nJ Pulse Research Articles

Spatiotemporal dissipation dynamics: a route to high-beam-quality and high-peak-power spatiotemporal mode-locked fiber lasers

Spatiotemporal mode-locking (STML) opens a new avenue for implementing high-energy, high-peak-power mode-locked fiber oscillators. However, the compromised beam quality poses a critical limitation to their broader applications. This study presents a method for enhancing the beam quality of STML fiber lasers by employing spatiotemporal dissipation involving the quenching and reabsorption effects of multimode erbium-doped fibers. The proposed technique introduces spatiotemporal saturable absorption, achieving high beam quality without the stringent conditions required for Kerr beam self-cleaning (BSC). Integrating spatiotemporal dissipation with Kerr BSC, we demonstrate an all-anomalous-dispersion Er-doped STML fiber laser, which produces solitons with 6.7 nJ pulse energy (the intracavity solitons with 25.8 nJ pulse energy and >52.8kW peak power), sub-500 fs pulse duration, and beam quality with M x 2/M y 2=1.23/1.20. To our knowledge, it is a record peak power for 1.5 µm band soliton lasers. Additionally, the approach enables the generation of noise-like pulses with M x 2/M y 2=1.04/1.13. This work not only advances our understanding of spatiotemporal dissipation dynamics in STML fiber lasers, but also paves the way toward high-performance STML fiber lasers, rendering them very attractive for applications.

Broadband THz Wave Generation and Detection in Organic Crystal PNPA at MHz Repetition Rates

AbstractOrganic nonlinear optical (NLO) crystals have emerged as efficient room‐temperature emitters of broadband THz radiation with high electric field strengths. Although initially confined to high‐pulse‐energy excitation in the millijoule range with kHz rates, recent efforts have focused on tailoring the physical properties of organic NLO materials for compatibility with popular MHz‐rate telecommunication wavelength lasers emitting nanojoule energy pulses. This is motivated by the large potential of such crystals for more portable and user‐safe spectroscopic systems, additionally complemented by their room‐temperature field‐sensitive THz detection capabilities. In this work, the MHz‐rate operation of the organic crystal PNPA ((E)‐4‐((4‐nitrobenzylidene)amino)‐N‐phenylaniline), which was recently discovered through data mining algorithms and reported to surpass the conversion efficiency of rivaling NLO crystals at 1 kHz repetition rate is demonstrated. Using a compact 200 mW Er:fiber laser producing 18 fs pulses at 50 MHz repetition rate, the THz field generation and detection capabilities of PNPA via performing gas phase spectroscopy in the 1.3–8.5 THz range are demonstrated. A dynamic range of 40 dB over 3.6 s and 70 dB over 2 h is obtained. The work extends the family of organic crystals compatible with telecommunication‐wavelength excitation using nJ pulses for spectroscopy beyond 5 THz.

Similariton-like Pulse Evolution in an Er-Doped Fiber Laser with Hybrid Mode Locking

An Er-doped all-fiber ultrashort pulse laser with positive total net-cavity group-velocity dispersion is demonstrated based on a hybrid mode-locking mechanism ensured by single-walled carbon–boron–nitrogen nanotubes with coaction of the nonlinear polarization evolution effect. The generation regime with a similariton-like spectrum is obtained. The spectrum width is ~31.5 nm, and the minimal pulse duration is ~294 fs at full width at half maximum. The average output power is ~3.2 mW, corresponding to 0.376 nJ pulse energy and 1.25 kW peak power. The fundamental pulse repetition rate is ~8.5 MHz, with a signal-to-noise ratio of 60 dB. The standard deviation of average output optical power stability, measured for 12 h, is about ~1% RMS, and the maximum level of relative intensity noise (RIN) does not exceed <−120 dBc/Hz in the 30 Hz–1 MHz frequency range. To prove the similariton-like regime generation, we also studied numerically and experimentally the pulse evolution during propagation through a laser resonator and output single-mode fiber with anomalous dispersion.

1 MW Peak‐Power Mamyshev Oscillator Started by a Passively Q‐Switched Microchip Laser

Ultrafast fiber lasers (UFLs) have become an attractive alternative to solid‐state lasers (SSL) due to their excellent beam quality, compactness, environmental stability, and easy thermal management. In the last decade, a significant research effort is spent to identify UFL architectures providing pulse energy, duration, and peak power comparable to those of complex and expensive, Ti:sapphire laser systems and semiconductor saturable absorber mirrors mode‐locked, Yb‐doped SSL. Lately, Mamyshev oscillators (MOs), relying on offset spectral filtering combined with nonlinear spectral broadening by self‐phase modulation, emerge as a promising solution and are rapidly becoming the state of the art for high energy/peak power UFLs based on large‐mode‐area (LMA) fibers. The focus of this work is the first demonstration of starting of the mode‐locking regime in an LMA MO with an affordable passively Q‐switched microchip laser. This solution was previously demonstrated only in low‐power MO based on single‐mode fibers, which are intrinsically easier to seed, if compared to high‐gain LMA UFLs, because of the lower amplified spontaneous emission noise floor. This starting technique in an easy‐to‐implement ring LMA MO at 1 μm is tested. The oscillator provides ≈50 nJ pulses at 12 MHz repetition rate with a minimum pulse duration of ≈50 fs after compression, resulting in MW peak power.

All-Solid-State Post-Compression of Low-Energy Pulses at High Repetition Rate

We demonstrate a proof of principle of a simple all-solid-state post-compression setup for low-energy, high-repetition-rate laser pulses, where spectral broadening was performed using a combination of highly nonlinear bulk materials in a simple single-pass geometry. The 75 fs, 210 nJ pulses from an amplified 76 MHz, 15.7 W Yb:KGW oscillator after sequential spectral broadening in ZnS and YAG samples of 2 mm and 15 mm thickness, respectively, were compressed to 37 fs by means of Gires–Tournois interferometric mirrors. The post-compressed pulses with an average power of 11.47 W demonstrated reasonable spatial-spectral homogeneity of the beam with the spectral overlap parameter V>83% and good beam quality with Mx2=1.28 and My2=1.14.

Spectrally tunable phase-biased NALM mode-locked Yb:fiber laser with nJ-level pulse energy

Applications of mode-locked fiber lasers benefit from robust and self-starting mode-locking, spectral tuning, high pulse energy and high average power. All-polarization-maintaining (PM) fiber lasers mode-locked with a phase-biased nonlinear amplifying loop mirror (NALM) have been shown to be very robust and reliably self-starting, and provide either spectral tuning or high pulse energy, but not both. We report on a simple method for concurrent spectral tuning and nanojoule-level pulse energy scaling of an all-PM phase-biased NALM mode-locked Yb:fiber laser, which we demonstrate over a 54 nm tuning range, reaching up to 1.67 nJ pulse energy and 126 mW average power. Unlike other laser configurations, our results show that net normal dispersion is not necessary or optimal for scaling the pulse energy of this type of mode-locked fiber laser.

50-fs pulse bursts via gain-managed nonlinear amplification

We report the first gain-managed nonlinear amplifier operating in burst mode, delivering 50-fs, 600- nJ pulses. Due to a complex interplay between nonlinearity and gain, the amplification is influenced non- trivially and collectively by all the pulses within a burst.

Resonant Fully Dielectric Metasurfaces for Ultrafast Terahertz Pulse Generation

In the framework of optical frequency conversion, metasurfaces have elevated the potential for effective interfacial nonlinear coefficients through various modes of field localization. For the generation of pulsed ultrafast terahertz (THz) signals, metasurfaces present a viable alternative in the domain of surface-scalable sources driven by low-power oscillators (using nJ pulses). However, recent innovations have predominantly relied on surface plasmons (metals) and, more broadly, on excitations within non-transparency windows—conditions that typically impose limitations on applications and the choice of platforms. Here, we demonstrate the utilization of a fully-dielectric, fully transparent semiconductor that exploits surface-nano-structure-mediated resonances alongside its inherent quadratic nonlinear response. Our system exhibits a remarkable 40-fold efficiency enhancement in comparison to the non-decorated substrate.

589 nm yellow laser pumped Kerr-lens mode-locked Alexandrite laser producing sub-50 fs pulses.

We report a femtosecond Kerr-lens mode-locked (KLM) Alexandrite laser resonantly pumped by a 589 nm yellow laser. The 4 nJ pulses as short as 42 fs were obtained corresponding to a peak power of 100 kW. With the repetition rate of 104 MHz, the average power of 420 mW was attained. The time-bandwidth product of generated laser pulse was measured to be 0.324 with a beam quality factor of M2 ≤ 1.13. The exceptional performance of visible femtosecond laser may find potential applications in various fields.

Noise-like pulses generation and its beam self-cleaning effect in an all-fiber multimode cavity with a figure-8 scheme

The beam profiles of multimode mode-locked fiber lasers are highly multimode, the speckled beam profiles limit their potential application. To improve the beam profiles of multimode mode-locked fiber lasers, we proposed an all-fiber figure-8 multimode cavity and experimentally demonstrated the generation of noise-like pulses (NLPs) and beam self-cleaning of NLPs in the cavity at 1.5 µm. The laser was mode locked by a nonlinear amplifying loop mirror, an Er/Yb co-doped fiber provided gain, and 50 m OM4 fiber introduced enough nonlinear phase shift difference. The scheme generated NLPs with 159 mW average power, 2.78 MHz repetition rate and 57.19 nJ pulse energy. The packet duration of the NLPs increased from 0.61 ns to 2.99 ns when the pump power was increased from 2 W to 9 W. Nonlinear beam self-cleaning with a near Gaussian beam profile output was achieved in the multimode fiber laser. The M2 was measured to be 2.41 at the pulse energy of 6.83 nJ. We also obtained spatiotemporal mode-locked pulses with 1.03 ps duration and speckled beam profiles. This is the first experimental demonstration of NLPs in multimode fiber lasers, and beam self-cleaning of NLPs was observed for the first time. The results enriched nonlinear dynamics in multimode fiber lasers.

Characterizing Passively Q-switched Fiber Laser in LiDAR Application

A LiDAR system consists of a Q-switched fiber laser that emits light pulses to measure the distance from the target. We have experimentally demonstrated a passively Q-switched erbium-doped fiber laser (EDFL) by employing graphene saturable absorber (SA). The SA was prepared by dipping a polyvinyl alcohol (PVA) thin film into the graphene solution. Once the SA was fabricated, it can be placed in the cavity to perform pulses and it is operating at 1558.92 nm. The shortest pulse received is 3.9 μs and generated at the repetition rate of 115 kHz. The pulses are stable between pump powers of 59.6mW and 127.1 mW. At the maximum pump power value of127.1 mW, thelaser cavity produced pulses with a 1.4mW output power and a 1.1nJ pulse energy.

Si-Cr Nano-Alloys Fabricated by Direct Femtosecond Laser Writing.

Ultra-short 230 fs laser pulses of 515 nm wavelength were tightly focused into 700 nm focal spots and utilised in opening ∼400 nm nano-holes in a Cr etch mask that was tens-of-nm thick. The ablation threshold was found to be 2.3 nJ/pulse, double that of plain silicon. Nano-holes irradiated with pulse energies below this threshold produced nano-disks, while higher energies produced nano-rings. Both these structures were not removed by either Cr or Si etch solutions. Subtle sub-1 nJ pulse energy control was harnessed to pattern large surface areas with controlled nano-alloying of Si and Cr. This work demonstrates vacuum-free large area patterning of nanolayers by alloying them at distinct locations with sub-diffraction resolution. Such metal masks with nano-hole opening can be used for formation of random patterns of nano-needles with sub-100 nm separation when applied to dry etching of Si.

Dual-tapered Mach Zehnder Interferometer for Dual-wavelength Q-Switched YDFL using Molybdenum Diselenide

A dual-wavelength Q-switched YDFL by utilizing MoSe2 thin film was successfully achieved in cavity ring. The dual synchronous wavelength output spectrum centered at 1035.8nm to 1040.2nm was achieved with repetition rate of 15.3 kHz to 35.2 kHz. Moreover, the maximum pulse energy was 2.8nJ and minimum pulse width was 1.8µs. In this paper, MoSe2 thin film capabilities as saturable absorber in 1-micron region was successfully achieved. Thus pave a new insight of transition metal chalcogenides (TMD) based photonics device.

Spectrally combined four-diode-pumped femtosecond Ti:sapphire laser with 16.3 nJ pulse and its application to video-rate coherent anti-Stokes Raman scattering spectro-microscopy.

We demonstrate the generation of high-energy femtosecond pulses by a spectrally combined four-diode-pumped Ti:sapphire laser with semi-conductor saturable absorber mirror mode locking. To achieve energy scaling, the laser cavity was extended using a design based on the Herriott multipass cell. The laser operates at a 17.5 MHz repetition rate and generates pulses with energies as high as 16.3 nJ and 80 fs in duration. The signal-to-noise ratio at the fundamental frequency showed an extinction ratio of >50 dB relative to the carrier. This compact single laser was applied to video-rate forward and backward coherent anti-Stokes Raman scattering spectro-microscopy with a pixel dwell time of 122 ns, which is the lowest dwell time ever achieved, to the best of our knowledge.

Realising high aspect ratio 10 nm feature size in laser materials processing in air at 800 nm wavelength in the far-field by creating a high purity longitudinal light field at focus

In semiconductor and data storage device manufacturing, it is desirable to produce feature sizes less than 30 nm with a high depth-to-width aspect ratio on the target material rapidly at a low cost. However, optical diffraction limits the smallest focused laser beam diameter to around half of the laser wavelength (λ/2). The existing approach to achieving nanoscale fabrication is mainly based on costly extreme ultraviolet (EUV) technology operating within the diffraction limit. In this paper, a new method is shown to achieve materials processing resolution down to 10 nm (λ/80) at an infrared laser wavelength of around 800 nm in the far-field, in air, well beyond the optical diffraction limit. A high-quality longitudinal field with a purity of 94.7% is generated to realise this super-resolution. Both experiments and theoretical modelling have been carried out to verify and understand the findings. The ablation craters induced on polished silicon, copper, and sapphire are compared for different types of light fields. Holes of 10–30 nm in diameter are produced on sapphire with a depth-to-width aspect ratio of over 16 and a zero taper with a single pulse at 100–120 nJ pulse energy. Such high aspect ratio sub-50 nm holes produced with single pulse laser irradiation are rarely seen in laser processing, indicating a new material removal mechanism with the longitudinal field. The working distance (lens to target) is around 170 µm, thus the material processing is in the far field. Tapered nano-holes can also be produced by adjusting the lens to the target distance.

Effect of femtosecond laser cutting parameters on the results of small-incision lenticule extraction.

To determine the effect of femtosecond laser cutting parameters on small-incision lenticule extraction (SMILE) results by evaluating cap thickness, interface light scattering, and visual and refractive outcomes. SynsLaser Clinic, Oslo, Norway. Retrospective. 58 right eyes treated with SMILE using a programmed cap thickness of 130 μm were divided into 2 groups according to laser settings: Group 1: 165 nJ pulse energy and 4.5 μm spot separation (n = 36); Group 2: 125 nJ pulse energy and 4.2 μm spot separation (n = 22). The cap thickness was measured within the central 5 mm of the horizontal meridian using spectral-domain optical coherence tomography. Postoperative interface light scattering was graded based on the percentage area showing light scattering: 0: no scattering; 1: ≤25%; 2: 26% to 50%; 3: 51% to 75%; and 4: >75%. At 3 months postoperatively, cap thickness was 138.9 ± 6.2 μm in Group 1 and 149.4 ± 3.5 μm in Group 2 ( P < .001). Interface scattering was 0.9 ± 1.0 in Group 1 and 0.3 ± 0.9 in Group 2 ( P < .05), with no scattering in 33.3% and 86.4% of the eyes, respectively. The postoperative spherical equivalent refraction was -0.03 ± 0.44 diopters (D) in Group 1 and -0.04 ± 0.31 D in Group 2. In Group 1, 83.3% of the eyes were within ± 0.5 D of the desired outcome, and 69.4% achieved an uncorrected distance visual acuity of 20/20 or better. In Group 2, these values were 95.5% and 86.4%, respectively. Lower pulse energy with tighter spots seems to reduce interface light scattering and improve refractive outcomes while also significantly increasing cap thickness.

Generation of 15 nJ pulse energy by a sub-150 fs thulium-doped fiber Mamyshev oscillator.

Mamyshev oscillators have pushed the frontiers in output parameters of ytterbium- and erbium-based ultrafast fiber oscillators in the spectral region around 1 µm and 1.5 µm within the last few years tremendously. In order to expand the superior performance toward the 2 µm spectral region, we present in this Letter an experimental investigation of the generation of high-energy pulses by a thulium-doped fiber Mamyshev oscillator. Generating highly energetic pulses is enabled by a tailored redshifted gain spectrum in a highly doped double-clad fiber. The oscillator emits pulses with an energy of up to 15 nJ, which can be compressed to 140 fs.

High energy and low noise soliton fiber laser comb based on nonlinear merging of Kelly sidebands.

Optical solitons in mode-locked laser cavities with dispersion-nonlinearity interaction, delivers pulses of light that retain their shape. Due to the nature of discretely distributed dispersion and nonlinearity, optical solitons can emit Kelly-sidebands via the frequency coupling of soliton and dispersive waves. In this paper, we generate a high-energy femtosecond laser comb, by using the intracavity Kelly radiations and 3rd order nonlinearities. By increasing the intracavity power, the soliton envelop and the Kelly-sidebands merge together via four-wave-mixing, forming a super-continuum spectrum, obtaining 3.18 nJ pulse energy. A supercontinuum span covering from 1100 nm to 2300 nm for further self-referenced f-2f stabilization can be directly achieved by using an amplification-free external supercontinuum technique. Our finding not only demonstrates a non-trivial frequency-time evolution based on 'erbium + χ(3)' nonlinear gains, but also offers a new opportunity to develop practically compact fiber frequency combs for frequency metrology or spectroscopy.

Aluminum oxide/polydimethylsiloxane-based Q-switched mode-locked erbium-doped fiber laser

A Q-switched mode-locked (QSML) erbium-doped fiber laser integrating aluminum oxide saturable absorber (Al2O3-SA) is demonstrated. With the help of polydimethylsiloxane polymer, Al2O3 powder was securely transferred on a tapered fiber surface and functioned as SA. A QSML pulse sequence was realized at a central wavelength of 1567.4 nm from 80 to 320 mW pump power with its envelope repetition rate ranging from 30.59 to 77.46 kHz. The short duration of 2.54 µs Q-switched envelope comprised of 8.3 ns ML pulses with 252 nJ pulse energy was realized at the maximum pump power of 320 mW. The high damage threshold of Al2O3-SA of beyond 7 GW/cm2 contributes to the future exploration of bulk metal oxide for high-energy optical pulse generation in near-infrared wavelengths.

Megawatt pulses from an all-fiber and self-starting femtosecond oscillator.

Mamyshev oscillators produce high-performance pulses, but technical and practical issues render them unsuitable for widespread use. Here we present a Mamyshev oscillator with several key design features that enable self-starting operation and unprecedented performance and simplicity from an all-fiber laser. The laser generates 110 nJ pulses that compress to 40 fs and 80 nJ with a grating pair. The pulse energy and duration are both the best achieved by a femtosecond all-fiber laser to date, to our knowledge, and the resulting peak power of 1.5 MW is 20 times higher than that of prior all-fiber, self-starting lasers. The simplicity of the design, ease of use, and pulse performance make this laser an attractive tool for practical applications.