states. At last, we calculate the electron edge Green's functions and analysis position dependence of the non-Fermi liquid behavior.

FL* Interpretation of a Dichotomy in the Spin Susceptibility of the Cuprates

We propose that some dichotomic Fermi liquid versus non-Fermi liquid behaviours of physical quantities in hole-doped cuprates can be explained in terms of the FL* fractionalized Fermi liquid concept, introduced some years ago, even beyond the region of underdoping. The particle excitations of this FL* system are the holon carrying charge, the spinon carrying spin 1/2, gauge fluctuations coupling them and the hole as a spinon–holon bound state or resonance due to gauge binding. In our proposal, physical responses have a Fermi-liquid-type behaviour if they are dominated by the hole resonance, whereas a non-Fermi liquid behaviour appears if they are dominated by spinon–spinon (and possibly also holon–holon) gauge interactions. The specific case of spin susceptibility in the so-called "strange metal phase" is discussed. The uniform susceptibility turns out to be hole-dominated, the spin-lattice relaxation rate in the Cu sites is spinon-dominated.

Valley-polarized nematic order in twisted moiré systems: In-plane orbital magnetism and crossover from non-Fermi liquid to Fermi liquid

The interplay between strong correlations and non-trivial topology in twisted moir\'e systems can give rise to a rich landscape of ordered states that intertwine the spin, valley, and charge degrees of freedom. In this paper, we investigate the properties of a system that displays long-range valley-polarized nematic order. Besides breaking the threefold rotational symmetry of the triangular moir\'e superlattice, this type of order also breaks twofold rotational and time-reversal symmetries, which leads to interesting properties. First, we develop a phenomenological model to describe the onset of this ordered state in twisted moir\'e systems and to explore its signatures in their thermodynamic and electronic properties. Its main manifestation is that it triggers the emergence of in-plane orbital magnetic moments oriented along high-symmetry lattice directions. We also investigate the properties of the valley-polarized nematic state at zero temperature. Due to the existence of a dangerously irrelevant coupling $\lambda$ in the six-state clock model that describes the putative valley-polarized nematic quantum critical point, the ordered state displays a pseudo-Goldstone mode. Using a two-patch model, we compute the fermionic self-energy to show that down to very low energies, the Yukawa-like coupling between the pseudo-Goldstone mode and the electronic degrees of freedom promotes the emergence of non-Fermi liquid behavior. Below a crossover energy scale $\Omega^{*}\sim\lambda^{3/2}$, however, Fermi liquid behavior is recovered. Finally, we discuss the applicability of these results to other non-trivial nematic states, such as the spin-polarized nematic phase.

Thermopower of a Luttinger-liquid-based Two-channel Charge Kondo Circuit: Nonperturbative Solution

Recently, the influence of electron-electron interactions on the thermoelectric transport in a two-channel charge Kondo circuit has been studied in [Phys. Rev. B 105, L121405 (2022)]. In this paper, we revisit the Luttinger-liquid-based model and discuss in details the limit where the spin field is noninteracting (\(g_\sigma = 1\)) and the interaction in the charge sector is repulsive (\(0&lt; g_\rho \leq 1\)). The thermoelectric transport coefficients are computed nonperturbatively with respect to the reflection amplitude at the quantum point contact. At low temperatures the thermopower shows the non-Fermi liquid behavior in the vicinity of the Coulomb peaks. We also demonstrate that repulsive interaction results in the enhancement of the thermoelectrical power.

Exact solution of the topological symplectic Kondo problem

The Kondo effect is an archetypical phenomenon in the physics of strongly correlated electron systems. Recent attention has focused on the application of Kondo physics to quantum information science by exploiting overscreened Kondo impurities with residual anyon-like impurity entropy. While this physics was proposed in the fine-tuned multi-channel Kondo setup or in the Majorana-based topological Kondo effect, we here study the Kondo effect with symplectic symmetry Sp(2k) and present details about the implementation which importantly only involves conventional s-wave superconductivity coupled to an array of resonant levels and neither requires perfect channel symmetry nor Majorana fermions. We carefully discuss the role of perturbations and show that a global Zeeman drives the system to a 2-channel SU(k) fixed point. Exact results for the residual entropy, specific heat and magnetization are derived using the thermodynamic Bethe Ansatz for Sp(2k). This solution not only proves the existence of a quantum critical ground state with anyon-like Hilbert space dimension, but also a particularly weak non-Fermi liquid behavior at criticality. We interpret the weakness of non-analyticities as a manifestation of suppressed density of states at the impurity causing only a very weak connection of putative anyons and conduction electrons. Given this weak connection, the simplicity of the design and the stability of the effect, we conjecture that the symplectic Kondo effect may be particularly suitable for quantum information applications.

Pair Density Wave Order from Electron Repulsion.

A pair density wave (PDW) is a superconductor whose order parameter is a periodic function of space, without an accompanying spatially uniform component. Since PDWs are not the outcome of a weak-coupling instability of a Fermi liquid, a generic pairing mechanism for PDW order has remained elusive. We describe and solve models having robust PDW phases. To access the intermediate coupling limit, we invoke large-N limits of Fermi liquids with repulsive BCS interactions that admit saddle point solutions. We show that the requirements for long-range PDW order are that the repulsive BCS couplings must be nonmonotonic in space and that their strength must exceed a threshold value. We obtain a phase diagram with both finite temperature transitions to PDW order and a T=0 quantum critical point, where non-Fermi liquid behavior occurs.

Non-Fermi Liquid Behavior in the Three-Dimensional Hubbard Model

We present a numerical study on the non-Fermi liquid behavior of a three-dimensional strongly correlated system. The Hubbard model in a simple cubic lattice is simulated by the dynamical cluster approximation; in particular, the quasi-particle weight is calculated at finite dopings for a range of temperatures. By fitting the quasi-particle weight to the marginal Fermi liquid form at finite doping near the putative quantum critical point, we find evidence of a separatrix between Fermi liquid and non-Fermi liquid regions. Our results suggest that a marginal Fermi liquid and possibly a quantum critical point exist in the non-symmetry broken solution of the three-dimensional interacting electron systems. We also calculate the spectral function, close to the half-filling, and we obtain evidence of pseudogap.

Parameter-free analytic continuation for quantum many-body calculations

We develop a reliable parameter-free analytic continuation method for quantum many-body calculations. Our method is based on a kernel grid, a causal spline, a regularization using the second-derivative roughness penalty, and the L-curve criterion. We also develop the L-curve averaged deviation to estimate the precision of our analytic continuation. To deal with statistically obtained data more efficiently, we further develop a bootstrap-averaged analytic continuation method. In the test using the exact imaginary-frequency Green's function with added statistical error, our method produces the spectral function that converges systematically to the exact one as the statistical error decreases. As an application, we simulate the two-orbital Hubbard model for various electron numbers with the dynamical-mean field theory in the imaginary time and obtain the real-frequency self-energy with our analytic continuation method, clearly identifying a non-Fermi liquid behavior as the electron number approaches the half filling from the quarter filling. Our analytic continuation can be used widely and it will facilitate drawing clear conclusions from imaginary-time quantum many-body calculations.

Crossed Luttinger liquid hidden in a quasi-two-dimensional material

Although the concept of Luttinger liquid (LL) that describes a one-dimensional (1D) interacting fermion system collapses in higher dimensions, it has been proposed to be closely related to many mysteries including the normal state of cuprate superconductor, unconventional metal, and quantum criticality. Therefore, the generalization of LL model to higher dimensions has attracted substantial research attention. Here we systematically investigate the electronic structure of a quasi-2D compound {\eta}-Mo4O11 using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation. Remarkably, we reveal a prototypical LL behavior originating from the crossing quasi-1D chain arrays hidden in the quasi-2D crystal structure. Our results suggest that {\eta}-Mo4O11 materializes the long sought-after crossed LL phase, where the orthogonal orbital components significantly reduce the coupling between intersecting quasi-1D chains and therefore maintain the essential properties of LL. Our finding not only presents a realization of 2D LL, but also provides a new angle to understand non-Fermi liquid behaviors in other 2D and 3D quantum materials.

Non-Fermi liquid behavior and quantum criticality in cubic heavy fermion systems with non-Kramers multipolar local moments

Notable non-Fermi liquid and quantum critical behaviors are observed in rare-earth metallic systems with non-Kramers local moments supporting a number of different multipolar moments. A prominent example is $\text{Pr(Ti,V)}_{2}\text{Al}_{20}$, where the non-Kramers doublet of the $\text{Pr}^{3+}$ ion allows quadrupolar and octupolar moments, but lacks a dipolar moment. Previous theoretical studies show that a single impurity Kondo problem with such an unusual local moment leads to novel non-Fermi liquid states. In this work, we investigate possible quantum critical behaviors arising from the competition between non-Fermi liquid states and multipolar-ordered phases induced by the RKKY interaction. We consider a local version of the corresponding Kondo lattice model, namely the Bose-Fermi Kondo model. Here, the multipolar local moments are coupled to fermionic and bosonic bath degrees of freedom representing the multipolar Kondo effect and RKKY interactions. Using a perturbative renormalization group (RG) study up to two loop order, we find critical points between non-Fermi liquid Kondo fixed points and a quadrupolar ordered fixed point. The critical points describe quantum critical behaviors at the corresponding phase transitions and can be distinguished by higher order corrections in the octupolar susceptibility that can be measured by ultrasound experiments. Our results imply the existence of a rich expansion of the phases and quantum critical behaviors in multipolar heavy fermion systems.

Heat Conductance Oscillations in Two Weakly Connected Charge Kondo Circuits

We revisit a model describing Seebeck effect on a weak link between two charge Kondo circuits, which has been proposed in the [Phys. Rev. B 97 (2018) 085403]. We calculate the thermoelectric coefficients in the perturbation theory assuming smallness of the reflection amplitudes of the quantum point contacts. We focus on the linear response equations for the heat conductance in three different scenarios as: Fermi liquid vs Fermi liquid, Fermi liquid vs non-Fermi liquid, non-Fermi liquid vs non-Fermi liquid. The oscillations of the heat conductance as a function of the gate voltage of each quantum dot are analysed in both Fermi liquid and non-Fermi liquid regimes. We discuss possible experimental realizations of the model to observe the signatures of the non-Fermi liquid behaviour in the heat conductance measurements.