Near-field Terahertz Research Articles

High-efficiency terahertz surface plasmon metacoupler empowered by bilayer bright–dark mode coupling

Conversion from free-space waves to surface plasmons has been well studied as a key aspect of plasmonics. In particular, efficient coupling and propagation of surface plasmons via phase gradient metasurfaces are of great current research interest. Hereby, we demonstrate a terahertz metacoupler based on a bilayer bright–dark mode coupling structure attaining near-perfect conversion efficiency (exceeding 95%) without considering absorption loss of the materials and maintaining a high conversion level even when the area of the excitation region changes. To validate our design, a fabricated metacoupler was assessed by scanning near-field terahertz microscopy. Our findings could pave the way for developing high-performance plasmonic devices encompassing ultra-thin and compact functional devices for a diverse range of applications, especially within the realm of high-speed terahertz communications.

Terahertz Near-Field Imaging of Buried Structures

Terahertz Near-Field Imaging of Buried Structures

Near-field terahertz electro-optical imaging based on a polarization image sensor

Abstract This paper presents a hyperspectral microscopy system that offers two-dimensional (2D) measurement of the spectral phase and amplitude information of terahertz (THz) radiation without the need for raster scanning. To achieve this, a new THz imaging method is introduced, wherein the distribution of the THz electric field is spatially measured using the electro-optic effect with a commercial polarization image sensor. This method enables the direct measurement of polarization components, eliminating the need for the polarization optics usually required in conventional electro-optical imaging. The performance of this imaging method is compared with a conventional 2D imaging system based on a standard visible camera. Finally, the sub-wavelength resolution capabilities of this new sensor are demonstrated by imaging a sample in the near field.

Near-field terahertz single-pixel imaging with ultralow sampling ratio

Near-field terahertz single-pixel imaging with ultralow sampling ratio

Unveiling enamel demineralization mechanisms by sensitive dielectric differentiation based on terahertz nanospectroscopy.

The early stage of dental caries, i.e. demineralization, has always been a topic of concern to dentists. Understanding the essential mechanism of its occurrence is of great significance for the prevention and treatment of dental caries. However, owing to limitations in resolution and the detection capabilities of diagnostic tools, the study of enamel demineralization has always been a challenge. Terahertz (THz) technology, especially the combination of scanning near-field optical microscopy (s-SNOM) and THz time-domain spectroscopy (TDS), due to its nanoscale resolution, has shown great advantages in the field of biological imaging. Here, a THz s-SNOM system is used to perform near-field imaging of enamel before and after demineralization at the nanoscale. It can be found that near-field signals decrease significantly after demineralization. This is due to the changes of the crystal lattice and the transfer of mineral ions during demineralization, which leads to a decrease in the permittivity of the enamel. The novel approach in this study reveals the essence of demineralization and lays the groundwork for additional research and potential interventions.

Continuous Template Growth of Large-Scale Tellurene Films on 1T'-MoTe2.

Use of a template triggers an epitaxial interaction with the depositing material during synthesis. Recent studies have demonstrated that two-dimensional tellurium (tellurene) can be directionally oriented when grown on transition metal dichalcogenide (TMD) templates. Specifically, employing a T-phase TMD, such as WTe2, restricts the growth direction even further due to its anisotropic nature, which allows for the synthesis of well-oriented tellurene films. Despite this, producing large-area epitaxial films still remains a significant challenge. Here, we report the continuous synthesis of a 1T'-MoTe2 template via chemical vapor deposition and tellurene via vapor transport. The interaction between helical Te and the 1T'-MoTe2 template facilitates the Te chains to collapse into ribbon shapes, enhancing lateral growth at a rate approximately 6 times higher than in the vertical direction, as confirmed by scanning electron microscopy and atomic force microscopy. Interestingly, despite the predominance of the lateral growth, cross-sectional transmission electron microscopy analysis of the tellurene ribbons revealed a consistent 60-degree incline at the edges. This suggests that the edges of the tellurene ribbons, where they contact the template surface, are favorable sites for additional Te absorption, which then stacks along the incline angle to expand. Furthermore, controlling the synthesis temperature, duration, and preheating time has facilitated the successful synthesis of tellurene films. The resultant tellurene exhibited hole mobility as high as ∼400 cm2/V s. After removing the underlying metallic template with plasma treatment, the film showed a current on/off ratio of ∼103. This ratio was confirmed by two-terminal field-effect transistor measurements and supported by near-field terahertz (THz) spectroscopy mapping.

Near-Field Terahertz Morphological Reconstruction Nanoscopy for Subsurface Imaging of Protein Layers.

Protein layers formed on solid surfaces have important applications in various fields. High-resolution characterization of the morphological structures of protein forms in the process of developing protein layers has significant implications for the control of the layer's quality as well as for the evaluation of the layer's performance. However, it remains challenging to precisely characterize all possible morphological structures of protein in various forms, including individuals, networks, and layers involved in the formation of protein layers with currently available methods. Here, we report a terahertz (THz) morphological reconstruction nanoscopy (THz-MRN), which can reveal the nanoscale three-dimensional structural information on a protein sample from its THz near-field image by exploiting an extended finite dipole model for a thin sample. THz-MRN allows for both surface imaging and subsurface imaging with a vertical resolution of ∼0.5 nm, enabling the characterization of various forms of proteins at the single-molecule level. We demonstrate the imaging and morphological reconstruction of single immunoglobulin G (IgG) molecules, their networks, a monolayer, and a heterogeneous double layer comprising an IgG monolayer and a horseradish peroxidase-conjugated anti-IgG layer. The established THz-MRN presents a useful approach for the label-free and nondestructive study of the formation of protein layers.

Spintronic terahertz metasurface emission characterized by scanning near-field nanoscopy

Abstract Understanding the ultrafast excitation, detection, transportation, and manipulation of nanoscale spin dynamics in the terahertz (THz) frequency range is critical to developing spintronic THz optoelectronic nanodevices. However, the diffraction limitation of the sub-millimeter waves – THz wavelengths – has impaired experimental investigation of spintronic THz nano-emission. Here, we present an approach to studying laser THz emission nanoscopy from W|CoFeB|Pt metasurfaces with ∼60-nm lateral spatial resolution. When comparing with statistic near-field THz time-domain spectroscopy with and without the heterostructures on fused silica substrates, we find that polarization- and phase-sensitive THz emission nanoscopy is more sensitive than the statistic THz scattering intensity nanoscopy. Our approach opens explorations of nanoscale ultrafast THz spintronic dynamics in optically excited metasurfaces.

Analysis of Near-Field Magnetic Responses on ZrTe5 through Cryogenic Magneto-THz Nano-Imaging

One manifestation of light-Weyl fermion interaction is the emergence of chiral magnetic effects under magnetic fields. Probing real space magnetic responses at terahertz (THz) scales is challenging but highly desired, as the local responses are less affected by the topologically trivial inhomogeneity that is ubiquitous in spatially averaged measurements. Here, we implement a cryogenic THz microscopy instrument under a magnetic field environment—a task only recently achieved. We explore the technical approach of this system and characterize the magnetic field’s influence on our AFM operation by statistical noise analysis. We find evidence for local near-field spatial variations in the topological semimetal ZrTe5 up to a 5-Tesla magnetic field and obtain near-field THz spectra to discuss their implications for future studies on the chiral magnetic effect.

A mini-review of signal processing techniques for RIS-assisted near field THz communication

Reflecting Intelligent Surfaces (RISs) are reshaping the landscape of wireless communications, particularly in the terahertz (THz) frequency bands, offering promising solutions to inherent challenges in the bands. THz communication boasts bandwidths exceeding 100 GHz, leading to data rates potentially in the terabits per second (Tbps) range, thereby making it an attractive proposition for wireless communications, imaging, and sensing. However, benefits come with challenges, including significant molecular absorption, scattering, diffraction, and hardware limitations. Moreover, as bandwidth in the THz range increases, so does the difficulty of signal processing at Nyquist rate. RIS emerges as a game-changer for 6G and beyond by providing programmable reflecting elements that can adaptively modify the phases and amplitudes of incident signals, enabling precision in directing THz waves and enhancing received signal strength. Such capabilities can significantly mitigate path loss and atmospheric absorption challenges. Furthermore, inherent pencil beamforming capabilities of RIS lead to optimized energy utilization. Major challenge in THz communications is the pressing needs for efficient algorithms for robust THz transceivers and optimizing RIS elements. This review describes the integration of RIS and near-field THz communications, highlighting their future potential and challenges for the next-generation wireless networks. In this article, a comprehensive understanding of the complexities and nuances of near-field propagation in 6G networks, especially as the technology shifts towards extremely large-scale antenna arrays (ELAA). Additionally, it will introduce the transformative potential of sub-Nyquist rate signal processing and artificial intelligence (AI) offering innovative solutions to address the inherent challenges of 6G communication, especially in channel estimation and beamforming strategies.

Ultrabroadband terahertz-band communications with self-healing bessel beams

The large available bandwidth at sub-terahertz and terahertz frequencies has the potential to enable very high data rates for wireless communications. Moreover, given the large electrical size of terahertz antenna apertures, many future terahertz communication systems will likely operate in the near field. However, due to their reliance on highly directional beams, terahertz systems are susceptible to blockage. Here, we propose using Bessel beams to overcome issues caused by blockage due to their diffraction-free nature and self-healing properties in the near field. We compare the performance of information-bearing Bessel beams and Gaussian beams with and without an obstacle. We later discuss the use of reconfigurable intelligent surfaces to construct terahertz Bessel beams. Finally, we propose a metric to quantify the quality of imperfectly generated terahertz Bessel beams and explore their ability to self-heal. The results demonstrate that Bessel beams are an attractive option for near-field terahertz communications, especially when mitigating the effects of partial blockage.

Parametric Sparse Channel Estimation for RIS-Assisted Terahertz Systems

To support extremely high data rates in 6G wireless networks, reconfigurable intelligent surface (RIS)-assisted terahertz (THz) communications have gained much attention in recent years. By manipulating the phase shifts of reflecting elements, the RIS can proactively adjust the wireless propagation environment of THz systems, thereby enhancing the overall throughput significantly. To realize the full potential of RIS-assisted THz systems, an acquisition of accurate channel information is of great importance. However, since the wavefront of the THz electromagnetic signal is spherical, the conventional channel estimation techniques using the planar wavefront assumption suffer from severe performance degradation in the near-field RIS-assisted THz systems. An aim of this work is to propose an efficient channel estimation technique for near-field RIS-assisted wideband THz systems. Key idea of the proposed polar-domain frequency-dependent RIS-assisted channel estimation (PF-RCE) scheme is to estimate the sparse multipath components (i.e., angles, distances, and path gains) of the near-field THz channel by exploiting the polar-domain sparsity and common support properties. We demonstrate from the numerical evaluations that PF-RCE achieves a significant performance gain over the conventional THz channel estimation schemes in terms of the normalized mean square error (NMSE).

Fourier Transformed Terahertz Spectroscopy Inspired Detection of Evanescent Orders in All Dielectric Sub-Wavelength Grating

Although evanescent orders offer interesting physics, the experimental detection of these modes are very challenging task because of their inherent characteristics. Evanescent orders are non-propagating in nature making it impossible to detect in the far-field. At the same time, near-field detection is also complicated because of the concurrence of propagating and non-propagating diffraction orders. In order to overcome these hindrances, we introduce Fourier transformed terahertz spectroscopy (FTTS) through near-field scanning terahertz microscopy (NSTM) to experimentally detect the non-propagating evanescent orders originating from a 1-dimensional dielectric grating for both the TE and TM configurations. Our studies demonstrate exponential decay of mode strengths away from the grating-air interface confirming them as evanescent waves. Identification of evanescent orders demonstrate the sound competences that FTTS can offer in exploring near-field systems. We believe, FTTS based approaches can pave new avenues on studying other near-field phenomena in terahertz photonic systems in near future.

Observation of Topological Transmission in Terahertz Domino Waveguide Array

In this paper, we propose on-chip terahertz domino waveguide array structures which can enable the topological effect and enhance the robustness of terahertz transmission. Terahertz topological effect (include topologically-protected edge states and binding states) is excited by constructing kink and antikink structures in designed domino waveguide arrays. Furthermore, the robustness of topological waveguide arrays is successfully demonstrated. The topological transmission effects have been experimentally demonstrated using scanning near-field terahertz microscopy. Our study provides a new approach to study the topological photonic transport of waveguide arrays in the terahertz regime and has potential application in terahertz integrated circuit.

Curved Synthetic Aperture Radar for Near-Field Terahertz Imaging

High resolution imaging technique will play an essential role in the future smart imaging applications to provide potential solutions for accurate detection, monitoring and classification of the target. The potential of synthetic aperture radar (SAR) systems to acquire high resolution images has opened new frontiers and led to its exploration in new applications. The conventional microwave radar imaging suffers limited range resolution in the sub-millimeter wave range and optical imaging methods are constrained by the diffraction limit. In the terahertz (THz) regime of the spectrum, the SAR systems could be operated in all the weather, all the time and are capable of penetrating through clouds, smoke, dust etc. to achieve high resolution images beyond the diffraction limit. The curved SAR presents a SAR system created by circularly encircling the target scene. The Circular SAR and Spiral SAR which are based on a circular and cylindrical spiral scanning trajectory, respectively are the scanning methods used for curved SAR. In this paper, we have explored a new toolbox that enables the rapid development of near-field THz-SAR imaging systems and generation of large near-field THz imaging scenarios with the goal to support and facilitate data driven research such as deep learning in the THz community through synthetically generated SAR images as well as its potential for THz based high resolution and 2D/3D near-field imaging application. Initially, the potential advantages of THz-SAR over Microwave SAR and optical imaging methods are presented. Further, a frequency modulated continuous wave (FMCW) radar testbed is simulated in multi-input multi-output (MIMO) configuration for the target frequency band. Moreover, the circular and cylindrical SAR scanning methods are explored for near-field imaging of point targets to obtain 2D and 3D THz-SAR images, respectively. Also, the radar images are reconstructed using the Back Propagation and Polar Formatting Algorithms, focusing on short range applications like indoor environments. Finally, the SAR performance evaluation metrics are reported and a roadmap for future work is presented.

Near-field terahertz nonlinear optics with blue light

The coupling of terahertz optical techniques to scattering-type scanning near-field microscopy (s-SNOM) has recently emerged as a valuable new paradigm for probing the properties of semiconductors and other materials on the nanoscale. Researchers have demonstrated a family of related techniques, including terahertz nanoscopy (elastic scattering, based on linear optics), time-resolved methods, and nanoscale terahertz emission spectroscopy. However, as with nearly all examples of s-SNOM since the technique’s inception in the mid-1990s, the wavelength of the optical source coupled to the near-field tip is long, usually at energies of 2.5 eV or less. Challenges in coupling of shorter wavelengths (i.e., blue light) to the nanotip has greatly inhibited the study of nanoscale phenomena in wide bandgap materials such as Si and GaN. Here, we describe the first experimental demonstration of s-SNOM using blue light. With femtosecond pulses at 410 nm, we generate terahertz pulses directly from bulk silicon, spatially resolved with nanoscale resolution, and show that these signals provide spectroscopic information that cannot be obtained using near-infrared excitation. We develop a new theoretical framework to account for this nonlinear interaction, which enables accurate extraction of material parameters. This work establishes a new realm of possibilities for the study of technologically relevant wide-bandgap materials using s-SNOM methods.

Studying Oral Tissue via Real-Time High-Resolution Terahertz Spectroscopic Imaging

Terahertz (THz) waves are extremely sensitive to water content and biological composition (proteins, genes, and metabolites), which are the key regulator of cancer development. Hence, the application of THz spectroscopy and imaging is promising in the field of biomedicine, especially in cancer diagnosis. Currently, the diagnosis of cancer patients (including tumor borders, tumor stage, etc.) mainly rely on optical microscope observation of pathological slices. The preparation of the slices is complicated and time consuming, and the microscopic field of view is small, which cannot effectively guide the precise removal of the tumor during the operation in time. To solve this problem, a label-free real-time high-resolution near-field THz spectroscopy imaging technique was developed. In this study, we successfully apply this technique to the oral tissue. Compared with conventional point-by-point scanning terahertz time-domain spectroscopy imaging, this technique can exhibit a real-time imaging rate (as high as 20 frames/s at 512 \ifmmode\times\else\texttimes\fi{} 1024 pixels) and a field of view approximately 5 mm in diameter with a spatial resolution up to \ensuremath{\lambda}/10 at 1 THz in near-field condition. The experimental results show that the terahertz spectroscopic imaging in this paper can clearly detect and identify not only biological tissues with different components, but also normal and cancerous tissues, as well as tissues with the same composition but different slice directions. This work lays an experimental foundation for the application of THz spectroscopy imaging to rapid label-free intraoperative diagnosis, and it provides a basis for promoting the wide application of THz technology in the biomedical field.

Quantitative Modeling of Near-Field Interactions in Terahertz Near-Field Microscopy

Terahertz scattering-scanning near-field optical microscopy (THz s-SNOM), combining the best features of terahertz technology and s-SNOM technology, has shown unique advantages in various applications. Consequently, building a model to characterize near-field interactions and investigate practical issues has become a popular topic in THz s-SNOM research. In this study, a finite element model (FEM) is proposed to quantify the near-field interactions, and to investigate the edge effect and antenna effect in THz s-SNOM. Our results indicate that the proposed model can give us a better understanding of the near-field interactions and direct the parameter design of the probe for THz s-SNOM.

Terahertz spoof surface plasmon polariton gradient index lens

Plasmonics takes advantage of surface plasmon polaritons (SPPs), which have the characteristics of strong subwavelength field confinement and enhancement. Plasmonic devices that confine light in regions with dimensions that are smaller than the wavelength have important application prospects in on-chip integrated circuits. Nonetheless, at terahertz frequencies, the weak confinement of SPPs and immature near-field technology hinder the development of related devices. Here, a highly confined SPP mode (spoof SPP) is implemented by structuring metal surfaces. Gradient index lenses with variable indices are constructed by fine-tuning the size of the pillars, and the characteristics of several different lenses are examined and explored by scanning near-field terahertz microscopy. Thus, terahertz waves are regulated and more possibilities are provided for further miniaturization and compactness of THz devices.

Aβ protein growth monitoring by structure-specific label-free THz spectroscopy.

A variety of different amyloid β (Aβ) protein aggregate forms have been linked with severity of Alzheimer's disease (AD) and its aggregation pathway can be a primary biomarker for diagnosis. Our group recently developed the water-based near-field terahertz (THz) spectroscopy technique to measure Aβ in solution (Heo et al., ACS Nano, 2020, 14 (6), 6548-6558). By noting monotonic conductance change with frequency in monomers following Drude tail and nonlinear conductance behaviors in oligomers and fibrils adopting the localization parameter in Smith model, we derived a structure-specific discrete metric that we termed dementia quotient (DQ), which is a structurally defined biophysical index of Aβ aggregation state with modified Drude-Smith model. Furthermore, we investigate Aβ protein dynamics to identify various morphological phase transitions from monomers to fibrils by monitoring the structure-specific DQ values under physiological conditions including body temperature and incubation medium (e.g., buffer versus Matrigel). Our method could ultimately facilitate the early AD diagnosis by clearly detecting of Aβ oligomer state in a nanomolar concentration (∼nm) of the proteins.