Abstract. The Indian capital megacity of Delhi is reeling under deteriorating air quality, and control measures are not yielding any significant changes, mainly due to a poor understanding of sources of emissions; hence, priority option in mitigation planning is lacking. In this paper, we have made an attempt to develop a spatially resolved technological high-resolution gridded (∼0.4km×0.4km) emission inventory for eight major pollutants of the Delhi region where high-resolution activity data of all possible major and unattended minor sources are generated by organizing a mega-campaign involving hundreds of volunteers. It is for the first time that we are able to estimate the decadal growth in emissions of various pollutants by comparing newly developed 2020 emissions with SAFAR (System of Air Quality and Weather Forecasting and Research) emissions of 2010 using the identical methodology and quantum of activity data. The estimated annual emissions for PM2.5, PM10, CO, NOx, VOC, SO2, BC, and OC over the Delhi National Capital Region (NCR) are estimated to be 123.8, 243.6, 799.0, 488.9, 730.0, 425.8, 33.6, and 20.3 Gg yr−1, respectively, for the year 2020. The decadal growth (2010–2020) in PM2.5 and PM10 is found to be marginal at 31 % and 3 %, respectively. The maximum growth is found to be in the transport sector followed by the industrial and other sectors. Maximum decadal growth found for the pollutants BC, OC, and NOx is 57 %, 34 %, and 91 %, respectively. The decadal shift of sectorial emissions with changing policies is examined. The complete dataset is available on Zenodo at https://doi.org/10.5281/zenodo.7715595 (Sahu et al., 2023).